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Title: The terahertz dynamics of simplest fluids probed by inelastic X-ray scattering

Abstract

More than two decades of inelastic X-ray scattering (IXS) studies on noble gases and alkali metals are reviewed to illustrate the advances they prompted in our understanding of the terahertz dynamics of simplest systems. The various literature results outline a remarkably coherent picture of common and distinctive behaviours of liquids and their crystalline counterparts. Furthermore, they draw a consistent and comprehensive picture of the evolution of collective modes at the crossover between the hydrodynamic and the single particle regime, their coupling with fast (sub-ps) relaxation processes and their gradual disappearance upon approaching microscopic scales. The gradual transition of the spectrum towards the single particle limit along with its coupling with collisional relaxations will be discussed in some detail. Lastly, less understood emerging topics will be discussed as the occurrence of polyamorphic crossovers, the onset of non-hydrodynamic modes and quantum effects on the spectrum, as well as recent IXS results challenging our vision of the supercritical phase as an intrinsically homogeneous thermodynamic domain.

Authors:
 [1]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1376121
Report Number(s):
BNL-114011-2017-JA
Journal ID: ISSN 0144-235X
Grant/Contract Number:  
SC00112704
Resource Type:
Accepted Manuscript
Journal Name:
International Reviews in Physical Chemistry
Additional Journal Information:
Journal Volume: 36; Journal Issue: 3; Journal ID: ISSN 0144-235X
Publisher:
Taylor & Francis
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Inelastic X-ray Scattering; Inelastic Neutron Scattering; Noble Gases; Relaxation Phenomena; Liquid and Supercritical Systems

Citation Formats

Cunsolo, Alessandro. The terahertz dynamics of simplest fluids probed by inelastic X-ray scattering. United States: N. p., 2017. Web. doi:10.1080/0144235X.2017.1331900.
Cunsolo, Alessandro. The terahertz dynamics of simplest fluids probed by inelastic X-ray scattering. United States. doi:10.1080/0144235X.2017.1331900.
Cunsolo, Alessandro. Mon . "The terahertz dynamics of simplest fluids probed by inelastic X-ray scattering". United States. doi:10.1080/0144235X.2017.1331900. https://www.osti.gov/servlets/purl/1376121.
@article{osti_1376121,
title = {The terahertz dynamics of simplest fluids probed by inelastic X-ray scattering},
author = {Cunsolo, Alessandro},
abstractNote = {More than two decades of inelastic X-ray scattering (IXS) studies on noble gases and alkali metals are reviewed to illustrate the advances they prompted in our understanding of the terahertz dynamics of simplest systems. The various literature results outline a remarkably coherent picture of common and distinctive behaviours of liquids and their crystalline counterparts. Furthermore, they draw a consistent and comprehensive picture of the evolution of collective modes at the crossover between the hydrodynamic and the single particle regime, their coupling with fast (sub-ps) relaxation processes and their gradual disappearance upon approaching microscopic scales. The gradual transition of the spectrum towards the single particle limit along with its coupling with collisional relaxations will be discussed in some detail. Lastly, less understood emerging topics will be discussed as the occurrence of polyamorphic crossovers, the onset of non-hydrodynamic modes and quantum effects on the spectrum, as well as recent IXS results challenging our vision of the supercritical phase as an intrinsically homogeneous thermodynamic domain.},
doi = {10.1080/0144235X.2017.1331900},
journal = {International Reviews in Physical Chemistry},
number = 3,
volume = 36,
place = {United States},
year = {2017},
month = {6}
}

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Works referenced in this record:

Observation of collective excitations in heavy water in the 108 cm−1 momentum range
journal, March 1978

  • Bosi, P.; Dupré, F.; Menzingee, F.
  • Lettere al Nuovo Cimento, Vol. 21, Issue 12
  • DOI: 10.1007/BF02763195

X-Ray Bragg Diffraction in Asymmetric Backscattering Geometry
journal, December 2006


Onset of depature from linearized hydrodynamic behavior in argon gas studied with neutron Brillouin scattering
journal, November 1990


Neutron Scattering from Liquid Helium at High Energies
journal, September 1968


A perfect crystal X-ray analyser with 1.5 meV energy resolution
journal, September 1996

