High- Tc Superconductivity in FeSe at High Pressure: Dominant Hole Carriers and Enhanced Spin Fluctuations

Sun, J. P.; Ye, G. Z.; Shahi, P.; Yan, J. -Q.; Matsuura, K.; Kontani, H.; Zhang, G. M.; Zhou, Q.; Sales, B. C.; Shibauchi, T.; Uwatoko, Y.; Singh, D. J.; Cheng, J. -G.

doi:10.1103/PhysRevLett.118.147004

Title: High- $T_{c}$ Superconductivity in FeSe at High Pressure: Dominant Hole Carriers and Enhanced Spin Fluctuations

Journal Article · 07 April 2017 · Physical Review Letters

DOI: https://doi.org/10.1103/PhysRevLett.118.147004 · OSTI ID:1376522

Sun, J. P. ^[1]; Ye, G. Z. ^[2]; Shahi, P. ^[1]; Yan, J. -Q. ^[3]; Matsuura, K. ^[4]; Kontani, H. ^[5]; Zhang, G. M. ^[6]; Zhou, Q. ^[7]; Sales, B. C. ^[3]; Shibauchi, T. ^[4]; Uwatoko, Y. ^[4]; Singh, D. J. ^[8]; Cheng, J. -G. ^[1]

Chinese Academy of Sciences (CAS), Beijing (China)
Chinese Academy of Sciences (CAS), Beijing (China); Yunnan Univ., Kunming (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tokyo (Japan)
Nagoya Univ. (Japan)
Tsinghua Univ., Beijing (China)
Yunnan Univ., Kunming (China)
Univ. of Missouri, Columbia, MO (United States)

The importance of electron-hole interband interactions is widely acknowledged for iron-pnictide superconductors with high transition temperatures (T_c). However, high-T_c superconductivity without hole carriers has been suggested in FeSe single-layer films and intercalated iron-selenides, raising a fundamental question whether iron pnictides and chalcogenides have different pairing mechanisms. Here, we study the properties of electronic structure in another high-T_c phase induced by pressure in bulk FeSe from magneto-transport measurements and first-principles calculations. With increasing pressure, the low-T_c superconducting phase transforms into high-T_c phase, where we find the normal-state Hall resistivity changes sign from negative to positive, demonstrating dominant hole carriers in striking contrast to other FeSe-derived high-T_c systems. Moreover, the Hall coefficient is remarkably enlarged and the magnetoresistance exhibits anomalous scaling behaviours, evidencing strongly enhanced interband spin fluctuations in the high-T_c phase. These results in FeSe highlight similarities with high-T_c phases of iron pnictides, constituting a step toward a unified understanding of iron-based superconductivity.

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1376522

Alternate ID(s):: OSTI ID: 1350795

Journal Information:: Physical Review Letters, Vol. 118, Issue 14; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (35)

