Antiferromagnetic Kondo lattice in the layered compound CePd1-xBi2 and comparison to the superconductor LaPd1-xBi2

Han, Fei; Wan, Xiangang; Phelan, Daniel; Stoumpos, Constantinos C.; Sturza, Mihai; Malliakas, Christos D.; Li, Qing'an; Han, Tian-Heng; Zhao, Qingbiao; Chung, Duck Young; Kanatzidis, Mercouri G.

doi:10.1103/PhysRevB.92.045112

Title: Antiferromagnetic Kondo lattice in the layered compound ${CePd}_{1 - x} {Bi}_{2}$ and comparison to the superconductor ${LaPd}_{1 - x} {Bi}_{2}$

Abstract

ZrCuSi₂-type CePd_1-xBi₂ crystals were obtained from excess Bi flux. Magnetic susceptibility measurements reveal that CePd_1-xBi₂ is a highly anisotropic antiferromagnet with transition temperature at 6 K, and a magnetic-field-induced metamagnetic transition at 5 T. An enhanced Sommerfeld coefficient of γ of 0.199 J-mol-Ce^-1K^-2 obtained from specific heat measurements suggests a moderate Kondo effect in CePd_1-xBi₂. In addition to the antiferromagnetic peak the resistivity curve shows a shoulder-like behavior which could be attributed to the presence of Kondo effect and crystal-electric-field effects in this compound. Magnetoresistance and Hall effect measurements suggest an interplay between Kondo and crystal-electric-field effects which reconstructs the Fermi surface topology of CePd_1-xBi₂ around 75 K. Electronic structure calculations reveal the Pd vacancies are important to the magnetic structure and enhance the crystal-electric-field effects which quench the orbital moment of Ce at low temperatures.

Authors:

Han, Fei ^[1]; Wan, Xiangang ^[2]; Phelan, Daniel ^[1]; Stoumpos, Constantinos C. ^[1]; Sturza, Mihai ^[1]; Malliakas, Christos D. ^[3]; Li, Qing'an ^[1]; Han, Tian-Heng ^[4]; Zhao, Qingbiao ^[1]; Chung, Duck Young ^[1]; Kanatzidis, Mercouri G. ^[3]

Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division
Nanjing Univ. (China). National Lab. of Solid State Microstructures
Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division; Northwestern Univ., Evanston, IL (United States). Dept. of Chemistry
Argonne National Lab. (ANL), Argonne, IL (United States). Materials Science Division; Univ. of Chicago, IL (United States). James Franck Inst. and Dept. of Physics

Publication Date:: Mon Jul 13 00:00:00 EDT 2015

Research Org.:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Natural Science Foundation of China (NSFC)

OSTI Identifier:: 1355774

Alternate Identifier(s):: OSTI ID: 1193901

Grant/Contract Number:: AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review. B, Condensed Matter and Materials Physics

Additional Journal Information:: Journal Volume: 92; Journal Issue: 4; Journal ID: ISSN 1098-0121

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Han, Fei, Wan, Xiangang, Phelan, Daniel, Stoumpos, Constantinos C., Sturza, Mihai, Malliakas, Christos D., Li, Qing'an, Han, Tian-Heng, Zhao, Qingbiao, Chung, Duck Young, and Kanatzidis, Mercouri G. Antiferromagnetic Kondo lattice in the layered compound CePd1-xBi2 and comparison to the superconductor LaPd1-xBi2.  United States: N. p., 2015. 
Web.  doi:10.1103/PhysRevB.92.045112.

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                    Han, Fei, Wan, Xiangang, Phelan, Daniel, Stoumpos, Constantinos C., Sturza, Mihai, Malliakas, Christos D., Li, Qing'an, Han, Tian-Heng, Zhao, Qingbiao, Chung, Duck Young, & Kanatzidis, Mercouri G. Antiferromagnetic Kondo lattice in the layered compound CePd1-xBi2 and comparison to the superconductor LaPd1-xBi2.  United States.  https://doi.org/10.1103/PhysRevB.92.045112

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                    Han, Fei, Wan, Xiangang, Phelan, Daniel, Stoumpos, Constantinos C., Sturza, Mihai, Malliakas, Christos D., Li, Qing'an, Han, Tian-Heng, Zhao, Qingbiao, Chung, Duck Young, and Kanatzidis, Mercouri G. Mon .  
"Antiferromagnetic Kondo lattice in the layered compound CePd1-xBi2 and comparison to the superconductor LaPd1-xBi2".  United States.  https://doi.org/10.1103/PhysRevB.92.045112.  https://www.osti.gov/servlets/purl/1355774.