  • Masciovecchio, C.; Bergmann, U.; Krisch, M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 117, Issue 3
  • DOI: 10.1016/0168-583X(96)00334-5

Slow-Neutron Scattering and Collective Motions in Liquid Lead
journal, December 1966


Generic mechanism for generating a liquid–liquid phase transition
journal, February 2001

  • Franzese, Giancarlo; Malescio, Gianpietro; Skibinsky, Anna
  • Nature, Vol. 409, Issue 6821
  • DOI: 10.1038/35055514

Ultrasonic and Light‐Scattering Studies of Carbon Tetrachloride
journal, August 1968

  • Carome, E. F.; Nichols, W. H.; Kunsitis‐Swyt, C. R.
  • The Journal of Chemical Physics, Vol. 49, Issue 3
  • DOI: 10.1063/1.1670185

Ultrasonic Shear and Longitudinal Measurements in Aqueous Glycerol
journal, May 1966

  • Slie, W. M.; Donfor, A. R.; Litovitz, T. A.
  • The Journal of Chemical Physics, Vol. 44, Issue 10
  • DOI: 10.1063/1.1726524

High-frequency dynamics of liquid and supercritical nitrogen
journal, January 2007


Collective modes in molten alkaline earth chlorides: III. Inelastic neutron scattering from molten MgCl 2 and CaCl 2
journal, February 1985


The phonon theory of liquid thermodynamics
journal, May 2012

  • Bolmatov, D.; Brazhkin, V. V.; Trachenko, K.
  • Scientific Reports, Vol. 2, Issue 1
  • DOI: 10.1038/srep00421

Zero Sound Mode in Normal Liquid He 3
journal, November 2007


Frequency-dependent shear modulus of glycerol near the glass transition
journal, July 1987


The single particle dynamics of iodine in the Sachs–Teller regime: An inelastic x-ray scattering study
journal, September 2010

  • Izzo, M. G.; Bencivenga, F.; Cunsolo, A.
  • The Journal of Chemical Physics, Vol. 133, Issue 12
  • DOI: 10.1063/1.3483689

Fingerprints of order and disorder on the high-frequency dynamics of liquids
journal, December 2010

  • Giordano, V. M.; Monaco, G.
  • Proceedings of the National Academy of Sciences, Vol. 107, Issue 51
  • DOI: 10.1073/pnas.1006319107

High frequency dynamics in liquids and supercritical fluids: A comparative inelastic x-ray scattering study
journal, February 2009

  • Bencivenga, F.; Cunsolo, A.; Krisch, M.
  • The Journal of Chemical Physics, Vol. 130, Issue 6
  • DOI: 10.1063/1.3073039

The Scattering of Slow Neutrons by Bound Protons. I. Methods of Calculation
journal, February 1947


High-frequency dynamics of vitreous GeSe 2
journal, September 2010


Brillouin neutron scattering of v-GeO 2
journal, August 2005


Generalized Hydrodynamics and Analysis of Current Correlation Functions
journal, October 1971

  • Ailawadi, Narinder K.; Rahman, Aneesur; Zwanzig, Robert
  • Physical Review A, Vol. 4, Issue 4
  • DOI: 10.1103/PhysRevA.4.1616

Investigation of collective excitations in liquid neon by means of neutron scattering at small scattering vectors
journal, November 1973


Polymorphic Phase Transitions in Liquids and Glasses
journal, January 1997


The bulk viscosity in dense fluids
journal, May 1988

  • Castillo, R.; Casta�eda, S.
  • International Journal of Thermophysics, Vol. 9, Issue 3
  • DOI: 10.1007/BF00513078

de Schepper et al. Respond.
journal, January 1985


Electrons in disordered systems and the theory of localization
journal, October 1974


The neutron scattering function for hard spheres
journal, June 1983


Deep-Inelastic Neutron Scattering Determination of the Single-Particle Kinetic Energy in Solid and Liquid H 3 e
journal, May 2001


Dynamics of supercooled liquids and the glass transition
journal, November 1984

  • Bengtzelius, U.; Gotze, W.; Sjolander, A.
  • Journal of Physics C: Solid State Physics, Vol. 17, Issue 33
  • DOI: 10.1088/0022-3719/17/33/005

