Physical properties of single crystalline RMg2Cu9 (R=Y,Ce-Nd,Gd-Dy,Yb) and the search for in-plane magnetic anisotropy in hexagonal systems

Kong, Tai; Meier, William R.; Lin, Qisheng; Saunders, Scott M.; Bud'ko, Sergey L.; Flint, Rebecca; Canfield, Paul C.

doi:10.1103/PhysRevB.94.144434

Title: Physical properties of single crystalline $R {Mg}_{2} {Cu}_{9}$ $(R = Y, Ce - Nd, Gd - Dy, Yb)$ and the search for in-plane magnetic anisotropy in hexagonal systems

Abstract

Single crystals of RMg₂Cu₉ (R=Y, Ce-Nd, Gd-Dy, Yb) were grown using a high-temperature solution growth technique and were characterized by measurements of room-temperature x-ray diffraction, temperature-dependent specific heat, and temperature- and field-dependent resistivity and anisotropic magnetization. YMg₂Cu₉ is a non-local-moment-bearing metal with an electronic specific heat coefficient, γ ~ 15 mJ/mol K². Yb is divalent and basically non-moment-bearing in YbMg2Cu9. Ce is trivalent in CeMg₂Cu₉ with two magnetic transitions being observed at 2.1 K and 1.5 K. PrMg₂Cu₉ does not exhibit any magnetic phase transition down to 0.5 K. The other members being studied (R = Nd, Gd-Dy) all exhibit antiferromagnetic transitions at low temperatures ranging from 3.2 K for NdMg₂Cu₉ to 11.9 K for TbMg₂Cu₉. Whereas GdMg₂Cu₉ is isotropic in its paramagnetic state due to zero angular momentum (L = 0), all the other local-moment-bearing members manifest an anisotropic, planar magnetization in their paramagnetic states. To further study this planar anisotropy, detailed angular-dependent magnetization was carried out on magnetically diluted (Y_0.99Tb_0.01)Mg₂Cu₉ and (Y_0.99Dy_0.01)Mg₂Cu₉. Despite the strong, planar magnetization anisotropy, the in-plane magnetic anisotropy is weak and field-dependent. Finally, a set of crystal electric field parameters are proposed to explain the observed magnetic anisotropy.

Authors:

Kong, Tai ^[1]; Meier, William R. ^[1]; Lin, Qisheng ^[1]; Saunders, Scott M. ^[1]; Bud'ko, Sergey L. ^[1]; Flint, Rebecca ^[1]; Canfield, Paul C. ^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)

Publication Date:: 2016-10-24

Research Org.:: Ames Lab., Ames, IA (United States)

Sponsoring Org.:: USDOE

OSTI Identifier:: 1347414

Alternate Identifier(s):: OSTI ID: 1329957

Report Number(s):: IS-J-9195
Journal ID: ISSN 2469-9950; PRBMDO; TRN: US1701336

Grant/Contract Number:: AC02-07CH11358; GBMF4411

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 94; Journal Issue: 14; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Kong, Tai, Meier, William R., Lin, Qisheng, Saunders, Scott M., Bud'ko, Sergey L., Flint, Rebecca, and Canfield, Paul C. Physical properties of single crystalline RMg2Cu9 (R=Y,Ce-Nd,Gd-Dy,Yb) and the search for in-plane magnetic anisotropy in hexagonal systems.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevB.94.144434.

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                    Kong, Tai, Meier, William R., Lin, Qisheng, Saunders, Scott M., Bud'ko, Sergey L., Flint, Rebecca, & Canfield, Paul C. Physical properties of single crystalline RMg2Cu9 (R=Y,Ce-Nd,Gd-Dy,Yb) and the search for in-plane magnetic anisotropy in hexagonal systems.  United States.  https://doi.org/10.1103/PhysRevB.94.144434

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                    Kong, Tai, Meier, William R., Lin, Qisheng, Saunders, Scott M., Bud'ko, Sergey L., Flint, Rebecca, and Canfield, Paul C. Mon .  
"Physical properties of single crystalline RMg2Cu9 (R=Y,Ce-Nd,Gd-Dy,Yb) and the search for in-plane magnetic anisotropy in hexagonal systems".  United States.  https://doi.org/10.1103/PhysRevB.94.144434.  https://www.osti.gov/servlets/purl/1347414.

