Cooling rate dependence of structural order in Al90Sm10 metallic glass

Sun, Yang; Zhang, Yue; Zhang, Feng; Ye, Zhuo; Ding, Zejun; Wang, Cai -Zhuang; Ho, Kai -Ming

doi:10.1063/1.4955223

Title: Cooling rate dependence of structural order in Al₉₀Sm₁₀ metallic glass

Abstract

Here, the atomic structure of Al₉₀Sm₁₀ metallic glass is studied using molecular dynamics simulations. By performing a long sub-T_g annealing, we developed a glass model closer to the experiments than the models prepared by continuous cooling. Using the cluster alignment method, we found that “3661” cluster is the dominating short-range order in the glass samples. The connection and arrangement of “3661” clusters, which define the medium-range order in the system, are enhanced significantly in the sub-T_g annealed sample as compared with the fast cooled glass samples. Unlike some strong binary glass formers such as Cu_64.5Zr_35.5, the clusters representing the short-range order do not form an interconnected interpenetrating network in Al₉₀Sm₁₀, which has only marginal glass formability.

Authors:

^[1]; Zhang, Yue ^[2]; Zhang, Feng ^[2]; Ye, Zhuo ^[2]; Ding, Zejun ^[3]; Wang, Cai -Zhuang ^[4]; Ho, Kai -Ming ^[5]

Univ. of Science and Technology of China, Anhui (China); Ames Lab., Ames, IA (United States)
Ames Lab., Ames, IA (United States)
Univ. of Science and Technology of China, Anhui (China)
Ames Lab. and Iowa State Univ., Ames, IA (United States)
Univ. of Science and Technology of China, Anhui (China); Ames Lab., Ames, IA (United States); Iowa State Univ., Ames, IA (United States)

Publication Date:: Thu Jul 07 00:00:00 EDT 2016

Research Org.:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1349898

Alternate Identifier(s):: OSTI ID: 1260852

Report Number(s):: IS-J-9247
Journal ID: ISSN 0021-8979; TRN: US1701794

Grant/Contract Number:: 2012CB933702; 11274288; 11574289; 201406340015; AC02-07CH11358

Resource Type:: Accepted Manuscript

Journal Name:: Journal of Applied Physics

Additional Journal Information:: Journal Volume: 120; Journal Issue: 1; Journal ID: ISSN 0021-8979

Publisher:: American Institute of Physics (AIP)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Sun, Yang, Zhang, Yue, Zhang, Feng, Ye, Zhuo, Ding, Zejun, Wang, Cai -Zhuang, and Ho, Kai -Ming. Cooling rate dependence of structural order in Al90Sm10 metallic glass.  United States: N. p., 2016. 
Web.  doi:10.1063/1.4955223.

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                    Sun, Yang, Zhang, Yue, Zhang, Feng, Ye, Zhuo, Ding, Zejun, Wang, Cai -Zhuang, & Ho, Kai -Ming. Cooling rate dependence of structural order in Al90Sm10 metallic glass.  United States.  https://doi.org/10.1063/1.4955223

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                    Sun, Yang, Zhang, Yue, Zhang, Feng, Ye, Zhuo, Ding, Zejun, Wang, Cai -Zhuang, and Ho, Kai -Ming. Thu .  
"Cooling rate dependence of structural order in Al90Sm10 metallic glass".  United States.  https://doi.org/10.1063/1.4955223.  https://www.osti.gov/servlets/purl/1349898.

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@article{osti_1349898,

  title        = {Cooling rate dependence of structural order in Al90Sm10 metallic glass},

  author       = {Sun, Yang and Zhang, Yue and Zhang, Feng and Ye, Zhuo and Ding, Zejun and Wang, Cai -Zhuang and Ho, Kai -Ming},

  abstractNote = {Here, the atomic structure of Al90Sm10 metallic glass is studied using molecular dynamics simulations. By performing a long sub-Tg annealing, we developed a glass model closer to the experiments than the models prepared by continuous cooling. Using the cluster alignment method, we found that “3661” cluster is the dominating short-range order in the glass samples. The connection and arrangement of “3661” clusters, which define the medium-range order in the system, are enhanced significantly in the sub-Tg annealed sample as compared with the fast cooled glass samples. Unlike some strong binary glass formers such as Cu64.5Zr35.5, the clusters representing the short-range order do not form an interconnected interpenetrating network in Al90Sm10, which has only marginal glass formability.},

  doi          = {10.1063/1.4955223},

  journal      = {Journal of Applied Physics},

  number       = 1,

  volume       = 120,

  place        = {United States},

  year         = {Thu Jul 07 00:00:00 EDT 2016},

  month        = {Thu Jul 07 00:00:00 EDT 2016}

}

Copy to clipboard

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Title: Cooling rate dependence of structural order in Al90Sm10 metallic glass

