DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: A non-LTE analysis of high energy density Kr plasmas on Z and NIF

Abstract

We report that multi-keV X-ray radiation sources have a wide range of applications, from biomedical studies and research on thermonuclear fusion to materials science and astrophysics. The refurbished Z pulsed power machine at the Sandia National Laboratories produces intense multi-keV X-rays from argon Z-pinches, but for a krypton Z-pinch, the yield decreases much faster with atomic number ZA than similar sources on the National Ignition Facility (NIF) laser at the Lawrence Livermore National Laboratory. To investigate whether fundamental energy deposition differences between pulsed power and lasers could account for the yield differences, we consider the Kr plasma on the two machines. The analysis assumes the plasma not in local thermodynamic equilibrium, with a detailed coupling between the hydrodynamics, the radiation field, and the ionization physics. While for the plasma parameters of interest the details of krypton’s M-shell are not crucial, both the L-shell and the K-shell must be modeled in reasonable detail, including the state-specific dielectronic recombination processes that significantly affect Kr’s ionization balance and the resulting X-ray spectrum. We present a detailed description of the atomic model, provide synthetic K- and L-shell spectra, and compare these with the available experimental data from the Z-machine and from NIF to showmore » that the K-shell yield behavior versus ZA is indeed related to the energy input characteristics. In conclusion, this work aims at understanding the probable causes that might explain the differences in the X-ray conversion efficiencies of several radiation sources on Z and« less

Authors:
 [1];  [2];  [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [3];  [3];  [3];  [3];  [3]; ORCiD logo [3];  [3];  [4]; ORCiD logo [5];  [5];  [5];  [5]; ORCiD logo [5];  [5]
  1. Naval Research Lab. (NRL), Washington, DC (United States). Plasma Physics Division
  2. Berkeley Research Associates, Beltsville, MD (United States)
  3. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  4. Engility Corporation, Chantilly, VA (United States)
  5. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Publication Date:
Research Org.:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1810679
Alternate Identifier(s):
OSTI ID: 1338408
Report Number(s):
LLNL-JRNL-692187; SAND-2016-12903J
Journal ID: ISSN 1070-664X; 818889; TRN: US2213075
Grant/Contract Number:  
AC52-07NA27344; AC04-94AL85000; AC04-94AL85000: AC52-07NA27344
Resource Type:
Accepted Manuscript
Journal Name:
Physics of Plasmas
Additional Journal Information:
Journal Volume: 23; Journal Issue: 10; Journal ID: ISSN 1070-664X
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
70 PLASMA PHYSICS AND FUSION TECHNOLOGY; plasma confinement; atomic physics; leptons; material science; hydrodynamics; chemical elements; x-ray spectroscopy; astrophysics; thermonuclear fusion; lasers

