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Title: Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control

Abstract

Nuclear forensic science seeks to identify the origin of nuclear materials found outside regulatory control. It is increasingly recognized as an integral part of a robust nuclear security program. Our review highlights areas of active, evolving research in nuclear forensics, with a focus on analytical techniques commonly employed in Earth and planetary sciences. Applications of nuclear forensics to uranium ore concentrates (UOCs) are discussed first. UOCs have become an attractive target for nuclear forensic researchers because of the richness in impurities compared to materials produced later in the fuel cycle. Furthermore, the development of chronometric methods for age dating nuclear materials is then discussed, with an emphasis on improvements in accuracy that have been gained from measurements of multiple radioisotopic systems. Finally, papers that report on casework are reviewed, to provide a window into current scientific practice.

Authors:
 [1];  [1];  [1];  [1];  [1];  [1]
  1. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Publication Date:
Research Org.:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1366959
Report Number(s):
LLNL-JRNL-683854
Journal ID: ISSN 0084-6597
Grant/Contract Number:  
AC52-07NA27344
Resource Type:
Accepted Manuscript
Journal Name:
Annual Review of Earth and Planetary Sciences
Additional Journal Information:
Journal Volume: 44; Journal Issue: 1; Journal ID: ISSN 0084-6597
Publisher:
Annual Reviews
Country of Publication:
United States
Language:
English
Subject:
38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY; 11 NUCLEAR FUEL CYCLE AND RUEL MATERIALS; 98 NUCLEAR DISARMAMENT, SAFEGUARDS AND PHYSICAL PROTECTION; nuclear forensics; nuclear trafficking; radiochronometry; uranium ore concentrate

Citation Formats

Kristo, Michael J., Gaffney, Amy M., Marks, Naomi, Knight, Kim, Cassata, William S., and Hutcheon, Ian D. Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control. United States: N. p., 2016. Web. doi:10.1146/annurev-earth-060115-012309.
Kristo, Michael J., Gaffney, Amy M., Marks, Naomi, Knight, Kim, Cassata, William S., & Hutcheon, Ian D. Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control. United States. doi:10.1146/annurev-earth-060115-012309.
Kristo, Michael J., Gaffney, Amy M., Marks, Naomi, Knight, Kim, Cassata, William S., and Hutcheon, Ian D. Wed . "Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control". United States. doi:10.1146/annurev-earth-060115-012309. https://www.osti.gov/servlets/purl/1366959.
@article{osti_1366959,
title = {Nuclear Forensic Science: Analysis of Nuclear Material Out of Regulatory Control},
author = {Kristo, Michael J. and Gaffney, Amy M. and Marks, Naomi and Knight, Kim and Cassata, William S. and Hutcheon, Ian D.},
abstractNote = {Nuclear forensic science seeks to identify the origin of nuclear materials found outside regulatory control. It is increasingly recognized as an integral part of a robust nuclear security program. Our review highlights areas of active, evolving research in nuclear forensics, with a focus on analytical techniques commonly employed in Earth and planetary sciences. Applications of nuclear forensics to uranium ore concentrates (UOCs) are discussed first. UOCs have become an attractive target for nuclear forensic researchers because of the richness in impurities compared to materials produced later in the fuel cycle. Furthermore, the development of chronometric methods for age dating nuclear materials is then discussed, with an emphasis on improvements in accuracy that have been gained from measurements of multiple radioisotopic systems. Finally, papers that report on casework are reviewed, to provide a window into current scientific practice.},
doi = {10.1146/annurev-earth-060115-012309},
journal = {Annual Review of Earth and Planetary Sciences},
number = 1,
volume = 44,
place = {United States},
year = {2016},
month = {5}
}

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Works referencing / citing this record:

Advances in age-dating of individual uranium particles by large geometry secondary ion mass spectrometry
journal, January 2019

  • Szakal, Christopher; Simons, David S.; Fassett, John D.
  • The Analyst, Vol. 144, Issue 14
  • DOI: 10.1039/c9an00774a

Advances in age-dating of individual uranium particles by large geometry secondary ion mass spectrometry
journal, January 2019

  • Szakal, Christopher; Simons, David S.; Fassett, John D.
  • The Analyst, Vol. 144, Issue 14
  • DOI: 10.1039/c9an00774a