Doubly magic Pb208 : High-spin states, isomers, and E3 collectivity in the yrast decay

Broda, R.; Janssens, R. V.  F.; Iskra, Ł. W.; Wrzesinski, J.; Fornal, B.; Carpenter, M. P.; Chiara, C. J.; Cieplicka-Oryńczak, N.; Hoffman, C. R.; Kondev, F. G.; Królas, W.; Lauritsen, T.; Podolyak, Zs.; Seweryniak, D.; Shand, C. M.; Szpak, B.; Walters, W. B.; Zhu, S.; Brown, B. A.

doi:10.1103/PhysRevC.95.064308

Title: Doubly magic ${}^{208}{Pb}$ : High-spin states, isomers, and $E 3$ collectivity in the yrast decay

Abstract

Yrast and near-yrast levels up to spin values in excess of I = 30h have been delineated in the doubly-magic ²⁰⁸Pb nucleus following deep-inelastic reactions involving ²⁰⁸Pb targets and, mostly, 430-MeV ⁴⁸Ca and 1440-MeV ²⁰⁸Pb beams. The level scheme was established up to an excitation energy of 16.4 MeV, based on multi-fold γ-ray coincidence relationships measured with the Gammasphere array. Below the well-known, 0.5-μs 10⁺ isomer, ten new transitions were added to earlier work. The delineation of the higher parts of the level sequence benefited from analyses involving a number of prompt- and delayed-coincidence conditions. Three new isomeric states were established along the yrast line with I ^π = 20^- (10342 keV), 23⁺ (11361 keV), and 28^- (13675 keV), and respective half-lives of 22(3), 12.7(2), and 60(6) ns. Gamma transitions were also identified preceding in time the 28^- isomer, however, only a few could be placed in the level scheme and no firm spin-parity quantum numbers could be proposed. In contrast, for most states below this 28^- isomer, firm spin-parity values were assigned, based on total electron-conversion coefficients, deduced for low-energy (<500 keV) transitions from γ-intensity balances, and on measured γ-ray angular distributions. The latter also enabled the quantitative determinationmore »« less

Authors:

Broda, R. ^[1]; Janssens, R. V. F. ^[2]; Iskra, Ł. W. ^[1]; Wrzesinski, J. ^[1]; Fornal, B. ^[1]; Carpenter, M. P. ^[2]; Chiara, C. J. ^[3]; Cieplicka-Oryńczak, N. ^[1]; Hoffman, C. R. ^[2]; Kondev, F. G. ^[4]; Królas, W. ^[1]; Lauritsen, T. ^[2]; Podolyak, Zs. ^[5]; Seweryniak, D. ^[2]; Shand, C. M. ^[5]; Szpak, B. ^[1]; Walters, W. B. ^[6]; Zhu, S. ^[2]; Brown, B. A. ^[7]

Polish Academy of Sciences (PAS), Krakow (Poland). Inst. of Nuclear Physics
Argonne National Lab. (ANL), Argonne, IL (United States). Physics Division
Argonne National Lab. (ANL), Argonne, IL (United States). Physics Division; Univ. of Maryland, College Park, MD (United States). Dept. of Chemistry and Biochemistry
Argonne National Lab. (ANL), Argonne, IL (United States). Nuclear Engineering Division
Univ. of Surrey, Guildford (United Kingdom). Dept. of Physics
Univ. of Maryland, College Park, MD (United States). Dept. of Chemistry and Biochemistry
Michigan State Univ., East Lansing, MI (United States). Dept. of Physics and Astronomy and National Superconducting Cyclotron Lab.

