Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer MoS 2

Yao, Kaiyuan; Yan, Aiming; Kahn, Salman; Suslu, Aslihan; Liang, Yufeng; Barnard, Edward S.; Tongay, Sefaattin; Zettl, Alex; Borys, Nicholas J.; Schuck, P. James

doi:10.1103/PhysRevLett.119.087401

Title: Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer ${MoS}_{2}$

Authors:: Yao, Kaiyuan; Yan, Aiming; Kahn, Salman; Suslu, Aslihan; Liang, Yufeng; Barnard, Edward S.; Tongay, Sefaattin; Zettl, Alex; Borys, Nicholas J.; Schuck, P. James

Publication Date:: 2017-08-25

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1376940

Grant/Contract Number:: AC02-05CH11231; AC02-05-CH11231; KC2207; KCWF16

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Physical Review Letters

Additional Journal Information:: Journal Name: Physical Review Letters Journal Volume: 119 Journal Issue: 8; Journal ID: ISSN 0031-9007

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Citation Formats


                    Yao, Kaiyuan, Yan, Aiming, Kahn, Salman, Suslu, Aslihan, Liang, Yufeng, Barnard, Edward S., Tongay, Sefaattin, Zettl, Alex, Borys, Nicholas J., and Schuck, P. James. Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer MoS 2.  United States: N. p., 2017. 
Web.  doi:10.1103/PhysRevLett.119.087401.

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                    Yao, Kaiyuan, Yan, Aiming, Kahn, Salman, Suslu, Aslihan, Liang, Yufeng, Barnard, Edward S., Tongay, Sefaattin, Zettl, Alex, Borys, Nicholas J., & Schuck, P. James. Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer MoS 2.  United States.  https://doi.org/10.1103/PhysRevLett.119.087401

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                    Yao, Kaiyuan, Yan, Aiming, Kahn, Salman, Suslu, Aslihan, Liang, Yufeng, Barnard, Edward S., Tongay, Sefaattin, Zettl, Alex, Borys, Nicholas J., and Schuck, P. James. Fri .  
"Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer MoS 2".  United States.  https://doi.org/10.1103/PhysRevLett.119.087401.

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@article{osti_1376940,

  title        = {Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer MoS 2},

  author       = {Yao, Kaiyuan and Yan, Aiming and Kahn, Salman and Suslu, Aslihan and Liang, Yufeng and Barnard, Edward S. and Tongay, Sefaattin and Zettl, Alex and Borys, Nicholas J. and Schuck, P. James},

  abstractNote = {},

  doi          = {10.1103/PhysRevLett.119.087401},

  journal      = {Physical Review Letters},

  number       = 8,

  volume       = 119,

  place        = {United States},

  year         = {2017},

  month        = {8}

}

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Title: Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer MoS 2

Citation Formats

Analytical approach to excitonic properties of MoS 2 journal, March 2014

Linear Scaling of the Exciton Binding Energy versus the Band Gap of Two-Dimensional Materials journal, August 2015

Photodetectors based on graphene, other two-dimensional materials and hybrid systems journal, October 2014

Emerging Photoluminescence in Monolayer MoS2 journal, April 2010

Carrier dynamics in semiconductors studied with time-resolved terahertz spectroscopy journal, June 2011

Observation of Excitonic Rydberg States in Monolayer MoS 2 and WS 2 by Photoluminescence Excitation Spectroscopy journal, April 2015

Dynamical Excitonic Effects in Doped Two-Dimensional Semiconductors journal, August 2016

Comment on “Linear Scaling of the Exciton Binding Energy versus the Band Gap of Two-Dimensional Materials” journal, May 2017

Population inversion and giant bandgap renormalization in atomically thin WS2 layers journal, June 2015

Influence of Excited Carriers on the Optical and Electronic Properties of MoS 2 journal, June 2014

Direct Imaging of Band Profile in Single Layer MoS 2 on Graphite: Quasiparticle Energy Gap, Metallic Edge States, and Edge Band Bending journal, April 2014

Observation of Rapid Exciton–Exciton Annihilation in Monolayer Molybdenum Disulfide journal, September 2014

Optical Spectrum of MoS 2 : Many-Body Effects and Diversity of Exciton States journal, November 2013

Absorption of light by excitons and trions in monolayers of metal dichalcogenide Mo S 2 : Experiments and theory journal, May 2014

Many-body correlations and excitonic effects in semiconductor spectroscopy journal, January 2006

Intervalley biexcitons and many-body effects in monolayer MoS 2 journal, September 2015

Atomically Thin MoS2 A New Direct-Gap Semiconductor journal, September 2010

Probing excitonic states in suspended two-dimensional semiconductors by photocurrent spectroscopy journal, October 2014

Defect-Induced Photoluminescence in Monolayer Semiconducting Transition Metal Dichalcogenides journal, January 2015

