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Title: Doping dependence of the magnetic excitations in La 2 - x Sr x CuO 4

Abstract

The magnetic correlations within the cuprates have undergone intense scrutiny as part of efforts to understand high-temperature superconductivity. We explore the evolution of the magnetic correlations along the nodal direction of the Brillouin zone in La2–xSrxCuO4, spanning the doping phase diagram from the antiferromagnetic Mott insulator at x = 0 to the metallic phase at x = 0.26. Magnetic excitations along this direction are found to be systematically softened and broadened with doping, at a higher rate than the excitations along the antinodal direction. This phenomenology is discussed in terms of the nature of the magnetism in the doped cuprates. As a result, survival of the high-energy magnetic excitations, even in the overdoped regime, indicates that these excitations are marginal to pairing, while the influence of the low-energy excitations remains ambiguous.

Authors:
 [1];  [1];  [2];  [1];  [3];  [4];  [5];  [5];  [6];  [6];  [7];  [1];  [8];  [8];  [5];  [1]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States)
  2. Diamond Light Source, Ltd., Oxfordshire (United Kingdom)
  3. Univ. of Bristol, Bristol (United Kingdom)
  4. Univ. Pierre et Marie Curie - Case 115, Paris Cedex 05 (France)
  5. Paul Scherrer Inst. (PSI), Villigen (Switzerland)
  6. National Synchrotron Radiation Research Center, Hsinchu (Taiwan)
  7. National Synchrotron Radiation Research Center, Hsinchu (Taiwan); National Tsing Hua Univ., Hsinchu (Taiwan)
  8. Brookhaven National Lab. (BNL), Upton, NY (United States); Yale Univ., New Haven, CT (United States)
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1345728
Alternate Identifier(s):
OSTI ID: 1344594
Report Number(s):
BNL-113511-2017-JA
Journal ID: ISSN 2469-9950; PRBMDO; R&D Project: PO011; MA509MACA; KC0201060; KC0203020; TRN: US1700848
Grant/Contract Number:  
SC00112704; 1047478
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 95; Journal Issue: 7; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Meyers, D., Miao, H., Walters, A. C., Bisogni, V., Springell, R. S., d'Astuto, M., Dantz, M., Pelliciari, J., Huang, H. Y., Okamoto, J., Huang, D. J., Hill, J. P., He, X., Bozovic, I., Schmitt, T., and Dean, M. P. M. Doping dependence of the magnetic excitations in La2-xSrxCuO4. United States: N. p., 2017. Web. doi:10.1103/PhysRevB.95.075139.
Meyers, D., Miao, H., Walters, A. C., Bisogni, V., Springell, R. S., d'Astuto, M., Dantz, M., Pelliciari, J., Huang, H. Y., Okamoto, J., Huang, D. J., Hill, J. P., He, X., Bozovic, I., Schmitt, T., & Dean, M. P. M. Doping dependence of the magnetic excitations in La2-xSrxCuO4. United States. https://doi.org/10.1103/PhysRevB.95.075139
Meyers, D., Miao, H., Walters, A. C., Bisogni, V., Springell, R. S., d'Astuto, M., Dantz, M., Pelliciari, J., Huang, H. Y., Okamoto, J., Huang, D. J., Hill, J. P., He, X., Bozovic, I., Schmitt, T., and Dean, M. P. M. Wed . "Doping dependence of the magnetic excitations in La2-xSrxCuO4". United States. https://doi.org/10.1103/PhysRevB.95.075139. https://www.osti.gov/servlets/purl/1345728.
@article{osti_1345728,
title = {Doping dependence of the magnetic excitations in La2-xSrxCuO4},
author = {Meyers, D. and Miao, H. and Walters, A. C. and Bisogni, V. and Springell, R. S. and d'Astuto, M. and Dantz, M. and Pelliciari, J. and Huang, H. Y. and Okamoto, J. and Huang, D. J. and Hill, J. P. and He, X. and Bozovic, I. and Schmitt, T. and Dean, M. P. M.},
abstractNote = {The magnetic correlations within the cuprates have undergone intense scrutiny as part of efforts to understand high-temperature superconductivity. We explore the evolution of the magnetic correlations along the nodal direction of the Brillouin zone in La2–xSrxCuO4, spanning the doping phase diagram from the antiferromagnetic Mott insulator at x = 0 to the metallic phase at x = 0.26. Magnetic excitations along this direction are found to be systematically softened and broadened with doping, at a higher rate than the excitations along the antinodal direction. This phenomenology is discussed in terms of the nature of the magnetism in the doped cuprates. As a result, survival of the high-energy magnetic excitations, even in the overdoped regime, indicates that these excitations are marginal to pairing, while the influence of the low-energy excitations remains ambiguous.},
doi = {10.1103/PhysRevB.95.075139},
journal = {Physical Review B},
number = 7,
volume = 95,
place = {United States},
year = {Wed Feb 15 00:00:00 EST 2017},
month = {Wed Feb 15 00:00:00 EST 2017}
}

