Faraday Rotation Due to Surface States in the Topological Insulator (Bi1–xSbx)2Te3
Abstract
For this research, using magneto-infrared spectroscopy, we have explored the charge dynamics of (Bi,Sb)2Te3 thin films on InP substrates. From the magneto-transmission data we extracted three distinct cyclotron resonance (CR) energies that are all apparent in the broad band Faraday rotation (FR) spectra. This comprehensive FR-CR data set has allowed us to isolate the response of the bulk states from the intrinsic surface states associated with both the top and bottom surfaces of the film. Finally, the FR data uncovered that electron- and hole-type Dirac Fermions reside on opposite surfaces of our films, which paves the way for observing many exotic quantum phenomena in topological insulators.
- Authors:
-
- Columbia Univ., New York, NY (United States). Department of Physics
- University of California-San Diego, La Jolla, CA (United States). Physics Department
- Pennsylvania State Univ., University Park, PA (United States). Dept of Physics
- Nordita, KTH Royal Institute of Technology and Stockholm University, Stokholm (Sweden); Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Institute for Materials Science
- Stony Brook Univ., NY (United States). Dept. of Physics and Astronomy; Brookhaven National Lab. (BNL), Upton, NY (United States). Department of Physics and RIKEN-BNL Research Cente
- Columbia Univ., New York, NY (United States). Department of Physics; University of California-San Diego, La Jolla, CA (United States). Physics Department
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Nuclear Physics (NP)
- OSTI Identifier:
- 1376104
- Report Number(s):
- BNL-113961-2017-JA
Journal ID: ISSN 1530-6984; KB0301020
- Grant/Contract Number:
- SC0012704; FG02-00ER45799; FG02-88ER40388
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 17; Journal Issue: 2; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; Bismuth antimony telluride; cyclotron resonance; Faraday rotation; topological insulators; topological surface states
Citation Formats
Shao, Yinming, Post, Kirk W., Wu, Jhih-Sheng, Dai, Siyuan, Frenzel, Alex J., Richardella, Anthony R., Lee, Joon Sue, Samarth, Nitin, Fogler, Michael M., Balatsky, Alexander V., Kharzeev, Dmitri E., and Basov, D. N. Faraday Rotation Due to Surface States in the Topological Insulator (Bi1–xSbx)2Te3. United States: N. p., 2016.
Web. doi:10.1021/acs.nanolett.6b04313.
Shao, Yinming, Post, Kirk W., Wu, Jhih-Sheng, Dai, Siyuan, Frenzel, Alex J., Richardella, Anthony R., Lee, Joon Sue, Samarth, Nitin, Fogler, Michael M., Balatsky, Alexander V., Kharzeev, Dmitri E., & Basov, D. N. Faraday Rotation Due to Surface States in the Topological Insulator (Bi1–xSbx)2Te3. United States. https://doi.org/10.1021/acs.nanolett.6b04313
Shao, Yinming, Post, Kirk W., Wu, Jhih-Sheng, Dai, Siyuan, Frenzel, Alex J., Richardella, Anthony R., Lee, Joon Sue, Samarth, Nitin, Fogler, Michael M., Balatsky, Alexander V., Kharzeev, Dmitri E., and Basov, D. N. Thu .
"Faraday Rotation Due to Surface States in the Topological Insulator (Bi1–xSbx)2Te3". United States. https://doi.org/10.1021/acs.nanolett.6b04313. https://www.osti.gov/servlets/purl/1376104.
