Measurement of the neutron-induced reaction cross sections
Abstract
The neutron-induced reaction cross sections of 242mAm were measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. A new neutron-capture cross section was determined, and the absolute scale was set according to a concurrent measurement of the well-known 242mAm(n,f) cross section. The (n,γ) cross section was measured from thermal energy to an incident energy of 1 eV at which point the data quality was limited by the reaction yield in the laboratory. Our new 242mAm fission cross section was normalized to ENDF/B-VII.1 to set the absolute scale, and it agreed well with the (n,f) cross section from thermal energy to 1 keV. Lastly, the average absolute capture-to-fission ratio was determined from thermal energy to En = 0.1 eV, and it was found to be 26(4)% as opposed to the ratio of 19% from the ENDF/B-VII.1 evaluation.
- Authors:
-
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
- North Carolina State Univ., Raleigh, NC (United States)
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Publication Date:
- Research Org.:
- Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- Contributing Org.:
- DANCE Collaboration
- OSTI Identifier:
- 1345338
- Alternate Identifier(s):
- OSTI ID: 1344190
- Report Number(s):
- LLNL-JRNL-700220
Journal ID: ISSN 2469-9985; PRVCAN; TRN: US1700707
- Grant/Contract Number:
- AC52-07NA27344; AC52-06NA25396
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review C
- Additional Journal Information:
- Journal Volume: 95; Journal Issue: 2; Journal ID: ISSN 2469-9985
- Publisher:
- APS
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 11 NUCLEAR FUEL CYCLE AND RUEL MATERIALS; 73 NUCLEAR PHYSICS AND RADIATION PHYSICS; 29 ENERGY PLANNING, POLICY AND ECONOMY
Citation Formats
Buckner, M. Q., Wu, C. Y., Henderson, R. A., Bucher, B., Wimer, N., Chyzh, A., Bredeweg, T. A., Baramsai, B., Couture, A., Jandel, M., Mosby, S., and Ullmann, J. L. Measurement of the Am242m neutron-induced reaction cross sections. United States: N. p., 2017.
Web. doi:10.1103/PhysRevC.95.024610.
Buckner, M. Q., Wu, C. Y., Henderson, R. A., Bucher, B., Wimer, N., Chyzh, A., Bredeweg, T. A., Baramsai, B., Couture, A., Jandel, M., Mosby, S., & Ullmann, J. L. Measurement of the Am242m neutron-induced reaction cross sections. United States. https://doi.org/10.1103/PhysRevC.95.024610
Buckner, M. Q., Wu, C. Y., Henderson, R. A., Bucher, B., Wimer, N., Chyzh, A., Bredeweg, T. A., Baramsai, B., Couture, A., Jandel, M., Mosby, S., and Ullmann, J. L. Fri .
"Measurement of the Am242m neutron-induced reaction cross sections". United States. https://doi.org/10.1103/PhysRevC.95.024610. https://www.osti.gov/servlets/purl/1345338.
@article{osti_1345338,
title = {Measurement of the Am242m neutron-induced reaction cross sections},
author = {Buckner, M. Q. and Wu, C. Y. and Henderson, R. A. and Bucher, B. and Wimer, N. and Chyzh, A. and Bredeweg, T. A. and Baramsai, B. and Couture, A. and Jandel, M. and Mosby, S. and Ullmann, J. L.},
abstractNote = {The neutron-induced reaction cross sections of 242mAm were measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. A new neutron-capture cross section was determined, and the absolute scale was set according to a concurrent measurement of the well-known 242mAm(n,f) cross section. The (n,γ) cross section was measured from thermal energy to an incident energy of 1 eV at which point the data quality was limited by the reaction yield in the laboratory. Our new 242mAm fission cross section was normalized to ENDF/B-VII.1 to set the absolute scale, and it agreed well with the (n,f) cross section from thermal energy to 1 keV. Lastly, the average absolute capture-to-fission ratio was determined from thermal energy to En = 0.1 eV, and it was found to be 26(4)% as opposed to the ratio of 19% from the ENDF/B-VII.1 evaluation.},
doi = {10.1103/PhysRevC.95.024610},
journal = {Physical Review C},
number = 2,
volume = 95,
place = {United States},
year = {Fri Feb 17 00:00:00 EST 2017},
month = {Fri Feb 17 00:00:00 EST 2017}
}
Web of Science
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