Citation Formats

Dasgupta, A., Clark, R. W., Ouart, N., Giuliani, J., Velikovich, A., Ampleford, D. J., Hansen, S. B., Jennings, C., Harvey-Thompson, A. J., Jones, B., Flanagan, T. M., Bell, K. S., Apruzese, J. P., Fournier, K. B., Scott, H. A., May, M. J., Barrios, M. A., Colvin, J. D., and Kemp, G. E. A non-LTE analysis of high energy density Kr plasmas on Z and NIF. United States: N. p., 2016. Web. doi:10.1063/1.4965243.
Dasgupta, A., Clark, R. W., Ouart, N., Giuliani, J., Velikovich, A., Ampleford, D. J., Hansen, S. B., Jennings, C., Harvey-Thompson, A. J., Jones, B., Flanagan, T. M., Bell, K. S., Apruzese, J. P., Fournier, K. B., Scott, H. A., May, M. J., Barrios, M. A., Colvin, J. D., & Kemp, G. E. A non-LTE analysis of high energy density Kr plasmas on Z and NIF. United States. https://doi.org/10.1063/1.4965243
Dasgupta, A., Clark, R. W., Ouart, N., Giuliani, J., Velikovich, A., Ampleford, D. J., Hansen, S. B., Jennings, C., Harvey-Thompson, A. J., Jones, B., Flanagan, T. M., Bell, K. S., Apruzese, J. P., Fournier, K. B., Scott, H. A., May, M. J., Barrios, M. A., Colvin, J. D., and Kemp, G. E. Thu . "A non-LTE analysis of high energy density Kr plasmas on Z and NIF". United States. https://doi.org/10.1063/1.4965243. https://www.osti.gov/servlets/purl/1810679.
@article{osti_1810679,
title = {A non-LTE analysis of high energy density Kr plasmas on Z and NIF},
author = {Dasgupta, A. and Clark, R. W. and Ouart, N. and Giuliani, J. and Velikovich, A. and Ampleford, D. J. and Hansen, S. B. and Jennings, C. and Harvey-Thompson, A. J. and Jones, B. and Flanagan, T. M. and Bell, K. S. and Apruzese, J. P. and Fournier, K. B. and Scott, H. A. and May, M. J. and Barrios, M. A. and Colvin, J. D. and Kemp, G. E.},
abstractNote = {We report that multi-keV X-ray radiation sources have a wide range of applications, from biomedical studies and research on thermonuclear fusion to materials science and astrophysics. The refurbished Z pulsed power machine at the Sandia National Laboratories produces intense multi-keV X-rays from argon Z-pinches, but for a krypton Z-pinch, the yield decreases much faster with atomic number ZA than similar sources on the National Ignition Facility (NIF) laser at the Lawrence Livermore National Laboratory. To investigate whether fundamental energy deposition differences between pulsed power and lasers could account for the yield differences, we consider the Kr plasma on the two machines. The analysis assumes the plasma not in local thermodynamic equilibrium, with a detailed coupling between the hydrodynamics, the radiation field, and the ionization physics. While for the plasma parameters of interest the details of krypton’s M-shell are not crucial, both the L-shell and the K-shell must be modeled in reasonable detail, including the state-specific dielectronic recombination processes that significantly affect Kr’s ionization balance and the resulting X-ray spectrum. We present a detailed description of the atomic model, provide synthetic K- and L-shell spectra, and compare these with the available experimental data from the Z-machine and from NIF to show that the K-shell yield behavior versus ZA is indeed related to the energy input characteristics. In conclusion, this work aims at understanding the probable causes that might explain the differences in the X-ray conversion efficiencies of several radiation sources on Z and},
doi = {10.1063/1.4965243},
journal = {Physics of Plasmas},
number = 10,
volume = 23,
place = {United States},
year = {Thu Oct 20 00:00:00 EDT 2016},
month = {Thu Oct 20 00:00:00 EDT 2016}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 4 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Two-dimensional radiation MHD modeling assessment of designs for argon gas puff distributions for future experiments on the refurbished Z machine
journal, September 2012


An analytic Voigt profile escape probability approximation
journal, November 1985


Spectroscopic analysis of Cu wire array implosions on the refurbished Z generator
journal, September 2012


X-ray power and yield measurements at the refurbished Z machine
journal, August 2014

  • Jones, M. C.; Ampleford, D. J.; Cuneo, M. E.
  • Review of Scientific Instruments, Vol. 85, Issue 8
  • DOI: 10.1063/1.4891316

Opacity and gradients in aluminum wire array z-pinch implosions on the Z pulsed power facility
journal, March 2014

  • Ampleford, D. J.; Hansen, S. B.; Jennings, C. A.
  • Physics of Plasmas, Vol. 21, Issue 3
  • DOI: 10.1063/1.4865224

K-shell X-ray sources at the Z Accelerator
journal, June 2010


The effect of gradients at stagnation on K-shell x-ray line emission in high-current Ar gas-puff implosions
journal, February 2015

  • Jones, B.; Apruzese, J. P.; Harvey-Thompson, A. J.
  • Physics of Plasmas, Vol. 22, Issue 2
  • DOI: 10.1063/1.4913350

Implosion dynamics and K-shell x-ray generation in large diameter stainless steel wire array Z pinches with various nesting configurations
journal, December 2008

