Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells
Abstract
A low-bandgap (1.33 eV) Sn-based MA0.5FA0.5Pb0.75Sn0.25I3 perovskite is developed via combined compositional, process, and interfacial engineering. It can deliver a high power conversion efficiency (PCE) of 14.19%. Lastly, a four-terminal all-perovskite tandem solar cell is demonstrated by combining this low-bandgap cell with a semitransparent MAPbI3 cell to achieve a high efficiency of 19.08%.
- Authors:
-
- Univ. of Washington, Seattle, WA (United States)
- Publication Date:
- Research Org.:
- Univ. of Washington, Seattle, WA (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- Contributing Org.:
- This work was supported by the Office of Naval Research (N00014-14-1-0246), the Asian Office of Aerospace R&D (FA2386-15-1-4106), and the Department of Energy SunShot (DE-EE0006710). A.K.-Y.J. thanks the Boeing-Johnson Foundation for financial support. Z.Y. thanks the financial support from Washington Research Foundation Innovation Fellowship. Part of this work was conducted at UW NNCI Washington Nanofabrication Facility and Molecular Analysis Facility (Supported in part by the National Science Foundation, Grant No. ECC-1542101) at University of Washington. The authors thank the material synthesis from Francis Lin. The authors also thank Chun-Chih Huang for the steady state PL measurement.
- OSTI Identifier:
- 1343608
- Report Number(s):
- DOE-UW-Jen-33
Journal ID: ISSN 0935-9648
- Grant/Contract Number:
- EE0006710
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 28; Journal Issue: 40; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY
Citation Formats
Yang, Zhibin, Rajagopal, Adharsh, Chueh, Chu -Chen, Jo, Sae Byeok, Liu, Bo, Zhao, Ting, and Jen, Alex K. -Y. Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells. United States: N. p., 2016.
Web. doi:10.1002/adma.201602696.
Yang, Zhibin, Rajagopal, Adharsh, Chueh, Chu -Chen, Jo, Sae Byeok, Liu, Bo, Zhao, Ting, & Jen, Alex K. -Y. Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells. United States. https://doi.org/10.1002/adma.201602696
Yang, Zhibin, Rajagopal, Adharsh, Chueh, Chu -Chen, Jo, Sae Byeok, Liu, Bo, Zhao, Ting, and Jen, Alex K. -Y. Mon .
"Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells". United States. https://doi.org/10.1002/adma.201602696. https://www.osti.gov/servlets/purl/1343608.
@article{osti_1343608,
title = {Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells},
author = {Yang, Zhibin and Rajagopal, Adharsh and Chueh, Chu -Chen and Jo, Sae Byeok and Liu, Bo and Zhao, Ting and Jen, Alex K. -Y.},
abstractNote = {A low-bandgap (1.33 eV) Sn-based MA0.5FA0.5Pb0.75Sn0.25I3 perovskite is developed via combined compositional, process, and interfacial engineering. It can deliver a high power conversion efficiency (PCE) of 14.19%. Lastly, a four-terminal all-perovskite tandem solar cell is demonstrated by combining this low-bandgap cell with a semitransparent MAPbI3 cell to achieve a high efficiency of 19.08%.},
doi = {10.1002/adma.201602696},
journal = {Advanced Materials},
number = 40,
volume = 28,
place = {United States},
year = {2016},
month = {8}
}
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- Werner, Jérémie; Niesen, Bjoern; Ballif, Christophe
- Advanced Materials Interfaces, Vol. 5, Issue 1
Enhanced Uniformity and Stability of Pb–Sn Perovskite Solar Cells via Me 4 NBr Passivation
journal, May 2019
- Du, Xingzhi; Qiu, Renzheng; Zou, Taoyu
- Advanced Materials Interfaces, Vol. 6, Issue 14
Integrating Properties Modification in the Synthesis of Metal Halide Perovskites
journal, November 2018
- Huang, Ke; Liu, Jinxin; Chang, Xuejiao
- Advanced Materials Technologies, Vol. 4, Issue 2
Plasmonic-Functionalized Broadband Perovskite Photodetector
journal, February 2018
- Du, Bowen; Yang, Wenqiang; Jiang, Qiao
- Advanced Optical Materials, Vol. 6, Issue 8
Efficient Monolithic Perovskite/Perovskite Tandem Solar Cells
journal, December 2016
- Forgács, Dávid; Gil-Escrig, Lidón; Pérez-Del-Rey, Daniel
- Advanced Energy Materials, Vol. 7, Issue 8
Carrier Interfacial Engineering by Bismuth Modification for Efficient and Thermoresistant Perovskite Solar Cells
journal, March 2018
- Chen, Cong; Liu, Dali; Zhang, Boxue
- Advanced Energy Materials, Vol. 8, Issue 20
Inorganic CsPb 1− x Sn x IBr 2 for Efficient Wide-Bandgap Perovskite Solar Cells
journal, May 2018
- Li, Nan; Zhu, Zonglong; Li, Jiangwei
- Advanced Energy Materials, Vol. 8, Issue 22
Perowskit-Solarzellen: atomare Ebene, Schichtqualität und Leistungsfähigkeit der Zellen
journal, February 2018
- Saliba, Michael; Correa-Baena, Juan-Pablo; Grätzel, Michael
- Angewandte Chemie, Vol. 130, Issue 10
Homogenous Alloys of Formamidinium Lead Triiodide and Cesium Tin Triiodide for Efficient Ideal‐Bandgap Perovskite Solar Cells
journal, July 2017
- Zong, Yingxia; Wang, Ning; Zhang, Lin
- Angewandte Chemie, Vol. 129, Issue 41
The detailed balance limit of perovskite/silicon and perovskite/CdTe tandem solar cells: Detailed balance limit of tandem solar cells
journal, February 2017
- Rühle, Sven
- physica status solidi (a), Vol. 214, Issue 5
Realizing High Efficiency over 20% of Low‐Bandgap Pb–Sn‐Alloyed Perovskite Solar Cells by In Situ Reduction of Sn 4+
journal, December 2019
- Jiang, Tingming; Chen, Zeng; Chen, Xu
- Solar RRL, Vol. 4, Issue 3
Impact of cesium on the phase and device stability of triple cation Pb–Sn double halide perovskite films and solar cells
journal, January 2018
- Tosado, Gabriella A.; Lin, Yi-Yu; Zheng, Erjin
- Journal of Materials Chemistry A, Vol. 6, Issue 36
Tin( iv ) dopant removal through anti-solvent engineering enabling tin based perovskite solar cells with high charge carrier mobilities
journal, January 2019
- Bandara, R. M. I.; Jayawardena, K. D. G. I.; Adeyemo, S. O.
