DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Efficient modeling of Bragg coherent x-ray nanobeam diffraction

Abstract

X-ray Bragg diffraction experiments that utilize tightly focused coherent beams produce complicated Bragg diffraction patterns that depend on scattering geometry, characteristics of the sample, and properties of the x-ray focusing optic. In this paper, we use a Fourier-transform-based method of modeling the 2D intensity distribution of a Bragg peak and apply it to the case of thin films illuminated with a Fresnel zone plate in three different Bragg scattering geometries. Finally, the calculations agree well with experimental coherent diffraction patterns, demonstrating that nanodiffraction patterns can be modeled at nonsymmetric Bragg conditions with this approach—a capability critical for advancing nanofocused x-ray diffraction microscopy.

Authors:
 [1];  [2];  [3];  [3];  [4];  [5];  [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
  2. Argonne National Lab. (ANL), Argonne, IL (United States). Center for Nanoscale Materials
  3. Aix-Marseille Univ., Marseille (France). CNRS. Fresnel Inst.
  4. Columbia Univ., New York, NY (United States). Dept. of Applied Physics and Mathematics
  5. Thomas J. Watson Research Center, Yorktown Heights, NY (United States). IBM Corporation
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States); Aix-Marseille Univ., Marseille (France)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Agency for Research (ANR) (France)
Contributing Org.:
Columbia Univ., New York, NY (United States); Thomas J. Watson Research Center, Yorktown Heights, NY (United States)
OSTI Identifier:
1356646
Alternate Identifier(s):
OSTI ID: 1222258
Grant/Contract Number:  
AC02-06CH11357; ANR-11-BS10-0005
Resource Type:
Accepted Manuscript
Journal Name:
Optics Letters
Additional Journal Information:
Journal Volume: 40; Journal Issue: 14; Journal ID: ISSN 0146-9592
Publisher:
Optical Society of America (OSA)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Diffractive optics; Far field diffraction; High numerical aperture optics; Ptychography; Scanning probe microscopy; X ray optics; Coherence; Synchrotron radiation

Citation Formats

Hruszkewycz, S. O., Holt, M. V., Allain, M., Chamard, V., Polvino, S. M., Murray, C. E., and Fuoss, P. H. Efficient modeling of Bragg coherent x-ray nanobeam diffraction. United States: N. p., 2015. Web. doi:10.1364/OL.40.003241.
Hruszkewycz, S. O., Holt, M. V., Allain, M., Chamard, V., Polvino, S. M., Murray, C. E., & Fuoss, P. H. Efficient modeling of Bragg coherent x-ray nanobeam diffraction. United States. https://doi.org/10.1364/OL.40.003241
Hruszkewycz, S. O., Holt, M. V., Allain, M., Chamard, V., Polvino, S. M., Murray, C. E., and Fuoss, P. H. Thu . "Efficient modeling of Bragg coherent x-ray nanobeam diffraction". United States. https://doi.org/10.1364/OL.40.003241. https://www.osti.gov/servlets/purl/1356646.
@article{osti_1356646,
title = {Efficient modeling of Bragg coherent x-ray nanobeam diffraction},
author = {Hruszkewycz, S. O. and Holt, M. V. and Allain, M. and Chamard, V. and Polvino, S. M. and Murray, C. E. and Fuoss, P. H.},
abstractNote = {X-ray Bragg diffraction experiments that utilize tightly focused coherent beams produce complicated Bragg diffraction patterns that depend on scattering geometry, characteristics of the sample, and properties of the x-ray focusing optic. In this paper, we use a Fourier-transform-based method of modeling the 2D intensity distribution of a Bragg peak and apply it to the case of thin films illuminated with a Fresnel zone plate in three different Bragg scattering geometries. Finally, the calculations agree well with experimental coherent diffraction patterns, demonstrating that nanodiffraction patterns can be modeled at nonsymmetric Bragg conditions with this approach—a capability critical for advancing nanofocused x-ray diffraction microscopy.},
doi = {10.1364/OL.40.003241},
journal = {Optics Letters},
number = 14,
volume = 40,
place = {United States},
year = {Thu Jul 02 00:00:00 EDT 2015},
month = {Thu Jul 02 00:00:00 EDT 2015}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Nanoscale Hard X-Ray Microscopy Methods for Materials Studies
journal, July 2013


Modeling of kinematic diffraction from a thin silicon film illuminated by a coherent, focused X-ray nanobeam
journal, April 2010

  • Ying, Andrew; Osting, Braxton; Noyan, I. C.
  • Journal of Applied Crystallography, Vol. 43, Issue 3
  • DOI: 10.1107/S0021889810008459

Quantitative Nanoscale Imaging of Lattice Distortions in Epitaxial Semiconductor Heterostructures Using Nanofocused X-ray Bragg Projection Ptychography
journal, September 2012

  • Hruszkewycz, S. O.; Holt, M. V.; Murray, C. E.
  • Nano Letters, Vol. 12, Issue 10
  • DOI: 10.1021/nl303201w

Coherent X-ray diffraction imaging of strain at the nanoscale
journal, April 2009

  • Robinson, Ian; Harder, Ross
  • Nature Materials, Vol. 8, Issue 4
  • DOI: 10.1038/nmat2400

Framework for three-dimensional coherent diffraction imaging by focused beam x-ray Bragg ptychography
journal, January 2011

  • Hruszkewycz, Stephan O.; Holt, Martin V.; Tripathi, Ash
  • Optics Letters, Vol. 36, Issue 12
  • DOI: 10.1364/OL.36.002227

Coherent Bragg nanodiffraction at the hard X-ray Nanoprobe beamline
journal, March 2014

  • Hruszkewycz, S. O.; Holt, M. V.; Maser, J.
  • Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 372, Issue 2010
  • DOI: 10.1098/rsta.2013.0118

Nanomembrane-based materials for Group IV semiconductor quantum electronics
journal, February 2014

  • Paskiewicz, D. M.; Savage, D. E.; Holt, M. V.
  • Scientific Reports, Vol. 4, Issue 1
  • DOI: 10.1038/srep04218

Works referencing / citing this record:

High-resolution three-dimensional structural microscopy by single-angle Bragg ptychography
journal, November 2016

  • Hruszkewycz, S. O.; Allain, M.; Holt, M. V.
  • Nature Materials, Vol. 16, Issue 2
  • DOI: 10.1038/nmat4798

Imaging nanoscale lattice variations by machine learning of x-ray diffraction microscopy data
journal, August 2016