Frequency‐Dependent Transport Coefficients in Fluid Mechanics
journal, July 1965

  • Zwanzig, Robert
  • The Journal of Chemical Physics, Vol. 43, Issue 2
  • DOI: 10.1063/1.1696795

Hydrodynamic time correlation functions for a Lennard-Jones fluid
journal, July 1988


Phonon-like excitation in secondary and tertiary structure of hydrated protein powders
journal, January 2011

  • Li, Mingda; Chu, Xiang-qiang; Fratini, Emiliano
  • Soft Matter, Vol. 7, Issue 21
  • DOI: 10.1039/c1sm05954h

Density fluctuations in liquid argon: Coherent dynamic structure factor along the 120-K isotherm obtained by neutron scattering
journal, May 1985


Half Width of Neutron Spectra
journal, December 1987


Electron-ion pseudopotentials in metals
journal, October 1966


Observation of New Short-Wavelength Collective Excitations in Heavy Water by Coherent Inelastic Neutron Scattering
journal, June 1985


Simulational analysis of the local structure in liquid germanium under pressure
journal, August 2002


Principle of Detailed Balance
journal, December 1951


Density fluctuations in classical monatomic liquids
journal, December 1971


The onset of shear modes in the high frequency spectrum of simple disordered systems: current knowledge and perspectives
journal, October 2015


The Ultrahigh Resolution IXS Beamline of NSLS-II: Recent Advances and Scientific Opportunities
journal, March 2013


Pressure-induced coordination changes in crystalline and vitreous GeO 2
journal, July 1989


The structure of amorphous, crystalline and liquid GeO 2
journal, October 2006

  • Micoulaut, M.; Cormier, L.; Henderson, G. S.
  • Journal of Physics: Condensed Matter, Vol. 18, Issue 45
  • DOI: 10.1088/0953-8984/18/45/R01

Evidence of Two Viscous Relaxation Processes in the Collective Dynamics of Liquid Lithium
journal, November 2000


Relaxation process in deeply supercooled water by Mandelstam-Brillouin scattering
journal, January 1989

  • Magazu, S.; Maisano, G.; Majolino, D.
  • The Journal of Physical Chemistry, Vol. 93, Issue 2
  • DOI: 10.1021/j100339a077

Brillouin light scattering from transverse and longitudinal acoustic waves in glycerol
journal, August 2004


The liquid-liquid phase transition in silicon revealed by snapshots of valence electrons
journal, August 2010

  • Beye, M.; Sorgenfrei, F.; Schlotter, W. F.
  • Proceedings of the National Academy of Sciences, Vol. 107, Issue 39
  • DOI: 10.1073/pnas.1006499107

Spectral Distribution of Scattered Light in a Simple Fluid
journal, January 1966


Mode-coupling effects in the density dependence of the shear viscosities of dense argon and methane
journal, November 1989

  • de Schepper, I. M.; van Loef, J. J.; Haffmans, A. F. E. M.
  • Journal of Statistical Physics, Vol. 57, Issue 3-4
  • DOI: 10.1007/BF01022825

Brillouin scattering study of the orientationally disordered phase of cyclohexanol
journal, July 1980


Exploiting the isomorphism between quantum theory and classical statistical mechanics of polyatomic fluids
journal, April 1981

  • Chandler, David; Wolynes, Peter G.
  • The Journal of Chemical Physics, Vol. 74, Issue 7
  • DOI: 10.1063/1.441588

Sound velocity in the inert gas liquids and the law of corresponding states
journal, September 1967

  • Aziz, R. A.; Bowman, D. H.; Lim, C. C.
  • Canadian Journal of Chemistry, Vol. 45, Issue 18
  • DOI: 10.1139/v67-335

Structural relaxation in supercooled water by time-resolved spectroscopy
journal, March 2004

  • Torre, Renato; Bartolini, Paolo; Righini, Roberto
  • Nature, Vol. 428, Issue 6980
  • DOI: 10.1038/nature02409

Viscoelastic behavior of helium at 39 K and 114 bar
journal, November 1991

  • Montfrooij, W.; de Graaf, L. A.; de Schepper, I. M.
  • Physical Review A, Vol. 44, Issue 10
  • DOI: 10.1103/PhysRevA.44.6559