Publication Date:: 2017-06-12

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Nuclear Physics (NP); Polish National Science Centre (NCN); National Science Foundation (NSF)

OSTI Identifier:: 1374540

Alternate Identifier(s):: OSTI ID: 1363716

Grant/Contract Number:: AC02-06CH11357; FG02-94ER40834; PHY-1404442

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review C

Additional Journal Information:: Journal Volume: 95; Journal Issue: 6; Journal ID: ISSN 2469-9985

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 73 NUCLEAR PHYSICS AND RADIATION PHYSICS

Citation Formats


                    Broda, R., Janssens, R. V.  F., Iskra, Ł. W., Wrzesinski, J., Fornal, B., Carpenter, M. P., Chiara, C. J., Cieplicka-Oryńczak, N., Hoffman, C. R., Kondev, F. G., Królas, W., Lauritsen, T., Podolyak, Zs., Seweryniak, D., Shand, C. M., Szpak, B., Walters, W. B., Zhu, S., and Brown, B. A. Doubly magic Pb208 : High-spin states, isomers, and E3 collectivity in the yrast decay.  United States: N. p., 2017. 
Web.  doi:10.1103/PhysRevC.95.064308.

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                    Broda, R., Janssens, R. V.  F., Iskra, Ł. W., Wrzesinski, J., Fornal, B., Carpenter, M. P., Chiara, C. J., Cieplicka-Oryńczak, N., Hoffman, C. R., Kondev, F. G., Królas, W., Lauritsen, T., Podolyak, Zs., Seweryniak, D., Shand, C. M., Szpak, B., Walters, W. B., Zhu, S., & Brown, B. A. Doubly magic Pb208 : High-spin states, isomers, and E3 collectivity in the yrast decay.  United States.  https://doi.org/10.1103/PhysRevC.95.064308

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                    Broda, R., Janssens, R. V.  F., Iskra, Ł. W., Wrzesinski, J., Fornal, B., Carpenter, M. P., Chiara, C. J., Cieplicka-Oryńczak, N., Hoffman, C. R., Kondev, F. G., Królas, W., Lauritsen, T., Podolyak, Zs., Seweryniak, D., Shand, C. M., Szpak, B., Walters, W. B., Zhu, S., and Brown, B. A. Mon .  
"Doubly magic Pb208 : High-spin states, isomers, and E3 collectivity in the yrast decay".  United States.  https://doi.org/10.1103/PhysRevC.95.064308.  https://www.osti.gov/servlets/purl/1374540.

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@article{osti_1374540,

  title        = {Doubly magic Pb208 : High-spin states, isomers, and E3 collectivity in the yrast decay},

  author       = {Broda, R. and Janssens, R. V.  F. and Iskra, Ł. W. and Wrzesinski, J. and Fornal, B. and Carpenter, M. P. and Chiara, C. J. and Cieplicka-Oryńczak, N. and Hoffman, C. R. and Kondev, F. G. and Królas, W. and Lauritsen, T. and Podolyak, Zs. and Seweryniak, D. and Shand, C. M. and Szpak, B. and Walters, W. B. and Zhu, S. and Brown, B. A.},

  abstractNote = {Yrast and near-yrast levels up to spin values in excess of I = 30h have been delineated in the doubly-magic 208Pb nucleus following deep-inelastic reactions involving 208Pb targets and, mostly, 430-MeV 48Ca and 1440-MeV 208Pb beams. The level scheme was established up to an excitation energy of 16.4 MeV, based on multi-fold γ-ray coincidence relationships measured with the Gammasphere array. Below the well-known, 0.5-μs 10+ isomer, ten new transitions were added to earlier work. The delineation of the higher parts of the level sequence benefited from analyses involving a number of prompt- and delayed-coincidence conditions. Three new isomeric states were established along the yrast line with I π = 20- (10342 keV), 23+ (11361 keV), and 28- (13675 keV), and respective half-lives of 22(3), 12.7(2), and 60(6) ns. Gamma transitions were also identified preceding in time the 28- isomer, however, only a few could be placed in the level scheme and no firm spin-parity quantum numbers could be proposed. In contrast, for most states below this 28- isomer, firm spin-parity values were assigned, based on total electron-conversion coefficients, deduced for low-energy (<500 keV) transitions from γ-intensity balances, and on measured γ-ray angular distributions. The latter also enabled the quantitative determination of mixing ratios. The transition probabilities extracted for all isomeric transitions in 208Pb have been reviewed and discussed in terms of the intrinsic structure of the initial and final levels involved. Particular emphasis was placed on the many observed E3 transitions as they often exhibit significant enhancements in strength (of the order of tens of W.u.) comparable to the one seen for the neutron j15/2→g9/2 E3 transition in 209Pb. In this context, the enhancement of the 725-keV E3 transition (56 W.u.) associated with the decay of the highest-lying 28- isomer observed in this work remains particularly challenging to explain. Large-scale shell-model calculations were performed with two approaches, a first one where the 1, 2, and 3 particle-hole excitations do not mix with one another, and another more complex one, in which such mixing takes place. We compared the calculated levels with the data and a general agreement is observed for most of the 208Pb level scheme. At the highest spins and energies, however, the 2 correspondence between theory and experiment is less satisfactory and the experimental yrast line appears to be more regular than the calculated one. This regularity is notable when the level energies are plotted versus the I(I+1) product and the observed, nearly linear, behavior was considered within a simple “rotational” interpretation. Furthermore, within this approximate picture, the extracted moment of inertia suggests that only the 76 valence nucleons participate in the “rotation” and that the 132Sn spherical core remains inert.},

