skip to main content
DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Near-unity photoluminescence quantum yield in MoS2

Authors:
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1355845
Grant/Contract Number:  
AC02-05Ch11231
Resource Type:
Published Article
Journal Name:
Science
Additional Journal Information:
Journal Name: Science Journal Volume: 350 Journal Issue: 6264; Journal ID: ISSN 0036-8075
Publisher:
American Association for the Advancement of Science (AAAS)
Country of Publication:
United States
Language:
English

Citation Formats

Amani, M., Lien, D. -H., Kiriya, D., Xiao, J., Azcatl, A., Noh, J., Madhvapathy, S. R., Addou, R., KC, S., Dubey, M., Cho, K., Wallace, R. M., Lee, S. -C., He, J. -H., Ager, J. W., Zhang, X., Yablonovitch, E., and Javey, A. Near-unity photoluminescence quantum yield in MoS2. United States: N. p., 2015. Web. doi:10.1126/science.aad2114.
Amani, M., Lien, D. -H., Kiriya, D., Xiao, J., Azcatl, A., Noh, J., Madhvapathy, S. R., Addou, R., KC, S., Dubey, M., Cho, K., Wallace, R. M., Lee, S. -C., He, J. -H., Ager, J. W., Zhang, X., Yablonovitch, E., & Javey, A. Near-unity photoluminescence quantum yield in MoS2. United States. doi:10.1126/science.aad2114.
Amani, M., Lien, D. -H., Kiriya, D., Xiao, J., Azcatl, A., Noh, J., Madhvapathy, S. R., Addou, R., KC, S., Dubey, M., Cho, K., Wallace, R. M., Lee, S. -C., He, J. -H., Ager, J. W., Zhang, X., Yablonovitch, E., and Javey, A. Thu . "Near-unity photoluminescence quantum yield in MoS2". United States. doi:10.1126/science.aad2114.
@article{osti_1355845,
title = {Near-unity photoluminescence quantum yield in MoS2},
author = {Amani, M. and Lien, D. -H. and Kiriya, D. and Xiao, J. and Azcatl, A. and Noh, J. and Madhvapathy, S. R. and Addou, R. and KC, S. and Dubey, M. and Cho, K. and Wallace, R. M. and Lee, S. -C. and He, J. -H. and Ager, J. W. and Zhang, X. and Yablonovitch, E. and Javey, A.},
abstractNote = {},
doi = {10.1126/science.aad2114},
journal = {Science},
number = 6264,
volume = 350,
place = {United States},
year = {2015},
month = {11}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: 10.1126/science.aad2114

Citation Metrics:
Cited by: 358 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Constructing metallic nanoroads on a MoS 2 monolayer via hydrogenation
journal, January 2014

  • Cai, Yongqing; Bai, Zhaoqiang; Pan, Hui
  • Nanoscale, Vol. 6, Issue 3
  • DOI: 10.1039/C3NR05218D

Many-Body Effects in Valleytronics: Direct Measurement of Valley Lifetimes in Single-Layer MoS 2
journal, December 2013

  • Mai, Cong; Barrette, Andrew; Yu, Yifei
  • Nano Letters, Vol. 14, Issue 1
  • DOI: 10.1021/nl403742j

Two-dimensional material nanophotonics
journal, November 2014


Defects activated photoluminescence in two-dimensional semiconductors: interplay between bound, charged and free excitons
journal, September 2013

  • Tongay, Sefaattin; Suh, Joonki; Ataca, Can
  • Scientific Reports, Vol. 3, Issue 1
  • DOI: 10.1038/srep02657

MoS 2 functionalization for ultra-thin atomic layer deposited dielectrics
journal, March 2014

  • Azcatl, Angelica; McDonnell, Stephen; K. C., Santosh
  • Applied Physics Letters, Vol. 104, Issue 11
  • DOI: 10.1063/1.4869149

Projector augmented-wave method
journal, December 1994


Strain-Induced Indirect to Direct Bandgap Transition in Multilayer WSe 2
journal, July 2014

  • Desai, Sujay B.; Seol, Gyungseon; Kang, Jeong Seuk
  • Nano Letters, Vol. 14, Issue 8
  • DOI: 10.1021/nl501638a

Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996


Inhibited and Enhanced Spontaneous Emission from Optically Thin AlGaAs/GaAs Double Heterostructures
journal, November 1988


Strong interlayer coupling in van der Waals heterostructures built from single-layer chalcogenides
journal, April 2014

  • Fang, H.; Battaglia, C.; Carraro, C.
  • Proceedings of the National Academy of Sciences, Vol. 111, Issue 17
  • DOI: 10.1073/pnas.1405435111

Strong Light-Matter Interactions in Heterostructures of Atomically Thin Films
journal, May 2013


Fast exciton annihilation by capture of electrons or holes by defects via Auger scattering in monolayer metal dichalcogenides
journal, April 2015


Defect-Dominated Doping and Contact Resistance in MoS 2
journal, February 2014

  • McDonnell, Stephen; Addou, Rafik; Buie, Creighton
  • ACS Nano, Vol. 8, Issue 3
  • DOI: 10.1021/nn500044q