Relaxation Equations for Depolarized Rayleigh and Brillouin Scattering in Liquids
journal, September 1971


Brillouin Scattering: Viscoelastic Measurements in Liquids
journal, January 1968

  • Pinnow, D. A.; Candau, S. J.; LaMacchia, J. T.
  • The Journal of the Acoustical Society of America, Vol. 43, Issue 1
  • DOI: 10.1121/1.1910742

Scattering of Slow Neutrons by a Liquid
journal, June 1958


Collective dynamics in liquid lead: Generalized propagating excitations
journal, April 2001


Is there any evidence of a positive sound dispersion in the high frequency dynamics of noble gases?
journal, March 2000


Atomic Motion in Liquid Argon
journal, September 1967


Comment on "Short-Wavelength Sound Modes in Liquid Argon"
journal, July 1984


Neutron scattering investigation of high-frequency dynamics in glassy glucose
journal, April 2012


The Widom line as the crossover between liquid-like and gas-like behaviour in supercritical fluids
journal, June 2010

  • Simeoni, G. G.; Bryk, T.; Gorelli, F. A.
  • Nature Physics, Vol. 6, Issue 7
  • DOI: 10.1038/nphys1683

Dielectric Relaxation in Glycerol, Propylene Glycol, and n ‐Propanol
journal, December 1951

  • Davidson, D. W.; Cole, R. H.
  • The Journal of Chemical Physics, Vol. 19, Issue 12
  • DOI: 10.1063/1.1748105

Transition from the collective to the single-particle regimes in a quantum fluid
journal, January 2003


Scattering of Neutrons by Phonons in an Aluminum Single Crystal
journal, October 1955


Relaxation processes in supercooled liquids
journal, March 1992


Unified phonon-based approach to the thermodynamics of solid, liquid and gas states
journal, December 2015


Kinetic theory of hard spheres
journal, August 1979

  • van Beijeren, H.; Ernst, M. H.
  • Journal of Statistical Physics, Vol. 21, Issue 2
  • DOI: 10.1007/BF01008695

Signature of a polyamorphic transition in the THz spectrum of vitreous GeO2
journal, October 2015

  • Cunsolo, Alessandro; Li, Yan; Kodituwakku, Chaminda N.
  • Scientific Reports, Vol. 5, Issue 1
  • DOI: 10.1038/srep14996

Macroscopic Separation of Dense Fluid Phase and Liquid Phase of Phosphorus
journal, October 2004


High-frequency transverse dynamics in glasses
journal, March 2003

  • Scopigno, T.; Pontecorvo, E.; Leonardo, R. Di
  • Journal of Physics: Condensed Matter, Vol. 15, Issue 11
  • DOI: 10.1088/0953-8984/15/11/345

Dynamical Crossover at the Liquid-Liquid Transformation of a Compressed Molten Alkali Metal
journal, August 2013


Thermodynamic behaviour of supercritical matter
journal, August 2013

  • Bolmatov, Dima; Brazhkin, V. V.; Trachenko, K.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3331

Overdamped Phonons in Fluid Helium at 4 K
journal, June 1995


Vibrational Collective Dynamics of Dry Proteins in the Terahertz Region
journal, March 2012

  • Paciaroni, Alessandro; Orecchini, Andrea; Haertlein, Michael
  • The Journal of Physical Chemistry B, Vol. 116, Issue 12
  • DOI: 10.1021/jp211190q

Supercooled liquids and the glass transition
journal, March 2001

  • Debenedetti, Pablo G.; Stillinger, Frank H.
  • Nature, Vol. 410, Issue 6825
  • DOI: 10.1038/35065704

Neutron Brillouin scattering in fluid neon
journal, January 1975


Transport, Collective Motion, and Brownian Motion
journal, March 1965


High-pressure phase transformations in liquids and amorphous solids
journal, August 2003


A first-order liquid–liquid phase transition in phosphorus
journal, January 2000

  • Katayama, Yoshinori; Mizutani, Takeshi; Utsumi, Wataru
  • Nature, Vol. 403, Issue 6766
  • DOI: 10.1038/35003143