Abstract

Citation Formats

‘Crystal Genes’ in Metallic Liquids and Glasses journal, March 2016

Icosahedral Short-Range Order in Deeply Undercooled Metallic Melts journal, July 2002

Solute–solute correlations responsible for the prepeak in structure factors of undercooled Al-rich liquids: a molecular dynamics study journal, May 2015

Glassy metals journal, April 1980

Effects of sub- T g annealing on Cu 64.5 Zr 35.5 glasses: A molecular dynamics study journal, February 2014

New analytical scattering-factor functions for free atoms and ions journal, May 1995

Structural Origins of the Excellent Glass Forming Ability of Pd 40 Ni 40 P 20 journal, April 2012

The Stability of Al11Sm3 (Al4Sm) Phases in the Al-Sm Binary System journal, June 2007

A structural model for metallic glasses journal, September 2004

Full icosahedra dominate local order in Cu64Zr34 metallic glass and supercooled liquid journal, May 2014

Amorphous, nanoquasicrystalline and nanocrystalline alloys in Al-based systems journal, December 1998

Correlation between the elastic modulus and the intrinsic plastic behavior of metallic glasses: The roles of atomic configuration and alloy composition journal, June 2009

Non-crystalline Structure in Solidified Gold–Silicon Alloys journal, September 1960

A geometric model for atomic configurations in amorphous Al alloys journal, May 2003

Bulk metallic glasses journal, June 2004

Stabilization of metallic supercooled liquid and bulk amorphous alloys journal, January 2000

Disordered, quasicrystalline and crystalline phases of densely packed tetrahedra journal, December 2009

Cooling rates dependence of medium-range order development in C u 64 . 5 Z r 35 . 5 metallic glass journal, February 2015

Rapid solidification and metallic glass formation – Experimental and theoretical limits journal, October 2007

Structure and Properties of Metallic Glasses journal, January 1978

Atomic packing and short-to-medium-range order in metallic glasses journal, January 2006

Direct observation of local atomic order in a metallic glass journal, November 2010

Supercooled liquids and the glass transition journal, March 2001

Development of interatomic potentials appropriate for simulation of devitrification of Al 90 Sm 10 alloy journal, April 2015

Atomistic cluster alignment method for local order mining in liquids and glasses journal, November 2010

Metallic Liquids and Glasses: Atomic Order and Global Packing journal, October 2010

New Amorphous Al-Ln (Ln=Pr, Nd, Sm or Gd) Alloys Prepared by Melt Spinning journal, September 1988

Processing of Bulk Metallic Glass journal, December 2009

Discovery of a metastable Al20Sm4 phase journal, March 2015

A theory of the electrical properties of liquid metals: III. the resistivity of binary alloys journal, January 1965

Local structure in marginal glass forming Al–Sm alloy journal, August 2010

A brief overview of bulk metallic glasses journal, September 2011

Packing Structures and Transitions in Liquids and Solids journal, September 1984

Metallic Glasses journal, March 1995

A new structural model for transition metal–metalloid glasses journal, November 1978

Initial crystallization in a nanostructured Al–Sm rare earth alloy journal, June 2010

Connectivity of icosahedral network and a dramatically growing static length scale in Cu-Zr binary metallic glasses journal, May 2013

Atomic-level structure and structure–property relationship in metallic glasses journal, May 2011

Eutectic-to-metallic glass transition in the Al–Sm system journal, October 2011

Packing of Spheres: Co-ordination of Randomly Packed Spheres journal, December 1960

Cooling rate dependence of structural order in Ni 62 Nb 38 metallic glass journal, January 2018

A comparative study of Sm networks in Al-10 at.%Sm glass and associated crystalline phases journal, January 2018

Pressure dependence of the structure of liquid NiTi: a molecular dynamics study journal, June 2019

Predicting Complex Relaxation Processes in Metallic Glass journal, September 2019

