Metal Thio- and Selenophosphates as Multifunctional van der Waals Layered Materials
Abstract
Since the discovery of Dirac physics in graphene, research in 2D materials has exploded with the aim of finding new materials and harnessing their unique and tunable electronic and optical properties. The follow-on work on 2D dielectrics and semiconductors has led to the emergence and development of hexagonal boron nitride, black phosphorus, and transition metal disulfides. However, the spectrum of good insulating materials is still very narrow. Likewise, 2D materials exhibiting correlated phenomena such as superconductivity, magnetism, and ferroelectricity have yet to be developed or discovered. These properties will significantly enrich the spectrum of functional 2D materials, particularly in the case of high phase-transition temperatures. They will also advance a fascinating fundamental frontier of size and proximity effects on correlated ground states. In this work, a broad family of layered metal thio(seleno)phosphate materials that are moderate- to wide-bandgap semiconductors with incipient ionic conductivity and a host of ferroic properties are reviewed. It is argued that this material class has the potential to merge the sought-after properties of complex oxides with electronic functions of 2D and quasi-2D electronic materials, as well as to create new avenues for both applied and fundamental materials research in structural and magnetic correlations.
- Authors:
-
- Air Force Research Lab. (AFRL), Wright-Patterson AFB, OH (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); UES Inc., Beavercreek, OH (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1842642
- Alternate Identifier(s):
- OSTI ID: 1375659
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 29; Journal Issue: 38; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 2D materials; ferroelectrics; ferroic materials; magnetic materials; metal thiophosphates
Citation Formats
Susner, Michael A., Chyasnavichyus, Marius, McGuire, Michael A., Ganesh, Panchapakesan, and Maksymovych, Petro. Metal Thio- and Selenophosphates as Multifunctional van der Waals Layered Materials. United States: N. p., 2017.
Web. doi:10.1002/adma.201602852.
Susner, Michael A., Chyasnavichyus, Marius, McGuire, Michael A., Ganesh, Panchapakesan, & Maksymovych, Petro. Metal Thio- and Selenophosphates as Multifunctional van der Waals Layered Materials. United States. https://doi.org/10.1002/adma.201602852
Susner, Michael A., Chyasnavichyus, Marius, McGuire, Michael A., Ganesh, Panchapakesan, and Maksymovych, Petro. Mon .
"Metal Thio- and Selenophosphates as Multifunctional van der Waals Layered Materials". United States. https://doi.org/10.1002/adma.201602852. https://www.osti.gov/servlets/purl/1842642.
@article{osti_1842642,
title = {Metal Thio- and Selenophosphates as Multifunctional van der Waals Layered Materials},
author = {Susner, Michael A. and Chyasnavichyus, Marius and McGuire, Michael A. and Ganesh, Panchapakesan and Maksymovych, Petro},
abstractNote = {Since the discovery of Dirac physics in graphene, research in 2D materials has exploded with the aim of finding new materials and harnessing their unique and tunable electronic and optical properties. The follow-on work on 2D dielectrics and semiconductors has led to the emergence and development of hexagonal boron nitride, black phosphorus, and transition metal disulfides. However, the spectrum of good insulating materials is still very narrow. Likewise, 2D materials exhibiting correlated phenomena such as superconductivity, magnetism, and ferroelectricity have yet to be developed or discovered. These properties will significantly enrich the spectrum of functional 2D materials, particularly in the case of high phase-transition temperatures. They will also advance a fascinating fundamental frontier of size and proximity effects on correlated ground states. In this work, a broad family of layered metal thio(seleno)phosphate materials that are moderate- to wide-bandgap semiconductors with incipient ionic conductivity and a host of ferroic properties are reviewed. It is argued that this material class has the potential to merge the sought-after properties of complex oxides with electronic functions of 2D and quasi-2D electronic materials, as well as to create new avenues for both applied and fundamental materials research in structural and magnetic correlations.},
doi = {10.1002/adma.201602852},
journal = {Advanced Materials},
number = 38,
volume = 29,
place = {United States},
year = {Mon Aug 21 00:00:00 EDT 2017},
month = {Mon Aug 21 00:00:00 EDT 2017}
}
Web of Science
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