@article{osti_1376104,
title = {Faraday Rotation Due to Surface States in the Topological Insulator (Bi1–xSbx)2Te3},
author = {Shao, Yinming and Post, Kirk W. and Wu, Jhih-Sheng and Dai, Siyuan and Frenzel, Alex J. and Richardella, Anthony R. and Lee, Joon Sue and Samarth, Nitin and Fogler, Michael M. and Balatsky, Alexander V. and Kharzeev, Dmitri E. and Basov, D. N.},
abstractNote = {For this research, using magneto-infrared spectroscopy, we have explored the charge dynamics of (Bi,Sb)2Te3 thin films on InP substrates. From the magneto-transmission data we extracted three distinct cyclotron resonance (CR) energies that are all apparent in the broad band Faraday rotation (FR) spectra. This comprehensive FR-CR data set has allowed us to isolate the response of the bulk states from the intrinsic surface states associated with both the top and bottom surfaces of the film. Finally, the FR data uncovered that electron- and hole-type Dirac Fermions reside on opposite surfaces of our films, which paves the way for observing many exotic quantum phenomena in topological insulators.},
doi = {10.1021/acs.nanolett.6b04313},
journal = {Nano Letters},
number = 2,
volume = 17,
place = {United States},
year = {Thu Dec 29 00:00:00 EST 2016},
month = {Thu Dec 29 00:00:00 EST 2016}
}
Web of Science
Works referenced in this record:
Parallel field magnetoresistance in topological insulator thin films
journal, July 2013
- Lin, C. J.; He, X. Y.; Liao, J.
- Physical Review B, Vol. 88, Issue 4
Topological insulators and superconductors
journal, October 2011
- Qi, Xiao-Liang; Zhang, Shou-Cheng
- Reviews of Modern Physics, Vol. 83, Issue 4
Evidence of the two surface states of (Bi0.53Sb0.47)2Te3 films grown by van der Waals epitaxy
journal, December 2013
- He, Liang; Kou, Xufeng; Lang, Murong
- Scientific Reports, Vol. 3, Issue 1
Landau Quantization and the Thickness Limit of Topological Insulator Thin Films of
journal, January 2012
- Jiang, Yeping; Wang, Yilin; Chen, Mu
- Physical Review Letters, Vol. 108, Issue 1
Theory of Kerr and Faraday rotations and linear dichroism in Topological Weyl Semimetals
journal, August 2015
- Kargarian, Mehdi; Randeria, Mohit; Trivedi, Nandini
- Scientific Reports, Vol. 5, Issue 1
Highly tunable electron transport in epitaxial topological insulator (Bi 1- x Sb x ) 2 Te 3 thin films
journal, September 2012
- He, Xiaoyue; Guan, Tong; Wang, Xiuxia
- Applied Physics Letters, Vol. 101, Issue 12
Optical Hall Conductivity in Ordinary and Graphene Quantum Hall Systems
journal, September 2009
- Morimoto, Takahiro; Hatsugai, Yasuhiro; Aoki, Hideo
- Physical Review Letters, Vol. 103, Issue 11
Universal Faraday Rotation in HgTe Wells with Critical Thickness
journal, September 2016
- Shuvaev, A.; Dziom, V.; Kvon, Z. D.
- Physical Review Letters, Vol. 117, Issue 11
Magneto-Optical Signature of Massless Kane Electrons in
journal, September 2016
- Akrap, A.; Hakl, M.; Tchoumakov, S.
- Physical Review Letters, Vol. 117, Issue 13
Quantized Faraday and Kerr rotation and axion electrodynamics of a 3D topological insulator
journal, December 2016
- Wu, L.; Salehi, M.; Koirala, N.
- Science, Vol. 354, Issue 6316
Quantum Faraday and Kerr rotations in graphene
journal, May 2013
- Shimano, R.; Yumoto, G.; Yoo, J. Y.
- Nature Communications, Vol. 4, Issue 1
High-Resolution Faraday Rotation and Electron-Phonon Coupling in Surface States of the Bulk-Insulating Topological Insulator
journal, November 2015
- Wu, Liang; Tse, Wang-Kong; Brahlek, M.
- Physical Review Letters, Vol. 115, Issue 21
Classical to quantum crossover of the cyclotron resonance in graphene: a study of the strength of intraband absorption
journal, September 2012
- Orlita, M.; Crassee, I.; Faugeras, C.
