Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids
Abstract
We present an optical technique based on ultrafast photoacoustics to determine the local temperature distribution profile in liquid samples in contact with a laser heated optical transducer. This ultrafast pump-probe experiment uses time-domain Brillouin scattering (TDBS) to locally determine the light scattering frequency shift. As the temperature influences the Brillouin scattering frequency, the TDBS signal probes the local laser-induced temperature distribution in the liquid. Here, we demonstrate the relevance and the sensitivity of this technique for the measurement of the absolute laser-induced temperature gradient of a glass forming liquid prototype, glycerol, at different laser pump powers—i.e., different steady state background temperatures. Complementarily, our experiments illustrate how this TDBS technique can be applied to measure thermal diffusion in complex multilayer systems in contact with a surrounding liquid.
- Authors:
-
- Univ. du Maine, Le Mans (France). Inst. Molecules et Materiaux du Mans
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Chemistry
- Univ. du Maine, Le Mans (France). Lab. d'Acoustique de l' Univ. du Maine
- Publication Date:
- Research Org.:
- Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1474332
- Alternate Identifier(s):
- OSTI ID: 1371600
- Grant/Contract Number:
- FG02-00ER15087
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Review of Scientific Instruments
- Additional Journal Information:
- Journal Volume: 88; Journal Issue: 7; Journal ID: ISSN 0034-6748
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; 47 OTHER INSTRUMENTATION
Citation Formats
Chaban, Ievgeniia, Shin, Hyun D., Klieber, Christoph, Busselez, Rémi, Gusev, Vitalyi E., Nelson, Keith A., and Pezeril, Thomas. Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids. United States: N. p., 2017.
Web. doi:10.1063/1.4993132.
Chaban, Ievgeniia, Shin, Hyun D., Klieber, Christoph, Busselez, Rémi, Gusev, Vitalyi E., Nelson, Keith A., & Pezeril, Thomas. Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids. United States. https://doi.org/10.1063/1.4993132
Chaban, Ievgeniia, Shin, Hyun D., Klieber, Christoph, Busselez, Rémi, Gusev, Vitalyi E., Nelson, Keith A., and Pezeril, Thomas. Tue .
"Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids". United States. https://doi.org/10.1063/1.4993132. https://www.osti.gov/servlets/purl/1474332.
@article{osti_1474332,
title = {Time-domain Brillouin scattering for the determination of laser-induced temperature gradients in liquids},
author = {Chaban, Ievgeniia and Shin, Hyun D. and Klieber, Christoph and Busselez, Rémi and Gusev, Vitalyi E. and Nelson, Keith A. and Pezeril, Thomas},
abstractNote = {We present an optical technique based on ultrafast photoacoustics to determine the local temperature distribution profile in liquid samples in contact with a laser heated optical transducer. This ultrafast pump-probe experiment uses time-domain Brillouin scattering (TDBS) to locally determine the light scattering frequency shift. As the temperature influences the Brillouin scattering frequency, the TDBS signal probes the local laser-induced temperature distribution in the liquid. Here, we demonstrate the relevance and the sensitivity of this technique for the measurement of the absolute laser-induced temperature gradient of a glass forming liquid prototype, glycerol, at different laser pump powers—i.e., different steady state background temperatures. Complementarily, our experiments illustrate how this TDBS technique can be applied to measure thermal diffusion in complex multilayer systems in contact with a surrounding liquid.},
doi = {10.1063/1.4993132},
journal = {Review of Scientific Instruments},
number = 7,
volume = 88,
place = {United States},
year = {Tue Jul 18 00:00:00 EDT 2017},
month = {Tue Jul 18 00:00:00 EDT 2017}
}
Web of Science
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