- Journal of Materials Chemistry C, Vol. 7, Issue 27
Enhancing electron diffusion length in narrow-bandgap perovskites for efficient monolithic perovskite tandem solar cells
text, January 2019
- Z., Ni,; J., Huang,; J., Zhao,
- The University of North Carolina at Chapel Hill University Libraries
Polyelemental, Multicomponent Perovskite Semiconductor Libraries through Combinatorial Screening
conference, March 2020
- Saliba, Michael
- 2nd nanoGe International Conference on Perovskite Thin Film Photovoltaics and Perovskite Photonics and Optoelectronics, Proceedings of the International Conference on Perovskite Thin Film Photovoltaics and Perovskite Photonics and Optoelectronics
Progress in Tandem Solar Cells Based on Hybrid Organic-Inorganic Perovskites
journal, March 2017
- Chen, Bo; Zheng, Xiaopeng; Bai, Yang
- Advanced Energy Materials, Vol. 7, Issue 14
Extending Photoresponse to the Near‐Infrared Region for Inverted Perovskite Solar Cells by Using a Low‐Bandgap Electron Transporting Material
journal, February 2020
- Wu, Fei; Gao, Wei; Zhu, Linna
- Solar RRL, Vol. 4, Issue 5
Tin(iv) dopant removal through anti-solvent engineering enabling tin based perovskite solar cells with high charge carrier mobilities
text, January 2019
- Bandara, Rmi; Jayawardena, Kdgi; Adeyemo, Stephanie
- Apollo - University of Cambridge Repository
Enhancing electron diffusion length in narrow-bandgap perovskites for efficient monolithic perovskite tandem solar cells
journal, October 2019
- Yang, Zhibin; Yu, Zhenhua; Wei, Haotong
- Nature Communications, Vol. 10, Issue 1
Polyelemental, Multicomponent Perovskite Semiconductor Libraries through Combinatorial Screening
conference, July 2019
- Saliba, Michael
- Proceedings of the nanoGe Fall Meeting 2019
Low‐Bandgap Mixed Tin‐Lead Perovskites and Their Applications in All‐Perovskite Tandem Solar Cells
journal, February 2019
- Wang, Changlei; Song, Zhaoning; Li, Chongwen
- Advanced Functional Materials, Vol. 29, Issue 47
Organic–Inorganic Copper (II)‐Based Perovskites: A Benign Approach toward Low‐Toxicity and Water‐Stable Light Absorbers for Photovoltaic Applications
journal, December 2019
- Ahmad, Khursheed; Mobin, Shaikh M.
- Energy Technology, Vol. 8, Issue 3
Opportunities and challenges for tandem solar cells using metal halide perovskite semiconductors
journal, July 2018
- Leijtens, Tomas; Bush, Kevin A.; Prasanna, Rohit
- Nature Energy, Vol. 3, Issue 10
Polyelemental, Multicomponent Perovskite Semiconductor Libraries through Combinatorial Screening
conference, November 2021
- Saliba, Michael
- nanoGe Fall Meeting 2019, Proceedings of the nanoGe Fall Meeting19
Compositionally Graded Absorber for Efficient and Stable Near-Infrared-Transparent Perovskite Solar Cells
journal, January 2018
- Fu, Fan; Pisoni, Stefano; Weiss, Thomas P.
- Advanced Science, Vol. 5, Issue 3
Sub-1.4eV bandgap inorganic perovskite solar cells with long-term stability
journal, January 2020
- Hu, Mingyu; Chen, Min; Guo, Peijun
- Nature Communications, Vol. 11, Issue 1
Perovskite solar cells: must lead be replaced – and can it be done?
journal, May 2018
- Zhang, Qi; Hao, Feng; Li, Jianbao
- Science and Technology of Advanced Materials, Vol. 19, Issue 1
Enhanced photovoltaic performance and stability with a new type of hollow 3D perovskite {en}FASnI 3
journal, August 2017
- Ke, Weijun; Stoumpos, Constantinos C.; Zhu, Menghua
- Science Advances, Vol. 3, Issue 8
Enhancing electron diffusion length in narrow-bandgap perovskites for efficient monolithic perovskite tandem solar cells
text, January 2019
- Z., Ni,; J., Huang,; J., Zhao,
- The University of North Carolina at Chapel Hill University Libraries