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Title: Operation of the Airmodus A11 nano Condensation Nucleus Counter at various inlet pressures and various operation temperatures, and design of a new inlet system

Abstract

Measuring sub-3 nm particles outside of controlled laboratory conditions is a challenging task, as many of the instruments are operated at their limits and are subject to changing ambient conditions. In this study, we advance the current understanding of the operation of the Airmodus A11 nano Condensation Nucleus Counter (nCNC), which consists of an A10 Particle Size Magnifier (PSM) and an A20 Condensation Particle Counter (CPC). The effect of the inlet line pressure on the measured particle concentration was measured, and two separate regions inside the A10, where supersaturation of working fluid can take place, were identified. The possibility of varying the lower cut-off diameter of the nCNC was investigated; by scanning the growth tube temperature, the range of the lower cut-off was extended from 1–2.5 to 1–6 nm. Here we present a new inlet system, which allows automated measurement of the background concentration of homogeneously nucleated droplets, minimizes the diffusion losses in the sampling line and is equipped with an electrostatic filter to remove ions smaller than approximately 4.5 nm. Lastly, our view of the guidelines for the optimal use of the Airmodus nCNC is provided.

Authors:
 [1];  [1];  [1];  [1];  [1];  [2];  [1];  [3];  [4];  [1];  [1]
  1. Univ. of Helsinki, Helsinki (Finland)
  2. Univ. of Helsinki, Helsinki (Finland); Univ. Paris-Diderot, Paris (France)
  3. Univ. of Helsinki, Helsinki (Finland); Paul Scherrer Inst. (PSI), Villigen (Switzerland)
  4. Airmodus Ltd., Helsinki (Finland)
Publication Date:
Research Org.:
Univ. of Helsinki, Helsinki (Finland). Dept. of Physics
Sponsoring Org.:
USDOE
OSTI Identifier:
1375412
Resource Type:
Accepted Manuscript
Journal Name:
Atmospheric Measurement Techniques (Online)
Additional Journal Information:
Journal Name: Atmospheric Measurement Techniques (Online); Journal Volume: 9; Journal Issue: 7; Journal ID: ISSN 1867-8548
Publisher:
European Geosciences Union
Country of Publication:
United States
Language:
English
Subject:
54 ENVIRONMENTAL SCIENCES

Citation Formats

Kangasluoma, Juha, Franchin, Alessandro, Duplissy, Jonahtan, Ahonen, Lauri, Korhonen, Frans, Attoui, Michel, Mikkila, Jyri, Lehtipalo, Katrianne, Vanhanen, Joonas, Kulmala, Markku, and Petaja, Tuukka. Operation of the Airmodus A11 nano Condensation Nucleus Counter at various inlet pressures and various operation temperatures, and design of a new inlet system. United States: N. p., 2016. Web. doi:10.5194/amt-9-2977-2016.
Kangasluoma, Juha, Franchin, Alessandro, Duplissy, Jonahtan, Ahonen, Lauri, Korhonen, Frans, Attoui, Michel, Mikkila, Jyri, Lehtipalo, Katrianne, Vanhanen, Joonas, Kulmala, Markku, & Petaja, Tuukka. Operation of the Airmodus A11 nano Condensation Nucleus Counter at various inlet pressures and various operation temperatures, and design of a new inlet system. United States. https://doi.org/10.5194/amt-9-2977-2016
Kangasluoma, Juha, Franchin, Alessandro, Duplissy, Jonahtan, Ahonen, Lauri, Korhonen, Frans, Attoui, Michel, Mikkila, Jyri, Lehtipalo, Katrianne, Vanhanen, Joonas, Kulmala, Markku, and Petaja, Tuukka. Thu . "Operation of the Airmodus A11 nano Condensation Nucleus Counter at various inlet pressures and various operation temperatures, and design of a new inlet system". United States. https://doi.org/10.5194/amt-9-2977-2016. https://www.osti.gov/servlets/purl/1375412.
@article{osti_1375412,
title = {Operation of the Airmodus A11 nano Condensation Nucleus Counter at various inlet pressures and various operation temperatures, and design of a new inlet system},
author = {Kangasluoma, Juha and Franchin, Alessandro and Duplissy, Jonahtan and Ahonen, Lauri and Korhonen, Frans and Attoui, Michel and Mikkila, Jyri and Lehtipalo, Katrianne and Vanhanen, Joonas and Kulmala, Markku and Petaja, Tuukka},
abstractNote = {Measuring sub-3 nm particles outside of controlled laboratory conditions is a challenging task, as many of the instruments are operated at their limits and are subject to changing ambient conditions. In this study, we advance the current understanding of the operation of the Airmodus A11 nano Condensation Nucleus Counter (nCNC), which consists of an A10 Particle Size Magnifier (PSM) and an A20 Condensation Particle Counter (CPC). The effect of the inlet line pressure on the measured particle concentration was measured, and two separate regions inside the A10, where supersaturation of working fluid can take place, were identified. The possibility of varying the lower cut-off diameter of the nCNC was investigated; by scanning the growth tube temperature, the range of the lower cut-off was extended from 1–2.5 to 1–6 nm. Here we present a new inlet system, which allows automated measurement of the background concentration of homogeneously nucleated droplets, minimizes the diffusion losses in the sampling line and is equipped with an electrostatic filter to remove ions smaller than approximately 4.5 nm. Lastly, our view of the guidelines for the optimal use of the Airmodus nCNC is provided.},
doi = {10.5194/amt-9-2977-2016},
journal = {Atmospheric Measurement Techniques (Online)},
number = 7,
volume = 9,
place = {United States},
year = {Thu Jul 14 00:00:00 EDT 2016},
month = {Thu Jul 14 00:00:00 EDT 2016}
}

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Molecular monodisperse mobility and mass standards from electrosprays of tetra-alkyl ammonium halides
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Sizing of neutral sub 3nm tungsten oxide clusters using Airmodus Particle Size Magnifier
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Role of sulphuric acid, ammonia and galactic cosmic rays in atmospheric aerosol nucleation
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  • Nature, Vol. 476, Issue 7361
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A large source of low-volatility secondary organic aerosol
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  • DOI: 10.1038/nature13032

Laboratory Verification of PH-CPC's Ability to Monitor Atmospheric Sub-3 nm Clusters
journal, January 2009


Laboratory Evaluation of a TSI Condensation Particle Counter (Model 3771) Under Airborne Measurement Conditions
journal, February 2011


Particle Size Magnifier for Nano-CN Detection
journal, March 2011


Condensational Growth of Ultrafine Aerosol Particles in a New Particle Size Magnifier
journal, January 1984


Ultrafine Aerosol Measurement Using a Condensation Nucleus Counter with Pulse Height Analysis
journal, January 1996


Major contribution of neutral clusters to new particle formation at the interface between the boundary layer and the free troposphere
journal, January 2015


High concentrations of sub-3 nm clusters and frequent new particle formation observed in the Po Valley, Italy, during the PEGASOS 2012 campaign
journal, November 2015


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journal, January 2013

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Estimating the influence of transport on aerosol size distributions during new particle formation events
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