Equivalence of the sound velocity in water and ice at mesoscopic wavelengths
journal, February 1996

  • Ruocco, G.; Sette, F.; Bergmann, U.
  • Nature, Vol. 379, Issue 6565
  • DOI: 10.1038/379521a0

Structural and Collisional Relaxations in Liquids and Supercritical Fluids
journal, February 2007


Dynamical properties of liquid water
journal, November 1996

  • Balucani, U.; Brodholt, J. P.; Vallauri, R.
  • Journal of Physics: Condensed Matter, Vol. 8, Issue 47
  • DOI: 10.1088/0953-8984/8/47/014

Is There Any Fast Sound in Water?
journal, November 2006


Observation of Umklapp processes in noncrystalline materials
journal, June 2001


Collective Ion Dynamics in Liquid Zinc: Evidence for Complex Dynamics in a Non-Free-Electron Liquid Metal
journal, May 2015


Structural‐Relaxation Dynamics in Liquids
journal, May 1970

  • Montrose, C. J.; Litovitz, T. A.
  • The Journal of the Acoustical Society of America, Vol. 47, Issue 5B
  • DOI: 10.1121/1.1912027

Noncritical behavior of density fluctuations in supercooled water
journal, September 1993


Symmetry breaking gives rise to energy spectra of three states of matter
journal, September 2013

  • Bolmatov, Dima; Musaev, Edvard T.; Trachenko, K.
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep02794

Disappearance of the sound-propagation gap in liquid argon at very high densities
journal, December 1987

  • Verkerk, P.; Well, A. A. van; Schepper, I. M. de
  • Journal of Physics C: Solid State Physics, Vol. 20, Issue 36
  • DOI: 10.1088/0022-3719/20/36/002

Fluctuation Analysis in Simple Fluids
journal, September 1970


Collective dynamics in liquid cesium near the melting point
journal, April 1992


Structural relaxation in the dynamics of glycerol: a joint visible, UV and x-ray inelastic scattering study
journal, January 2006


On the generalized bulk viscosity behavior
journal, October 2001

  • Bertolini, D.; Tani, A.
  • The Journal of Chemical Physics, Vol. 115, Issue 14
  • DOI: 10.1063/1.1409957

High frequency dynamics in liquid nickel: An inelastic x-ray scattering study
journal, June 2008

  • Cazzato, S.; Scopigno, T.; Hosokawa, S.
  • The Journal of Chemical Physics, Vol. 128, Issue 23
  • DOI: 10.1063/1.2925256

Sound propagation in fluids and neutron spectra
journal, June 1984


Rubberlike Dynamics in Sulphur above the λ -Transition Temperature
journal, December 2005


Liquidlike Behavior of Supercritical Fluids
journal, December 2006


The mixed longitudinal–transverse nature of collective modes in water
journal, May 2010


Phonon spectroscopy by inelastic x-ray scattering
journal, January 2000


Quantum effects in the dynamics of He probed by inelastic x-ray scattering
journal, July 2001


The possibility of transverse excitation modes in liquid Ga
journal, February 2008


Wave Number Dependence of the Relaxation Time for the Longitudinal Mode in Simple Liquid
journal, July 1973

  • Machida, Mitsunobu; Murase, Chiaki
  • Progress of Theoretical Physics, Vol. 50, Issue 1
  • DOI: 10.1143/PTP.50.1

Density fluctuations in liquid neon studied by neutron scattering
journal, October 1985


Transverse dynamics of water across the melting point: A parallel neutron and x-ray inelastic scattering study
journal, May 2012


Two liquid states of matter: A dynamic line on a phase diagram
journal, March 2012


Experimental Determination of the Structural Relaxation in Liquid Water
journal, January 1999


The Scattering of Neutrons by Systems of Heavy Nuclei
journal, May 1952


High frequency dynamics and structural relaxation process in liquid ammonia
journal, August 2007

  • Giura, P.; Angelini, R.; Datchi, F.
  • The Journal of Chemical Physics, Vol. 127, Issue 8
  • DOI: 10.1063/1.2753161

Stretched exponential relaxation in molecular and electronic glasses
journal, September 1996