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Cited by: 24 works
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Works referenced in this record:

Persistence of High-Frequency Spin Fluctuations in Overdoped Superconducting La 2 x Sr x CuO 4 ( x = 0.22 )
journal, August 2007


Extracting paramagnon excitations from resonant inelastic x-ray scattering experiments
journal, June 2016


Two energy scales in the spin excitations of the high-temperature superconductor La2−xSrxCuO4
journal, February 2007

  • Vignolle, B.; Hayden, S. M.; McMorrow, D. F.
  • Nature Physics, Vol. 3, Issue 3
  • DOI: 10.1038/nphys546

Magnetic energy change available to superconducting condensation in optimally doped YBa2Cu3O6.95
journal, August 2006

  • Woo, Hyungje; Dai, Pengcheng; Hayden, S. M.
  • Nature Physics, Vol. 2, Issue 9
  • DOI: 10.1038/nphys394

Collective Nature of Spin Excitations in Superconducting Cuprates Probed by Resonant Inelastic X-Ray Scattering
journal, May 2015


Magnetic excitations in stripe-ordered La 1.875 Ba 0.125 CuO 4 studied using resonant inelastic x-ray scattering
journal, July 2013


Resonant inelastic x-ray scattering studies of elementary excitations
journal, June 2011

  • Ament, Luuk J. P.; van Veenendaal, Michel; Devereaux, Thomas P.
  • Reviews of Modern Physics, Vol. 83, Issue 2
  • DOI: 10.1103/RevModPhys.83.705

The effect of collective spin-1 excitations on electronic spectra in high- T c superconductors
journal, January 2006


Persistence of magnetic excitations in La2−xSrxCuO4 from the undoped insulator to the heavily overdoped non-superconducting metal
journal, August 2013

  • Dean, M. P. M.; Dellea, G.; Springell, R. S.
  • Nature Materials, Vol. 12, Issue 11
  • DOI: 10.1038/nmat3723

Direct Relation between the Low-Energy Spin Excitations and Superconductivity of Overdoped High- T c Superconductors
journal, May 2004


Itinerant effects and enhanced magnetic interactions in Bi-based multilayer cuprates
journal, December 2014


Highly efficient beamline and spectrometer for inelastic soft X-ray scattering at high resolution
journal, January 2014


Spin excitations in a single La2CuO4 layer
journal, September 2012

  • Dean, M. P. M.; Springell, R. S.; Monney, C.
  • Nature Materials, Vol. 11, Issue 10
  • DOI: 10.1038/nmat3409

Magnetic Excitations and Phase Separation in the Underdoped La 2 x Sr x CuO 4 Superconductor Measured by Resonant Inelastic X-Ray Scattering
journal, February 2010


Persistent spin excitations in doped antiferromagnets revealed by resonant inelastic light scattering
journal, February 2014

  • Jia, C. J.; Nowadnick, E. A.; Wohlfeld, K.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4314

Testing the itinerancy of spin dynamics in superconducting Bi2Sr2CaCu2O8+δ
journal, August 2009

  • Xu, Guangyong; Gu, G. D.; Hücker, M.
  • Nature Physics, Vol. 5, Issue 9
  • DOI: 10.1038/nphys1360

Quantum magnetic excitations from stripes in copper oxide superconductors
journal, June 2004

  • Tranquada, J. M.; Woo, H.; Perring, T. G.
  • Nature, Vol. 429, Issue 6991
  • DOI: 10.1038/nature02574

The structure of the high-energy spin excitations in a high-transition-temperature superconductor
journal, June 2004

  • Hayden, S. M.; Mook, H. A.; Dai, Pengcheng
  • Nature, Vol. 429, Issue 6991
  • DOI: 10.1038/nature02576

Raman and fluorescence characteristics of resonant inelastic X-ray scattering from doped superconducting cuprates
journal, January 2016

  • Huang, H. Y.; Jia, C. J.; Chen, Z. Y.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep19657

