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Title: Study of aluminum particle combustion in solid propellant plumes using digital in-line holography and imaging pyrometry

Abstract

The combustion of molten metals is an important area of study with applications ranging from solid aluminized rocket propellants to fireworks displays. Our work uses digital in-line holography (DIH) to experimentally quantify the three-dimensional position, size, and velocity of aluminum particles during combustion of ammonium perchlorate (AP) based solid-rocket propellants. Additionally, spatially resolved particle temperatures are simultaneously measured using two-color imaging pyrometry. To allow for fast characterization of the properties of tens of thousands of particles, automated data processing routines are proposed. In using these methods, statistics from aluminum particles with diameters ranging from 15 to 900 µm are collected at an ambient pressure of 83 kPa. In the first set of DIH experiments, increasing initial propellant temperature is shown to enhance the agglomeration of nascent aluminum at the burning surface, resulting in ejection of large molten aluminum particles into the exhaust plume. The resulting particle number and volume distributions are quantified. In the second set of simultaneous DIH and pyrometry experiments, particle size and velocity relationships as well as temperature statistics are explored. The average measured temperatures are found to be 2640 ± 282 K, which compares well with previous estimates of the range of particle and gas-phase temperatures.more » The novel methods proposed here represent new capabilities for simultaneous quantification of the joint size, velocity, and temperature statistics during the combustion of molten metal particles. The proposed techniques are expected to be useful for detailed performance assessment of metalized solid-rocket propellants.« less

Authors:
ORCiD logo [1];  [1];  [1];  [1];  [1];  [1];  [2]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Naval Air Warfare Center Weapons Division, China Lake, CA (United States)
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA); California Inst. of Technology
OSTI Identifier:
1356857
Alternate Identifier(s):
OSTI ID: 1413352
Report Number(s):
SAND2017-4477J
Journal ID: ISSN 0010-2180; PII: S0010218017301505
Grant/Contract Number:  
AC04-94AL85000
Resource Type:
Accepted Manuscript
Journal Name:
Combustion and Flame
Additional Journal Information:
Journal Volume: 182; Journal Issue: C; Journal ID: ISSN 0010-2180
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Aluminum particle combustion; Ammonium perchlorate; Metalized solid propellant; Digital in-line holography; Imaging pyrometer

Citation Formats

Chen, Yi, Guildenbecher, Daniel R., Hoffmeister, Kathryn N. G., Cooper, Marcia A., Stauffacher, Howard L., Oliver, Michael S., and Washburn, Ephraim B.. Study of aluminum particle combustion in solid propellant plumes using digital in-line holography and imaging pyrometry. United States: N. p., 2017. Web. https://doi.org/10.1016/j.combustflame.2017.04.016.
Chen, Yi, Guildenbecher, Daniel R., Hoffmeister, Kathryn N. G., Cooper, Marcia A., Stauffacher, Howard L., Oliver, Michael S., & Washburn, Ephraim B.. Study of aluminum particle combustion in solid propellant plumes using digital in-line holography and imaging pyrometry. United States. https://doi.org/10.1016/j.combustflame.2017.04.016
Chen, Yi, Guildenbecher, Daniel R., Hoffmeister, Kathryn N. G., Cooper, Marcia A., Stauffacher, Howard L., Oliver, Michael S., and Washburn, Ephraim B.. Fri . "Study of aluminum particle combustion in solid propellant plumes using digital in-line holography and imaging pyrometry". United States. https://doi.org/10.1016/j.combustflame.2017.04.016. https://www.osti.gov/servlets/purl/1356857.
@article{osti_1356857,
title = {Study of aluminum particle combustion in solid propellant plumes using digital in-line holography and imaging pyrometry},
author = {Chen, Yi and Guildenbecher, Daniel R. and Hoffmeister, Kathryn N. G. and Cooper, Marcia A. and Stauffacher, Howard L. and Oliver, Michael S. and Washburn, Ephraim B.},
abstractNote = {The combustion of molten metals is an important area of study with applications ranging from solid aluminized rocket propellants to fireworks displays. Our work uses digital in-line holography (DIH) to experimentally quantify the three-dimensional position, size, and velocity of aluminum particles during combustion of ammonium perchlorate (AP) based solid-rocket propellants. Additionally, spatially resolved particle temperatures are simultaneously measured using two-color imaging pyrometry. To allow for fast characterization of the properties of tens of thousands of particles, automated data processing routines are proposed. In using these methods, statistics from aluminum particles with diameters ranging from 15 to 900 µm are collected at an ambient pressure of 83 kPa. In the first set of DIH experiments, increasing initial propellant temperature is shown to enhance the agglomeration of nascent aluminum at the burning surface, resulting in ejection of large molten aluminum particles into the exhaust plume. The resulting particle number and volume distributions are quantified. In the second set of simultaneous DIH and pyrometry experiments, particle size and velocity relationships as well as temperature statistics are explored. The average measured temperatures are found to be 2640 ± 282 K, which compares well with previous estimates of the range of particle and gas-phase temperatures. The novel methods proposed here represent new capabilities for simultaneous quantification of the joint size, velocity, and temperature statistics during the combustion of molten metal particles. The proposed techniques are expected to be useful for detailed performance assessment of metalized solid-rocket propellants.},
doi = {10.1016/j.combustflame.2017.04.016},
journal = {Combustion and Flame},
number = C,
volume = 182,
place = {United States},
year = {2017},
month = {5}
}