Why Does Undoped FeSe Become a High- T c Superconductor under Pressure? Imai, T.; Ahilan, K.; Ning, F. L. Physical Review Letters, Vol. 102, Issue 17 https://doi.org/10.1103/PhysRevLett.102.177005	journal	April 2009
Superconductivity in the PbO-type structure -FeSe Hsu, F. -C.; Luo, J. -Y.; Yeh, K. -W. Proceedings of the National Academy of Sciences, Vol. 105, Issue 38 https://doi.org/10.1073/pnas.0807325105	journal	September 2008
Evolution of High-Temperature Superconductivity from a Low- T c Phase Tuned by Carrier Concentration in FeSe Thin Flakes Lei, B.; Cui, J. H.; Xiang, Z. J. Physical Review Letters, Vol. 116, Issue 7 https://doi.org/10.1103/PhysRevLett.116.077002	journal	February 2016
Crystal and Electronic Structure of FeSe at High Pressure and Low Temperature Kumar, Ravhi S.; Zhang, Yi; Sinogeikin, Stanislav The Journal of Physical Chemistry B, Vol. 114, Issue 39 https://doi.org/10.1021/jp1060446	journal	October 2010
Problems with reconciling density functional theory calculations with experiment in ferropnictides Mazin, I. I.; Johannes, M. D.; Boeri, L. Physical Review B, Vol. 78, Issue 8 https://doi.org/10.1103/PhysRevB.78.085104	journal	August 2008
Evolution from non-Fermi- to Fermi-liquid transport via isovalent doping in BaFe 2 ( As 1 − x P x ) 2 superconductors Kasahara, S.; Shibauchi, T.; Hashimoto, K. Physical Review B, Vol. 81, Issue 18 https://doi.org/10.1103/PhysRevB.81.184519	journal	May 2010
Unconventional Superconductivity with a Sign Reversal in the Order Parameter of LaFeAsO 1 − x F x Mazin, I. I.; Singh, D. J.; Johannes, M. D. Physical Review Letters, Vol. 101, Issue 5 https://doi.org/10.1103/PhysRevLett.101.057003	journal	July 2008
Unconventional Hall Effect in Pnictides from Interband Interactions Fanfarillo, L.; Cappelluti, E.; Castellani, C. Physical Review Letters, Vol. 109, Issue 9 https://doi.org/10.1103/PhysRevLett.109.096402	journal	August 2012
Pressure-induced high- T c superconducting phase in FeSe: Correlation between anion height and T c Okabe, H.; Takeshita, N.; Horigane, K. Physical Review B, Vol. 81, Issue 20 https://doi.org/10.1103/PhysRevB.81.205119	journal	May 2010
Transport phenomena in a three-dimensional system close to the magnetic quantum critical point: The conserving approximation with current vertex corrections Onari, Seiichiro; Kontani, Hiroshi; Tanaka, Yukio Physical Review B, Vol. 73, Issue 22 https://doi.org/10.1103/PhysRevB.73.224434	journal	June 2006
Orbital-dependent Fermi surface shrinking as a fingerprint of nematicity in FeSe Fanfarillo, Laura; Mansart, Joseph; Toulemonde, Pierre Physical Review B, Vol. 94, Issue 15 https://doi.org/10.1103/PhysRevB.94.155138	journal	October 2016
Dichotomy of the electronic structure and superconductivity between single-layer and double-layer FeSe/SrTiO3 films Liu, Xu; Liu, Defa; Zhang, Wenhao Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms6047	journal	September 2014
Pressure Induced Static Magnetic Order in Superconducting FeSe 1 − x Bendele, M.; Amato, A.; Conder, K. Physical Review Letters, Vol. 104, Issue 8 https://doi.org/10.1103/PhysRevLett.104.087003	journal	February 2010
Electronic and magnetic phase diagram of β-Fe1.01Se with superconductivity at 36.7 K under pressure Medvedev, S.; McQueen, T. M.; Troyan, I. A. Nature Materials, Vol. 8, Issue 8 https://doi.org/10.1038/nmat2491	journal	June 2009
Observation of a Hidden Hole-Like Band Approaching the Fermi Level in K-Doped Iron Selenide Superconductor Sunagawa, Masanori; Terashima, Kensei; Hamada, Takahiro Journal of the Physical Society of Japan, Vol. 85, Issue 7 https://doi.org/10.7566/JPSJ.85.073704	journal	July 2016
Thermopower, Hall tensor, and relaxation time approximation for elemental zinc Chaput, L.; Pécheur, P.; Scherrer, H. Physical Review B, Vol. 75, Issue 4 https://doi.org/10.1103/PhysRevB.75.045116	journal	January 2007
Fermi surface reconstruction in FeSe under high pressure Terashima, Taichi; Kikugawa, Naoki; Kiswandhi, Andhika Physical Review B, Vol. 93, Issue 9 https://doi.org/10.1103/PhysRevB.93.094505	journal	March 2016
