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Title: 2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications

Abstract

The rise of two-dimensional (2D) materials research took place following the isolation of graphene in 2004. These new 2D materials include transition metal dichalcogenides, mono-elemental 2D sheets, and several carbide- and nitride-based materials. The number of publications related to these emerging materials has been drastically increasing over the last five years. Thus, through this comprehensive review, we aim to discuss the most recent groundbreaking discoveries as well as emerging opportunities and remaining challenges. This review starts out by delving into the improved methods of producing these new 2D materials via controlled exfoliation, metal organic chemical vapor deposition, and wet chemical means. We look into recent studies of doping as well as the optical properties of 2D materials and their heterostructures. Recent advances towards applications of these materials in 2D electronics are also reviewed, and include the tunnel MOSFET and ways to reduce the contact resistance for fabricating high-quality devices. Finally, several unique and innovative applications recently explored are discussed as well as perspectives of this exciting and fast moving field.

Authors:
 [1];  [1];  [2];  [2];  [2];  [3];  [4];  [5];  [6];  [7];  [8];  [9];  [10];  [11];  [4]; ORCiD logo [12];  [13];  [14];  [15];  [16] more »;  [3];  [17];  [18];  [19];  [20] « less
  1. Pennsylvania State Univ., University Park, PA (United States). Dept of Physics; Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials
  2. Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Materials Sciences and Engineering
  3. Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Chemistry
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Science (CNMS)
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Foundry
  6. Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
  7. Univ. of Pittsburgh, PA (United States). Dept. of Chemical and Petroleum Engineering
  8. Univ. of Regensburg (Germany). Inst. fur Experimentelle und Angewandte Physik; Columbia Univ., New York, NY (United States). Dept. of Physics and Electrical Engineering
  9. Univ. of Kansas, Lawrence, KS (United States). Dept. of Physics and Astronomy
  10. Univ. of Virginia, Charlottesville, VA (United States). Dept. of Materials Science and Engineering
  11. Stanford Univ., CA (United States). Dept. of Materials Science and Engineering; SLAC National Accelerator Lab., Menlo Park, CA (United States)
  12. Univ. of Arizona, Tucson, AZ (United States). Dept. of Physics
  13. Univ. of Pennsylvania, Philadelphia, PA (United States). Dept. of Physics and Astronomy
  14. Lehigh Univ., Bethlehem, PA (United States). Dept. of Electrical and Computer Engineering
  15. Univ. of Chicago, IL (United States). Dept. of Chemistry and Inst. of Molecular Engineering
  16. Rutgers Univ., Piscataway, NJ (United States). Dept. of Materials Science and Engineering; Rutgers Univ., Piscataway, NJ (United States). Dept. of Electrical and Computer Engineering
  17. Univ. of California, Berkeley, CA (United States). Dept. of Electrical Engineering and Computer Sciences; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
  18. Northwestern Univ., Evanston, IL (United States). Dept. of Materials Science and Engineering; Northwestern Univ., Evanston, IL (United States). Dept of Chemistry
  19. Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Materials Sciences and Engineering; Pennsylvania State Univ., University Park, PA (United States). Center for Atomically Thin Multifunctional Coatings (ATOMIC)
  20. Pennsylvania State Univ., University Park, PA (United States). Dept of Physics; Pennsylvania State Univ., University Park, PA (United States). Center for 2-Dimensional and Layered Materials; Pennsylvania State Univ., University Park, PA (United States). Dept of Materials Sciences and Engineering; Pennsylvania State Univ., University Park, PA (United States). Dept of Chemistry; Pennsylvania State Univ., University Park, PA (United States). Center for Atomically Thin Multifunctional Coatings (ATOMIC)
Publication Date:
Research Org.:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1360213
Alternate Identifier(s):
OSTI ID: 1468337
Grant/Contract Number:  
AC02-76SF00515; AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
2D Materials
Additional Journal Information:
Journal Volume: 3; Journal Issue: 4; Journal ID: ISSN 2053-1583
Publisher:
IOP Publishing
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE

