Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by Fe impurities [Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by modest Fe substitution]

Zhu, M.; Wang, Y.; Li, P. G.; Ge, J. J.; Tian, W.; Keavney, D.; Mao, Z. Q.; Ke, X.

doi:10.1103/PhysRevB.95.174430

Title: Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by Fe impurities [Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by modest Fe substitution]

Abstract

We report the magnetic and electronic properties of the bilayer ruthenate Sr₃Ru₂O₇ upon Fe substitution for Ru. We find that Sr₃(Ru_1-xFe_x)₂O₇ shows spin-glass-like phase below 4 K for x = 0.01 and commensurate E-type antiferromagnetically ordered insulating ground state characterized by the propagation vector q_c = (0.25 0.25 0) for x ≥ 0.03, in contrast to the paramagnetic metallic state in the parent compound with strong spin fluctuations occurring at wave vectors q = (0.09 0 0) and (0.25 0 0). The observed antiferromagnetic ordering is quasitwo-dimensional with very short correlation length along the c axis, a feature similar to the Mndoped Sr₃Ru₂O₇. Lastly, our results suggest that this ordered ground state is associated with the intrinsic magnetic instability in the pristine compound, which can be readily tipped by the local magnetic coupling between the 3d orbitals of the magnetic dopants and Ru 4d orbitals.

Authors:

Zhu, M. ^[1]; Wang, Y. ^[2]; Li, P. G. ^[2]; Ge, J. J. ^[2]; Tian, W. ^[3]; Keavney, D. ^[4]; Mao, Z. Q. ^[2]; Ke, X. ^[1]

Michigan State Univ., East Lansing, MI (United States)
Tulane Univ., New Orleans, LA (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

Publication Date:: Fri May 19 00:00:00 EDT 2017

Research Org.:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Org.:: National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22), Experimental Program to Stimulate Competitive Research (EPSCoR); USDOE

OSTI Identifier:: 1363902

Alternate Identifier(s):: OSTI ID: 1357936

Grant/Contract Number:: AC02-06CH11357; SC0012432

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 95; Journal Issue: 17; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Zhu, M., Wang, Y., Li, P. G., Ge, J. J., Tian, W., Keavney, D., Mao, Z. Q., and Ke, X. Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by Fe impurities [Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by modest Fe substitution].  United States: N. p., 2017. 
Web.  doi:10.1103/PhysRevB.95.174430.

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                    Zhu, M., Wang, Y., Li, P. G., Ge, J. J., Tian, W., Keavney, D., Mao, Z. Q., & Ke, X. Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by Fe impurities [Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by modest Fe substitution].  United States.  https://doi.org/10.1103/PhysRevB.95.174430

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                    Zhu, M., Wang, Y., Li, P. G., Ge, J. J., Tian, W., Keavney, D., Mao, Z. Q., and Ke, X. Fri .  
"Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by Fe impurities [Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by modest Fe substitution]".  United States.  https://doi.org/10.1103/PhysRevB.95.174430.  https://www.osti.gov/servlets/purl/1363902.

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@article{osti_1363902,

  title        = {Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by Fe impurities [Tipping the magnetic instability in paramagnetic Sr3Ru2O7 by modest Fe substitution]},

  author       = {Zhu, M. and Wang, Y. and Li, P. G. and Ge, J. J. and Tian, W. and Keavney, D. and Mao, Z. Q. and Ke, X.},

  abstractNote = {We report the magnetic and electronic properties of the bilayer ruthenate Sr3Ru2O7 upon Fe substitution for Ru. We find that Sr3(Ru1-xFex)2O7 shows spin-glass-like phase below 4 K for x = 0.01 and commensurate E-type antiferromagnetically ordered insulating ground state characterized by the propagation vector qc = (0.25 0.25 0) for x ≥ 0.03, in contrast to the paramagnetic metallic state in the parent compound with strong spin fluctuations occurring at wave vectors q = (0.09 0 0) and (0.25 0 0). The observed antiferromagnetic ordering is quasitwo-dimensional with very short correlation length along the c axis, a feature similar to the Mndoped Sr3Ru2O7. Lastly, our results suggest that this ordered ground state is associated with the intrinsic magnetic instability in the pristine compound, which can be readily tipped by the local magnetic coupling between the 3d orbitals of the magnetic dopants and Ru 4d orbitals.},

  doi          = {10.1103/PhysRevB.95.174430},

  journal      = {Physical Review B},

  number       = 17,

  volume       = 95,

  place        = {United States},

  year         = {Fri May 19 00:00:00 EDT 2017},

  month        = {Fri May 19 00:00:00 EDT 2017}

}

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Title: Tipping the magnetic instability in paramagnetic S r 3 R u 2 O 7 by Fe impurities [Tipping the magnetic instability in paramagnetic S r 3 R u 2 O 7 by modest Fe substitution]

