DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Statistical properties of Pu 243 , and Pu 242 (n,γ) cross section calculation

Abstract

The level density and γ-ray strength function (γSF) of Pu243 have been measured in the quasicontinuum using the Oslo method. Excited states in Pu243 were populated using the Pu242(d,p) reaction. The level density closely follows the constant-temperature level density formula for excitation energies above the pairing gap. The γSF displays a double-humped resonance at low energy as also seen in previous investigations of actinide isotopes. The structure is interpreted as the scissors resonance and has a centroid of ωSR=2.42(5) MeV and a total strength of BSR=10.1(15)μN2, which is in excellent agreement with sum-rule estimates. The measured level density and γSF were used to calculate the Pu242(n,γ) cross section in a neutron energy range for which there were previously no measured data.

Authors:
 [1];  [2];  [2];  [2];  [3];  [4];  [5];  [2];  [2];  [5];  [2];  [2];  [2];  [2];  [2];  [3];  [2];  [6];  [2];  [2] more »;  [2];  [2];  [2];  [7];  [8];  [6];  [3] « less
  1. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Berkeley, CA (United States)
  2. Univ. of Oslo, Oslo (Norway)
  3. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  4. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  5. Univ. of California, Berkeley, CA (United States)
  6. Institut de Physique Nucleaire d'Orsay, Orsay Cedex (France)
  7. Ohio Univ., Athens, OH (United States)
  8. iThemba LABS, Somerset West (South Africa)
Publication Date:
Research Org.:
Ohio Univ., Athens, OH (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC)
OSTI Identifier:
1338840
Alternate Identifier(s):
OSTI ID: 1236515; OSTI ID: 1430666
Grant/Contract Number:  
NA0002905; W-7405-Eng-48; AC52-07NA27344; AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review C
Additional Journal Information:
Journal Volume: 93; Journal Issue: 1; Journal ID: ISSN 2469-9985
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; gamma strength function; pygmy resonance

Citation Formats

Laplace, T. A., Zeiser, F., Guttormsen, M., Larsen, A. C., Bleuel, D. L., Bernstein, L. A., Goldblum, B. L., Siem, S., Garotte, F. L. Bello, Brown, J. A., Campo, L. Crespo, Eriksen, T. K., Giacoppo, F., Gorgen, A., Hadynska-Klek, K., Henderson, R. A., Klintefjord, M., Lebois, M., Renstrom, T., Rose, S. J., Sahin, E., Tornyi, T. G., Tveten, G. M., Voinov, A., Wiedeking, M., Wilson, J. N., and Younes, W. Statistical properties of Pu243 , and Pu242(n,γ) cross section calculation. United States: N. p., 2016. Web. doi:10.1103/PhysRevC.93.014323.
Laplace, T. A., Zeiser, F., Guttormsen, M., Larsen, A. C., Bleuel, D. L., Bernstein, L. A., Goldblum, B. L., Siem, S., Garotte, F. L. Bello, Brown, J. A., Campo, L. Crespo, Eriksen, T. K., Giacoppo, F., Gorgen, A., Hadynska-Klek, K., Henderson, R. A., Klintefjord, M., Lebois, M., Renstrom, T., Rose, S. J., Sahin, E., Tornyi, T. G., Tveten, G. M., Voinov, A., Wiedeking, M., Wilson, J. N., & Younes, W. Statistical properties of Pu243 , and Pu242(n,γ) cross section calculation. United States. https://doi.org/10.1103/PhysRevC.93.014323
Laplace, T. A., Zeiser, F., Guttormsen, M., Larsen, A. C., Bleuel, D. L., Bernstein, L. A., Goldblum, B. L., Siem, S., Garotte, F. L. Bello, Brown, J. A., Campo, L. Crespo, Eriksen, T. K., Giacoppo, F., Gorgen, A., Hadynska-Klek, K., Henderson, R. A., Klintefjord, M., Lebois, M., Renstrom, T., Rose, S. J., Sahin, E., Tornyi, T. G., Tveten, G. M., Voinov, A., Wiedeking, M., Wilson, J. N., and Younes, W. Fri . "Statistical properties of Pu243 , and Pu242(n,γ) cross section calculation". United States. https://doi.org/10.1103/PhysRevC.93.014323. https://www.osti.gov/servlets/purl/1338840.
@article{osti_1338840,
title = {Statistical properties of Pu243 , and Pu242(n,γ) cross section calculation},
author = {Laplace, T. A. and Zeiser, F. and Guttormsen, M. and Larsen, A. C. and Bleuel, D. L. and Bernstein, L. A. and Goldblum, B. L. and Siem, S. and Garotte, F. L. Bello and Brown, J. A. and Campo, L. Crespo and Eriksen, T. K. and Giacoppo, F. and Gorgen, A. and Hadynska-Klek, K. and Henderson, R. A. and Klintefjord, M. and Lebois, M. and Renstrom, T. and Rose, S. J. and Sahin, E. and Tornyi, T. G. and Tveten, G. M. and Voinov, A. and Wiedeking, M. and Wilson, J. N. and Younes, W.},
abstractNote = {The level density and γ-ray strength function (γSF) of Pu243 have been measured in the quasicontinuum using the Oslo method. Excited states in Pu243 were populated using the Pu242(d,p) reaction. The level density closely follows the constant-temperature level density formula for excitation energies above the pairing gap. The γSF displays a double-humped resonance at low energy as also seen in previous investigations of actinide isotopes. The structure is interpreted as the scissors resonance and has a centroid of ωSR=2.42(5) MeV and a total strength of BSR=10.1(15)μN2, which is in excellent agreement with sum-rule estimates. The measured level density and γSF were used to calculate the Pu242(n,γ) cross section in a neutron energy range for which there were previously no measured data.},
doi = {10.1103/PhysRevC.93.014323},
journal = {Physical Review C},
number = 1,
volume = 93,
place = {United States},
year = {Fri Jan 29 00:00:00 EST 2016},
month = {Fri Jan 29 00:00:00 EST 2016}
}