  doi          = {10.1103/PhysRevC.95.064308},

  journal      = {Physical Review C},

  number       = 6,

  volume       = 95,

  place        = {United States},

  year         = {2017},

  month        = {6}

}

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Works referencing / citing this record:

Two-neutron and core-excited states in ${}^{210}{Pb}$ : Tracing $E 3$ collectivity and evidence for a new $β$ -decaying isomer in ${}^{210}{Tl}$
journal, August 2018

Broda, R.; Iskra, Ł. W.; Janssens, R. V. F.
Physical Review C, Vol. 98, Issue 2
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Description of one-particle one-hole configurations coupled to the $3^{-}$ yrast state in the doubly magic nucleus ${}^{208}{Pb}$
journal, March 2019

Heusler, A.; Jolos, R. V.; von Brentano, P.
Physical Review C, Vol. 99, Issue 3
DOI: 10.1103/physrevc.99.034323

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Title: Doubly magic Pb 208 : High-spin states, isomers, and E 3 collectivity in the yrast decay

Abstract

Citation Formats

Electromagnetic decay of 10+ states and yrast isomers in 208Pb journal, April 1989

High-spin yrast structure of Hg 204 from the decay of a four-hole, 22 + isomer journal, October 2015

Double-Octupole States in P 208 b journal, December 2000

Effective Charge of the π h 11 / 2 Orbital and the Electric Field Gradient of Hg from the Yrast Structure of H 206 g journal, November 2001

Study of excited states in 208 Pb by particle- γ coincidences with the 207 Pb ( d , p ) 208 Pb and 209 Bi ( t , α ) 208 Pb reactions journal, September 1997

High-spin states and isomers in the one-proton-hole and three-neutron-hole 204 Tl isotope journal, July 2011

Nuclear Data Sheets for A = 208 journal, August 2007

The $\pi h_{11/2}^{-1}\nu i_{13/2}^{-2}$ three-hole isomeric state and octupole core excitation in the 205 Tl nucleus journal, April 2003

Bonn potential and shell-model calculations for N = 126 isotones journal, November 1999

High resolution electron scattering from high spin states in Pb 208 journal, June 1992

High-spin states in 208Pb journal, May 2001

Particle octupole-vibration coupling near 208Pb journal, July 2000

Yrast structure of the two-proton- and three-neutron-hole nucleus Hg 203 from the decay of a 53 / 2 + isomer journal, June 2011

?-decay of the particle-hole states with the highest spins in208Pb journal, December 1993

Derivation of wave functions and matrix elements of the residual interaction in 208 Pb from experimental data journal, May 1999

On the origin of the 2485 keV?-ray observed in near-barrier collisions of various heavy ions with208Pb journal, March 1992

Yrast structure of 206 Bi: Isomeric states and one-proton-particle, three-neutron-hole excitations journal, November 2012

Complete identification of states in Pb 208 below E x = 6.2 MeV journal, May 2016

