Self-Assembled Fe-N-Doped Carbon Nanotube Aerogels with Single-Atom Catalyst Feature as High-Efficiency Oxygen Reduction Electrocatalysts
Abstract
In this study, self-assembled M–N-doped carbon nanotube aerogels with single-atom catalyst feature are for the first time reported through one-step hydrothermal route and subsequent facile annealing treatment. By taking advantage of the porous nanostructures, 1D nanotubes as well as single-atom catalyst feature, the resultant Fe–N-doped carbon nanotube aerogels exhibit excellent oxygen reduction reaction electrocatalytic performance even better than commercial Pt/C in alkaline solution.
- Authors:
-
- School of Mechanical and Materials Engineering, Washington State University, Pullman WA 99164 USA
- Center for Functional Nanomaterials, Brookhaven National Laboratory, Upton NY 11973 USA
- Environmental Molecular Science Laboratory, Pacific Northwest National Laboratory, Richland WA 99354 USA
- Energy and Environmental Directory, Pacific Northwest National Laboratory, Richland WA 99354 USA
- School of Mechanical and Materials Engineering, Washington State University, Pullman WA 99164 USA; Environmental Molecular Science Laboratory, Pacific Northwest National Laboratory, Richland WA 99354 USA
- Publication Date:
- Research Org.:
- Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1347291
- Report Number(s):
- BNL-113588-2017-JA
Journal ID: ISSN 1613-6810; R&D Project: 16060; 16060; KC0403020
- Grant/Contract Number:
- SC00112704; AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Small
- Additional Journal Information:
- Journal Volume: 13; Journal Issue: 15; Journal ID: ISSN 1613-6810
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 77 NANOSCIENCE AND NANOTECHNOLOGY; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; Aerogels; transition metal–nitrogen–carbon structures; single-atom catalysts; nonprecious metal catalysts; oxygen reduction reaction
Citation Formats
Zhu, Chengzhou, Fu, Shaofang, Song, Junhua, Shi, Qiurong, Su, Dong, Engelhard, Mark H., Li, Xiaolin, Xiao, Dongdong, Li, Dongsheng, Estevez, Luis, Du, Dan, and Lin, Yuehe. Self-Assembled Fe-N-Doped Carbon Nanotube Aerogels with Single-Atom Catalyst Feature as High-Efficiency Oxygen Reduction Electrocatalysts. United States: N. p., 2017.
Web. doi:10.1002/smll.201603407.
Zhu, Chengzhou, Fu, Shaofang, Song, Junhua, Shi, Qiurong, Su, Dong, Engelhard, Mark H., Li, Xiaolin, Xiao, Dongdong, Li, Dongsheng, Estevez, Luis, Du, Dan, & Lin, Yuehe. Self-Assembled Fe-N-Doped Carbon Nanotube Aerogels with Single-Atom Catalyst Feature as High-Efficiency Oxygen Reduction Electrocatalysts. United States. https://doi.org/10.1002/smll.201603407
Zhu, Chengzhou, Fu, Shaofang, Song, Junhua, Shi, Qiurong, Su, Dong, Engelhard, Mark H., Li, Xiaolin, Xiao, Dongdong, Li, Dongsheng, Estevez, Luis, Du, Dan, and Lin, Yuehe. Mon .
"Self-Assembled Fe-N-Doped Carbon Nanotube Aerogels with Single-Atom Catalyst Feature as High-Efficiency Oxygen Reduction Electrocatalysts". United States. https://doi.org/10.1002/smll.201603407. https://www.osti.gov/servlets/purl/1347291.
@article{osti_1347291,
title = {Self-Assembled Fe-N-Doped Carbon Nanotube Aerogels with Single-Atom Catalyst Feature as High-Efficiency Oxygen Reduction Electrocatalysts},
author = {Zhu, Chengzhou and Fu, Shaofang and Song, Junhua and Shi, Qiurong and Su, Dong and Engelhard, Mark H. and Li, Xiaolin and Xiao, Dongdong and Li, Dongsheng and Estevez, Luis and Du, Dan and Lin, Yuehe},
abstractNote = {In this study, self-assembled M–N-doped carbon nanotube aerogels with single-atom catalyst feature are for the first time reported through one-step hydrothermal route and subsequent facile annealing treatment. By taking advantage of the porous nanostructures, 1D nanotubes as well as single-atom catalyst feature, the resultant Fe–N-doped carbon nanotube aerogels exhibit excellent oxygen reduction reaction electrocatalytic performance even better than commercial Pt/C in alkaline solution.},
doi = {10.1002/smll.201603407},
journal = {Small},
number = 15,
volume = 13,
place = {United States},
year = {Mon Feb 06 00:00:00 EST 2017},
month = {Mon Feb 06 00:00:00 EST 2017}
}
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