Absence of a Holelike Fermi Surface for the Iron-Based K 0.8 Fe 1.7 Se 2 Superconductor Revealed by Angle-Resolved Photoemission Spectroscopy Qian, T.; Wang, X. -P.; Jin, W. -C. Physical Review Letters, Vol. 106, Issue 18 https://doi.org/10.1103/PhysRevLett.106.187001	journal	May 2011
Electronic structure and superconductivity of FeSe-related superconductors Liu, Xu; Zhao, Lin; He, Shaolong Journal of Physics: Condensed Matter, Vol. 27, Issue 18 https://doi.org/10.1088/0953-8984/27/18/183201	journal	April 2015
Lifting of xz / yz orbital degeneracy at the structural transition in detwinned FeSe Shimojima, T.; Suzuki, Y.; Sonobe, T. Physical Review B, Vol. 90, Issue 12 https://doi.org/10.1103/PhysRevB.90.121111	journal	September 2014
Magnetotransport study of the pressure-induced antiferromagnetic phase in FeSe Terashima, Taichi; Kikugawa, Naoki; Kasahara, Shigeru Physical Review B, Vol. 93, Issue 18 https://doi.org/10.1103/PhysRevB.93.180503	journal	May 2016
BoltzTraP. A code for calculating band-structure dependent quantities Madsen, Georg K. H.; Singh, David J. Computer Physics Communications, Vol. 175, Issue 1 https://doi.org/10.1016/j.cpc.2006.03.007	journal	July 2006
Dichotomy between the Hole and Electron Behavior in Multiband Superconductor FeSe Probed by Ultrahigh Magnetic Fields Watson, M. D.; Yamashita, T.; Kasahara, S. Physical Review Letters, Vol. 115, Issue 2 https://doi.org/10.1103/PhysRevLett.115.027006	journal	July 2015
The Electron-Pairing Mechanism of Iron-Based Superconductors Wang, F.; Lee, D. -H. Science, Vol. 332, Issue 6026 https://doi.org/10.1126/science.1200182	journal	April 2011
Integrated-fin gasket for palm cubic-anvil high pressure apparatus Cheng, J. -G.; Matsubayashi, K.; Nagasaki, S. Review of Scientific Instruments, Vol. 85, Issue 9 https://doi.org/10.1063/1.4896473	journal	September 2014
Electric transport of a single-crystal iron chalcogenide FeSe superconductor: Evidence of symmetry-breakdown nematicity and additional ultrafast Dirac cone-like carriers Huynh, K. K.; Tanabe, Y.; Urata, T. Physical Review B, Vol. 90, Issue 14 https://doi.org/10.1103/PhysRevB.90.144516	journal	October 2014
Anomalous Fermi surface in FeSe seen by Shubnikov–de Haas oscillation measurements Terashima, Taichi; Kikugawa, Naoki; Kiswandhi, Andhika Physical Review B, Vol. 90, Issue 14 https://doi.org/10.1103/PhysRevB.90.144517	journal	October 2014
Unusual band renormalization in the simplest iron-based superconductor FeSe 1 − x Maletz, J.; Zabolotnyy, V. B.; Evtushinsky, D. V. Physical Review B, Vol. 89, Issue 22 https://doi.org/10.1103/PhysRevB.89.220506	journal	June 2014
Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe Sun, J. P.; Matsuura, K.; Ye, G. Z. Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms12146	journal	July 2016
Common electronic origin of superconductivity in (Li,Fe)OHFeSe bulk superconductor and single-layer FeSe/SrTiO3 films Zhao, Lin; Liang, Aiji; Yuan, Dongna Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms10608	journal	February 2016
Reconstruction of Band Structure Induced by Electronic Nematicity in an FeSe Superconductor Nakayama, K.; Miyata, Y.; Phan, G. N. Physical Review Letters, Vol. 113, Issue 23 https://doi.org/10.1103/PhysRevLett.113.237001	journal	December 2014
Non-Fermi Liquid Behavior in the Magnetotransport of Ce M In ₅ ( M : Co and Rh): Striking Similarity between Quasi Two-Dimensional Heavy Fermion and High- T _c Cuprates Nakajima, Y.; Shishido, H.; Nakai, H. Journal of the Physical Society of Japan, Vol. 76, Issue 2 https://doi.org/10.1143/JPSJ.76.024703	journal	February 2007
Strong cooperative coupling of pressure-induced magnetic order and nematicity in FeSe Kothapalli, K.; Böhmer, A. E.; Jayasekara, W. T. Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms12728	journal	September 2016
Quantum oscillations in the parent magnetic phase of an iron arsenide high temperature superconductor Sebastian, Suchitra E.; Gillett, J.; Harrison, N. Journal of Physics: Condensed Matter, Vol. 20, Issue 42 https://doi.org/10.1088/0953-8984/20/42/422203	journal	September 2008
Pressure Induced Stripe-Order Antiferromagnetism and First-Order Phase Transition in Fese Wang, P. S.; Sun, S. S.; Cui, Y. Physical Review Letters, Vol. 117, Issue 23 https://doi.org/10.1103/PhysRevLett.117.237001	journal	November 2016