Citation Formats

Lin, Zhong, McCreary, Amber, Briggs, Natalie, Subramanian, Shruti, Zhang, Kehao, Sun, Yifan, Li, Xufan, Borys, Nicholas J., Yuan, Hongtao, Fullerton-Shirey, Susan K., Chernikov, Alexey, Zhao, Hui, McDonnell, Stephen, Lindenberg, Aaron M., Xiao, Kai, LeRoy, Brian J., Drndić, Marija, Hwang, James C. M., Park, Jiwoong, Chhowalla, Manish, Schaak, Raymond E., Javey, Ali, Hersam, Mark C., Robinson, Joshua, and Terrones, Mauricio. 2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications. United States: N. p., 2016. Web. doi:10.1088/2053-1583/3/4/042001.
Lin, Zhong, McCreary, Amber, Briggs, Natalie, Subramanian, Shruti, Zhang, Kehao, Sun, Yifan, Li, Xufan, Borys, Nicholas J., Yuan, Hongtao, Fullerton-Shirey, Susan K., Chernikov, Alexey, Zhao, Hui, McDonnell, Stephen, Lindenberg, Aaron M., Xiao, Kai, LeRoy, Brian J., Drndić, Marija, Hwang, James C. M., Park, Jiwoong, Chhowalla, Manish, Schaak, Raymond E., Javey, Ali, Hersam, Mark C., Robinson, Joshua, & Terrones, Mauricio. 2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications. United States. https://doi.org/10.1088/2053-1583/3/4/042001
Lin, Zhong, McCreary, Amber, Briggs, Natalie, Subramanian, Shruti, Zhang, Kehao, Sun, Yifan, Li, Xufan, Borys, Nicholas J., Yuan, Hongtao, Fullerton-Shirey, Susan K., Chernikov, Alexey, Zhao, Hui, McDonnell, Stephen, Lindenberg, Aaron M., Xiao, Kai, LeRoy, Brian J., Drndić, Marija, Hwang, James C. M., Park, Jiwoong, Chhowalla, Manish, Schaak, Raymond E., Javey, Ali, Hersam, Mark C., Robinson, Joshua, and Terrones, Mauricio. Thu . "2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications". United States. https://doi.org/10.1088/2053-1583/3/4/042001. https://www.osti.gov/servlets/purl/1360213.
@article{osti_1360213,
title = {2D materials advances: from large scale synthesis and controlled heterostructures to improved characterization techniques, defects and applications},
author = {Lin, Zhong and McCreary, Amber and Briggs, Natalie and Subramanian, Shruti and Zhang, Kehao and Sun, Yifan and Li, Xufan and Borys, Nicholas J. and Yuan, Hongtao and Fullerton-Shirey, Susan K. and Chernikov, Alexey and Zhao, Hui and McDonnell, Stephen and Lindenberg, Aaron M. and Xiao, Kai and LeRoy, Brian J. and Drndić, Marija and Hwang, James C. M. and Park, Jiwoong and Chhowalla, Manish and Schaak, Raymond E. and Javey, Ali and Hersam, Mark C. and Robinson, Joshua and Terrones, Mauricio},
abstractNote = {The rise of two-dimensional (2D) materials research took place following the isolation of graphene in 2004. These new 2D materials include transition metal dichalcogenides, mono-elemental 2D sheets, and several carbide- and nitride-based materials. The number of publications related to these emerging materials has been drastically increasing over the last five years. Thus, through this comprehensive review, we aim to discuss the most recent groundbreaking discoveries as well as emerging opportunities and remaining challenges. This review starts out by delving into the improved methods of producing these new 2D materials via controlled exfoliation, metal organic chemical vapor deposition, and wet chemical means. We look into recent studies of doping as well as the optical properties of 2D materials and their heterostructures. Recent advances towards applications of these materials in 2D electronics are also reviewed, and include the tunnel MOSFET and ways to reduce the contact resistance for fabricating high-quality devices. Finally, several unique and innovative applications recently explored are discussed as well as perspectives of this exciting and fast moving field.},
doi = {10.1088/2053-1583/3/4/042001},
journal = {2D Materials},
number = 4,
volume = 3,
place = {United States},
year = {Thu Dec 08 00:00:00 EST 2016},
month = {Thu Dec 08 00:00:00 EST 2016}
}

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Observation of charge transfer in mixed-dimensional heterostructures formed by transition metal dichalcogenide monolayers and PbS quantum dots
journal, December 2019

  • Zereshki, Peymon; Tavakoli, Mohammad Mahdi; Valencia-Acuna, Pavel
  • Physical Review B, Vol. 100, Issue 23
  • DOI: 10.1103/physrevb.100.235411

Nanoreinforcements of Two-Dimensional Nanomaterials for Flame Retardant Polymeric Composites: An Overview
journal, December 2019