- New Journal of Physics, Vol. 14, Issue 9
Ambipolar field effect in the ternary topological insulator (BixSb1–x)2Te3 by composition tuning
journal, October 2011
- Kong, Desheng; Chen, Yulin; Cha, Judy J.
- Nature Nanotechnology, Vol. 6, Issue 11
Topological field theory of time-reversal invariant insulators
journal, November 2008
- Qi, Xiao-Liang; Hughes, Taylor L.; Zhang, Shou-Cheng
- Physical Review B, Vol. 78, Issue 19, Article No. 195424
Quasiclassical cyclotron resonance of Dirac fermions in highly doped graphene
journal, October 2010
- Witowski, A. M.; Orlita, M.; Stȩpniewski, R.
- Physical Review B, Vol. 82, Issue 16
Magneto-optical conductivity in a topological insulator
journal, July 2013
- Li, Zhou; Carbotte, J. P.
- Physical Review B, Vol. 88, Issue 4
A tunable topological insulator in the spin helical Dirac transport regime
journal, July 2009
- Hsieh, D.; Xia, Y.; Qian, D.
- Nature, Vol. 460, Issue 7259
Multicomponent magneto-optical conductivity of multilayer graphene on SiC
journal, July 2011
- Crassee, I.; Levallois, J.; van der Marel, D.
- Physical Review B, Vol. 84, Issue 3
Landau-level broadening due to electron-impurity interaction in graphene in strong magnetic fields
journal, August 2010
- Yang, C. H.; Peeters, F. M.; Xu, W.
- Physical Review B, Vol. 82, Issue 7
Magneto-optical conductivity in graphene
journal, December 2006
- Gusynin, V. P.; Sharapov, S. G.; Carbotte, J. P.
- Journal of Physics: Condensed Matter, Vol. 19, Issue 2
Landau Quantization of Topological Surface States in
journal, August 2010
- Cheng, Peng; Song, Canli; Zhang, Tong
- Physical Review Letters, Vol. 105, Issue 7
Infrared Spectroscopy of Landau Levels of Graphene
journal, May 2007
- Jiang, Z.; Henriksen, E. A.; Tung, L. C.
- Physical Review Letters, Vol. 98, Issue 19
Colloquium: Topological insulators
journal, November 2010
- Hasan, M. Z.; Kane, C. L.
- Reviews of Modern Physics, Vol. 82, Issue 4, p. 3045-3067
Exciton Condensation and Charge Fractionalization in a Topological Insulator Film
journal, August 2009
- Seradjeh, B.; Moore, J. E.; Franz, M.
- Physical Review Letters, Vol. 103, Issue 6
Optical conductivity of bismuth-based topological insulators
journal, July 2012
- Di Pietro, P.; Vitucci, F. M.; Nicoletti, D.
- Physical Review B, Vol. 86, Issue 4
Topological magnetoelectric effects in thin films of topological insulators
journal, August 2015
- Morimoto, Takahiro; Furusaki, Akira; Nagaosa, Naoto
- Physical Review B, Vol. 92, Issue 8
Electrodynamics of correlated electron materials
journal, June 2011
- Basov, D. N.; Averitt, Richard D.; van der Marel, Dirk
- Reviews of Modern Physics, Vol. 83, Issue 2
Realization of a vertical topological p–n junction in epitaxial Sb2Te3/Bi2Te3 heterostructures
journal, November 2015
- Eschbach, Markus; Młyńczak, Ewa; Kellner, Jens
- Nature Communications, Vol. 6, Issue 1
Giant Faraday rotation in single- and multilayer graphene
journal, November 2010
- Crassee, Iris; Levallois, Julien; Walter, Andrew L.
- Nature Physics, Vol. 7, Issue 1
Band structure engineering in (Bi1−xSbx)2Te3 ternary topological insulators
journal, September 2011
- Zhang, Jinsong; Chang, Cui-Zu; Zhang, Zuocheng
- Nature Communications, Vol. 2, Issue 1
Investigation of the highest valence band in (Bi1-xSbx)2Te3 crystals
journal, November 1977
- Köhler, H.; Freudenberger, A.
