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Title: High-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses

Abstract

Electrons ejected from atoms and subsequently driven to high energies in strong laser fields enable techniques from attosecond pulse generation to imaging with rescattered electrons. Analogous processes govern strong-field electron emission from nanostructures, where long wavelength radiation and large local field enhancements hold the promise for producing electrons with substantially higher energies, allowing for higher resolution time-resolved imaging. Here we report on the use of single-cycle terahertz pulses to drive electron emission from unbiased nano-tips. Energies exceeding 5 keV are observed, substantially greater than previously attained at higher drive frequencies. Despite large differences in the magnitude of the respective local fields, we find that the maximum electron energies are only weakly dependent on the tip radius, for 10 nm<1,000 nm. As a result, due to the single-cycle nature of the field, the high-energy electron emission is predicted to be confined to a single burst, potentially enabling a variety of applications.

Authors:
 [1];  [1]
  1. Univ. of Virginia, Charlottesville, VA (United States)
Publication Date:
Research Org.:
Univ. of Virginia, Charlottesville, VA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1361204
Grant/Contract Number:  
FG02-00ER15053; SC0012462
Resource Type:
Accepted Manuscript
Journal Name:
Nature Communications
Additional Journal Information:
Journal Volume: 7; Journal ID: ISSN 2041-1723
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; 36 MATERIALS SCIENCE; applied physics; techniques and instrumentation; terahertz optics

Citation Formats

Li, Sha, and Jones, R. R. High-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses. United States: N. p., 2016. Web. doi:10.1038/ncomms13405.
Li, Sha, & Jones, R. R. High-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses. United States. https://doi.org/10.1038/ncomms13405
Li, Sha, and Jones, R. R. Thu . "High-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses". United States. https://doi.org/10.1038/ncomms13405. https://www.osti.gov/servlets/purl/1361204.
@article{osti_1361204,
title = {High-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses},
author = {Li, Sha and Jones, R. R.},
abstractNote = {Electrons ejected from atoms and subsequently driven to high energies in strong laser fields enable techniques from attosecond pulse generation to imaging with rescattered electrons. Analogous processes govern strong-field electron emission from nanostructures, where long wavelength radiation and large local field enhancements hold the promise for producing electrons with substantially higher energies, allowing for higher resolution time-resolved imaging. Here we report on the use of single-cycle terahertz pulses to drive electron emission from unbiased nano-tips. Energies exceeding 5 keV are observed, substantially greater than previously attained at higher drive frequencies. Despite large differences in the magnitude of the respective local fields, we find that the maximum electron energies are only weakly dependent on the tip radius, for 10 nm<1,000 nm. As a result, due to the single-cycle nature of the field, the high-energy electron emission is predicted to be confined to a single burst, potentially enabling a variety of applications.},
doi = {10.1038/ncomms13405},
journal = {Nature Communications},
number = ,
volume = 7,
place = {United States},
year = {Thu Nov 10 00:00:00 EST 2016},
month = {Thu Nov 10 00:00:00 EST 2016}
}

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Works referenced in this record:

Attosecond science
journal, June 2007

  • Corkum, P. B.; Krausz, Ferenc
  • Nature Physics, Vol. 3, Issue 6
  • DOI: 10.1038/nphys620

Attosecond physics
journal, February 2009


Steering Attosecond Electron Wave Packets with Light
journal, July 2002


Sub-laser-cycle electron pulses for probing molecular dynamics
journal, June 2002

  • Niikura, Hiromichi; Légaré, F.; Hasbani, R.
  • Nature, Vol. 417, Issue 6892
  • DOI: 10.1038/nature00787

Time-resolved atomic inner-shell spectroscopy
journal, October 2002

  • Drescher, M.; Hentschel, M.; Kienberger, R.
  • Nature, Vol. 419, Issue 6909
  • DOI: 10.1038/nature01143