High-frequency dynamics of glass-forming polybutadiene
journal, April 1999


High-pressure x-ray diffraction of SiO 2 glass
journal, August 1992


Microscopic relaxation in supercritical and liquid neon
journal, February 2001

  • Cunsolo, A.; Pratesi, G.; Verbeni, R.
  • The Journal of Chemical Physics, Vol. 114, Issue 5
  • DOI: 10.1063/1.1334613

Collective dynamics in molten potassium: An inelastic x-ray scattering study
journal, May 2004

  • Monaco, A.; Scopigno, T.; Benassi, P.
  • The Journal of Chemical Physics, Vol. 120, Issue 17
  • DOI: 10.1063/1.1689641

Solvent structure and perturbations in solutions of chemical and biological importance
journal, January 1994


The interatomic structure of water at supercritical temperatures
journal, December 1993

  • Postorino, P.; Tromp, R. H.; Ricci, M-A.
  • Nature, Vol. 366, Issue 6456
  • DOI: 10.1038/366668a0

Transverse Acoustic Excitations in Liquid Ga
journal, March 2009


Brillouin scattering in neopentane
journal, December 1977


Classical Electrodynamics
journal, November 1962

  • Jackson, John David; Levitt, L. C.
  • Physics Today, Vol. 15, Issue 11
  • DOI: 10.1063/1.3057859

Coexistence of Monatomic and Diatomic Molecular Fluid Character in Liquid Gallium
journal, February 1993


First observations of phonon dispersion curves with inelastic x‐ray scattering (invited)
journal, July 1989

  • Burkel, E.; Dorner, B.; Illini, Th.
  • Review of Scientific Instruments, Vol. 60, Issue 7
  • DOI: 10.1063/1.1141055

Adiabatic and isothermal sound waves: The case of supercritical nitrogen
journal, July 2006


Shear propagation in the terahertz dynamics of water-glycerol mixtures
journal, November 2013

  • Cunsolo, Alessandro; Kodituwakku, Chaminda N.; Bencivenga, Filippo
  • The Journal of Chemical Physics, Vol. 139, Issue 18
  • DOI: 10.1063/1.4827108

Non-symmetrical dielectric relaxation behaviour arising from a simple empirical decay function
journal, January 1970

  • Williams, Graham; Watts, David C.
  • Transactions of the Faraday Society, Vol. 66
  • DOI: 10.1039/tf9706600080

A self-consistent mode-coupling theory for dynamical correlations in quantum liquids: Rigorous formulation
journal, April 2002

  • Rabani, Eran; Reichman, David R.
  • The Journal of Chemical Physics, Vol. 116, Issue 14
  • DOI: 10.1063/1.1458545

Non-analytic dispersion relations in liquid argon
journal, August 1984


Hydrogen bonding in supercritical water
journal, September 1994

  • Chialvo, Ariel A.; Cummings, Peter T.
  • The Journal of Chemical Physics, Vol. 101, Issue 5
  • DOI: 10.1063/1.467432

Brillouin Scattering and Dispersion and Attenuation of Hypersonic Thermal Waves in Liquid Carbon Tetrachloride
journal, March 1971

  • Stegeman, G. I. A.; Gornall, W. S.; Volterra, V.
  • The Journal of the Acoustical Society of America, Vol. 49, Issue 3C
  • DOI: 10.1121/1.1912459

Brillouin scattering of neutrons from liquids
journal, January 1967

  • Dorner, B.; Plesser, Th.; Stiller, H.
  • Discussions of the Faraday Society, Vol. 43
  • DOI: 10.1039/df9674300160

Structural and Microscopic Relaxation Processes in Liquid Hydrogen Fluoride
journal, June 2002


Liquid dynamics and inelastic scattering of neutrons
journal, January 1959


Phonon-like and single-particle dynamics in liquid lithium
journal, April 2000


The relationship between liquid, supercooled and glassy water
journal, November 1998

  • Mishima, Osamu; Stanley, H. Eugene
  • Nature, Vol. 396, Issue 6709
  • DOI: 10.1038/24540

Inelastic collective dynamics of liquid rubidium with increasing temperature by neutron scattering studies
journal, November 2006


Kinetic theory of the eigenmodes of classical fluids and neutron scattering
journal, December 1984