Observation of Excitonic Rydberg States in Monolayer MoS 2 and WS 2 by Photoluminescence Excitation Spectroscopy
journal, April 2015

  • Hill, Heather M.; Rigosi, Albert F.; Roquelet, Cyrielle
  • Nano Letters, Vol. 15, Issue 5
  • DOI: 10.1021/nl504868p

Surface Defects on Natural MoS 2
journal, May 2015

  • Addou, Rafik; Colombo, Luigi; Wallace, Robert M.
  • ACS Applied Materials & Interfaces, Vol. 7, Issue 22
  • DOI: 10.1021/acsami.5b01778

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996


Strain and structure heterogeneity in MoS2 atomic layers grown by chemical vapour deposition
journal, November 2014

  • Liu, Zheng; Amani, Matin; Najmaei, Sina
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms6246

Intensity enhancement in textured optical sheets for solar cells
journal, February 1982

  • Yablonovitch, E.; Cody, G. D.
  • IEEE Transactions on Electron Devices, Vol. 29, Issue 2
  • DOI: 10.1109/T-ED.1982.20700

Induced-emission cross sections in neodymium laser glasses
journal, April 1974


Inhomogeneous Electron Gas
journal, November 1964


Ultrahigh spontaneous emission quantum efficiency, 99.7% internally and 72% externally, from AlGaAs/GaAs/AlGaAs double heterostructures
journal, January 1993

  • Schnitzer, I.; Yablonovitch, E.; Caneau, C.
  • Applied Physics Letters, Vol. 62, Issue 2
  • DOI: 10.1063/1.109348

Impurities and Electronic Property Variations of Natural MoS 2 Crystal Surfaces
journal, August 2015


Stability and electronic structures of native defects in single-layer MoS 2
journal, May 2014


Chloride Molecular Doping Technique on 2D Materials: WS 2 and MoS 2
journal, October 2014

  • Yang, Lingming; Majumdar, Kausik; Liu, Han
  • Nano Letters, Vol. 14, Issue 11
  • DOI: 10.1021/nl502603d

Band-tail parameter modeling in semiconductor materials
journal, July 1998


Atomically Thin MoS2 A New Direct-Gap Semiconductor
journal, September 2010


Low-temperature photocarrier dynamics in monolayer MoS 2
journal, September 2011

  • Korn, T.; Heydrich, S.; Hirmer, M.
  • Applied Physics Letters, Vol. 99, Issue 10
  • DOI: 10.1063/1.3636402

Hydrogen sorption by molybdenum sulphide catalysts
journal, January 1980

  • Wright, Christopher J.; Sampson, Christopher; Fraser, David
  • Journal of the Chemical Society, Faraday Transactions 1: Physical Chemistry in Condensed Phases, Vol. 76, Issue 0
  • DOI: 10.1039/f19807601585

Near-Unity Quantum Yields of Biexciton Emission from CdSe / CdS Nanocrystals Measured Using Single-Particle Spectroscopy
journal, May 2011


Non-Radiative Transitions in Semiconductors
journal, January 1970


Hopping transport through defect-induced localized states in molybdenum disulphide
journal, October 2013

  • Qiu, Hao; Xu, Tao; Wang, Zilu
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3642

Exciton dynamics and annihilation in WS 2 2D semiconductors
journal, January 2015


Ultrafast Dynamics of Defect-Assisted Electron–Hole Recombination in Monolayer MoS 2
journal, December 2014

  • Wang, Haining; Zhang, Changjian; Rana, Farhan
  • Nano Letters, Vol. 15, Issue 1
  • DOI: 10.1021/nl503636c

Pressure-induced semiconducting to metallic transition in multilayered molybdenum disulphide
journal, May 2014

  • Nayak, Avinash P.; Bhattacharyya, Swastibrata; Zhu, Jie
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4731

Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS 2
journal, August 2014


Auger recombination of excitons in one-dimensional systems
journal, June 2006


Monolayer semiconductor nanocavity lasers with ultralow thresholds
journal, March 2015

  • Wu, Sanfeng; Buckley, Sonia; Schaibley, John R.
  • Nature, Vol. 520, Issue 7545
  • DOI: 10.1038/nature14290

Theory of neutral and charged excitons in monolayer transition metal dichalcogenides
journal, July 2013

  • Berkelbach, Timothy C.; Hybertsen, Mark S.; Reichman, David R.
  • Physical Review B, Vol. 88, Issue 4
  • DOI: 10.1103/PhysRevB.88.045318

Bandgap, Mid-Gap States, and Gating Effects in MoS 2
journal, July 2014

  • Lu, Chih-Pin; Li, Guohong; Mao, Jinhai
  • Nano Letters, Vol. 14, Issue 8
  • DOI: 10.1021/nl501659n

Control of valley polarization in monolayer MoS2 by optical helicity
journal, June 2012


Valley polarization in MoS2 monolayers by optical pumping
journal, June 2012

  • Zeng, Hualing; Dai, Junfeng; Yao, Wang
  • Nature Nanotechnology, Vol. 7, Issue 8
  • DOI: 10.1038/nnano.2012.95

Self-Consistent Equations Including Exchange and Correlation Effects
journal, November 1965