Magnetic response in the underdoped cuprates
journal, September 2012


The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering
journal, November 2014

  • Braicovich, L.; Minola, M.; Dellea, G.
  • Review of Scientific Instruments, Vol. 85, Issue 11
  • DOI: 10.1063/1.4900959

From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015

  • Keimer, B.; Kivelson, S. A.; Norman, M. R.
  • Nature, Vol. 518, Issue 7538
  • DOI: 10.1038/nature14165

SAXES, a high resolution spectrometer for resonant x-ray emission in the 400–1600eV energy range
journal, November 2006

  • Ghiringhelli, G.; Piazzalunga, A.; Dallera, C.
  • Review of Scientific Instruments, Vol. 77, Issue 11
  • DOI: 10.1063/1.2372731

First-principles calculations of phonon dispersion and lattice dynamics in La 2 CuO 4
journal, April 1999


Insights into the high temperature superconducting cuprates from resonant inelastic X-ray scattering
journal, February 2015


Correlated electrons in high-temperature superconductors
journal, July 1994


Anisotropic softening of magnetic excitations along the nodal direction in superconducting cuprates
journal, December 2014

  • Guarise, M.; Piazza, B. Dalla; Berger, H.
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms6760

Collective spin excitations in the singlet-correlated band model: a comparison with resonant inelastic x-ray scattering
journal, July 2013


Lattice symmetry breaking in cuprate superconductors: stripes, nematics, and superconductivity
journal, November 2009


Intense paramagnon excitations in a large family of high-temperature superconductors
journal, July 2011

  • Le Tacon, M.; Ghiringhelli, G.; Chaloupka, J.
  • Nature Physics, Vol. 7, Issue 9
  • DOI: 10.1038/nphys2041

Self-energy effects in electronic Raman spectra of doped cuprates due to magnetic fluctuations
journal, June 2013


High-resolution soft X-ray beamline ADRESS at the Swiss Light Source for resonant inelastic X-ray scattering and angle-resolved photoelectron spectroscopies
journal, July 2010

  • Strocov, V. N.; Schmitt, T.; Flechsig, U.
  • Journal of Synchrotron Radiation, Vol. 17, Issue 5
  • DOI: 10.1107/S0909049510019862

Theoretical determination of strong electron-phonon coupling in YBa 2 Cu 3 O 7
journal, May 1990


Bimagnon studies in cuprates with resonant inelastic x-ray scattering at the O K edge. II. Doping effect in La 2 x Sr x CuO 4
journal, June 2012


Progress in Neutron Scattering Studies of Spin Excitations in High- T c Cuprates
journal, January 2012

  • Fujita, Masaki; Hiraka, Haruhiro; Matsuda, Masaaki
  • Journal of the Physical Society of Japan, Vol. 81, Issue 1
  • DOI: 10.1143/JPSJ.81.011007

Atomic-layer engineering of superconducting oxides: yesterday, today, tomorrow
journal, March 2001

  • Bozovic, I.
  • IEEE Transactions on Appiled Superconductivity, Vol. 11, Issue 1
  • DOI: 10.1109/77.919617

Doping a Mott insulator: Physics of high-temperature superconductivity
journal, January 2006

  • Lee, Patrick A.; Nagaosa, Naoto; Wen, Xiao-Gang
  • Reviews of Modern Physics, Vol. 78, Issue 1
  • DOI: 10.1103/RevModPhys.78.17

Quenched Magnon excitations by oxygen sublattice reconstruction in (SrCuO2)n/(SrTiO3)2 superlattices
journal, September 2016

  • Dantz, M.; Pelliciari, J.; Samal, D.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep32896

Signatures of strong correlation effects in resonant inelastic x-ray scattering studies on cuprates
journal, August 2016


The Spin Excitation Spectrum in Superconducting YBa2Cu3O6.85
journal, May 2000


Spin Waves and Electronic Interactions in La 2 CuO 4
journal, June 2001


Anomalous High-Energy Spin Excitations in the High- T c Superconductor-Parent Antiferromagnet La 2 CuO 4
journal, December 2010


Infrared signatures of hole and spin stripes in La 2 x Sr x Cu O 4
journal, November 2005


A common thread: The pairing interaction for unconventional superconductors
journal, October 2012


High-Energy Kink in the Single-Particle Spectra of the Two-Dimensional Hubbard Model
journal, December 2007


Works referencing / citing this record:

Damped spin excitations in a doped cuprate superconductor with orbital hybridization
text, January 2017