Cited By (15)

Hall coefficient signals orbital differentiation in the Hund’s metal Sr2RuO4 Zingl, Manuel; Mravlje, Jernej; Aichhorn, Markus npj Quantum Materials, Vol. 4, Issue 1 https://doi.org/10.1038/s41535-019-0175-y	journal	July 2019
Separate tuning of nematicity and spin fluctuations to unravel the origin of superconductivity in FeSe Baek, Seung-Ho; Ok, Jong Mok; Kim, Jun Sung npj Quantum Materials, Vol. 5, Issue 1 https://doi.org/10.1038/s41535-020-0211-y	journal	January 2020
Quenched nematic criticality and two superconducting domes in an iron-based superconductor Reiss, Pascal; Graf, David; Haghighirad, Amir A. Nature Physics, Vol. 16, Issue 1 https://doi.org/10.1038/s41567-019-0694-2	journal	October 2019
Photoinduced possible superconducting state with long-lived disproportionate band filling in FeSe Suzuki, Takeshi; Someya, Takashi; Hashimoto, Takahiro Communications Physics, Vol. 2, Issue 1 https://doi.org/10.1038/s42005-019-0219-4	journal	September 2019
Enhancement of superconductivity in FeNb _x Se _0.95 by hole carrier doping Ma, Qingshuang; Lan, Feng; Qiu, Wenbin Journal of Materials Chemistry C, Vol. 7, Issue 32 https://doi.org/10.1039/c9tc02664a	journal	January 2019
Majority carrier type inversion in the FeSe family and a ‘doped semimetal’ scheme in iron-based superconductors Ovchenkov, Y. A.; Chareev, D. A.; Kulbachinskii, V. A. Superconductor Science and Technology, Vol. 32, Issue 6 https://doi.org/10.1088/1361-6668/ab1387	journal	May 2019
The fabrication of high-quality superconducting FeSe _1−x S _x films via pulsed laser deposition Ma, Qingshuang; Lan, Feng; Qiu, Wenbin Superconductor Science and Technology, Vol. 33, Issue 3 https://doi.org/10.1088/1361-6668/ab66e6	journal	January 2020
Theory of two-fluid metallicity in superconducting FeSe at high pressure Craco, L.; Leoni, S. Physical Review B, Vol. 100, Issue 12 https://doi.org/10.1103/physrevb.100.121101	journal	September 2019
Extreme anisotropy and anomalous transport properties of heavily electron doped Li x ( NH 3 ) y Fe 2 Se 2 single crystals Sun, Shanshan; Wang, Shaohua; Yu, Rong Physical Review B, Vol. 96, Issue 6 https://doi.org/10.1103/physrevb.96.064512	journal	August 2017
Realization of continuous electron doping in bulk iron selenides and identification of a new superconducting zone Sun, R. J.; Quan, Y.; Jin, S. F. Physical Review B, Vol. 98, Issue 21 https://doi.org/10.1103/physrevb.98.214508	journal	December 2018
Highly-Tunable Crystal Structure and Physical Properties in FeSe-Based Superconductors Zhou, Kaiyao; Wang, Junjie; Song, Yanpeng Crystals, Vol. 9, Issue 11 https://doi.org/10.3390/cryst9110560	journal	October 2019
Dome of magnetic order inside the nematic phase of sulfur-substituted FeSe under pressure Xiang, Li; Kaluarachchi, Udhara S.; Böhmer, Anna E. arXiv https://doi.org/10.48550/arxiv.1704.04999	text	January 2017
Flux growth in a horizontal configuration: an analogue to vapor transport growth Yan, J. -Q.; Sales, B. C.; Susner, M. A. arXiv https://doi.org/10.48550/arxiv.1706.02339	text	January 2017
Majority carrier type inversion in FeSe family and "doped semimetal" scheme in iron-based superconductors Ovchenkov, Y. A.; Chareev, D. A.; Kulbachinskii, V. A. arXiv https://doi.org/10.48550/arxiv.1808.03551	text	January 2018
Synergy and competition between superconductivity and antiferromagnetism in FeSe under pressure Chen, Guan-Yu; Wang, Enyu; Zhu, Xiyu arXiv https://doi.org/10.48550/arxiv.1811.11599	text	January 2018

Similar Records

Publisher's Note: High-temperature superconductivity stabilized by electron-hole interband coupling in collapsed tetragonal phase of

{KFe}_{2} {As}_{2}

under high pressure [Phys. Rev. B 91 , 060508(R) (2015)]

Journal Article · 2015 · Physical Review. B, Condensed Matter and Materials Physics · OSTI ID:1335147

Nakajima, Yasuyuki; Wang, Renxiong; Metz, Tristin; +6 more

{}^{77}{Se}

NMR investigation of the

K_{x}

_{2 - y}

_{2}

high-

T_{c}

superconductor (

T_{c} = 33

Journal Article · 2011 · Physical Review. B, Condensed Matter and Materials Physics · OSTI ID:1385538

Torchetti, D. A.; Fu, M.; Christensen, D. C.; +4 more

Long-range magnetic order in hydroxide-layer-doped

({Li}_{1 - x - y} {Fe}_{x} {Mn}_{y} OD) FeSe

Journal Article · 2020 · Physical Review Materials · OSTI ID:1606363

Wilfong, Brandon; Zhou, Xiuquan; Zheng, Huafei; +6 more

Related Subjects

75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY

Title: High- T c Superconductivity in FeSe at High Pressure: Dominant Hole Carriers and Enhanced Spin Fluctuations

Citation Formats

References (35)

Cited By (15)

Similar Records

Related Subjects

Title: High- $T_{c}$ Superconductivity in FeSe at High Pressure: Dominant Hole Carriers and Enhanced Spin Fluctuations