Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction
Abstract
Metamagnetism occuring inside a ferromagnetic phase is peculiar. Therefore, Sr4Ru3O10, a T C = 105 K ferromagnet, has attracted much attention in recent years, because it develops a pronounced metamagnetic anomaly below T C for magnetic fields applied in the crystallographic ab-plane. The metamagnetic transition moves to higher fields for lower temperatures and splits into a double anomaly at critical fields Hc1 = 2.3 T and Hc2 = 2.8 T, respectively. Here, we report a detailed study of the different components of the magnetization vector as a function of temperature, applied magnetic field, and varying angle in Sr4Ru3O10. We discover for the first time a reduction of the magnetic moment in the plane of rotation at the metamagnetic transition. The anomaly shifts to higher fields by rotating the field from H ⊥ c to H || c. We compare our experimental findings with numerical simulations based on spin reorientation models taking into account magnetocrystalline anisotropy, Zeeman effect and antisymmetric exchange interactions. While Magnetocrystalline anisotropy combined with a Zeeman term are sufficient to explain a metamagnetic transition in Sr4Ru3O10, a Dzyaloshinskii-Moriya term is crucial to account for the reduction of the magnetic moment as observed in the experiments.
- Authors:
-
[1];
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Univ. of Texas, Dallas, TX (United States). Dept. of Physics
- Univ. of Johannesburg (South Africa). Dept. of Physics
- Univ. of Salerno, Fisciano (Italy). CNR-SPIN Inst. Sede Secondaria di Salerno
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); National Research Foundation (NRF) (South Africa)
- Contributing Org.:
- Florida State Univ., Tallahassee, FL (United States); Univ. of Texas, Dallas, TX (United States); Univ. of Salerno, Fisciano (Italy)
- OSTI Identifier:
- 1369197
- Report Number(s):
- LA-UR-17-20729
Journal ID: ISSN 2045-2322
- Grant/Contract Number:
- AC52-06NA25396; DMR-1157490; 93549
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 7; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; magnetism, metamagnetis, strontium ruthenate
Citation Formats
Weickert, Franziska, Civale, Leonardo, Maiorov, Boris, Jaime, Marcelo, Salamon, Myron B., Carleschi, Emanuela, Strydom, André M., Fittipaldi, Rosalba, Granata, Veronica, and Vecchione, Antonio. Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction. United States: N. p., 2017.
Web. doi:10.1038/s41598-017-03648-2.
Weickert, Franziska, Civale, Leonardo, Maiorov, Boris, Jaime, Marcelo, Salamon, Myron B., Carleschi, Emanuela, Strydom, André M., Fittipaldi, Rosalba, Granata, Veronica, & Vecchione, Antonio. Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction. United States. https://doi.org/10.1038/s41598-017-03648-2
Weickert, Franziska, Civale, Leonardo, Maiorov, Boris, Jaime, Marcelo, Salamon, Myron B., Carleschi, Emanuela, Strydom, André M., Fittipaldi, Rosalba, Granata, Veronica, and Vecchione, Antonio. Tue .
"Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction". United States. https://doi.org/10.1038/s41598-017-03648-2. https://www.osti.gov/servlets/purl/1369197.
@article{osti_1369197,
title = {Missing magnetism in Sr4Ru3O10: Indication for Antisymmetric Exchange Interaction},
author = {Weickert, Franziska and Civale, Leonardo and Maiorov, Boris and Jaime, Marcelo and Salamon, Myron B. and Carleschi, Emanuela and Strydom, André M. and Fittipaldi, Rosalba and Granata, Veronica and Vecchione, Antonio},
abstractNote = {Metamagnetism occuring inside a ferromagnetic phase is peculiar. Therefore, Sr4Ru3O10, a T C = 105 K ferromagnet, has attracted much attention in recent years, because it develops a pronounced metamagnetic anomaly below T C for magnetic fields applied in the crystallographic ab-plane. The metamagnetic transition moves to higher fields for lower temperatures and splits into a double anomaly at critical fields Hc1 = 2.3 T and Hc2 = 2.8 T, respectively. Here, we report a detailed study of the different components of the magnetization vector as a function of temperature, applied magnetic field, and varying angle in Sr4Ru3O10. We discover for the first time a reduction of the magnetic moment in the plane of rotation at the metamagnetic transition. The anomaly shifts to higher fields by rotating the field from H ⊥ c to H || c. We compare our experimental findings with numerical simulations based on spin reorientation models taking into account magnetocrystalline anisotropy, Zeeman effect and antisymmetric exchange interactions. While Magnetocrystalline anisotropy combined with a Zeeman term are sufficient to explain a metamagnetic transition in Sr4Ru3O10, a Dzyaloshinskii-Moriya term is crucial to account for the reduction of the magnetic moment as observed in the experiments.},
doi = {10.1038/s41598-017-03648-2},
journal = {Scientific Reports},
number = ,
volume = 7,
place = {United States},
year = {Tue Jun 20 00:00:00 EDT 2017},
month = {Tue Jun 20 00:00:00 EDT 2017}
}
Free Publicly Available Full Text
Publisher's Version of Record
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 9 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Spin-triplet superconductivity in Sr2RuO4 identified by 17O Knight shift
journal, December 1998
- Ishida, K.; Mukuda, H.; Kitaoka, Y.