Attosecond spectroscopy in condensed matter
journal, October 2007

  • Cavalieri, A. L.; Müller, N.; Uphues, Th.
  • Nature, Vol. 449, Issue 7165
  • DOI: 10.1038/nature06229

Delay in Photoemission
journal, June 2010


Real-time observation of valence electron motion
journal, August 2010

  • Goulielmakis, Eleftherios; Loh, Zhi-Heng; Wirth, Adrian
  • Nature, Vol. 466, Issue 7307
  • DOI: 10.1038/nature09212

Laser-Induced Electron Tunneling and Diffraction
journal, June 2008


Imaging ultrafast molecular dynamics with laser-induced electron diffraction
journal, March 2012

  • Blaga, Cosmin I.; Xu, Junliang; DiChiara, Anthony D.
  • Nature, Vol. 483, Issue 7388
  • DOI: 10.1038/nature10820

Diffraction using laser-driven broadband electron wave packets
journal, August 2014

  • Xu, Junliang; Blaga, Cosmin I.; Zhang, Kaikai
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5635

Field-driven photoemission from nanostructures quenches the quiver motion
journal, March 2012


Tip-Enhanced Strong-Field Photoemission
journal, September 2010


Localized Multiphoton Emission of Femtosecond Electron Pulses from Metal Nanotips
journal, January 2007


Attosecond control of electrons emitted from a nanoscale metal tip
journal, July 2011

  • Krüger, Michael; Schenk, Markus; Hommelhoff, Peter
  • Nature, Vol. 475, Issue 7354
  • DOI: 10.1038/nature10196

Strong-Field Above-Threshold Photoemission from Sharp Metal Tips
journal, December 2010


Attosecond physics in photoemission from a metal nanotip
journal, March 2012

  • Krüger, M.; Schenk, M.; Förster, M.
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 45, Issue 7
  • DOI: 10.1088/0953-4075/45/7/074006

Electron rescattering at metal nanotips induced by ultrashort laser pulses
journal, July 2012


Interaction of ultrashort laser pulses with metal nanotips: a model system for strong-field phenomena
journal, August 2012


Optical Control of Field-Emission Sites by Femtosecond Laser Pulses
journal, December 2009


Controlled near-field enhanced electron acceleration from dielectric nanospheres with intense few-cycle laser fields
journal, April 2011

  • Zherebtsov, Sergey; Fennel, Thomas; Plenge, Jürgen
  • Nature Physics, Vol. 7, Issue 8
  • DOI: 10.1038/nphys1983

High-harmonic generation by resonant plasmon field enhancement
journal, June 2008

  • Kim, Seungchul; Jin, Jonghan; Kim, Young-Jin
  • Nature, Vol. 453, Issue 7196
  • DOI: 10.1038/nature07012

Plasmonic generation of ultrashort extreme-ultraviolet light pulses
journal, October 2011


Extreme-ultraviolet light generation in plasmonic nanostructures
journal, March 2013

  • Sivis, M.; Duwe, M.; Abel, B.
  • Nature Physics, Vol. 9, Issue 5
  • DOI: 10.1038/nphys2590

Terahertz control of nanotip photoemission
journal, May 2014

  • Wimmer, L.; Herink, G.; Solli, D. R.
  • Nature Physics, Vol. 10, Issue 6
  • DOI: 10.1038/nphys2974

An ultrafast terahertz scanning tunnelling microscope
journal, July 2013


Basic and applied studies of field emission at microwave frequencies
journal, January 1963

  • Charbonnier, F. M.; Barbour, J. P.; Garrett, L. F.
  • Proceedings of the IEEE, Vol. 51, Issue 7
  • DOI: 10.1109/PROC.1963.2379

Field emission in a microwave field
journal, March 1995

  • Fursey, George N.
  • Journal of Vacuum Science & Technology B: Microelectronics and Nanometer Structures, Vol. 13, Issue 2
  • DOI: 10.1116/1.588354