Journal Article:

Citation Metrics:
Cited by: 20 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

EMPIRE: Nuclear Reaction Model Code System for Data Evaluation
journal, December 2007


JENDL-4.0: A New Library for Nuclear Science and Engineering
journal, January 2011

  • Shibata, Keiichi; Iwamoto, Osamu; Nakagawa, Tsuneo
  • Journal of Nuclear Science and Technology, Vol. 48, Issue 1
  • DOI: 10.1080/18811248.2011.9711675

Nuclear data sensitivity, uncertainty and target accuracy assessment for future nuclear systems
journal, May 2006


Modern Nuclear Data Evaluation with the TALYS Code System
journal, December 2012


Skyrme-Hartree-Fock-Bogoliubov Nuclear Mass Formulas: Crossing the 0.6 MeV Accuracy Threshold with Microscopically Deduced Pairing
journal, April 2009


Modeling of the n + 242 Pu Reactions for Fast Reactor Applications
journal, June 2009

  • Rich, E.; Tudora, A.; Noguere, G.
  • Nuclear Science and Engineering, Vol. 162, Issue 2
  • DOI: 10.13182/NSE162-178

Photonuclear cross sections of Pu-239 using neutron capture gamma rays, near threshold
journal, April 1993


Electrodeposition of U and Pu on thin C and Ti substrates
journal, November 2011

  • Henderson, R. A.; Gostic, J. M.; Burke, J. T.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 655, Issue 1
  • DOI: 10.1016/j.nima.2011.06.023

Parameter-free description of orbital magnetic dipole strength
journal, January 2005


Experimental level densities of atomic nuclei
journal, December 2015

  • Guttormsen, M.; Aiche, M.; Bello Garrote, F. L.
  • The European Physical Journal A, Vol. 51, Issue 12
  • DOI: 10.1140/epja/i2015-15170-4

Level density and γ -ray strength function in the odd-odd Np 238 nucleus
journal, April 2014


Global coupled-channel optical potential for nucleon–actinide interaction from 1 keV to 200 MeV
journal, May 2004

  • Soukhovitskii, Efrem Sh; Chiba, Satoshi; Lee, Jeong-Yeon
  • Journal of Physics G: Nuclear and Particle Physics, Vol. 30, Issue 7
  • DOI: 10.1088/0954-3899/30/7/007