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@article{osti_1355774,

  title        = {Antiferromagnetic Kondo lattice in the layered compound CePd1-xBi2 and comparison to the superconductor LaPd1-xBi2},

  author       = {Han, Fei and Wan, Xiangang and Phelan, Daniel and Stoumpos, Constantinos C. and Sturza, Mihai and Malliakas, Christos D. and Li, Qing'an and Han, Tian-Heng and Zhao, Qingbiao and Chung, Duck Young and Kanatzidis, Mercouri G.},

  abstractNote = {ZrCuSi2-type CePd1-xBi2 crystals were obtained from excess Bi flux. Magnetic susceptibility measurements reveal that CePd1-xBi2 is a highly anisotropic antiferromagnet with transition temperature at 6 K, and a magnetic-field-induced metamagnetic transition at 5 T. An enhanced Sommerfeld coefficient of γ of 0.199 J-mol-Ce-1K-2 obtained from specific heat measurements suggests a moderate Kondo effect in CePd1-xBi2. In addition to the antiferromagnetic peak the resistivity curve shows a shoulder-like behavior which could be attributed to the presence of Kondo effect and crystal-electric-field effects in this compound. Magnetoresistance and Hall effect measurements suggest an interplay between Kondo and crystal-electric-field effects which reconstructs the Fermi surface topology of CePd1-xBi2 around 75 K. Electronic structure calculations reveal the Pd vacancies are important to the magnetic structure and enhance the crystal-electric-field effects which quench the orbital moment of Ce at low temperatures.},

  doi          = {10.1103/PhysRevB.92.045112},

  journal      = {Physical Review. B, Condensed Matter and Materials Physics},

  number       = 4,

  volume       = 92,

  place        = {United States},

  year         = {Mon Jul 13 00:00:00 EDT 2015},

  month        = {Mon Jul 13 00:00:00 EDT 2015}

}

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Works referencing / citing this record:

Magnetic field-tuned Fermi liquid in a Kondo insulator
journal, December 2019

Kushwaha, Satya K.; Chan, Mun K.; Park, Joonbum
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Title: Antiferromagnetic Kondo lattice in the layered compound CePd 1 - x Bi 2 and comparison to the superconductor LaPd 1 - x Bi 2

Abstract

Citation Formats

The Kondo lattice and weak antiferromagnetism journal, July 1977

Magnetic Property of a New Kondo Lattice Intermetallic Compound: CeCu 6 journal, April 1984

On the magnetic ordering of CeAl2 journal, November 1977

Magnetic and electronic properties of CeB6 journal, January 1980

Superconductivity and strong intrinsic defects in LaPd 1 − x Bi 2 journal, October 2013

The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds journal, November 2005

X-ray and Neutron Structure Determination and Magnetic Properties of New Quaternary Phases RE 0.67 Ni 2 Ga 5+ n - x Ge x and RE 0.67 Ni 2 Ga 5+ n - x Si x ( n = 0, 1; RE = Y, Sm, Gd, Tb, Dy, Ho, Er, Tm) Synthesized in Liquid Ga journal, July 2002

A short history of SHELX journal, December 2007

Heat Capacity Measurements on Small Samples at Low Temperatures journal, February 1972

Scaling of the temperature dependent Hall effect in La 2 − x Sr x CuO 4 journal, April 1994

Iron-Based Layered Superconductor La[O 1- x F x ]FeAs ( x = 0.05−0.12) with T c = 26 K journal, March 2008

High-temperature superconductivity in iron-based materials journal, August 2010

Substitution effect on the magnetic and transport properties of CeNi 0.8−x Mn x Bi 2 journal, August 2014

Crystal and magnetic structures of the superconductor CeNi 0 . 8 Bi 2 journal, June 2011

Anisotropic electrical and magnetic properties of Ce T Sb 2 ( T = Cu , Au, and Ni) single crystals journal, August 2003

Matrix Elements and Operator Equivalents Connected with the Magnetic Properties of Rare Earth Ions journal, March 1952

The theory of paramagnetic relaxation journal, January 1967

Exchange interactions in magnetic insulators journal, February 1976

Crystal Field and Metamagnetic Behavior of Rare-Earth Orthoaluminates: DyAlO3 journal, June 1990

Modeling optical spectra and Van Vleck paramagnetism in Er3+:YAlO3 journal, January 2009

Coexistence of Light and Heavy Carriers Associated with Superconductivity and Antiferromagnetism in CeNi 0.8 Bi 2 with a Bi Square Net journal, February 2011

Crystalline electric fields and the ground state of Ce 3 Rh 4 Pb 13 journal, August 2007

Magnetic properties of the heavy-fermion antiferromagnet CeMg 3 journal, April 2011

Specific heat of concentrated kondo systems: (La, Ce)Al2 and CeAl2 journal, December 1978

Magnetic and transport properties of the antiferromagnetic Kondo-lattice compound CeNiBi 2 journal, March 2002

Low-temperature heat capacity and magnetic properties of the R Ni X 2 compounds ( R =La, Ce; X =Si, Ge, Sn) journal, May 1991

Antiferromagnetic transitions in the Kondo lattice system Ce 2 Ni 3 Ge 5 journal, October 2000

Antiferromagnetic Kondo-lattice systems Ce 2 Rh 3 Ge 5 and Ce 2 Ir 3 Ge 5 with moderate heavy-fermion behavior journal, October 1999

Influence of the Crystalline Field on the Kondo Effect of Alloys and Compounds with Cerium Impurities journal, June 1972

In-Plane Magnetoresistance Obeys Kohler’s Rule in the Pseudogap Phase of Cuprate Superconductors journal, October 2014

