Ultrafast Plasmonic Control of Second Harmonic Generation
Abstract
Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher harmonic conversion efficiencies per unit volume than those attainable in bulk materials. Here we demonstrate efficient second-harmonic generation (SHG) in a serrated nanogap plasmonic geometry that generates steep electric field gradients on a dielectric metasurface. An ultrafast control pulse is used to control plasmon-induced electric fields in a thin-film material with inversion symmetry that, without plasmonic enhancement, does not exhibit an even-order nonlinear optical response. The temporal evolution of the plasmonic near-field is characterized with ~100 as resolution using a novel nonlinear interferometric technique. The serrated nanogap is a unique platform in which to investigate optically controlled, plasmonically enhanced harmonic generation in dielectric materials on an ultrafast time scale. Lastly, this metamaterial geometry can also be readily extended to all-optical control of other nonlinear phenomena, such as four-wave mixing and sum- and difference-frequency generation, in a wide variety of dielectric materials.
- Authors:
-
- Vanderbilt Univ., Nashville, TN (United States). Dept. of Physics and Astronomy; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Computational Sciences and Engineering Division
- Vanderbilt Univ., Nashville, TN (United States). Dept. of Physics and Astronomy; Univ. of Virginia, Charlottesville, VA (United States). Dept. of Physics
- Vanderbilt Univ., Nashville, TN (United States). Dept. of Physics and Astronomy
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Computational Sciences and Engineering Division
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Oak Ridge Leadership Computing Facility (OLCF)
- Sponsoring Org.:
- USDOE Laboratory Directed Research and Development (LDRD) Program; National Science Foundation (NSF); USDOE Office of Science (SC)
- OSTI Identifier:
- 1364273
- Grant/Contract Number:
- AC05-00OR22725; FG02-01ER45916
- Resource Type:
- Accepted Manuscript
- Journal Name:
- ACS Photonics
- Additional Journal Information:
- Journal Volume: 3; Journal Issue: 8; Journal ID: ISSN 2330-4022
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; interferometry; metasurfaces; nonlinear optics; optical control; plasmonic enhancement
Citation Formats
Davidson, Roderick B., Yanchenko, Anna, Ziegler, Jed I., Avanesyan, Sergey M., Lawrie, Benjamin J., and Haglund, Richard F. Ultrafast Plasmonic Control of Second Harmonic Generation. United States: N. p., 2016.
Web. doi:10.1021/acsphotonics.6b00034.
Davidson, Roderick B., Yanchenko, Anna, Ziegler, Jed I., Avanesyan, Sergey M., Lawrie, Benjamin J., & Haglund, Richard F. Ultrafast Plasmonic Control of Second Harmonic Generation. United States. https://doi.org/10.1021/acsphotonics.6b00034
Davidson, Roderick B., Yanchenko, Anna, Ziegler, Jed I., Avanesyan, Sergey M., Lawrie, Benjamin J., and Haglund, Richard F. Wed .
"Ultrafast Plasmonic Control of Second Harmonic Generation". United States. https://doi.org/10.1021/acsphotonics.6b00034. https://www.osti.gov/servlets/purl/1364273.
@article{osti_1364273,
title = {Ultrafast Plasmonic Control of Second Harmonic Generation},
author = {Davidson, Roderick B. and Yanchenko, Anna and Ziegler, Jed I. and Avanesyan, Sergey M. and Lawrie, Benjamin J. and Haglund, Richard F.},
abstractNote = {Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher harmonic conversion efficiencies per unit volume than those attainable in bulk materials. Here we demonstrate efficient second-harmonic generation (SHG) in a serrated nanogap plasmonic geometry that generates steep electric field gradients on a dielectric metasurface. An ultrafast control pulse is used to control plasmon-induced electric fields in a thin-film material with inversion symmetry that, without plasmonic enhancement, does not exhibit an even-order nonlinear optical response. The temporal evolution of the plasmonic near-field is characterized with ~100 as resolution using a novel nonlinear interferometric technique. The serrated nanogap is a unique platform in which to investigate optically controlled, plasmonically enhanced harmonic generation in dielectric materials on an ultrafast time scale. Lastly, this metamaterial geometry can also be readily extended to all-optical control of other nonlinear phenomena, such as four-wave mixing and sum- and difference-frequency generation, in a wide variety of dielectric materials.},
doi = {10.1021/acsphotonics.6b00034},
journal = {ACS Photonics},
number = 8,
volume = 3,
place = {United States},
year = {Wed Jun 01 00:00:00 EDT 2016},
month = {Wed Jun 01 00:00:00 EDT 2016}
}
Web of Science
Works referenced in this record:
Nonlinear plasmonics
journal, November 2012
- Kauranen, Martti; Zayats, Anatoly V.