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@article{osti_1347414,

  title        = {Physical properties of single crystalline RMg2Cu9 (R=Y,Ce-Nd,Gd-Dy,Yb) and the search for in-plane magnetic anisotropy in hexagonal systems},

  author       = {Kong, Tai and Meier, William R. and Lin, Qisheng and Saunders, Scott M. and Bud'ko, Sergey L. and Flint, Rebecca and Canfield, Paul C.},

  abstractNote = {Single crystals of RMg2Cu9 (R=Y, Ce-Nd, Gd-Dy, Yb) were grown using a high-temperature solution growth technique and were characterized by measurements of room-temperature x-ray diffraction, temperature-dependent specific heat, and temperature- and field-dependent resistivity and anisotropic magnetization. YMg2Cu9 is a non-local-moment-bearing metal with an electronic specific heat coefficient, γ ~ 15 mJ/mol K2. Yb is divalent and basically non-moment-bearing in YbMg2Cu9. Ce is trivalent in CeMg2Cu9 with two magnetic transitions being observed at 2.1 K and 1.5 K. PrMg2Cu9 does not exhibit any magnetic phase transition down to 0.5 K. The other members being studied (R = Nd, Gd-Dy) all exhibit antiferromagnetic transitions at low temperatures ranging from 3.2 K for NdMg2Cu9 to 11.9 K for TbMg2Cu9. Whereas GdMg2Cu9 is isotropic in its paramagnetic state due to zero angular momentum (L = 0), all the other local-moment-bearing members manifest an anisotropic, planar magnetization in their paramagnetic states. To further study this planar anisotropy, detailed angular-dependent magnetization was carried out on magnetically diluted (Y0.99Tb0.01)Mg2Cu9 and (Y0.99Dy0.01)Mg2Cu9. Despite the strong, planar magnetization anisotropy, the in-plane magnetic anisotropy is weak and field-dependent. Finally, a set of crystal electric field parameters are proposed to explain the observed magnetic anisotropy.},

  doi          = {10.1103/PhysRevB.94.144434},

  journal      = {Physical Review B},

  number       = 14,

  volume       = 94,

  place        = {United States},

  year         = {2016},

  month        = {10}

}

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Title: Physical properties of single crystalline R Mg 2 Cu 9 ( R = Y , Ce - Nd , Gd - Dy , Yb ) and the search for in-plane magnetic anisotropy in hexagonal systems

Abstract

Citation Formats

Angular dependence of metamagnetic transitions in DyAgSb 2 journal, January 1999

Anisotropy and metamagnetism in the RNi2Ge2 (R=Y, La–Nd, Sm–Lu) series journal, October 1999

An empirical correction for absorption anisotropy journal, January 1995

Crystalline electric-field effects in single-crystal HoNi 2 B 2 C journal, February 1996

EXPGUI , a graphical user interface for GSAS journal, April 2001

Diamagnetic Corrections and Pascal's Constants journal, April 2008

Ferromagnetic spin fluctuations in quasi-2D—EuCu9Mg2 journal, October 2010

Angular dependence of metamagnetic transitions in HoNi 2 B 2 C journal, January 1997

High-temperature solution growth of intermetallic single crystals and quasicrystals journal, May 2001

The effect of a crystalline electric field on the magnetic transition temperatures of rare-earth rhodium borides journal, August 1982

Crystal-field effects of paramagnetic Curie temperature journal, June 1971

Magnetic properties of cerium monopnictides journal, February 1983

Calorimetric study of the antiferromagnetic transition in ytterbium sesquioxide journal, January 1994

Crystal-field effects and the magnetic properties of rare-earth rhodium borides journal, June 1984

Resistive Anomalies at Magnetic Critical Points journal, March 1968

Magnetic phase diagram of flux-grown single crystals of CeSb journal, May 2000

Specific heat in some gadolinium compounds. I. Experimental journal, June 1991

Crystalline electric field effects on the paramagnetic susceptibility of polycrystalline materials journal, June 1983

Theory of the coupling between conduction electrons and moments of 3d and 4f ions in metals journal, March 1978

Drastic annealing effects in transport properties of single crystals of the YbNi 2 B 2 C heavy fermion system journal, October 2002

Magnetic excitations in crystal-field split 4f systems journal, January 1985

Thermodynamic and transport properties of RAgGe (R=Tb–Lu) single crystals journal, June 2004

Thermodynamic and Transport Properties of CeMg 2 Cu 9 under Pressure journal, August 2004

Growth of single crystals from metallic fluxes journal, June 1992

Interactions indirectes entre couches 4f dans les métaux de terres rares journal, January 1962

Microscopic model for the magnetic subsystem in HoNi 2 B 2 C journal, March 1998

Systematic study of anisotropic transport and magnetic properties of RAgSb2 (R=Y, La–Nd, Sm, Gd–Tm) journal, October 1999

Pressure study of an antiferromagnet, CeMg 2 Cu 9 journal, March 2002

Angular-dependent planar metamagnetism in the hexagonal compounds TbPtIn and TmAgGe journal, January 2005