Linear-response theory and lattice dynamics: A muffin-tin-orbital approach journal, December 1996

First-principles calculations of the electronic structure and spectra of strongly correlated systems: the LDA + U method journal, January 1997

First-principles study on the electronic structure of journal, January 2007

Superconductivity in the Presence of Strong Pauli Paramagnetism: Ce Cu 2 Si 2 journal, December 1979

Magnetic field-tuned Fermi liquid in a Kondo insulator journal, December 2019

Kondo Insulator to Semimetal Transformation Tuned by Spin-Orbit Coupling text, January 2016

Title: Antiferromagnetic Kondo lattice in the layered compound ${CePd}_{1 - x} {Bi}_{2}$ and comparison to the superconductor ${LaPd}_{1 - x} {Bi}_{2}$

The Kondo lattice and weak antiferromagnetism
journal, July 1977

Magnetic Property of a New Kondo Lattice Intermetallic Compound: CeCu ₆
journal, April 1984

On the magnetic ordering of CeAl2
journal, November 1977

Magnetic and electronic properties of CeB6
journal, January 1980

Superconductivity and strong intrinsic defects in LaPd $_{1 - x}$ Bi $_{2}$
journal, October 2013

The Metal Flux: A Preparative Tool for the Exploration of Intermetallic Compounds
journal, November 2005

X-ray and Neutron Structure Determination and Magnetic Properties of New Quaternary Phases RE _0.67 Ni ₂ Ga ₅₊ _n _- _x Ge _x and RE _0.67 Ni ₂ Ga ₅₊ _n _- _x Si _x ( n = 0, 1; RE = Y, Sm, Gd, Tb, Dy, Ho, Er, Tm) Synthesized in Liquid Ga
journal, July 2002

A short history of SHELX
journal, December 2007

Heat Capacity Measurements on Small Samples at Low Temperatures
journal, February 1972

Scaling of the temperature dependent Hall effect in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$
journal, April 1994

Iron-Based Layered Superconductor La[O _1- _x F _x ]FeAs ( x = 0.05−0.12) with T _c = 26 K
journal, March 2008

High-temperature superconductivity in iron-based materials
journal, August 2010

Substitution effect on the magnetic and transport properties of CeNi _0.8−x Mn _x Bi ₂
journal, August 2014

Crystal and magnetic structures of the superconductor CeNi $_{0.8}$ Bi $_{2}$
journal, June 2011

Anisotropic electrical and magnetic properties of $Ce T {Sb}_{2}$ $(T = Cu,$ Au, and Ni) single crystals
journal, August 2003

Matrix Elements and Operator Equivalents Connected with the Magnetic Properties of Rare Earth Ions
journal, March 1952

The theory of paramagnetic relaxation
journal, January 1967

Exchange interactions in magnetic insulators
journal, February 1976

Crystal Field and Metamagnetic Behavior of Rare-Earth Orthoaluminates: DyAlO3
journal, June 1990

Modeling optical spectra and Van Vleck paramagnetism in Er3+:YAlO3
journal, January 2009

Coexistence of Light and Heavy Carriers Associated with Superconductivity and Antiferromagnetism in ${CeNi}_{0.8} {Bi}_{2}$ with a Bi Square Net
journal, February 2011

Crystalline electric fields and the ground state of ${Ce}_{3} {Rh}_{4} {Pb}_{13}$
journal, August 2007

Magnetic properties of the heavy-fermion antiferromagnet CeMg $_{3}$
journal, April 2011

Specific heat of concentrated kondo systems: (La, Ce)Al2 and CeAl2
journal, December 1978

Magnetic and transport properties of the antiferromagnetic Kondo-lattice compound ${CeNiBi}_{2}$
journal, March 2002

Low-temperature heat capacity and magnetic properties of the R Ni $X_{2}$ compounds ( R =La, Ce; X =Si, Ge, Sn)
journal, May 1991

Antiferromagnetic transitions in the Kondo lattice system ${Ce}_{2} {Ni}_{3} {Ge}_{5}$
journal, October 2000

Antiferromagnetic Kondo-lattice systems ${Ce}_{2} {Rh}_{3} {Ge}_{5}$ and ${Ce}_{2} {Ir}_{3} {Ge}_{5}$ with moderate heavy-fermion behavior
journal, October 1999

Influence of the Crystalline Field on the Kondo Effect of Alloys and Compounds with Cerium Impurities
journal, June 1972

In-Plane Magnetoresistance Obeys Kohler’s Rule in the Pseudogap Phase of Cuprate Superconductors
journal, October 2014

Linear-response theory and lattice dynamics: A muffin-tin-orbital approach
journal, December 1996

First-principles calculations of the electronic structure and spectra of strongly correlated systems: the LDA + U method
journal, January 1997

First-principles study on the electronic structure of
journal, January 2007

Superconductivity in the Presence of Strong Pauli Paramagnetism: Ce ${Cu}_{2}$ ${Si}_{2}$
journal, December 1979

Magnetic field-tuned Fermi liquid in a Kondo insulator
journal, December 2019

Kondo Insulator to Semimetal Transformation Tuned by Spin-Orbit Coupling
text, January 2016