Monolayer excitonic laser journal, October 2015

Large excitonic effects in monolayers of molybdenum and tungsten dichalcogenides journal, September 2012

Electrical control of neutral and charged excitons in a monolayer semiconductor journal, February 2013

Electronic Structure and Luminescence of Quasi-Freestanding MoS 2 Nanopatches on Au(111) journal, July 2016

Atomically thin p–n junctions with van der Waals heterointerfaces journal, August 2014

Giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor journal, August 2014

Trion-Induced Negative Photoconductivity in Monolayer MoS 2 journal, October 2014

Identifying different stacking sequences in few-layer CVD-grown Mo S 2 by low-energy atomic-resolution scanning transmission electron microscopy journal, January 2016

Defects activated photoluminescence in two-dimensional semiconductors: interplay between bound, charged and free excitons journal, September 2013

Exciton radiative lifetime in transition metal dichalcogenide monolayers journal, May 2016

Tightly Bound Excitons in Monolayer WSe 2 journal, July 2014

The quasiparticle zoo journal, December 2016

Extraordinary Sunlight Absorption and One Nanometer Thick Photovoltaics Using Two-Dimensional Monolayer Materials journal, July 2013

Voltage-controlled quantum light from an atomically thin semiconductor journal, May 2015

2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications journal, December 2016

Anomalous Above-Gap Photoexcitations and Optical Signatures of Localized Charge Puddles in Monolayer Molybdenum Disulfide journal, February 2017

Multi-terminal transport measurements of MoS2 using a van der Waals heterostructure device platform journal, April 2015

Optical identification of sulfur vacancies: Bound excitons at the edges of monolayer tungsten disulfide journal, April 2017

Atomic-Scale Spectroscopy of Gated Monolayer MoS 2 journal, April 2016

Electrical Tuning of Exciton Binding Energies in Monolayer WS 2 journal, September 2015

Carrier Plasmon Induced Nonlinear Band Gap Renormalization in Two-Dimensional Semiconductors journal, February 2015

Terahertz-induced exciton signatures in semiconductors: Terahertz-induced exciton signatures in semiconductors journal, June 2013

Tightly bound trions in monolayer MoS2 journal, December 2012

Phase-engineered low-resistance contacts for ultrathin MoS2 transistors journal, August 2014

Evolution of Electronic Structure in Atomically Thin Sheets of WS 2 and WSe 2 journal, December 2012

Engineering Bandgaps of Monolayer MoS 2 and WS 2 on Fluoropolymer Substrates by Electrostatically Tuned Many-Body Effects journal, May 2016

Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS 2 journal, August 2014

Many-body aspects of the optical spectra of bulk and low-dimensional doped semiconductors journal, May 1987

Monolayer semiconductor nanocavity lasers with ultralow thresholds journal, March 2015

Single-layer MoS2 transistors journal, January 2011

Photocarrier relaxation pathway in two-dimensional semiconducting transition metal dichalcogenides journal, July 2014

High Performance Multilayer MoS2Transistors with Scandium Contacts journal, December 2012

Quasiparticle band structures and optical properties of strained monolayer MoS 2 and WS 2 journal, April 2013

Control of valley polarization in monolayer MoS2 by optical helicity journal, June 2012

Quasiparticle band structure calculation of monolayer, bilayer, and bulk MoS 2 journal, May 2012

All Chemical Vapor Deposition Synthesis and Intrinsic Bandgap Observation of MoS 2 /Graphene Heterostructures journal, October 2015

Title: Optically Discriminating Carrier-Induced Quasiparticle Band Gap and Exciton Energy Renormalization in Monolayer ${MoS}_{2}$

Analytical approach to excitonic properties of MoS $_{2}$
journal, March 2014

Linear Scaling of the Exciton Binding Energy versus the Band Gap of Two-Dimensional Materials
journal, August 2015

Photodetectors based on graphene, other two-dimensional materials and hybrid systems
journal, October 2014

Emerging Photoluminescence in Monolayer MoS₂
journal, April 2010

Carrier dynamics in semiconductors studied with time-resolved terahertz spectroscopy
journal, June 2011

Observation of Excitonic Rydberg States in Monolayer MoS ₂ and WS ₂ by Photoluminescence Excitation Spectroscopy
journal, April 2015

Dynamical Excitonic Effects in Doped Two-Dimensional Semiconductors
journal, August 2016

Comment on “Linear Scaling of the Exciton Binding Energy versus the Band Gap of Two-Dimensional Materials”
journal, May 2017

Population inversion and giant bandgap renormalization in atomically thin WS2 layers
journal, June 2015

Influence of Excited Carriers on the Optical and Electronic Properties of MoS ₂
journal, June 2014