  • Lu, Shaolin; Hong, Wei; Chen, Xudong
  • Advances in Polymer Technology, Vol. 2019
  • DOI: 10.1155/2019/4273253

Optical Properties and Photocarrier Dynamics of Bi 2 O 2 Se Monolayer and Nanoplates
journal, March 2020

  • Liu, Shuangyan; Tan, Congwei; He, Dawei
  • Advanced Optical Materials, Vol. 8, Issue 6
  • DOI: 10.1002/adom.201901567

Batch production of 6-inch uniform monolayer molybdenum disulfide catalyzed by sodium in glass
journal, March 2018


Electrostatically driven scalable synthesis of MoS 2 –graphene hybrid films assisted by hydrophobins
journal, January 2017

  • Kaur, Jasneet; Vergara, Alessandro; Rossi, Manuela
  • RSC Adv., Vol. 7, Issue 79
  • DOI: 10.1039/c7ra09878b

Wafer-recyclable, environment-friendly transfer printing for large-scale thin-film nanoelectronics
journal, July 2018

  • Wie, Dae Seung; Zhang, Yue; Kim, Min Ku
  • Proceedings of the National Academy of Sciences, Vol. 115, Issue 31
  • DOI: 10.1073/pnas.1806640115

The Role of Graphene and Other 2D Materials in Solar Photovoltaics
journal, September 2018


Temperature‐induced phonon behavior in titanium disulfide (TiS 2 ) nanosheets
journal, May 2019

  • Dużyńska, A.; Judek, J.; Wilczyński, K.
  • Journal of Raman Spectroscopy, Vol. 50, Issue 8
  • DOI: 10.1002/jrs.5637

Centimeter-scale Green Integration of Layer-by-Layer 2D TMD vdW Heterostructures on Arbitrary Substrates by Water-Assisted Layer Transfer
journal, February 2019


CMOS-compatible batch processing of monolayer MoS 2 MOSFETs
journal, March 2018

  • Xiong, Kuanchen; Kim, Hyun; Marstell, Roderick J.
  • Journal of Physics D: Applied Physics, Vol. 51, Issue 15
  • DOI: 10.1088/1361-6463/aab4ba

Mobility and Decay Dynamics of Charge Carriers in One-Dimensional Selenium van der Waals Solid
journal, August 2017

  • Bhaskar, Prashant; Achtstein, Alexander W.; Diedenhofen, Silke L.
  • The Journal of Physical Chemistry C, Vol. 121, Issue 34
  • DOI: 10.1021/acs.jpcc.7b05183

Charge Mobility and Recombination Mechanisms in Tellurium van der Waals Solid
journal, December 2018

  • Bhaskar, Prashant; Achtstein, Alexander W.; Vermeulen, Martien J. W.
  • The Journal of Physical Chemistry C, Vol. 123, Issue 1
  • DOI: 10.1021/acs.jpcc.8b09665

Probing Exfoliated Graphene Layers and Their Lithiation with Microfocused X-rays
journal, May 2019


Batch production of 6-inch uniform monolayer molybdenum disulfide catalyzed by sodium in glass
journal, March 2018


Fabrication of Subnanometer-Precision Nanopores in Hexagonal Boron Nitride
journal, November 2017


Growth of ‘W’ doped molybdenum disulfide on graphene transferred molybdenum substrate
journal, May 2018


Centimeter-scale Green Integration of Layer-by-Layer 2D TMD vdW Heterostructures on Arbitrary Substrates by Water-Assisted Layer Transfer
journal, February 2019


Review Article: Progress in fabrication of transition metal dichalcogenides heterostructure systems
journal, May 2017

  • Dong, Rui; Kuljanishvili, Irma
  • Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 35, Issue 3
  • DOI: 10.1116/1.4982736

Transport and Field Emission Properties of MoS2 Bilayers
journal, March 2018

  • Urban, Francesca; Passacantando, Maurizio; Giubileo, Filippo
  • Nanomaterials, Vol. 8, Issue 3
  • DOI: 10.3390/nano8030151

Feasible Route for a Large Area Few-Layer MoS2 with Magnetron Sputtering
journal, August 2018


Electronic and Optical Properties of Two-Dimensional Tellurene: From First-Principles Calculations
journal, July 2019


Defect Engineering in 2D Materials: Precise Manipulation and Improved Functionalities
journal, December 2019