Appraisal of the Kuo-Herling shell-model interaction and application to A =210–212 nuclei journal, February 1991

Nuclear Data Sheets for A = 209 journal, May 2015

Two-particle states in 210Pb, 210Bi and 210Po with realistic forces journal, February 1972

Hard-to-reach nuclei studied with deep-inelastic heavy-ion reactions journal, April 2003

Spectroscopic studies with the use of deep-inelastic heavy-ion reactions journal, May 2006

The GAMMASPHERE journal, December 1990

Review of metastable states in heavy nuclei journal, May 2016

γ Spectroscopy of 209Pb with deep inelastic reactions journal, March 1998

Bonn Potential and Shell-Model Calculations for N=126 Isotones text, January 1999

Two-neutron and core-excited states in Pb 210 : Tracing E 3 collectivity and evidence for a new β -decaying isomer in Tl 210 journal, August 2018

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Title: Doubly magic ${}^{208}{Pb}$ : High-spin states, isomers, and $E 3$ collectivity in the yrast decay

Electromagnetic decay of 10+ states and yrast isomers in 208Pb
journal, April 1989

High-spin yrast structure of ${}^{204}{Hg}$ from the decay of a four-hole, $22^{+}$ isomer
journal, October 2015

Double-Octupole States in ${}^{208}P b$
journal, December 2000

Effective Charge of the $π h_{11 / 2}$ Orbital and the Electric Field Gradient of Hg from the Yrast Structure of ${}^{206}H g$
journal, November 2001

Study of excited states in $^{208}$ Pb by particle- $γ$ coincidences with the $^{207} Pb {(d, p)}^{208} Pb$ and $^{209} Bi (t, α)^{208} Pb$ reactions
journal, September 1997

High-spin states and isomers in the one-proton-hole and three-neutron-hole $^{204}$ Tl isotope
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Nuclear Data Sheets for A = 208
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The $\pi h_{11/2}^{-1}\nu i_{13/2}^{-2}$ three-hole isomeric state and octupole core excitation in the 205 Tl nucleus
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Bonn potential and shell-model calculations for $N = 126$ isotones
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High resolution electron scattering from high spin states in ${}^{208}{Pb}$
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High-spin states in 208Pb
journal, May 2001

Particle octupole-vibration coupling near 208Pb
journal, July 2000

Yrast structure of the two-proton- and three-neutron-hole nucleus ${}^{203}{Hg}$ from the decay of a $53 / 2^{+}$ isomer
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?-decay of the particle-hole states with the highest spins in208Pb
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Derivation of wave functions and matrix elements of the residual interaction in $^{208} Pb$ from experimental data
journal, May 1999

On the origin of the 2485 keV?-ray observed in near-barrier collisions of various heavy ions with208Pb
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Yrast structure of $^{206}$ Bi: Isomeric states and one-proton-particle, three-neutron-hole excitations
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Appraisal of the Kuo-Herling shell-model interaction and application to A =210–212 nuclei
journal, February 1991

Nuclear Data Sheets for A = 209
journal, May 2015

Two-particle states in 210Pb, 210Bi and 210Po with realistic forces
journal, February 1972

Hard-to-reach nuclei studied with deep-inelastic heavy-ion reactions
journal, April 2003

Spectroscopic studies with the use of deep-inelastic heavy-ion reactions
journal, May 2006

The GAMMASPHERE
journal, December 1990

Review of metastable states in heavy nuclei
journal, May 2016

γ Spectroscopy of 209Pb with deep inelastic reactions
journal, March 1998

Bonn Potential and Shell-Model Calculations for N=126 Isotones
text, January 1999

Two-neutron and core-excited states in ${}^{210}{Pb}$ : Tracing $E 3$ collectivity and evidence for a new $β$ -decaying isomer in ${}^{210}{Tl}$
journal, August 2018

Description of one-particle one-hole configurations coupled to the $3^{-}$ yrast state in the doubly magic nucleus ${}^{208}{Pb}$
journal, March 2019