Short-Wavelength Collective Excitations in Liquid Rubidium Observed by Coherent Neutron Scattering
journal, January 1974


A theoretical study of the static structure and thermodynamics of liquid lithium
journal, June 1993

  • Gonzalez, L. E.; Gonzalez, D. J.; Silbert, M.
  • Journal of Physics: Condensed Matter, Vol. 5, Issue 26
  • DOI: 10.1088/0953-8984/5/26/003

Ultrasonic investigation of the glass transition in glycerol
journal, July 1986

  • Jeong, Yoon H.; Nagel, Sidney R.; Bhattacharya, S.
  • Physical Review A, Vol. 34, Issue 1
  • DOI: 10.1103/PhysRevA.34.602

Liquid alkali metals at the melting point: Structural and dynamical properties
journal, February 1993

  • Balucani, Umberto; Torcini, Alessandro; Vallauri, Renzo
  • Physical Review B, Vol. 47, Issue 6
  • DOI: 10.1103/PhysRevB.47.3011

Dynamics of Dense Supercritical Neon at the Transition from Hydrodynamical to Single-Particle Regimes
journal, April 1998


Thermophysical Properties of Fluid H 2 O
journal, January 1984

  • Kestin, J.; Sengers, J. V.; Kamgar‐Parsi, B.
  • Journal of Physical and Chemical Reference Data, Vol. 13, Issue 1
  • DOI: 10.1063/1.555707

Generalized collective modes for the Lennard-Jones fluid
journal, February 1995


Microscopic dynamics in liquid metals: The experimental point of view
journal, September 2005

  • Scopigno, Tullio; Ruocco, Giancarlo; Sette, Francesco
  • Reviews of Modern Physics, Vol. 77, Issue 3
  • DOI: 10.1103/RevModPhys.77.881

Theory of inelastic x-ray scattering from condensed matter
journal, August 2001


Evidence of Anomalous Acoustic Behavior from Brillouin Scattering in Supercooled Water
journal, March 1984


Propagation of sound in water. A molecular-dynamics study
journal, July 1974


High-contrast sub-millivolt inelastic X-ray scattering for nano- and mesoscale science
journal, June 2014

  • Shvyd’ko, Yuri; Stoupin, Stanislav; Shu, Deming
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5219

High-frequency longitudinal and transverse dynamics in water
journal, January 2005


Transverse excitations in liquid Sn
journal, February 2013


Propagating microscopic temperature fluctuations in a dense helium fluid at 13.3 K
journal, February 1992


Collective acoustic modes as renormalized damped oscillators: Unified description of neutron and x-ray scattering data from classical fluids
journal, June 2006


The Scattering of Slow Neutrons by Molecular Gases
journal, July 1941


Sound and heat revolutions in phononics
journal, November 2013


Brillouin scattering studies of normal and supercooled water
journal, November 1976

  • Rouch, J.; Lai, C. C.; Chen, S. H.
  • The Journal of Chemical Physics, Vol. 65, Issue 10
  • DOI: 10.1063/1.432853

Theory of Transport Coefficients for Moderately Dense Gases
journal, April 1969


Collective excitations in supercritical fluids: Analytical and molecular dynamics study of “positive” and “negative” dispersion
journal, July 2010

  • Bryk, Taras; Mryglod, Ihor; Scopigno, Tullio
  • The Journal of Chemical Physics, Vol. 133, Issue 2
  • DOI: 10.1063/1.3442412

Renormalized Kinetic Theory of Dense Fluids
journal, October 1979


Short-Wavelength Sound Modes in Liquid Argon
journal, March 1983


Ultrasonic Shear and Compressional Relaxation in Liquid Glycerol
journal, September 1957

  • Piccirelli, Robert; Litovitz, T. A.
  • The Journal of the Acoustical Society of America, Vol. 29, Issue 9
  • DOI: 10.1121/1.1909121

A Continued-Fraction Representation of the Time-Correlation Functions
journal, September 1965


High Frequency Sound Waves in Vitreous Silica
journal, February 1998


Viscoelastic behavior of water in the terahertz-frequency range: An inelastic x-ray scattering study
journal, November 1999


The dynamic properties of monatomic liquids
journal, April 1975


Revealing the Mechanism of the Viscous-to-Elastic Crossover in Liquids
journal, July 2015