- Nature, Vol. 396, Issue 6712
Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7
journal, October 2001
- Grigera, S. A.
- Science, Vol. 294, Issue 5541
Spin-orbital nature of the high-field magnetic state in the
journal, March 2016
- Granata, Veronica; Capogna, Lucia; Forte, Filomena
- Physical Review B, Vol. 93, Issue 11
Magnetic Interactions in Ternary Ruthenium Oxides
journal, September 1966
- Callaghan, Alan; Moeller, Carl W.; Ward, Roland
- Inorganic Chemistry, Vol. 5, Issue 9
Magnetic properties of SrRuO 3 Single Crystal
journal, December 1976
- Kanbayasi, Akio
- Journal of the Physical Society of Japan, Vol. 41, Issue 6
Anisotropy of magnetoresistivities in : Evidence for an orbital-selective metamagnetic transition
journal, May 2010
- Fobes, D.; Liu, T. J.; Qu, Z.
- Physical Review B, Vol. 81, Issue 17
Anisotropic optical conductivity of Sr Ru O
journal, June 2012
- Mirri, C.; Vitucci, F. M.; Di Pietro, P.
- Physical Review B, Vol. 85, Issue 23
Changes in Magnetization of Single‐Crystal Dysprosium, Erbium, and Holmium in High Magnetic Fields
journal, March 1964
- Flippen, R. B.
- Journal of Applied Physics, Vol. 35, Issue 3
Correlated-electron theory of strongly anisotropic metamagnets
journal, December 1997
- Held, K.; Ulmke, M.; Blümer, N.
- Physical Review B, Vol. 56, Issue 22
Partially disordered antiferromagnetism and multiferroic behavior in a frustrated Ising system
journal, March 2016
- Mun, Eundeok; Weickert, Franziska; Kim, Jaewook
- Physical Review B, Vol. 93, Issue 10
Collective electron ferronmagnetism
journal, April 1938
- Stoner, Edmund Clifton
- Proceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences, Vol. 165, Issue 922, p. 372-414
Collective electron metamagnetism
journal, November 1962
- Wohlfarth, E. P.; Rhodes, P.
- Philosophical Magazine, Vol. 7, Issue 83
Itinerant metamagnetism
journal, August 1988
- Levitin, R. Z.; Markosyan, A. S.
- Soviet Physics Uspekhi, Vol. 31, Issue 8
Charge instabilities at the metamagnetic transition of itinerant electron systems
journal, September 2005
- Honerkamp, Carsten
- Physical Review B, Vol. 72, Issue 11
Pronounced first-order metamagnetic transition in the paramagnetic heavy-fermion system CeTiGe
journal, February 2012
- Deppe, M.; Lausberg, S.; Weickert, F.
- Physical Review B, Vol. 85, Issue 6
Metamagnetism of itinerant electrons in multi-layer ruthenates
journal, March 2004
- Binz, B.; Sigrist, M.
- Europhysics Letters (EPL), Vol. 65, Issue 6
Universal signatures of the metamagnetic quantum critical endpoint: Application to
journal, April 2010
- Weickert, Franziska; Brando, Manuel; Steglich, Frank
- Physical Review B, Vol. 81, Issue 13
Multiple First-Order Metamagnetic Transitions and Quantum Oscillations in Ultrapure
journal, April 2004
- Perry, R. S.; Kitagawa, K.; Grigera, S. A.
- Physical Review Letters, Vol. 92, Issue 16
Disorder-Sensitive Phase Formation Linked to Metamagnetic Quantum Criticality
journal, November 2004
- Grigera, S. A.
- Science, Vol. 306, Issue 5699
Metamagnetic Quantum Criticality in Studied by Thermal Expansion
journal, April 2006
- Gegenwart, P.; Weickert, F.; Garst, M.
- Physical Review Letters, Vol. 96, Issue 13
Phase diagram of the electronic states of trilayered ruthenate
journal, March 2007
- Fobes, D.; Yu, M. H.; Zhou, M.
- Physical Review B, Vol. 75, Issue 9
Anomalous itinerant magnetism in single-crystal : A thermodynamic and transport investigation
journal, January 2007
- Cao, G.; Chikara, S.; Brill, J. W.
- Physical Review B, Vol. 75, Issue 2
Magnetic, electrical transport, and thermoelectric properties of : Evidence for a field-induced electronic phase transition at low temperatures
journal, September 2007
- Xu, Zhuan; Xu, Xiangfan; Freitas, Rafael S.
