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Title: Exploratory study of fission product yield determination from photofission of Pu 239 at 11 MeV with monoenergetic photons

Abstract

Here, measurements of fission product yields play an important role for the understanding of fundamental aspects of the fission process. Recently, neutron-induced fission product-yield data of 239Pu at energies below 4 MeV revealed an unexpected energy dependence of certain fission fragments. In order to investigate whether this observation is prerogative to neutron-induced fission, a program has been initiated to measure fission product yields in photoinduced fission. Here we report on the first ever photofission product yield measurement with monoenergetic photons produced by Compton back-scattering of FEL photons. The experiment was performed at the High-Intensity Gamma-ray Source at Triangle Universities Nuclear Laboratory on 239Pu at Eγ = 11 MeV. In this exploratory study the yield of eight fission products ranging from 91Sr to 143Ce has been obtained.

Authors:
 [1];  [1];  [1];  [2]
  1. Duke Univ., Durham, NC (United States)
  2. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Publication Date:
Research Org.:
Duke Univ., Durham, NC (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1349999
Alternate Identifier(s):
OSTI ID: 1343783
Grant/Contract Number:  
NA0001838; FG02-97ER41033; AC52-07NA27344
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review C
Additional Journal Information:
Journal Volume: 95; Journal Issue: 2; Journal ID: ISSN 2469-9985
Publisher:
APS
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; fission; photofission; fission product yields

Citation Formats

Bhike, Megha, Tornow, W., Krishichayan, -, and Tonchev, A. P. Exploratory study of fission product yield determination from photofission of Pu239 at 11 MeV with monoenergetic photons. United States: N. p., 2017. Web. doi:10.1103/PhysRevC.95.024608.
Bhike, Megha, Tornow, W., Krishichayan, -, & Tonchev, A. P. Exploratory study of fission product yield determination from photofission of Pu239 at 11 MeV with monoenergetic photons. United States. https://doi.org/10.1103/PhysRevC.95.024608
Bhike, Megha, Tornow, W., Krishichayan, -, and Tonchev, A. P. Tue . "Exploratory study of fission product yield determination from photofission of Pu239 at 11 MeV with monoenergetic photons". United States. https://doi.org/10.1103/PhysRevC.95.024608. https://www.osti.gov/servlets/purl/1349999.
@article{osti_1349999,
title = {Exploratory study of fission product yield determination from photofission of Pu239 at 11 MeV with monoenergetic photons},
author = {Bhike, Megha and Tornow, W. and Krishichayan, - and Tonchev, A. P.},
abstractNote = {Here, measurements of fission product yields play an important role for the understanding of fundamental aspects of the fission process. Recently, neutron-induced fission product-yield data of 239Pu at energies below 4 MeV revealed an unexpected energy dependence of certain fission fragments. In order to investigate whether this observation is prerogative to neutron-induced fission, a program has been initiated to measure fission product yields in photoinduced fission. Here we report on the first ever photofission product yield measurement with monoenergetic photons produced by Compton back-scattering of FEL photons. The experiment was performed at the High-Intensity Gamma-ray Source at Triangle Universities Nuclear Laboratory on 239Pu at Eγ = 11 MeV. In this exploratory study the yield of eight fission products ranging from 91Sr to 143Ce has been obtained.},
doi = {10.1103/PhysRevC.95.024608},
journal = {Physical Review C},
number = 2,
volume = 95,
place = {United States},
year = {Tue Feb 14 00:00:00 EST 2017},
month = {Tue Feb 14 00:00:00 EST 2017}
}

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Works referenced in this record:

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Works referencing / citing this record:

Review on the progress in nuclear fission—experimental methods and theoretical descriptions
journal, September 2018