  • Bolmatov, Dima; Zhernenkov, Mikhail; Zav’yalov, Dmitry
  • The Journal of Physical Chemistry Letters, Vol. 6, Issue 15
  • DOI: 10.1021/acs.jpclett.5b01338

Inelastic X-ray scattering determination of the dynamic structure factor of liquid lithium
journal, November 1999


Dynamical processes in hard-sphere fluids
journal, June 1987

  • Kamgar-Parsi, B.; Cohen, E. G. D.; de Schepper, I. M.
  • Physical Review A, Vol. 35, Issue 11
  • DOI: 10.1103/PhysRevA.35.4781

Mixing of Longitudinal and Transverse Dynamics in Liquid Water
journal, September 1997


Deep Inelastic Atomic Scattering of X Rays in Liquid Neon
journal, May 2002


Comparison of Dielectric and Mechanical Relaxation in Associated Liquids
journal, August 1963

  • Litovitz, T. A.; McDuffie, G. E.
  • The Journal of Chemical Physics, Vol. 39, Issue 3
  • DOI: 10.1063/1.1734316

Некоторые вопросы молекулярного рассеяния света в жидкостях
journal, January 1957


Microscopic collective dynamics in liquid p a r a H 2
journal, December 1999


Biophysical Applications of Quasi-Elastic and Inelastic Neutron Scattering
journal, June 1984


The dispersive behavior of collective excitations in fluids: An experimental test for the generalized collective modes theory
journal, March 2012

  • Bencivenga, F.; Cunsolo, A.
  • The Journal of Chemical Physics, Vol. 136, Issue 11
  • DOI: 10.1063/1.3693624

Evolution of vibrational excitations in glassy systems
journal, January 2000


Neutron scattering study of thermally excited density fluctuations in a dense classical fluid
journal, November 1978


Velocity dispersion and viscous relaxation in supercooled water
journal, September 1996

  • Cunsolo, A.; Nardone, M.
  • The Journal of Chemical Physics, Vol. 105, Issue 10
  • DOI: 10.1063/1.472263

Diamond anvil cell and high-pressure physical investigations
journal, January 1983


Brillouin Scattering in Simple Liquids: Argon and Neon
journal, October 1969


Relaxation Processes in Harmonic Glasses?
journal, June 2000


Transition from Normal to Fast Sound in Liquid Water
journal, July 1996


Collective modes in fluids and neutron scattering
journal, July 1980


Slow-Neutron Scattering by Molecules
journal, April 1957


Momentum distributions and final-state effects in neutron scattering
journal, September 1994


Small Energy Transfer Scattering of Cold Neutrons from Liquid Argon
journal, October 1967


Inelastic x-ray scattering study of liquid Ga: Implications for the short-range order
journal, August 2011


Signatures of quantum behavior in the microscopic dynamics of liquid hydrogen and deuterium
journal, September 2005

  • Cunsolo, A.; Colognesi, D.; Sampoli, M.
  • The Journal of Chemical Physics, Vol. 123, Issue 11
  • DOI: 10.1063/1.2033807

Microscopic structure and collective modes in liquid hydrogen: A preliminary inelastic X-ray scattering study
journal, February 2002


Formation of Glasses from Liquids and Biopolymers
journal, March 1995


Shear Relaxation Times of Simple Fluids
journal, April 1966

  • Mountain, Raymond D.; Zwanzig, Robert
  • The Journal of Chemical Physics, Vol. 44, Issue 7
  • DOI: 10.1063/1.1727124

    Works referencing / citing this record:

    Excitation spectra in fluids: How to analyze them properly
    journal, July 2019

    • Kryuchkov, Nikita P.; Mistryukova, Lukiya A.; Brazhkin, Vadim V.
    • Scientific Reports, Vol. 9, Issue 1
    • DOI: 10.1038/s41598-019-46979-y

    Excitation spectra in fluids: How to analyze them properly
    journal, July 2019

    • Kryuchkov, Nikita P.; Mistryukova, Lukiya A.; Brazhkin, Vadim V.
    • Scientific Reports, Vol. 9, Issue 1
    • DOI: 10.1038/s41598-019-46979-y