Field emission at terahertz frequencies: AC-tunneling and ultrafast carrier dynamics
journal, December 2014


Ultrafast low-energy electron diffraction in transmission resolves polymer/graphene superstructure dynamics
journal, July 2014


The effects of a static electric field on high-order harmonic generation
journal, May 1998

  • Wang, Bingbing; Li, Xiaofeng; Fu, Panming
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 31, Issue 9
  • DOI: 10.1088/0953-4075/31/9/012

Electron Emission in Intense Electric Fields
journal, May 1928

  • Fowler, R. H.; Nordheim, L.
  • Proceedings of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 119, Issue 781
  • DOI: 10.1098/rspa.1928.0091

Probing of Optical Near-Fields by Electron Rescattering on the 1 nm Scale
journal, September 2013

  • Thomas, Sebastian; Krüger, Michael; Förster, Michael
  • Nano Letters, Vol. 13, Issue 10
  • DOI: 10.1021/nl402407r

Electric Field Enhancement Factors Around a Metallic, End-Capped Cylinder
journal, July 2006


Large optical field enhancement for nanotips with large opening angles
journal, June 2015

  • Thomas, Sebastian; Wachter, Georg; Lemell, Christoph
  • New Journal of Physics, Vol. 17, Issue 6, Article No. 063010
  • DOI: 10.1088/1367-2630/17/6/063010

Tip-based source of femtosecond electron pulses at 30 keV
journal, March 2014

  • Hoffrogge, Johannes; Paul Stein, Jan; Krüger, Michael
  • Journal of Applied Physics, Vol. 115, Issue 9
  • DOI: 10.1063/1.4867185

Terahertz-driven linear electron acceleration
journal, October 2015

  • Nanni, Emilio A.; Huang, Wenqian R.; Hong, Kyung-Han
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms9486

Generation of high-power terahertz pulses by tilted-pulse-front excitation and their application possibilities
journal, January 2008

  • Hebling, János; Yeh, Ka-Lo; Hoffmann, Matthias C.
  • Journal of the Optical Society of America B, Vol. 25, Issue 7
  • DOI: 10.1364/JOSAB.25.0000B6

Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3
journal, February 2011

  • Hirori, H.; Doi, A.; Blanchard, F.
  • Applied Physics Letters, Vol. 98, Issue 9
  • DOI: 10.1063/1.3560062

Single-shot terahertz-field-driven X-ray streak camera
journal, August 2009


Applications of electrostatic capacitance and charging
journal, December 2013

  • Sandu, Titus; Boldeiu, George; Moagar-Poladian, Victor
  • Journal of Applied Physics, Vol. 114, Issue 22
  • DOI: 10.1063/1.4847495

Time-resolved atomic inner-shell spectroscopy
journal, October 2002

  • Drescher, M.; Hentschel, M.; Kienberger, R.
  • Nature, Vol. 419, Issue 6909
  • DOI: 10.1038/nature01143

Attosecond spectroscopy in condensed matter
journal, October 2007

  • Cavalieri, A. L.; Müller, N.; Uphues, Th.
  • Nature, Vol. 449, Issue 7165
  • DOI: 10.1038/nature06229

Field-driven photoemission from nanostructures quenches the quiver motion
journal, March 2012


Static-electric-field effects on high harmonic generation
journal, June 1996


Laser-Photofield Emission from Needle Cathodes for Low-Emittance Electron Beams
journal, February 2008


Local Capacitor Model for Plasmonic Electric Field Enhancement
journal, March 2009


Energy Distribution Curves of Ultrafast Laser-Induced Field Emission and Their Implications for Electron Dynamics
journal, August 2011


Strong Field Acceleration and Steering of Ultrafast Electron Pulses from a Sharp Metallic Nanotip
journal, December 2012


Ionization of Excited Atoms by Intense Single-Cycle THz Pulses
journal, April 2014