- Physical Review B, Vol. 76, Issue 9
Electronic and magnetic properties of triple-layered ruthenate Sr4Ru3O10 single crystals grown by a floating-zone method
journal, June 2005
- Zhou, M.; Hooper, J.; Fobes, D.
- Materials Research Bulletin, Vol. 40, Issue 6
Orbital-dependent metamagnetic response in
journal, March 2007
- Jo, Y. J.; Balicas, L.; Kikugawa, N.
- Physical Review B, Vol. 75, Issue 9
Nature of Spin-Reorientation Transitions
journal, April 1968
- Horner, H.; Varma, C. M.
- Physical Review Letters, Vol. 20, Issue 16
A thermodynamic theory of “weak” ferromagnetism of antiferromagnetics
journal, January 1958
- Dzyaloshinsky, I.
- Journal of Physics and Chemistry of Solids, Vol. 4, Issue 4
Anisotropic Superexchange Interaction and Weak Ferromagnetism
journal, October 1960
- Moriya, Tôru
- Physical Review, Vol. 120, Issue 1
A simple law governing coupled magnetic orders in perovskites
journal, July 2012
- Bellaiche, L.; Gui, Zhigang; Kornev, Igor A.
- Journal of Physics: Condensed Matter, Vol. 24, Issue 31
Crystal Growth of a Lamellar Sr 3 Ru 2 O 7 –Sr 4 Ru 3 O 10 Eutectic System
journal, December 2007
- Fittipaldi, Rosalba; Sisti, Daniela; Vecchione, Antonio
- Crystal Growth & Design, Vol. 7, Issue 12
Demagnetizing Factors of the General Ellipsoid
journal, June 1945
- Osborn, J. A.
- Physical Review, Vol. 67, Issue 11-12
A thermodynamic theory of “weak” ferromagnetism of antiferromagnetics
journal, January 1958
- Dzyaloshinsky, I.
- Journal of Physics and Chemistry of Solids, Vol. 4, Issue 4
Electronic and magnetic properties of triple-layered ruthenate Sr4Ru3O10 single crystals grown by a floating-zone method
journal, June 2005
- Zhou, M.; Hooper, J.; Fobes, D.
- Materials Research Bulletin, Vol. 40, Issue 6
Magnetic Interactions in Ternary Ruthenium Oxides
journal, September 1966
- Callaghan, Alan; Moeller, Carl W.; Ward, Roland
- Inorganic Chemistry, Vol. 5, Issue 9
Changes in Magnetization of Single‐Crystal Dysprosium, Erbium, and Holmium in High Magnetic Fields
journal, March 1964
- Flippen, R. B.
- Journal of Applied Physics, Vol. 35, Issue 3
Collective electron metamagnetism
journal, November 1962
- Wohlfarth, E. P.; Rhodes, P.
- Philosophical Magazine, Vol. 7, Issue 83
Neutron diffraction study of triple-layered Sr 4 Ru 3 O 10
journal, January 2013
- Granata, Veronica; Capogna, Lucia; Reehuis, Manfred
- Journal of Physics: Condensed Matter, Vol. 25, Issue 5
Collective electron ferronmagnetism
journal, April 1938
- Stoner, Edmund Clifton
- Proceedings of the Royal Society of London. Series A. Mathematical and Physical Sciences, Vol. 165, Issue 922, p. 372-414
Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7
journal, October 2001
- Grigera, S. A.
- Science, Vol. 294, Issue 5541
Disorder-Sensitive Phase Formation Linked to Metamagnetic Quantum Criticality
journal, November 2004
- Grigera, S. A.
- Science, Vol. 306, Issue 5699
Metamagnetism of itinerant electrons in multi-layer ruthenates
journal, March 2004
- Binz, B.; Sigrist, M.
- Europhysics Letters (EPL), Vol. 65, Issue 6
Works referencing / citing this record:
Temperature- and field-driven spin reorientations in triple-layer ruthenate Sr4Ru3O10
journal, March 2018
- Zhu, M.; Li, P. G.; Wang, Y.
- Scientific Reports, Vol. 8, Issue 1
Suppression of the orbital magnetic moment driven by electronic correlations in
journal, September 2019
- Forte, Filomena; Capogna, Lucia; Granata, Veronica
- Physical Review B, Vol. 100, Issue 10
Temperature- and field-driven spin reorientations in triple-layer ruthenate Sr$_4$Ru$_3$O$_{10}$
preprint, January 2018
- Zhu, M.; Li, P. G.; Wang, Y.
- arXiv
In-depth study of the $H -T$ phase diagram of Sr4Ru3O10 by magnetization experiments
text, January 2017
- Weickert, F.; Civale, L.; Maiorov, B.
- arXiv
Temperature- and field-driven spin reorientations in triple-layer ruthenate Sr$_4$Ru$_3$O$_{10}$
preprint, January 2018
- Zhu, M.; Li, P. G.; Wang, Y.
- arXiv