Sulfiphilic nickel phosphosulfide enabled Li2S impregnation in 3D graphene cages for Li-S batteries
Abstract
A 3D graphene cage with a thin layer of electrodeposited nickel phosphosulfide for Li2S impregnation, using ternary nickel phosphosulphide as a highly conductive coating layer for stabilized polysulfide chemistry, is accomplished by the combination of theoretical and experimental studies. As a result, the 3D interconnected graphene cage structure leads to high capacity, good rate capability and excellent cycling stability in a Li2S cathode.
- Authors:
-
- Stanford Univ., Stanford, CA (United States)
- Stanford Univ., Stanford, CA (United States); SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1352541
- Alternate Identifier(s):
- OSTI ID: 1401267
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 29; Journal Issue: 12; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 25 ENERGY STORAGE; lithium-sulfur batteries; graphene cage; sulfiphilic; nickel phosphosulfide; lithium sulfide
Citation Formats
Zhou, Guangmin, Sun, Jie, Jin, Yang, Chen, Wei, Zu, Chenxi, Zhang, Rufan, Qiu, Yongcai, Zhao, Jie, Zhuo, Denys, Liu, Yayuan, Tao, Xinyong, Liu, Wei, Yan, Kai, Lee, Hye Ryoung, and Cui, Yi. Sulfiphilic nickel phosphosulfide enabled Li2S impregnation in 3D graphene cages for Li-S batteries. United States: N. p., 2017.
Web. doi:10.1002/adma.201603366.
Zhou, Guangmin, Sun, Jie, Jin, Yang, Chen, Wei, Zu, Chenxi, Zhang, Rufan, Qiu, Yongcai, Zhao, Jie, Zhuo, Denys, Liu, Yayuan, Tao, Xinyong, Liu, Wei, Yan, Kai, Lee, Hye Ryoung, & Cui, Yi. Sulfiphilic nickel phosphosulfide enabled Li2S impregnation in 3D graphene cages for Li-S batteries. United States. https://doi.org/10.1002/adma.201603366
Zhou, Guangmin, Sun, Jie, Jin, Yang, Chen, Wei, Zu, Chenxi, Zhang, Rufan, Qiu, Yongcai, Zhao, Jie, Zhuo, Denys, Liu, Yayuan, Tao, Xinyong, Liu, Wei, Yan, Kai, Lee, Hye Ryoung, and Cui, Yi. Mon .
"Sulfiphilic nickel phosphosulfide enabled Li2S impregnation in 3D graphene cages for Li-S batteries". United States. https://doi.org/10.1002/adma.201603366. https://www.osti.gov/servlets/purl/1352541.
@article{osti_1352541,
title = {Sulfiphilic nickel phosphosulfide enabled Li2S impregnation in 3D graphene cages for Li-S batteries},
author = {Zhou, Guangmin and Sun, Jie and Jin, Yang and Chen, Wei and Zu, Chenxi and Zhang, Rufan and Qiu, Yongcai and Zhao, Jie and Zhuo, Denys and Liu, Yayuan and Tao, Xinyong and Liu, Wei and Yan, Kai and Lee, Hye Ryoung and Cui, Yi},
abstractNote = {A 3D graphene cage with a thin layer of electrodeposited nickel phosphosulfide for Li2S impregnation, using ternary nickel phosphosulphide as a highly conductive coating layer for stabilized polysulfide chemistry, is accomplished by the combination of theoretical and experimental studies. As a result, the 3D interconnected graphene cage structure leads to high capacity, good rate capability and excellent cycling stability in a Li2S cathode.},
doi = {10.1002/adma.201603366},
journal = {Advanced Materials},
number = 12,
volume = 29,
place = {United States},
year = {Mon Jan 30 00:00:00 EST 2017},
month = {Mon Jan 30 00:00:00 EST 2017}
}
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