Energy and fuels from electrochemical interfaces
Abstract
Advances in electrocatalysis at solid–liquid interfaces are vital for driving the technological innovations that are needed to deliver reliable, affordable and environmentally friendly energy. Here, in this paper, we highlight the key achievements in the development of new materials for efficient hydrogen and oxygen production in electrolysers and, in reverse, their use in fuel cells. A key issue addressed here is the degree to which the fundamental understanding of the synergy between covalent and non-covalent interactions can form the basis for any predictive ability in tailor-making real-world catalysts. Common descriptors such as the substrate–hydroxide binding energy and the interactions in the double layer between hydroxide-oxides and H---OH are found to control individual parts of the hydrogen and oxygen electrochemistry that govern the efficiency of water-based energy conversion and storage systems. Lastly, links between aqueous- and organic-based environments are also established, encouraging the 'fuel cell' and 'battery' communities to move forward together.
- Authors:
-
- Argonne National Lab. (ANL), Lemont, IL (United States). Materials Science Division
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office
- OSTI Identifier:
- 1352573
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Materials
- Additional Journal Information:
- Journal Volume: 16; Journal Issue: 1; Journal ID: ISSN 1476-1122
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 25 ENERGY STORAGE; 36 MATERIALS SCIENCE
Citation Formats
Stamenkovic, Vojislav R., Strmcnik, Dusan, Lopes, Pietro P., and Markovic, Nenad M. Energy and fuels from electrochemical interfaces. United States: N. p., 2016.
Web. doi:10.1038/NMAT4738.
Stamenkovic, Vojislav R., Strmcnik, Dusan, Lopes, Pietro P., & Markovic, Nenad M. Energy and fuels from electrochemical interfaces. United States. https://doi.org/10.1038/NMAT4738
Stamenkovic, Vojislav R., Strmcnik, Dusan, Lopes, Pietro P., and Markovic, Nenad M. Tue .
"Energy and fuels from electrochemical interfaces". United States. https://doi.org/10.1038/NMAT4738. https://www.osti.gov/servlets/purl/1352573.
@article{osti_1352573,
title = {Energy and fuels from electrochemical interfaces},
author = {Stamenkovic, Vojislav R. and Strmcnik, Dusan and Lopes, Pietro P. and Markovic, Nenad M.},
abstractNote = {Advances in electrocatalysis at solid–liquid interfaces are vital for driving the technological innovations that are needed to deliver reliable, affordable and environmentally friendly energy. Here, in this paper, we highlight the key achievements in the development of new materials for efficient hydrogen and oxygen production in electrolysers and, in reverse, their use in fuel cells. A key issue addressed here is the degree to which the fundamental understanding of the synergy between covalent and non-covalent interactions can form the basis for any predictive ability in tailor-making real-world catalysts. Common descriptors such as the substrate–hydroxide binding energy and the interactions in the double layer between hydroxide-oxides and H---OH are found to control individual parts of the hydrogen and oxygen electrochemistry that govern the efficiency of water-based energy conversion and storage systems. Lastly, links between aqueous- and organic-based environments are also established, encouraging the 'fuel cell' and 'battery' communities to move forward together.},
doi = {10.1038/NMAT4738},
journal = {Nature Materials},
number = 1,
volume = 16,
place = {United States},
year = {2016},
month = {12}
}
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Electrocatalytic transformation of HF impurity to H2 and LiF in lithium-ion batteries
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Recent advances in understanding of the mechanism and control of Li 2 O 2 formation in aprotic Li–O 2 batteries
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Three-dimensional supramolecular phosphomolybdate architecture-derived Mo-based electrocatalytic system for overall water splitting
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A metal-vacancy-solid-solution NiAlP nanowall array bifunctional electrocatalyst for exceptional all-pH overall water splitting
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Robust graphene-wrapped PtNi nanosponge for enhanced oxygen reduction reaction performance
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Strain effects on Co,N co-decorated graphyne catalysts for overall water splitting electrocatalysis
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Design strategies for developing non-precious metal based bi-functional catalysts for alkaline electrolyte based zinc–air batteries
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Simple synthesis of a vacancy-rich NiO 2D/3D dendritic self-supported electrode for efficient overall water splitting
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Breaking the volcano-plot limits for Pt-based electrocatalysts by selective tuning adsorption of multiple intermediates
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Adsorbate-driven reactive interfacial Pt-NiO 1− x nanostructure formation on the Pt 3 Ni(111) alloy surface
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Ultrathin Transition Metal Dichalcogenide/3d Metal Hydroxide Hybridized Nanosheets to Enhance Hydrogen Evolution Activity
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Recent Advances on Controlled Synthesis and Engineering of Hollow Alloyed Nanotubes for Electrocatalysis
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In Situ and Operando Characterization of Proton Exchange Membrane Fuel Cells
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Design of Efficient Bifunctional Oxygen Reduction/Evolution Electrocatalyst: Recent Advances and Perspectives
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The Hydrogen Evolution Reaction in Alkaline Solution: From Theory, Single Crystal Models, to Practical Electrocatalysts
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Negative Charging of Transition‐Metal Phosphides via Strong Electronic Coupling for Destabilization of Alkaline Water
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Fabrication of a Single-Atom Platinum Catalyst for the Hydrogen Evolution Reaction: A New Protocol by Utilization of H x MoO 3− x with Plasmon Resonance
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Gallic acid-assisted synthesis of Pd uniformly anchored on porous N-rGO as efficient electrocatalyst for microbial fuel cells
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Rational design of atomically dispersed nickel active sites in β-Mo 2 C for the hydrogen evolution reaction at all pH values
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Defect engineering in earth-abundant electrocatalysts for CO 2 and N 2 reduction
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Insights into the spontaneous formation of hybrid PdO x /PEDOT films: electroless deposition and oxygen reduction activity
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NiCo 2 O 4 nanoarray on CNT sponge: a bifunctional oxygen electrode material for rechargeable Zn–air batteries
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Investigation of the correlation between the phase structure and activity of Ni–Mo–O derived electrocatalysts for the hydrogen evolution reaction
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Recent advances in graphene-based platinum and palladium electrocatalysts for the methanol oxidation reaction
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The Advanced Designs of High-Performance Platinum-Based Electrocatalysts: Recent Progresses and Challenges
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Elucidation of the Oxygen Reduction Volcano in Alkaline Media using a Copper-Platinum(111) Alloy
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Highly Tunable Heterojunctions from Multimetallic Sulfide Nanoparticles and Silver Nanowires
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