DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber

Abstract

Ultrafast control of the polarization state of light may enable a plethora of applications in optics, chemistry and biology. However, conventional polarizing elements, such as polarizers and waveplates, are either static or possess only gigahertz switching speeds. Here, with the aid of high-mobility indium-doped cadmium oxide (CdO) as the gateway plasmonic material, we realize a high-quality factor Berreman-type perfect absorber at a wavelength of 2.08 μm. On sub-bandgap optical pumping, the perfect absorption resonance strongly redshifts because of the transient increase of the ensemble-averaged effective electron mass of CdO, which leads to an absolute change in the p-polarized reflectance from 1.0 to 86.3%. As a result, by combining the exceedingly high modulation depth with the polarization selectivity of the perfect absorber, we experimentally demonstrate a reflective polarizer with a polarization extinction ratio of 91 that can be switched on and off within 800 fs.

Authors:
ORCiD logo [1];  [2];  [2]; ORCiD logo [1];  [1];  [2];  [1];  [1]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. North Carolina State Univ., Raleigh, NC (United States)
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1361213
Report Number(s):
SAND-2017-3063J
Journal ID: ISSN 1749-4885; nphoton.2017.64
Grant/Contract Number:  
AC04-94AL85000
Resource Type:
Accepted Manuscript
Journal Name:
Nature Photonics
Additional Journal Information:
Journal Volume: 11; Journal Issue: 6; Journal ID: ISSN 1749-4885
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; metamaterials; nanophotonics and plasmonics; ultrafast photonics

Citation Formats

Yang, Yuanmu, Kelley, Kyle, Sachet, Edward, Campione, Salvatore, Luk, Ting S., Maria, Jon -Paul, Sinclair, Michael B., and Brener, Igal. Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber. United States: N. p., 2017. Web. doi:10.1038/nphoton.2017.64.
Yang, Yuanmu, Kelley, Kyle, Sachet, Edward, Campione, Salvatore, Luk, Ting S., Maria, Jon -Paul, Sinclair, Michael B., & Brener, Igal. Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber. United States. https://doi.org/10.1038/nphoton.2017.64
Yang, Yuanmu, Kelley, Kyle, Sachet, Edward, Campione, Salvatore, Luk, Ting S., Maria, Jon -Paul, Sinclair, Michael B., and Brener, Igal. Mon . "Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber". United States. https://doi.org/10.1038/nphoton.2017.64. https://www.osti.gov/servlets/purl/1361213.
@article{osti_1361213,
title = {Femtosecond optical polarization switching using a cadmium oxide-based perfect absorber},
author = {Yang, Yuanmu and Kelley, Kyle and Sachet, Edward and Campione, Salvatore and Luk, Ting S. and Maria, Jon -Paul and Sinclair, Michael B. and Brener, Igal},
abstractNote = {Ultrafast control of the polarization state of light may enable a plethora of applications in optics, chemistry and biology. However, conventional polarizing elements, such as polarizers and waveplates, are either static or possess only gigahertz switching speeds. Here, with the aid of high-mobility indium-doped cadmium oxide (CdO) as the gateway plasmonic material, we realize a high-quality factor Berreman-type perfect absorber at a wavelength of 2.08 μm. On sub-bandgap optical pumping, the perfect absorption resonance strongly redshifts because of the transient increase of the ensemble-averaged effective electron mass of CdO, which leads to an absolute change in the p-polarized reflectance from 1.0 to 86.3%. As a result, by combining the exceedingly high modulation depth with the polarization selectivity of the perfect absorber, we experimentally demonstrate a reflective polarizer with a polarization extinction ratio of 91 that can be switched on and off within 800 fs.},
doi = {10.1038/nphoton.2017.64},
journal = {Nature Photonics},
number = 6,
volume = 11,
place = {United States},
year = {Mon May 01 00:00:00 EDT 2017},
month = {Mon May 01 00:00:00 EDT 2017}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 198 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Nonlinear phononics as an ultrafast route to lattice control
journal, August 2011

  • Först, M.; Manzoni, C.; Kaiser, S.
  • Nature Physics, Vol. 7, Issue 11
  • DOI: 10.1038/nphys2055

Coherent terahertz control of antiferromagnetic spin waves
journal, November 2010


Molecular Orientation and Alignment by Intense Single-Cycle THz Pulses
journal, October 2011


All-Optical Magnetic Recording with Circularly Polarized Light
journal, July 2007


40-GHz electro-optic polarization modulator for fiber optic communications systems
conference, December 2004

  • Bull, Jeffrey D.; Jaeger, Nicolas A.; Kato, Hiroshi
  • Photonics North, SPIE Proceedings
  • DOI: 10.1117/12.567640

