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Title: Magnetic switching in granular FePt layers promoted by near-field laser enhancement

Light-matter interaction at the nanoscale in magnetic materials is a topic of intense research in view of potential applications in next-generation high-density magnetic recording. Laser-assisted switching provides a pathway for overcoming the material constraints of high-anisotropy and high-packing density media, though much about the dynamics of the switching process remains unexplored. We use ultrafast small-angle X-ray scattering at an X-ray free-electron laser to probe the magnetic switching dynamics of FePt nanoparticles embedded in a carbon matrix following excitation by an optical femtosecond laser pulse. We observe that the combination of laser excitation and applied static magnetic field, 1 order of magnitude smaller than the coercive field, can overcome the magnetic anisotropy barrier between “up” and “down” magnetization, enabling magnetization switching. This magnetic switching is found to be inhomogeneous throughout the material with some individual FePt nanoparticles neither switching nor demagnetizing. The origin of this behavior is identified as the near-field modification of the incident laser radiation around FePt nanoparticles. Furthermore, the fraction of not-switching nanoparticles is influenced by the heat flow between FePt and a heat-sink layer.
Authors:
 [1] ; ORCiD logo [2] ;  [3] ;  [4] ;  [5] ;  [5] ;  [5] ;  [5] ;  [2] ;  [2] ;  [2] ;  [2] ;  [2] ;  [6] ;  [7] ;  [7] ;  [8] ;  [8] ;  [9] ;  [9] more »;  [10] ;  [2] ;  [2] ;  [2] « less
  1. SLAC National Accelerator Lab., Menlo Park, CA (United States); Univ. of Amsterdam, Amsterdam (The Netherlands)
  2. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States); European XFEL GmbH, Schenefeld (Germany)
  4. Eidgenossische Technische Hochschule (ETH) Zurich, Zurich (Switzerland)
  5. SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States)
  6. Temple Univ., Philadelphia, PA (United States)
  7. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  8. HGST a Western Digital Co., San Jose, CA (United States)
  9. National Institute for Materials Science, Tsukuba (Japan)
  10. Univ. of California San Diego, La Jolla, CA (United States)
Publication Date:
Grant/Contract Number:
AC02-05CH11231; AC02-76SF00515; MURI
Type:
Accepted Manuscript
Journal Name:
Nano Letters
Additional Journal Information:
Journal Volume: 17; Journal Issue: 4; Journal ID: ISSN 1530-6984
Publisher:
American Chemical Society
Research Org:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; FePt; magnetic switching; pump−probe; ultrafast magnetism; X-ray scattering
OSTI Identifier:
1361059