Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies
Abstract
Anisotropic colloidal quasi-two-dimensional nanoplates (NPLs) hold great promise as functional materials due to their combination of low dimensional optoelectronic properties and versatility through colloidal synthesis. Recently, lead-halide perovskites have emerged as important optoelectronic materials with excellent efficiencies in photovoltaic and light-emitting applications. Here we report the synthesis of quantum confined all inorganic cesium lead halide nanoplates in the perovskite crystal structure that are also highly luminescent (PLQY 84%). The controllable self-assembly of nanoplates either into stacked columnar phases or crystallographic-oriented thin-sheet structures is demonstrated. Furthermore, the broad accessible emission range, high native quantum yields, and ease of self-assembly make perovskite NPLs an ideal platform for fundamental optoelectronic studies and the investigation of future devices.
- Authors:
-
- Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Univ. of California, Berkeley, CA (United States)
- Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Kavli Energy NanoScience Institute, Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1351533
- Report Number(s):
- LBNL-1004421
Journal ID: ISSN 0002-7863; ir:1004421
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of the American Chemical Society
- Additional Journal Information:
- Journal Volume: 137; Journal Issue: 51; Journal ID: ISSN 0002-7863
- Publisher:
- American Chemical Society (ACS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Bekenstein, Yehonadav, Koscher, Brent A., Eaton, Samuel W., Yang, Peidong, and Alivisatos, A. Paul. Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies. United States: N. p., 2015.
Web. doi:10.1021/jacs.5b11199.
Bekenstein, Yehonadav, Koscher, Brent A., Eaton, Samuel W., Yang, Peidong, & Alivisatos, A. Paul. Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies. United States. https://doi.org/10.1021/jacs.5b11199
Bekenstein, Yehonadav, Koscher, Brent A., Eaton, Samuel W., Yang, Peidong, and Alivisatos, A. Paul. Tue .
"Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies". United States. https://doi.org/10.1021/jacs.5b11199. https://www.osti.gov/servlets/purl/1351533.
@article{osti_1351533,
title = {Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies},
author = {Bekenstein, Yehonadav and Koscher, Brent A. and Eaton, Samuel W. and Yang, Peidong and Alivisatos, A. Paul},
abstractNote = {Anisotropic colloidal quasi-two-dimensional nanoplates (NPLs) hold great promise as functional materials due to their combination of low dimensional optoelectronic properties and versatility through colloidal synthesis. Recently, lead-halide perovskites have emerged as important optoelectronic materials with excellent efficiencies in photovoltaic and light-emitting applications. Here we report the synthesis of quantum confined all inorganic cesium lead halide nanoplates in the perovskite crystal structure that are also highly luminescent (PLQY 84%). The controllable self-assembly of nanoplates either into stacked columnar phases or crystallographic-oriented thin-sheet structures is demonstrated. Furthermore, the broad accessible emission range, high native quantum yields, and ease of self-assembly make perovskite NPLs an ideal platform for fundamental optoelectronic studies and the investigation of future devices.},
doi = {10.1021/jacs.5b11199},
journal = {Journal of the American Chemical Society},
number = 51,
volume = 137,
place = {United States},
year = {2015},
month = {12}
}
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