- Nature Photonics, Vol. 6, Issue 11
Active nanoplasmonic metamaterials
journal, June 2012
- Hess, O.; Pendry, J. B.; Maier, S. A.
- Nature Materials, Vol. 11, Issue 7
High-speed plasmonic phase modulators
journal, February 2014
- Melikyan, A.; Alloatti, L.; Muslija, A.
- Nature Photonics, Vol. 8, Issue 3
Efficient forward second-harmonic generation from planar archimedean nanospirals
journal, January 2015
- Davidson II, Roderick B.; Ziegler, Jed I.; Vargas, Guillermo
- Nanophotonics, Vol. 4, Issue 1
Multiresonant Broadband Optical Antennas As Efficient Tunable Nanosources of Second Harmonic Light
journal, January 2012
- Aouani, Heykel; Navarro-Cia, Miguel; Rahmani, Mohsen
- Nano Letters, Vol. 12, Issue 9
Three-Dimensional Nanostructures as Highly Efficient Generators of Second Harmonic Light
journal, December 2011
- Zhang, Yu; Grady, Nathaniel K.; Ayala-Orozco, Ciceron
- Nano Letters, Vol. 11, Issue 12
Multipolar second harmonic generation from planar arrays of Au nanoparticles
journal, January 2012
- Capretti, Antonio; Walsh, Gary F.; Minissale, Salvatore
- Optics Express, Vol. 20, Issue 14
Size-dependent second-harmonic generation from gold nanoparticles
journal, March 2014
- Capretti, Antonio; Pecora, Emanuele F.; Forestiere, Carlo
- Physical Review B, Vol. 89, Issue 12
Giant nonlinear response from plasmonic metasurfaces coupled to intersubband transitions
journal, July 2014
- Lee, Jongwon; Tymchenko, Mykhailo; Argyropoulos, Christos
- Nature, Vol. 511, Issue 7507
Third-harmonic-upconversion enhancement from a single semiconductor nanoparticle coupled to a plasmonic antenna
journal, March 2014
- Aouani, Heykel; Rahmani, Mohsen; Navarro-Cía, Miguel
- Nature Nanotechnology, Vol. 9, Issue 4
Spatiotemporal control of nanooptical excitations
journal, March 2010
- Aeschlimann, M.; Bauer, M.; Bayer, D.
- Proceedings of the National Academy of Sciences, Vol. 107, Issue 12
Tailoring Spatiotemporal Light Confinement in Single Plasmonic Nanoantennas
journal, January 2012
- Hanke, Tobias; Cesar, Julijan; Knittel, Vanessa
- Nano Letters, Vol. 12, Issue 2
Electrically Controlled Nonlinear Generation of Light with Plasmonics
journal, September 2011
- Cai, W.; Vasudev, A. P.; Brongersma, M. L.
- Science, Vol. 333, Issue 6050
Electrifying photonic metamaterials for tunable nonlinear optics
journal, August 2014
- Kang, Lei; Cui, Yonghao; Lan, Shoufeng
- Nature Communications, Vol. 5, Issue 1
Near-Field Two-Photon-Induced Photoluminescence from Single Gold Nanorods and Imaging of Plasmon Modes
journal, July 2005
- Imura, Kohei; Nagahara, Tetsuhiko; Okamoto, Hiromi
- The Journal of Physical Chemistry B, Vol. 109, Issue 27
Terahertz-field-induced second harmonic generation through Pockels effect in zinc telluride crystal
journal, January 2014
- Cornet, Marion; Degert, Jérôme; Abraham, Emmanuel
- Optics Letters, Vol. 39, Issue 20
Multiple Independent Comb Shaping (MICS): Phase-only generation of optical pulse sequences
journal, January 2009
- Pestov, Dmitry; Lozovoy, Vadim V.; Dantus, Marcos
- Optics Express, Vol. 17, Issue 16
Optical Constants of the Noble Metals
journal, December 1972
- Johnson, P. B.; Christy, R. W.
- Physical Review B, Vol. 6, Issue 12, p. 4370-4379
Works referencing / citing this record:
Nanofocusing in SOI-based hybrid plasmonic metal slot waveguides
journal, January 2018
- Güsken, Nicholas A.; Nielsen, Michael P.; Nguyen, Ngoc B.
- Optics Express, Vol. 26, Issue 23
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation
journal, January 2019
- Huang, Zhijin; Lu, Huihui; Xiong, Hanqing
- Nanomaterials, Vol. 9, Issue 1
ALD assisted nanoplasmonic slot waveguide for on-chip enhanced Raman spectroscopy
journal, November 2018
- Raza, Ali; Clemmen, Stéphane; Wuytens, Pieter
- APL Photonics, Vol. 3, Issue 11
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation
journal, January 2019
- Huang, Zhijin; Lu, Huihui; Xiong, Hanqing
- Nanomaterials, Vol. 9, Issue 1