Rotation of laser beam polarization in acousto-optic devices
journal, March 1975

  • Eklund, H.; Roos, A.; Eng, S. T.
  • Optical and Quantum Electronics, Vol. 7, Issue 2
  • DOI: 10.1007/BF00631587

Off-resonant magnetization dynamics phase-locked to an intense phase-stable terahertz transient
journal, August 2013


Nanoplasmonics: past, present, and glimpse into future
journal, January 2011


Ultrafast active plasmonics
journal, December 2008

  • MacDonald, Kevin F.; Sámson, Zsolt L.; Stockman, Mark I.
  • Nature Photonics, Vol. 3, Issue 1, p. 55-58
  • DOI: 10.1038/nphoton.2008.249

Designed ultrafast optical nonlinearity in a plasmonic nanorod metamaterial enhanced by nonlocality
journal, January 2011


Nonlinear Fano-Resonant Dielectric Metasurfaces
journal, October 2015


Tuning of Magnetic Optical Response in a Dielectric Nanoparticle by Ultrafast Photoexcitation of Dense Electron–Hole Plasma
journal, August 2015


Ultrafast Dynamics of Surface Plasmons in InAs by Time-Resolved Infrared Nanospectroscopy
journal, July 2014

  • Wagner, Martin; McLeod, Alexander S.; Maddox, Scott J.
  • Nano Letters, Vol. 14, Issue 8
  • DOI: 10.1021/nl501558t

Transient GaAs Plasmonic Metasurfaces at Terahertz Frequencies
journal, December 2016


Ultrafast and Nanoscale Plasmonic Phenomena in Exfoliated Graphene Revealed by Infrared Pump–Probe Nanoscopy
journal, January 2014

  • Wagner, Martin; Fei, Zhe; McLeod, Alexander S.
  • Nano Letters, Vol. 14, Issue 2
  • DOI: 10.1021/nl4042577

Ultrafast optical switching of infrared plasmon polaritons in high-mobility graphene
journal, March 2016


Femtosecond photo-switching of interface polaritons in black phosphorus heterostructures
journal, December 2016

  • Huber, Markus A.; Mooshammer, Fabian; Plankl, Markus
  • Nature Nanotechnology, Vol. 12, Issue 3
  • DOI: 10.1038/nnano.2016.261

Epsilon-near-zero Al-doped ZnO for ultrafast switching at telecom wavelengths
journal, January 2015


Ultrafast Nonlinear Response of Bulk Plasmons in Highly Doped ZnO Layers
journal, September 2015


Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films
journal, April 2015

  • Luk, Ting S.; de Ceglia, Domenico; Liu, Sheng
  • Applied Physics Letters, Vol. 106, Issue 15, Article No. 151103
  • DOI: 10.1063/1.4917457

Ultrafast switching of tunable infrared plasmons in indium tin oxide nanorod arrays with large absolute amplitude
journal, February 2016

  • Guo, Peijun; Schaller, Richard D.; Ketterson, John B.
  • Nature Photonics, Vol. 10, Issue 4
  • DOI: 10.1038/nphoton.2016.14

Large optical nonlinearity of indium tin oxide in its epsilon-near-zero region
journal, April 2016


Enhanced Nonlinear Refractive Index in ε -Near-Zero Materials
journal, June 2016


Dynamic Reflection Phase and Polarization Control in Metasurfaces
journal, December 2016


Dysprosium-doped cadmium oxide as a gateway material for mid-infrared plasmonics
journal, February 2015

  • Sachet, Edward; Shelton, Christopher T.; Harris, Joshua S.
  • Nature Materials, Vol. 14, Issue 4
  • DOI: 10.1038/nmat4203

Alternative Plasmonic Materials: Beyond Gold and Silver
journal, May 2013

  • Naik, Gururaj V.; Shalaev, Vladimir M.; Boltasseva, Alexandra
  • Advanced Materials, Vol. 25, Issue 24
  • DOI: 10.1002/adma.201205076

Directional perfect absorption using deep subwavelength low-permittivity films
journal, August 2014

  • Luk, Ting S.; Campione, Salvatore; Kim, Iltai
  • Physical Review B, Vol. 90, Issue 8, Article No. 085411
  • DOI: 10.1103/PhysRevB.90.085411

Berreman mode and epsilon near zero mode
journal, January 2012

  • Vassant, Simon; Hugonin, Jean-Paul; Marquier, Francois
  • Optics Express, Vol. 20, Issue 21, p. 23971-23977
  • DOI: 10.1364/OE.20.023971