Abstract

Citation Formats

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Layered Ruthenium Oxides: From Band Metal to Mott Insulator journal, September 1998

Structure-property coupling in Sr 3 (Ru 1 − x Mn x ) 2 O 7 journal, November 2011

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Observation of a Metallic Antiferromagnetic Phase and Metal to Nonmetal Transition in Ca 3 Ru 2 O 7 journal, March 1997

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Competition Between Antiferromagnetism and Ferromagnetism in Sr2RuO4 Probed by Mn and Co Doping journal, October 2013

Spin-Orbital Order Modified by Orbital Dilution in Transition-Metal Oxides: From Spin Defects to Frustrated Spins Polarizing Host Orbitals journal, March 2015

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Title: Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by Fe impurities [Tipping the magnetic instability in paramagnetic $S r_{3} R u_{2} O_{7}$ by modest Fe substitution]

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journal, April 2017

Complexity in Strongly Correlated Electronic Systems
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Symmetry-Based Computational Tools for Magnetic Crystallography
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Revised effective ionic radii and systematic studies of interatomic distances in halides and chalcogenides
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journal, July 2008

Recent advances in magnetic structure determination by neutron powder diffraction
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Single-bilayer $E$ -type antiferromagnetism in Mn-substituted Sr $_{3}$ Ru $_{2}$ O $_{7}$ : Neutron scattering study
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Magnetic phase diagram of ${Ca}_{2 - x} {Sr}_{x} {RuO}_{4}$ governed by structural distortions
journal, June 2001

Ground state in ${Sr}_{3} {Ru}_{2} O_{7} :$ Fermi liquid close to a ferromagnetic instability
journal, September 2000

Evidence for Incommensurate Spin Fluctuations in ${Sr}_{2} {RuO}_{4}$
journal, October 1999

Strongly Correlated Electronic Materials: Present and Future
journal, November 2008

The physics of manganites: Structure and transport
journal, August 2001

Metamagnetic Quantum Criticality Revealed by ${}^{17}O − NMR$ in the Itinerant Metamagnet ${Sr}_{3} {Ru}_{2} O_{7}$
journal, September 2005

Spin Valve Effect and Magnetoresistivity in Single Crystalline ${Ca}_{3} {Ru}_{2} O_{7}$
journal, June 2008

Magnetoelectric Hexaferrites
journal, March 2012

Multiferroics: a magnetic twist for ferroelectricity
journal, January 2007

Doping a Mott insulator: Physics of high-temperature superconductivity
journal, January 2006

Field-tunable spin-density-wave phases in Sr3Ru2O7
journal, January 2015

Observation of two-dimensional spin fluctuations in the bilayer ruthenate ${Sr}_{3} {Ru}_{2} O_{7}$ by inelastic neutron scattering
journal, January 2003

Commensurate-incommensurate magnetic phase transition in the Fe-doped bilayer ruthenate ${Ca}_{3} {Ru}_{2} O_{7}$
journal, June 2014

The superconductivity of ${Sr}_{2} {RuO}_{4}$ and the physics of spin-triplet pairing
journal, May 2003

Observation of a Metallic Antiferromagnetic Phase and Metal to Nonmetal Transition in ${Ca}_{3} {Ru}_{2} O_{7}$
journal, March 1997

Magnetic ordering in ${Sr}_{2} {RuO}_{4}$ induced by nonmagnetic impurities
journal, April 2001

Competition Between Antiferromagnetism and Ferromagnetism in Sr2RuO4 Probed by Mn and Co Doping
journal, October 2013

Spin-Orbital Order Modified by Orbital Dilution in Transition-Metal Oxides: From Spin Defects to Frustrated Spins Polarizing Host Orbitals
journal, March 2015

Formation of a Nematic Fluid at High Fields in Sr3Ru2O7
journal, January 2007

Origins of colossal magnetoresistance in perovskite-type manganese oxides (invited)
journal, January 1996

Magnetic Field-Tuned Quantum Criticality in the Metallic Ruthenate Sr3Ru2O7
journal, October 2001

Emergent electronic and magnetic state in Ca $_{3}$ Ru $_{2}$ O $_{7}$ induced by Ti doping
journal, November 2011

Incommensurate magnetic ordering in Ti-doped ${Sr}_{3} {Ru}_{2} O_{7}$
journal, February 2009

Impurity-induced transition to a Mott insulator in ${Sr}_{3} {Ru}_{2} O_{7}$
journal, September 2005