Energy and fuels from electrochemical interfaces

Stamenkovic, Vojislav R.; Strmcnik, Dusan; Lopes, Pietro P.; Markovic, Nenad M.

doi:10.1038/NMAT4738

Title: Energy and fuels from electrochemical interfaces

Journal Article · 19 December 2016 · Nature Materials

DOI: https://doi.org/10.1038/NMAT4738 · OSTI ID:1352573

Stamenkovic, Vojislav R. ^[1]; Strmcnik, Dusan ^[1]; Lopes, Pietro P. ^[1]; Markovic, Nenad M. ^[1]

Argonne National Lab. (ANL), Lemont, IL (United States). Materials Science Division

Advances in electrocatalysis at solid–liquid interfaces are vital for driving the technological innovations that are needed to deliver reliable, affordable and environmentally friendly energy. Here, in this paper, we highlight the key achievements in the development of new materials for efficient hydrogen and oxygen production in electrolysers and, in reverse, their use in fuel cells. A key issue addressed here is the degree to which the fundamental understanding of the synergy between covalent and non-covalent interactions can form the basis for any predictive ability in tailor-making real-world catalysts. Common descriptors such as the substrate–hydroxide binding energy and the interactions in the double layer between hydroxide-oxides and H---OH are found to control individual parts of the hydrogen and oxygen electrochemistry that govern the efficiency of water-based energy conversion and storage systems. Lastly, links between aqueous- and organic-based environments are also established, encouraging the 'fuel cell' and 'battery' communities to move forward together.

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Research Organization:: Argonne National Laboratory (ANL)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Fuel Cell Technologies Program (EE-3F); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1352573

Journal Information:: Nature Materials, Journal Name: Nature Materials Journal Issue: 1 Vol. 16; ISSN 1476-1122

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Rapid Synthesis of 3D Porous Nitrogen-Doped Carbon Nanospheres (N-CNSs) and Carbon Nanoboxes (CNBs) for Supercapacitor Electrodes Zhou, Xing-hai; Cao, Lei; Li, Zhen-huan Journal of The Electrochemical Society, Vol. 165, Issue 5 https://doi.org/10.1149/2.0761805jes	journal	January 2018
The Role of Non-Metallic and Metalloid Elements on the Electrocatalytic Activity of Cobalt and Nickel Catalysts for the Oxygen Evolution Reaction Masa, Justus; Schuhmann, Wolfgang FID GEO https://doi.org/10.23689/fidgeo-4447	text	January 2019
Sustainable Residential Energy Supply: A Literature Review-Based Morphological Analysis Arens, Stefan; Schlüters, Sunke; Hanke, Benedikt Energies, Vol. 13, Issue 2 https://doi.org/10.3390/en13020432	journal	January 2020
The Reactivity and Stability of Polyoxometalate Water Oxidation Electrocatalysts Gao, Dandan; Trentin, Ivan; Schwiedrzik, Ludwig Molecules, Vol. 25, Issue 1 https://doi.org/10.3390/molecules25010157	journal	December 2019

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