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Anisotropic magnetization and resistivity of single crystalline RNi1−xBi2±y (R=La–Nd, Sm, Gd–Dy) journal, March 2013

Thermodynamic and transport properties of single crystalline RCo2Ge2 (R=Y, La–Nd, Sm–Tm) journal, May 2014

Magnetic and transport properties of single-grain R − M g − Z n icosahedral quasicrystals [ R = Y , ( Y 1 − x Gd x ) , ( Y 1 − x Tb x ) , Tb, Dy, Ho, and Er] journal, January 1999

Angular dependence of metamagnetic transitions in RNi2B2C (R = Er, Ho, Dy, and Tb) journal, November 1997

Rare-earth ions in a hexaognal field I journal, November 1970

Relation between the specific heat and susceptibility of an antiferromagnet journal, October 1962

Ising model with solitons, phasons, and "the devil's staircase" journal, June 1980

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Title: Physical properties of single crystalline $R {Mg}_{2} {Cu}_{9}$ $(R = Y, Ce - Nd, Gd - Dy, Yb)$ and the search for in-plane magnetic anisotropy in hexagonal systems

Angular dependence of metamagnetic transitions in ${DyAgSb}_{2}$
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An empirical correction for absorption anisotropy
journal, January 1995

Crystalline electric-field effects in single-crystal ${HoNi}_{2}$ $B_{2}$ C
journal, February 1996

EXPGUI , a graphical user interface for GSAS
journal, April 2001

Diamagnetic Corrections and Pascal's Constants
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Angular dependence of metamagnetic transitions in ${HoNi}_{2}$ $B_{2}$ C
journal, January 1997

High-temperature solution growth of intermetallic single crystals and quasicrystals
journal, May 2001

The effect of a crystalline electric field on the magnetic transition temperatures of rare-earth rhodium borides
journal, August 1982

Crystal-field effects of paramagnetic Curie temperature
journal, June 1971

Magnetic properties of cerium monopnictides
journal, February 1983

Calorimetric study of the antiferromagnetic transition in ytterbium sesquioxide
journal, January 1994

Crystal-field effects and the magnetic properties of rare-earth rhodium borides
journal, June 1984

Resistive Anomalies at Magnetic Critical Points
journal, March 1968

Magnetic phase diagram of flux-grown single crystals of CeSb
journal, May 2000

Specific heat in some gadolinium compounds. I. Experimental
journal, June 1991

Crystalline electric field effects on the paramagnetic susceptibility of polycrystalline materials
journal, June 1983

Theory of the coupling between conduction electrons and moments of 3d and 4f ions in metals
journal, March 1978

Drastic annealing effects in transport properties of single crystals of the ${YbNi}_{2} B_{2} C$ heavy fermion system
journal, October 2002

Magnetic excitations in crystal-field split 4f systems
journal, January 1985

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journal, June 2004

Thermodynamic and Transport Properties of CeMg ₂ Cu ₉ under Pressure
journal, August 2004

Growth of single crystals from metallic fluxes
journal, June 1992

Interactions indirectes entre couches 4f dans les métaux de terres rares
journal, January 1962

Microscopic model for the magnetic subsystem in ${HoNi}_{2} B_{2} C$
journal, March 1998

Systematic study of anisotropic transport and magnetic properties of RAgSb2 (R=Y, La–Nd, Sm, Gd–Tm)
journal, October 1999

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journal, March 2002

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journal, January 2005

Rare earth–copper–magnesium compounds RECu9Mg2 (RE=Y, La–Nd, Sm–Ho, Yb) with ordered CeNi3-type structure
journal, October 2006

Anisotropic magnetization and resistivity of single crystalline RNi1−xBi2±y (R=La–Nd, Sm, Gd–Dy)
journal, March 2013

Thermodynamic and transport properties of single crystalline RCo2Ge2 (R=Y, La–Nd, Sm–Tm)
journal, May 2014

Magnetic and transport properties of single-grain $R - M g - Z n$ icosahedral quasicrystals [ $R = Y,$ $(Y_{1 - x} {Gd}_{x}),$ $(Y_{1 - x} {Tb}_{x}),$ Tb, Dy, Ho, and Er]
journal, January 1999

Angular dependence of metamagnetic transitions in RNi2B2C (R = Er, Ho, Dy, and Tb)
journal, November 1997

Rare-earth ions in a hexaognal field I
journal, November 1970

Relation between the specific heat and susceptibility of an antiferromagnet
journal, October 1962

Ising model with solitons, phasons, and "the devil's staircase"
journal, June 1980

Field induced magnetic structures in TbNi2Si2
journal, June 1991

Fulde–Ferrell State in Spin–Orbit-Coupled Superconductor: Application to Dresselhaus SOC
journal, May 2018

New materials physics
journal, November 2019