Direct Imaging of Band Profile in Single Layer MoS ₂ on Graphite: Quasiparticle Energy Gap, Metallic Edge States, and Edge Band Bending
journal, April 2014

Observation of Rapid Exciton–Exciton Annihilation in Monolayer Molybdenum Disulfide
journal, September 2014

Optical Spectrum of ${MoS}_{2}$ : Many-Body Effects and Diversity of Exciton States
journal, November 2013

Absorption of light by excitons and trions in monolayers of metal dichalcogenide $Mo S_{2}$ : Experiments and theory
journal, May 2014

Many-body correlations and excitonic effects in semiconductor spectroscopy
journal, January 2006

Intervalley biexcitons and many-body effects in monolayer ${MoS}_{2}$
journal, September 2015

Atomically Thin ${MoS}_{2}$ A New Direct-Gap Semiconductor
journal, September 2010

Probing excitonic states in suspended two-dimensional semiconductors by photocurrent spectroscopy
journal, October 2014

Defect-Induced Photoluminescence in Monolayer Semiconducting Transition Metal Dichalcogenides
journal, January 2015

Monolayer excitonic laser
journal, October 2015

Large excitonic effects in monolayers of molybdenum and tungsten dichalcogenides
journal, September 2012

Electrical control of neutral and charged excitons in a monolayer semiconductor
journal, February 2013

Electronic Structure and Luminescence of Quasi-Freestanding MoS ₂ Nanopatches on Au(111)
journal, July 2016

Atomically thin p–n junctions with van der Waals heterointerfaces
journal, August 2014

Giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor
journal, August 2014

Trion-Induced Negative Photoconductivity in Monolayer ${MoS}_{2}$
journal, October 2014

Identifying different stacking sequences in few-layer CVD-grown $Mo S_{2}$ by low-energy atomic-resolution scanning transmission electron microscopy
journal, January 2016

Defects activated photoluminescence in two-dimensional semiconductors: interplay between bound, charged and free excitons
journal, September 2013

Exciton radiative lifetime in transition metal dichalcogenide monolayers
journal, May 2016

Tightly Bound Excitons in Monolayer ${WSe}_{2}$
journal, July 2014

The quasiparticle zoo
journal, December 2016

Extraordinary Sunlight Absorption and One Nanometer Thick Photovoltaics Using Two-Dimensional Monolayer Materials
journal, July 2013

Voltage-controlled quantum light from an atomically thin semiconductor
journal, May 2015

2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications
journal, December 2016

Anomalous Above-Gap Photoexcitations and Optical Signatures of Localized Charge Puddles in Monolayer Molybdenum Disulfide
journal, February 2017

Multi-terminal transport measurements of MoS2 using a van der Waals heterostructure device platform
journal, April 2015

Optical identification of sulfur vacancies: Bound excitons at the edges of monolayer tungsten disulfide
journal, April 2017

Atomic-Scale Spectroscopy of Gated Monolayer MoS ₂
journal, April 2016

Electrical Tuning of Exciton Binding Energies in Monolayer ${WS}_{2}$
journal, September 2015

Carrier Plasmon Induced Nonlinear Band Gap Renormalization in Two-Dimensional Semiconductors
journal, February 2015

Terahertz-induced exciton signatures in semiconductors: Terahertz-induced exciton signatures in semiconductors
journal, June 2013

Tightly bound trions in monolayer MoS2
journal, December 2012

Phase-engineered low-resistance contacts for ultrathin MoS₂ transistors
journal, August 2014

Evolution of Electronic Structure in Atomically Thin Sheets of WS ₂ and WSe ₂
journal, December 2012

Engineering Bandgaps of Monolayer MoS ₂ and WS ₂ on Fluoropolymer Substrates by Electrostatically Tuned Many-Body Effects
journal, May 2016

Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer ${WS}_{2}$
journal, August 2014

Many-body aspects of the optical spectra of bulk and low-dimensional doped semiconductors
journal, May 1987

Monolayer semiconductor nanocavity lasers with ultralow thresholds
journal, March 2015

Single-layer MoS₂ transistors
journal, January 2011

Photocarrier relaxation pathway in two-dimensional semiconducting transition metal dichalcogenides
journal, July 2014

High Performance Multilayer MoS₂Transistors with Scandium Contacts
journal, December 2012

Quasiparticle band structures and optical properties of strained monolayer MoS $_{2}$ and WS $_{2}$
journal, April 2013

Control of valley polarization in monolayer MoS2 by optical helicity
journal, June 2012

Quasiparticle band structure calculation of monolayer, bilayer, and bulk MoS $_{2}$
journal, May 2012

All Chemical Vapor Deposition Synthesis and Intrinsic Bandgap Observation of MoS ₂ /Graphene Heterostructures
journal, October 2015