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Title: Novel preparation of N-doped SnO 2 nanoparticles via laser-assisted pyrolysis: Demonstration of exceptional lithium storage properties

Abstract

Here, laser pyrolyzed SnO 2 nanoparticles with an option of nitrogen (N) doping are prepared using a cost-effective method. The electrochemical performance of N-doped samples is tested for the first time in Li-ion batteries where the sample with 3% of N-dopant exhibits optimum performance with a capacity of 522 mAh g active material –1 that can be obtained at 10 A g –1 (6.7C).

Authors:
 [1];  [2];  [3];  [4];  [4];  [5];  [6];  [1];  [7];  [4];  [4]
  1. Nanyang Technological Univ. (Singapore); IRAMIS, Gif sur Yvette (France)
  2. IRAMIS, Gif sur Yvette (France)
  3. Oregon State Univ., Corvallis, OR (United States)
  4. Nanyang Technological Univ. (Singapore)
  5. Northwestern Synchrotron Research Center at the Advance Photon Source, Argonne, IL (United States)
  6. Argonne National Lab. (ANL), Argonne, IL (United States)
  7. LITEN, Grenoble (France)
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
Singapore National Science Foundation; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22), Scientific User Facilities Division
OSTI Identifier:
1365391
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 29; Journal Issue: 6; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 77 NANOSCIENCE AND NANOTECHNOLOGY; 25 ENERGY STORAGE; SnO2; X-ray absorption spectroscopy; laser-pyrolysis; lithium ion batteries; nitrogen doping

Citation Formats

Wang, Luyuan Paul, Leconte, Yann, Feng, Zhenxing, Wei, Chao, Zhao, Yi, Ma, Qing, Xu, Wenqian, Bourrioux, Samantha, Azais, Philippe, Srinivasan, Madhavi, and Xu, Zhichuan J. Novel preparation of N-doped SnO2 nanoparticles via laser-assisted pyrolysis: Demonstration of exceptional lithium storage properties. United States: N. p., 2016. Web. doi:10.1002/adma.201603286.
Wang, Luyuan Paul, Leconte, Yann, Feng, Zhenxing, Wei, Chao, Zhao, Yi, Ma, Qing, Xu, Wenqian, Bourrioux, Samantha, Azais, Philippe, Srinivasan, Madhavi, & Xu, Zhichuan J. Novel preparation of N-doped SnO2 nanoparticles via laser-assisted pyrolysis: Demonstration of exceptional lithium storage properties. United States. doi:10.1002/adma.201603286.
Wang, Luyuan Paul, Leconte, Yann, Feng, Zhenxing, Wei, Chao, Zhao, Yi, Ma, Qing, Xu, Wenqian, Bourrioux, Samantha, Azais, Philippe, Srinivasan, Madhavi, and Xu, Zhichuan J. Mon . "Novel preparation of N-doped SnO2 nanoparticles via laser-assisted pyrolysis: Demonstration of exceptional lithium storage properties". United States. doi:10.1002/adma.201603286. https://www.osti.gov/servlets/purl/1365391.
@article{osti_1365391,
title = {Novel preparation of N-doped SnO2 nanoparticles via laser-assisted pyrolysis: Demonstration of exceptional lithium storage properties},
author = {Wang, Luyuan Paul and Leconte, Yann and Feng, Zhenxing and Wei, Chao and Zhao, Yi and Ma, Qing and Xu, Wenqian and Bourrioux, Samantha and Azais, Philippe and Srinivasan, Madhavi and Xu, Zhichuan J.},
abstractNote = {Here, laser pyrolyzed SnO2 nanoparticles with an option of nitrogen (N) doping are prepared using a cost-effective method. The electrochemical performance of N-doped samples is tested for the first time in Li-ion batteries where the sample with 3% of N-dopant exhibits optimum performance with a capacity of 522 mAh gactive material –1 that can be obtained at 10 A g–1 (6.7C).},
doi = {10.1002/adma.201603286},
journal = {Advanced Materials},
number = 6,
volume = 29,
place = {United States},
year = {2016},
month = {12}
}

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Cited by: 14 works
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Works referenced in this record:

Issues and challenges facing rechargeable lithium batteries
journal, November 2001

  • Tarascon, J.-M.; Armand, M.
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In Situ Observation of the Electrochemical Lithiation of a Single SnO2 Nanowire Electrode
journal, December 2010


Electrochemical and In Situ X-Ray Diffraction Studies of the Reaction of Lithium with Tin Oxide Composites
journal, January 1997

  • Courtney, Ian A.; Dahn, J. R.
  • Journal of The Electrochemical Society, Vol. 144, Issue 6, p. 2045-2052
  • DOI: 10.1149/1.1837740