Theory of epsilon-near-zero modes in ultrathin films
journal, March 2015

  • Campione, Salvatore; Brener, Igal; Marquier, Francois
  • Physical Review B, Vol. 91, Issue 12, Article No. 121408(R)
  • DOI: 10.1103/PhysRevB.91.121408

Bandgap and effective mass of epitaxial cadmium oxide
journal, January 2008

  • Jefferson, P. H.; Hatfield, S. A.; Veal, T. D.
  • Applied Physics Letters, Vol. 92, Issue 2
  • DOI: 10.1063/1.2833269

Ultra-high modulation depth exceeding 2,400% in optically controlled topological surface plasmons
journal, October 2015

  • Sim, Sangwan; Jang, Houk; Koirala, Nikesh
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9814

Transient photoconductivity in GaAs as measured by time-resolved terahertz spectroscopy
journal, December 2000

  • Beard, Matthew C.; Turner, Gordon M.; Schmuttenmaer, Charles A.
  • Physical Review B, Vol. 62, Issue 23
  • DOI: 10.1103/PhysRevB.62.15764

Eliminate coherence spike in reflection-type pump-probe measurements
journal, January 2009


Measurement of the Stokes parameters of light
journal, January 1977

  • Berry, H. G.; Gabrielse, G.; Livingston, A. E.
  • Applied Optics, Vol. 16, Issue 12
  • DOI: 10.1364/AO.16.003200

Coherent terahertz control of antiferromagnetic spin waves
text, January 2011

  • Kampfrath, Tobias; Sell, Alexander; Klatt, Gregor
  • Universität Regensburg
  • DOI: 10.5283/epub.19114

Femtosecond photo-switching of interface polaritons in black phosphorus heterostructures
text, January 2017

  • Huber, Markus A.; Mooshammer, Fabian; Plankl, Markus
  • Universität Regensburg
  • DOI: 10.5283/epub.35076

Works referencing / citing this record:

Broadband, High‐Speed, and Large‐Amplitude Dynamic Optical Switching with Yttrium‐Doped Cadmium Oxide
journal, December 2019

  • Saha, Soham; Diroll, Benjamin T.; Shank, Joshua
  • Advanced Functional Materials, Vol. 30, Issue 7
  • DOI: 10.1002/adfm.201908377

All‐Dielectric Active Terahertz Photonics Driven by Bound States in the Continuum
journal, July 2019

  • Han, Song; Cong, Longqing; Srivastava, Yogesh Kumar
  • Advanced Materials, Vol. 31, Issue 37
  • DOI: 10.1002/adma.201901921

Self-Assembled Nanostructured Photonic-Plasmonic Metasurfaces for High-Resolution Optical Thermometry
journal, May 2018

  • Baraldi, Giorgio; García Pardo, Marina; Gonzalo, José
  • Advanced Materials Interfaces, Vol. 5, Issue 12
  • DOI: 10.1002/admi.201800241

Epsilon-Near-Zero Photonics: A New Platform for Integrated Devices
journal, March 2018

  • Niu, Xinxiang; Hu, Xiaoyong; Chu, Saisai
  • Advanced Optical Materials, Vol. 6, Issue 10
  • DOI: 10.1002/adom.201701292

Transient Electronic Depletion and Lattice Expansion Induced Ultrafast Bandedge Plasmons
journal, November 2019


Light-Induced Tuning and Reconfiguration of Nanophotonic Structures: Light-Induced Tuning and Reconfiguration of Nanophotonic Structures
journal, August 2017

  • Makarov, Sergey V.; Zalogina, Anastasia S.; Tajik, Mohammad
  • Laser & Photonics Reviews, Vol. 11, Issue 5
  • DOI: 10.1002/lpor.201700108

All-optical active THz metasurfaces for ultrafast polarization switching and dynamic beam splitting
journal, July 2018

  • Cong, Longqing; Srivastava, Yogesh Kumar; Zhang, Huifang
  • Light: Science & Applications, Vol. 7, Issue 1
  • DOI: 10.1038/s41377-018-0024-y

Manipulation of polarizations for broadband terahertz waves emitted from laser plasma filaments
journal, August 2018


Ultrafast and energy-efficient all-optical switching with graphene-loaded deep-subwavelength plasmonic waveguides
journal, November 2019


High-harmonic generation from an epsilon-near-zero material
journal, July 2019


Nonlinear optical effects in epsilon-near-zero media
journal, June 2019


Near-zero-index materials for photonics
journal, September 2019

  • Kinsey, Nathaniel; DeVault, Clayton; Boltasseva, Alexandra
  • Nature Reviews Materials, Vol. 4, Issue 12
  • DOI: 10.1038/s41578-019-0133-0