�ber die Gesamtst�rke der von einem Zustande ausgehenden Absorptionslinien
journal, December 1925


Extraction of level density and γ strength function from primary γ spectra
journal, June 2000

  • Schiller, A.; Bergholt, L.; Guttormsen, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 447, Issue 3
  • DOI: 10.1016/S0168-9002(99)01187-0

ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data
journal, December 2011


Orbital and spin scissors modes in superfluid nuclei
journal, June 2015


ENDF/B-VII.0: Next Generation Evaluated Nuclear Data Library for Nuclear Science and Technology
journal, December 2006


The SiRi particle-telescope system
journal, August 2011

  • Guttormsen, M.; Bürger, A.; Hansen, T. E.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 648, Issue 1
  • DOI: 10.1016/j.nima.2011.05.055

A statistical analysis of excited nuclear states
journal, May 1959


Systematics of nuclear level density parameters
journal, October 2005


Erratum: Systematics of nuclear level density parameters [Phys. Rev. C 72, 044311 (2005)]
journal, April 2006


Scissors resonance in the quasicontinuum of Th, Pa, and U isotopes
journal, January 2014


A Composite Nuclear-Level Density Formula with Shell Corrections
journal, August 1965

  • Gilbert, A.; Cameron, A. G. W.
  • Canadian Journal of Physics, Vol. 43, Issue 8
  • DOI: 10.1139/p65-139

γ -ray strength function and pygmy resonance in rare earth nuclei
journal, March 2001


Photofission and photoneutron cross sections and photofission neutron multiplicities for U 233 , U 234 , Np 237 , and Pu 239
journal, December 1986


Analysis of possible systematic errors in the Oslo method
journal, March 2011


Statistical Gamma-Decay at Low Angular Momentum
journal, January 1990


Sum rules and giant resonances in nuclei
journal, April 1989


Nuclear Data Sheets for A = 243
journal, September 2014


�ber die Zahl der Dispersionselektronen, die einem station�ren Zustand zugeordnet sind
journal, December 1925

  • Reiche, F.; Thomas, W.
  • Zeitschrift f�r Physik, Vol. 34, Issue 1
  • DOI: 10.1007/BF01328494

Constant-temperature level densities in the quasicontinuum of Th and U isotopes
journal, August 2013


Giant resonance in the total photoabsorption cross section of Z ≈ 90 nuclei
journal, November 1976


The r-process of stellar nucleosynthesis: Astrophysics and nuclear physics achievements and mysteries
journal, September 2007


Observation of Large Scissors Resonance Strength in Actinides
journal, October 2012


The first generation of γ-rays from hot nuclei
journal, April 1987

  • Guttormsen, M.; Ramsøy, T.; Rekstad, J.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 255, Issue 3
  • DOI: 10.1016/0168-9002(87)91221-6

The unfolding of continuum γ-ray spectra
journal, June 1996

  • Guttormsen, M.; Tveter, T. S.; Bergholt, L.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 374, Issue 3
  • DOI: 10.1016/0168-9002(96)00197-0

Test of gamma-ray strength functions in nuclear reaction model calculations
journal, May 1990


Total Neutron Cross Section of 242 Pu
journal, June 1970

  • Young, T. E.; Reeder, S. D.
  • Nuclear Science and Engineering, Vol. 40, Issue 3
  • DOI: 10.13182/NSE70-A20190

Neutron Capture Cross-Section Ratios of Plutonium-240 and Plutonium-242 Versus Gold-197 in the Energy Range from 50 to 250 keV
journal, January 1979

  • Wisshak, K.; Käppeler, F.
  • Nuclear Science and Engineering, Vol. 69, Issue 1
  • DOI: 10.13182/NSE79-A21283

Works referencing / citing this record:

Dynamic high energy density plasma environments at the National Ignition Facility for nuclear science research
journal, February 2018

  • Cerjan, Ch J.; Bernstein, L.; Hopkins, L. Berzak
  • Journal of Physics G: Nuclear and Particle Physics, Vol. 45, Issue 3
  • DOI: 10.1088/1361-6471/aa8693