Journal Article:

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Cited by: 39 works
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Works referenced in this record:

Burning Aluminum Particles Inside a Laboratory-Scale Solid Rocket Motor
journal, May 2002

  • Melcher, John C.; Krier, Herman; Burton, Rodney L.
  • Journal of Propulsion and Power, Vol. 18, Issue 3
  • DOI: 10.2514/2.5977

Numerical Simulation of Single Aluminum Particle Combustion (Review)
journal, November 2005

  • Beckstead, M. W.; Liang, Y.; Pudduppakkam, K. V.
  • Combustion, Explosion, and Shock Waves, Vol. 41, Issue 6
  • DOI: 10.1007/s10573-005-0077-0

Aluminum agglomeration reduction in a composite propellant using tailored Al/PTFE particles
journal, January 2014


Metal particle combustion and nanotechnology
journal, January 2009

  • Yetter, Richard A.; Risha, Grant A.; Son, Steven F.
  • Proceedings of the Combustion Institute, Vol. 32, Issue 2
  • DOI: 10.1016/j.proci.2008.08.013

Experimental study of stages in aluminium particle combustion in air
journal, June 1996


PLIF species and ratiometric temperature measurements of aluminum particle combustion in O2, CO2 and N2O oxidizers, and comparison with model calculations
journal, January 1998


Formation of charged aggregates of Al2O3 nanoparticles by combustion of aluminum droplets in air
journal, July 2004


Light deviation based optical techniques applied to solid propellant combustion
conference, October 2012


Application of Optical Diagnostics to Particle Measurements in Solid Propellant Rocket Motors and Exhaust Plumes
journal, July 1993


Motor and plume particle size measurements in solid propellant micromotors
journal, May 1994

  • Laredo, D.; McCrorie, J. D.; Vaughn, J. K.
  • Journal of Propulsion and Power, Vol. 10, Issue 3
  • DOI: 10.2514/3.23750

Quantitative, three-dimensional imaging of aluminum drop combustion in solid propellant plumes via digital in-line holography
journal, January 2014

  • Guildenbecher, Daniel R.; Cooper, Marcia A.; Gill, Walter
  • Optics Letters, Vol. 39, Issue 17
  • DOI: 10.1364/OL.39.005126

High-speed (20  kHz) digital in-line holography for transient particle tracking and sizing in multiphase flows
journal, January 2016

  • Guildenbecher, Daniel R.; Cooper, Marcia A.; Sojka, Paul E.
  • Applied Optics, Vol. 55, Issue 11
  • DOI: 10.1364/AO.55.002892

Refinement of particle detection by the hybrid method in digital in-line holography
journal, January 2014

  • Gao, Jian; Guildenbecher, Daniel R.; Engvall, Luke
  • Applied Optics, Vol. 53, Issue 27
  • DOI: 10.1364/AO.53.00G130

Accurate measurement of out-of-plane particle displacement from the cross correlation of sequential digital in-line holograms
journal, January 2013

  • Guildenbecher, Daniel R.; Reu, Phillip L.; Stuaffacher, Howard Lee
  • Optics Letters, Vol. 38, Issue 20
  • DOI: 10.1364/OL.38.004015

The simulation of the combustion of micrometer-sized aluminum particles with oxygen and carbon dioxide
journal, March 2010


Infrared Emitted Intensity Measurements from Burning Aluminum Droplets in Solid Propellants
journal, December 2008


Temperature Measurements of Aluminum Particles Burning in Carbon Dioxide
journal, February 2005

  • Glumac, Nick; Krier, Herman; Bazyn, Tim
  • Combustion Science and Technology, Vol. 177, Issue 3
  • DOI: 10.1080/00102200590909030

Temperature measurements in metalized propellant combustion using hybrid fs/ps coherent anti-Stokes Raman scattering
journal, January 2016

  • Kearney, Sean P.; Guildenbecher, Daniel R.
  • Applied Optics, Vol. 55, Issue 18
  • DOI: 10.1364/AO.55.004958

Measurements of particle flame temperatures using three-color optical pyrometry
journal, February 1996


Combustion of nanoaluminum at elevated pressure and temperature behind reflected shock waves
journal, June 2006


Invited Article: Quantitative imaging of explosions with high-speed cameras
journal, May 2016

  • McNesby, Kevin L.; Homan, Barrie E.; Benjamin, Richard A.
  • Review of Scientific Instruments, Vol. 87, Issue 5
  • DOI: 10.1063/1.4949520

A model of composite solid-propellant combustion based on multiple flames
journal, December 1970