Excitation of epsilon-near-zero resonance in ultra-thin indium tin oxide shell embedded nanostructured optical fiber
journal, February 2018


Viscoelastic optical nonlocality of low-loss epsilon-near-zero nanofilms
journal, June 2018


Ultrafast and broadband optical nonlinearity in aluminum doped zinc oxide colloidal nanocrystals
journal, January 2019

  • Tian, Xiangling; Luo, Hongyu; Wei, Rongfei
  • Nanoscale, Vol. 11, Issue 29
  • DOI: 10.1039/c9nr04337c

Ultrafast and large optical nonlinearity of a TiSe 2 saturable absorber in the 2 μm wavelength region
journal, January 2019

  • Wei, Rongfei; Tian, Xiangling; Yang, Lupeng
  • Nanoscale, Vol. 11, Issue 46
  • DOI: 10.1039/c9nr06374a

Ultrafast active control of UV light with plasmonic resonance on aluminum nanostripes
journal, May 2018

  • Wang, Kuidong; Li, Runze; Hsiao, Hui-Hsin
  • Applied Physics Letters, Vol. 112, Issue 19
  • DOI: 10.1063/1.5027432

Complexities of atomic structure at CdO/MgO and CdO/Al 2O 3 interfaces
journal, November 2018

  • Grimley, Everett D.; Wynn, Alex P.; Kelley, Kyle P.
  • Journal of Applied Physics, Vol. 124, Issue 20
  • DOI: 10.1063/1.5053752

Multichannel remote polarization control enabled by nanostructured liquid crystalline networks
journal, May 2019

  • Zanotto, Simone; Sgrignuoli, Fabrizio; Nocentini, Sara
  • Applied Physics Letters, Vol. 114, Issue 20
  • DOI: 10.1063/1.5096648

Study of second and third harmonic generation from an indium tin oxide nanolayer: Influence of nonlocal effects and hot electrons
journal, January 2020

  • Rodríguez-Suné, L.; Scalora, M.; Johnson, A. S.
  • APL Photonics, Vol. 5, Issue 1
  • DOI: 10.1063/1.5129627

Ultra-fast transient plasmonics using transparent conductive oxides
journal, January 2018


Two-fluid hydrodynamic model for semiconductors
journal, March 2018


Ultrafast switching of optical singularity eigenstates with compact integrable liquid crystal structures
journal, January 2018

  • Liu, Yikun; Liang, Haowen; Chen, Chun-Wei
  • Optics Express, Vol. 26, Issue 22
  • DOI: 10.1364/oe.26.028818

Theoretical study of bicharacteristic waveguide for fundamental-mode phase-matched SHG from MIR to NIR
journal, January 2019

  • Huang, Tianye; Xu, Guizhen; Pan, Jianxing
  • Optics Express, Vol. 27, Issue 11
  • DOI: 10.1364/oe.27.015236

High-contrast optical switching using an epsilon-near-zero material coupled to a Bragg microcavity
journal, January 2019


All-optical active THz metasurfaces for ultrafast polarization switching and dynamic beam splitting.
text, January 2018

  • Cong, Longqing; Srivastava, Yogesh Kumar; Zhang, Huifang
  • Apollo - University of Cambridge Repository
  • DOI: 10.17863/cam.66497

Viscoelastic optical nonlocality of low-loss epsilon-near-zero nanofilms
preprint, January 2017


Two-fluid hydrodynamic model for semiconductors
text, January 2017


Generalized Brewster Angle Effect in Thin-Film Optical Absorbers and Its Application for Graphene Hydrogen Sensing
journal, June 2019


All-optical active THz metasurfaces for ultrafast polarization switching and dynamic beam splitting
journal, July 2018

  • Cong, Longqing; Srivastava, Yogesh Kumar; Zhang, Huifang
  • Light: Science & Applications, Vol. 7, Issue 1
  • DOI: 10.1038/s41377-018-0024-y

Covert infrared image encoding through imprinted plasmonic cavities
journal, November 2018

  • Franklin, Daniel; Modak, Sushrut; Vázquez-Guardado, Abraham
  • Light: Science & Applications, Vol. 7, Issue 1
  • DOI: 10.1038/s41377-018-0095-9

Optically Active Plasmonic Metasurfaces based on the Hybridization of In-Plane Coupling and Out-of-Plane Coupling
journal, May 2018


Recent Advances in Tunable and Reconfigurable Metamaterials
journal, October 2018

  • Bang, Sanghun; Kim, Jeonghyun; Yoon, Gwanho
  • Micromachines, Vol. 9, Issue 11
  • DOI: 10.3390/mi9110560