- Physica Status Solidi (b), Vol. 84, Issue 1
Electrodynamics of high- superconductors
journal, August 2005
- Basov, D. N.; Timusk, T.
- Reviews of Modern Physics, Vol. 77, Issue 2
Terahertz spectroscopy on Faraday and Kerr rotations in a quantum anomalous Hall state
journal, July 2016
- Okada, Ken N.; Takahashi, Youtarou; Mogi, Masataka
- Nature Communications, Vol. 7, Issue 1
Sum-Rule Constraints on the Surface State Conductance of Topological Insulators
journal, September 2015
- Post, K. W.; Chapler, B. C.; Liu, M. K.
- Physical Review Letters, Vol. 115, Issue 11
Magneto-optical Kramers-Kronig analysis
journal, March 2015
- Levallois, Julien; Nedoliuk, Ievgeniia O.; Crassee, Iris
- Review of Scientific Instruments, Vol. 86, Issue 3
Magneto-optical Faraday and Kerr effects in topological insulator films and in other layered quantized Hall systems
journal, November 2011
- Tse, Wang-Kong; MacDonald, A. H.
- Physical Review B, Vol. 84, Issue 20
Carrier Scattering from Dynamical Magnetoconductivity in Quasineutral Epitaxial Graphene
journal, November 2011
- Orlita, M.; Faugeras, C.; Grill, R.
- Physical Review Letters, Vol. 107, Issue 21
Works referencing / citing this record:
Chiral Spin Mode on the Surface of a Topological Insulator
journal, September 2017
- Kung, H. -H.; Maiti, S.; Wang, X.
- Physical Review Letters, Vol. 119, Issue 13
rf Quantum Capacitance of the Topological Insulator in the Bulk Depleted Regime for Field-Effect Transistors
journal, February 2018
- Inhofer, A.; Duffy, J.; Boukhicha, M.
- Physical Review Applied, Vol. 9, Issue 2
Terahertz Faraday and Kerr rotation spectroscopy of films in high magnetic fields up to 30 tesla
journal, September 2019
- Li, Xinwei; Yoshioka, Katsumasa; Xie, Ming
- Physical Review B, Vol. 100, Issue 11
Interband absorption edge in the topological insulators
journal, December 2017
- Dubroka, A.; Caha, O.; Hronček, M.
- Physical Review B, Vol. 96, Issue 23
Optical signatures of Dirac nodal lines in NbAs 2
journal, December 2018
- Shao, Yinming; Sun, Zhiyuan; Wang, Ying
- Proceedings of the National Academy of Sciences, Vol. 116, Issue 4
Observation of Extrinsic Photo-Induced Inverse Spin Hall Effect in a GaAs/AlGaAs Two-Dimensional Electron Gas
journal, October 2018
- Yu, Jinling; Zeng, Xiaolin; Wang, Yumeng
- Nanoscale Research Letters, Vol. 13, Issue 1
Chiral Spin Mode on the Surface of a Topological Insulator
text, January 2017
- Kung, H. -H.; Maiti, S.; Wang, X.
- arXiv
Helicity-dependent photocurrent of the top and bottom Dirac surface states of epitaxial thin films of three-dimensional topological insulators
journal, December 2019
- Yu, Jinling; Zhu, Kejing; Zeng, Xiaolin
- Physical Review B, Vol. 100, Issue 23
Observation of chiral surface excitons in a topological insulator Bi 2 Se 3
journal, February 2019
- Kung, H. -H.; Goyal, A. P.; Maslov, D. L.
- Proceedings of the National Academy of Sciences, Vol. 116, Issue 10
Optical Signatures of Dirac Nodal-lines in NbAs$_2$
text, January 2018
- Shao, Yinming; Sun, Zhiyuan; Wang, Ying
- arXiv