Energy and fuels from electrochemical interfaces

Stamenkovic, Vojislav R.; Strmcnik, Dusan; Lopes, Pietro P.; Markovic, Nenad M.

doi:10.1038/NMAT4738

Title: Energy and fuels from electrochemical interfaces

Journal Article · 20 December 2016 · Nature Materials

DOI: https://doi.org/10.1038/NMAT4738 · OSTI ID:1352573

Stamenkovic, Vojislav R. ^[1]; Strmcnik, Dusan ^[1]; Lopes, Pietro P. ^[1]; Markovic, Nenad M. ^[1]

Argonne National Lab. (ANL), Lemont, IL (United States). Materials Science Division

Advances in electrocatalysis at solid–liquid interfaces are vital for driving the technological innovations that are needed to deliver reliable, affordable and environmentally friendly energy. Here, in this paper, we highlight the key achievements in the development of new materials for efficient hydrogen and oxygen production in electrolysers and, in reverse, their use in fuel cells. A key issue addressed here is the degree to which the fundamental understanding of the synergy between covalent and non-covalent interactions can form the basis for any predictive ability in tailor-making real-world catalysts. Common descriptors such as the substrate–hydroxide binding energy and the interactions in the double layer between hydroxide-oxides and H---OH are found to control individual parts of the hydrogen and oxygen electrochemistry that govern the efficiency of water-based energy conversion and storage systems. Lastly, links between aqueous- and organic-based environments are also established, encouraging the 'fuel cell' and 'battery' communities to move forward together.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Sustainable Transportation Office. Hydrogen Fuel Cell Technologies Office (HFTO)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1352573

Journal Information:: Nature Materials, Vol. 16, Issue 1; ISSN 1476-1122

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1308 works

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