Field Emission Tip as a Nanometer Source of Free Electron Femtosecond Pulses
journal, February 2006


Ultrafast Electron Pulses from a Tungsten Tip Triggered by Low-Power Femtosecond Laser Pulses
journal, December 2006


Strong-field above-threshold photoemission from sharp metal tips
conference, May 2011

  • Schenk, M.; Kruger, M.; Hommelhoff, P.
  • 12th European Quantum Electronics Conference CLEO EUROPE/EQEC, 2011 Conference on Lasers and Electro-Optics Europe and 12th European Quantum Electronics Conference (CLEO EUROPE/EQEC)
  • DOI: 10.1109/cleoe.2011.5943576

Steering Attosecond Electron Wave Packets with Light
journal, July 2002


Laser-Induced Electron Tunneling and Diffraction
journal, June 2008


Nitrogen plasma formation through terahertz-induced ultrafast electron field emission
journal, January 2015

  • Iwaszczuk, Krzysztof; Zalkovskij, Maksim; Strikwerda, Andrew C.
  • Optica, Vol. 2, Issue 2
  • DOI: 10.1364/optica.2.000116

Optical Control of Field-Emission Sites by Femtosecond Laser Pulses
text, January 2009


Probing of optical near-fields by electron rescattering on the 1 nm scale
text, January 2012


Large optical field enhancement for nanotips with large opening angles
text, January 2014


Works referencing / citing this record:

Laser‐Driven Strong‐Field Terahertz Sources
journal, September 2019

  • Fülöp, József András; Tzortzakis, Stelios; Kampfrath, Tobias
  • Advanced Optical Materials, Vol. 8, Issue 3
  • DOI: 10.1002/adom.201900681

Ultrafast terahertz control of extreme tunnel currents through single atoms on a silicon surface
journal, February 2017

  • Jelic, Vedran; Iwaszczuk, Krzysztof; Nguyen, Peter H.
  • Nature Physics, Vol. 13, Issue 6
  • DOI: 10.1038/nphys4047

Sub-cycle dynamics in relativistic nanoplasma acceleration
journal, May 2019


Plasmon-induced nonlinear response of silver atomic chains
journal, January 2018

  • Yan, Lei; Guan, Mengxue; Meng, Sheng
  • Nanoscale, Vol. 10, Issue 18
  • DOI: 10.1039/c8nr02086h

Quantized conductance observed during sintering of silver nanoparticles by intense terahertz pulses
journal, April 2018

  • Takano, Keisuke; Harada, Hirofumi; Yoshimura, Masashi
  • Applied Physics Letters, Vol. 112, Issue 16
  • DOI: 10.1063/1.5022706

Attosecond physics phenomena at nanometric tips
journal, August 2018

  • Krüger, Michael; Lemell, Christoph; Wachter, Georg
  • Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 51, Issue 17
  • DOI: 10.1088/1361-6455/aac6ac

Subcycle mid-infrared coherent transients at 4  MHz repetition rate applicable to light-wave-driven scanning tunneling microscopy
journal, January 2019

  • Yoshioka, Katsumasa; Igarashi, Ippo; Yoshida, Shoji
  • Optics Letters, Vol. 44, Issue 21
  • DOI: 10.1364/ol.44.005350

Segmented terahertz electron accelerator and manipulator (STEAM)
text, January 2018

  • Zhang, Dongfang; Fallahi, Arya; Hemmer, Michael
  • Deutsches Elektronen-Synchrotron, DESY, Hamburg
  • DOI: 10.3204/pubdb-2018-01613

Segmented terahertz electron accelerator and manipulator (STEAM)
journal, April 2018


Laser‐driven strong‐field Terahertz sources
text, January 2019

  • Fülöp, József András; Tzortzakis, Stelios; Kampfrath, Tobias
  • Freie Universität Berlin
  • DOI: 10.17169/refubium-26582

Segmented Terahertz Electron Accelerator and Manipulator (STEAM)
text, January 2017