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Title: Insight into the phase evolution of a NiMgAl catalyst from the reduction stage to the post-reaction stage during the dry reforming of methane [Insight into the phase evolution of NiMgAl catalyst from reduction to post-reaction for dry reforming of methane]

Herein, phase evolution of a NiMgAl oxide catalyst at the reduction stage was qualitatively analysed and quantitatively determined by employing the continuous changes in its XRD intensity and TPR information. In conclusion, the stable crystallite size of both the active metal and spinel support was responsible for the long stability of the NiMgAl catalyst without carbon deposition during the DRM reaction.
Authors:
 [1] ;  [1] ;  [1] ;  [2] ;  [1] ; ORCiD logo [1]
  1. Mississippi State Univ., Mississippi State, MS (United States)
  2. Argonne National Lab. (ANL), Argonne, IL (United States)
Publication Date:
Grant/Contract Number:
AC02-06CH11357
Type:
Accepted Manuscript
Journal Name:
ChemComm
Additional Journal Information:
Journal Volume: 53; Journal Issue: 44; Journal ID: ISSN 1359-7345
Publisher:
Royal Society of Chemistry
Research Org:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org:
U.S. Department of Agriculture (USDA); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22), Scientific User Facilities Division
Country of Publication:
United States
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
OSTI Identifier:
1372485

Bao, Zhenghong, Zhan, Yiqiu, Street, Jason, Xu, Wenqian, To, Filip, and Yu, Fei. Insight into the phase evolution of a NiMgAl catalyst from the reduction stage to the post-reaction stage during the dry reforming of methane [Insight into the phase evolution of NiMgAl catalyst from reduction to post-reaction for dry reforming of methane]. United States: N. p., Web. doi:10.1039/C7CC03094K.
Bao, Zhenghong, Zhan, Yiqiu, Street, Jason, Xu, Wenqian, To, Filip, & Yu, Fei. Insight into the phase evolution of a NiMgAl catalyst from the reduction stage to the post-reaction stage during the dry reforming of methane [Insight into the phase evolution of NiMgAl catalyst from reduction to post-reaction for dry reforming of methane]. United States. doi:10.1039/C7CC03094K.
Bao, Zhenghong, Zhan, Yiqiu, Street, Jason, Xu, Wenqian, To, Filip, and Yu, Fei. 2017. "Insight into the phase evolution of a NiMgAl catalyst from the reduction stage to the post-reaction stage during the dry reforming of methane [Insight into the phase evolution of NiMgAl catalyst from reduction to post-reaction for dry reforming of methane]". United States. doi:10.1039/C7CC03094K. https://www.osti.gov/servlets/purl/1372485.
@article{osti_1372485,
title = {Insight into the phase evolution of a NiMgAl catalyst from the reduction stage to the post-reaction stage during the dry reforming of methane [Insight into the phase evolution of NiMgAl catalyst from reduction to post-reaction for dry reforming of methane]},
author = {Bao, Zhenghong and Zhan, Yiqiu and Street, Jason and Xu, Wenqian and To, Filip and Yu, Fei},
abstractNote = {Herein, phase evolution of a NiMgAl oxide catalyst at the reduction stage was qualitatively analysed and quantitatively determined by employing the continuous changes in its XRD intensity and TPR information. In conclusion, the stable crystallite size of both the active metal and spinel support was responsible for the long stability of the NiMgAl catalyst without carbon deposition during the DRM reaction.},
doi = {10.1039/C7CC03094K},
journal = {ChemComm},
number = 44,
volume = 53,
place = {United States},
year = {2017},
month = {5}
}