Microstructure evolution during near- T g annealing and its effect on shear banding in model alloys journal, December 2019

Recent Topics on the Structure and Crystallization of Al-based Glassy Alloys journal, January 2019

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Effects of Si solute on the glass formation and atomic structure of Pd liquid text, January 2018

Title: Cooling rate dependence of structural order in Al₉₀Sm₁₀ metallic glass

‘Crystal Genes’ in Metallic Liquids and Glasses
journal, March 2016

Icosahedral Short-Range Order in Deeply Undercooled Metallic Melts
journal, July 2002

Solute–solute correlations responsible for the prepeak in structure factors of undercooled Al-rich liquids: a molecular dynamics study
journal, May 2015

Glassy metals
journal, April 1980

Effects of sub- T _g annealing on Cu _64.5 Zr _35.5 glasses: A molecular dynamics study
journal, February 2014

New analytical scattering-factor functions for free atoms and ions
journal, May 1995

Structural Origins of the Excellent Glass Forming Ability of ${Pd}_{40} {Ni}_{40} P_{20}$
journal, April 2012

The Stability of Al11Sm3 (Al4Sm) Phases in the Al-Sm Binary System
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A structural model for metallic glasses
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Full icosahedra dominate local order in Cu64Zr34 metallic glass and supercooled liquid
journal, May 2014

Amorphous, nanoquasicrystalline and nanocrystalline alloys in Al-based systems
journal, December 1998

Correlation between the elastic modulus and the intrinsic plastic behavior of metallic glasses: The roles of atomic configuration and alloy composition
journal, June 2009

Non-crystalline Structure in Solidified Gold–Silicon Alloys
journal, September 1960

A geometric model for atomic configurations in amorphous Al alloys
journal, May 2003

Bulk metallic glasses
journal, June 2004

Stabilization of metallic supercooled liquid and bulk amorphous alloys
journal, January 2000

Disordered, quasicrystalline and crystalline phases of densely packed tetrahedra
journal, December 2009

Cooling rates dependence of medium-range order development in $C u_{64.5} Z r_{35.5}$ metallic glass
journal, February 2015

Rapid solidification and metallic glass formation – Experimental and theoretical limits
journal, October 2007

Structure and Properties of Metallic Glasses
journal, January 1978

Atomic packing and short-to-medium-range order in metallic glasses
journal, January 2006

Direct observation of local atomic order in a metallic glass
journal, November 2010

Supercooled liquids and the glass transition
journal, March 2001

Development of interatomic potentials appropriate for simulation of devitrification of Al ₉₀ Sm ₁₀ alloy
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Atomistic cluster alignment method for local order mining in liquids and glasses
journal, November 2010

Metallic Liquids and Glasses: Atomic Order and Global Packing
journal, October 2010

New Amorphous Al-Ln (Ln=Pr, Nd, Sm or Gd) Alloys Prepared by Melt Spinning
journal, September 1988

Processing of Bulk Metallic Glass
journal, December 2009

Discovery of a metastable Al20Sm4 phase
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A theory of the electrical properties of liquid metals: III. the resistivity of binary alloys
journal, January 1965

Local structure in marginal glass forming Al–Sm alloy
journal, August 2010

A brief overview of bulk metallic glasses
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Packing Structures and Transitions in Liquids and Solids
journal, September 1984

Metallic Glasses
journal, March 1995

A new structural model for transition metal–metalloid glasses
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Initial crystallization in a nanostructured Al–Sm rare earth alloy
journal, June 2010

Connectivity of icosahedral network and a dramatically growing static length scale in Cu-Zr binary metallic glasses
journal, May 2013

Atomic-level structure and structure–property relationship in metallic glasses
journal, May 2011

Eutectic-to-metallic glass transition in the Al–Sm system
journal, October 2011

Packing of Spheres: Co-ordination of Randomly Packed Spheres
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Cooling rate dependence of structural order in Ni ₆₂ Nb ₃₈ metallic glass
journal, January 2018

A comparative study of Sm networks in Al-10 at.%Sm glass and associated crystalline phases
journal, January 2018

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Predicting Complex Relaxation Processes in Metallic Glass
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Recent Topics on the Structure and Crystallization of Al-based Glassy Alloys
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Effects of Si solute on the glass formation and atomic structure of Pd liquid
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