  • Beckstead, M. W.; Derr, R. L.; Price, C. F.
  • AIAA Journal, Vol. 8, Issue 12
  • DOI: 10.2514/3.6087

Diffusion flame calculations for composite propellants predicting particle-size effects
journal, May 2010


New Aluminum Agglomeration Models and Their Use in Solid-Propellant-Rocket Simularions
journal, September 2005

  • Jackson, T. L.; Najjar, F.; Buckmaster, J.
  • Journal of Propulsion and Power, Vol. 21, Issue 5
  • DOI: 10.2514/1.11888

Effect of nano-aluminium in plateau-burning and catalyzed composite solid propellant combustion
journal, August 2009


A pocket model for aluminum agglomeration in composite propellants
journal, May 1983


The three-dimensional numerical simulation of aluminized composite solid propellant combustion
journal, December 2007


Modeling of Heterogeneous Propellant Combustion: A Survey
journal, May 2012


The Simulation of the Combustion of Micrometer-Sized Aluminum Particles with Steam
journal, June 2008

  • Washburn, E. B.; Trivedi, J. N.; Catoire, L.
  • Combustion Science and Technology, Vol. 180, Issue 8
  • DOI: 10.1080/00102200802125594

Combustion response of an aluminum droplet burning in air
journal, January 2011

  • Gallier, Stany; Sibe, Fabien; Orlandi, Olivier
  • Proceedings of the Combustion Institute, Vol. 33, Issue 2
  • DOI: 10.1016/j.proci.2010.05.046

On possibility of vapor-phase combustion for fine aluminum particles
journal, November 2009


Emission spectroscopy of flame fronts in aluminum suspensions
journal, January 2007

  • Goroshin, Samuel; Mamen, Jorin; Higgins, Andrew
  • Proceedings of the Combustion Institute, Vol. 31, Issue 2
  • DOI: 10.1016/j.proci.2006.07.175

Emission and laser absorption spectroscopy of flat flames in aluminum suspensions
journal, June 2017


Characterization of a gas burner to simulate a propellant flame and evaluate aluminum particle combustion
journal, April 2008


Emissivity of Aluminum-Oxide Particle Clouds: Application to Pyrometry of Explosive Fireballs
journal, April 2010

  • Lynch, Patrick; Krier, Herman; Glumac, Nick
  • Journal of Thermophysics and Heat Transfer, Vol. 24, Issue 2
  • DOI: 10.2514/1.43853

Optical Depth Effects on Aluminum Oxide Spectral Emissivity
journal, January 2015

  • Kalman, Joseph; Allen, David; Glumac, Nick
  • Journal of Thermophysics and Heat Transfer, Vol. 29, Issue 1
  • DOI: 10.2514/1.T4260

On the mechanism of asymmetric aluminum particle combustion
journal, June 1999


Combustion characteristics of micron-sized aluminum particles in oxygenated environments
journal, October 2011


    Works referencing / citing this record:

    Spatially focused microwave ignition of metallized energetic materials
    journal, February 2020

    • Kline, Dylan J.; Rehwoldt, Miles C.; Turner, Charles J.
    • Journal of Applied Physics, Vol. 127, Issue 5
    • DOI: 10.1063/1.5134089

    Comparison of simulation and experiments for multimode aerodynamic breakup of a liquid metal column in a shock-induced cross-flow
    journal, August 2019

    • Arienti, Marco; Ballard, Matthew; Sussman, Mark
    • Physics of Fluids, Vol. 31, Issue 8
    • DOI: 10.1063/1.5099589

    Theoretical study on combustion of non-spherical particles in nano-aluminized propellant in air
    journal, March 2019


    Agglomerate Sizing in Aluminized Propellants Using Digital Inline Holography and Traditional Diagnostics
    journal, July 2018

    • Powell, Michael S.; Gunduz, Ibrahim W.; Shang, Weixiao
    • Journal of Propulsion and Power, Vol. 34, Issue 4
    • DOI: 10.2514/1.b36859

    Ultra-high-speed Pulse-burst Phase Conjugate Digital In-line Holography for Imaging Through Shock-wave Distortions
    conference, January 2019

    • Chen, Yi; Heyborne, Jeffery; Guildenbecher, Daniel R.
    • AIAA Scitech 2019 Forum
    • DOI: 10.2514/6.2019-1602

    Reaction kinetics and a physical model of the charring layer by depositing Al 2 O 3 at ultra-high temperatures
    journal, January 2018

    • Guan, Yi-Wen; Li, Jiang; Liu, Yang
    • Physical Chemistry Chemical Physics, Vol. 20, Issue 37
    • DOI: 10.1039/c8cp04169e

    Imaging Aluminum Particles in Solid-Propellant Flames Using 5 kHz LIF of Al Atoms
    journal, July 2019

    • Vilmart, Gautier; Dorval, Nelly; Devillers, Robin
    • Materials, Vol. 12, Issue 15
    • DOI: 10.3390/ma12152421