  • Jones, Brent; Coverdale, Christine A.; Deeney, Christopher
  • Physics of Plasmas, Vol. 15, Issue 12
  • DOI: 10.1063/1.3049909

Multi-keV x-ray conversion efficiency in laser-produced plasmas
journal, May 2003

  • Back, C. A.; Davis, J.; Grun, J.
  • Physics of Plasmas, Vol. 10, Issue 5
  • DOI: 10.1063/1.1566750

Multi-keV x-ray source development experiments on the National Ignition Facility
journal, August 2010

  • Fournier, K. B.; May, M. J.; Colvin, J. D.
  • Physics of Plasmas, Vol. 17, Issue 8
  • DOI: 10.1063/1.3458904

Backlighter development at the National Ignition Facility (NIF): Zinc to zirconium
journal, September 2013


Efficient argon K -shell radiation from a Z pinch at currents >15 MA
journal, July 2001

  • Sze, H.; Coleman, P. L.; Banister, J.
  • Physics of Plasmas, Vol. 8, Issue 7
  • DOI: 10.1063/1.1373418

A probabilistic model for continuum transport in dense, optically thick plasmas
journal, March 1995

  • Clark, R. W.; Davis, J.; Apruzese, J. P.
  • Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 53, Issue 3
  • DOI: 10.1016/0022-4073(95)90062-4

Bright x-ray stainless steel K-shell source development at the National Ignition Facility
journal, June 2015

  • May, M. J.; Fournier, K. B.; Colvin, J. D.
  • Physics of Plasmas, Vol. 22, Issue 6
  • DOI: 10.1063/1.4922751

The physics of radiation transport in dense plasmas
journal, May 2002

  • Apruzese, J. P.; Davis, J.; Whitney, K. G.
  • Physics of Plasmas, Vol. 9, Issue 5
  • DOI: 10.1063/1.1446038

Fokker-Planck analysis of short-pulse laser heating in the hot-spot-model approximation
journal, December 1994


Demonstration of a 13-keV Kr K -shell x-ray source at the National Ignition Facility
journal, September 2013


K-α emission spectroscopic analysis from a Cu Z-pinch
journal, June 2013


Influence of L‐shell dynamics on K‐shell yields for imploding krypton Z‐pinch plasmas
journal, May 1995

  • Davis, J.; Giuliani, J. L.; Mulbrandon, M.
  • Physics of Plasmas, Vol. 2, Issue 5
  • DOI: 10.1063/1.871325

Architecture, implementation, and testing of a multiple-shell gas injection system for high current implosions on the Z accelerator
journal, June 2013

  • Krishnan, Mahadevan; Elliott, Kristi Wilson; Madden, Robert E.
  • Review of Scientific Instruments, Vol. 84, Issue 6
  • DOI: 10.1063/1.4809511

Measurement of the $\sim$0.1- to $>$ 10-keV Energy Distribution for an Argon Z -Pinch at the 15-MA Level
journal, February 2007

  • Coleman, Philip L.; Apruzese, J. P.; Velikovich, Alexander L.
  • IEEE Transactions on Plasma Science, Vol. 35, Issue 1
  • DOI: 10.1109/TPS.2006.889273

The physics basis for ignition using indirect-drive targets on the National Ignition Facility
journal, February 2004

  • Lindl, John D.; Amendt, Peter; Berger, Richard L.
  • Physics of Plasmas, Vol. 11, Issue 2
  • DOI: 10.1063/1.1578638

K-shell radiation physics in low- to moderate-atomic-number z-pinch plasmas on the Z accelerator
journal, May 2006

  • Jones, B.; Deeney, C.; Coverdale, C. A.
  • Journal of Quantitative Spectroscopy and Radiative Transfer, Vol. 99, Issue 1-3
  • DOI: 10.1016/j.jqsrt.2005.05.027

A Renewed Capability for Gas Puff Science on Sandia's Z Machine
journal, May 2014

  • Jones, Brent; Jennings, Christopher A.; Lamppa, Derek C.
  • IEEE Transactions on Plasma Science, Vol. 42, Issue 5
  • DOI: 10.1109/TPS.2013.2287180

Contrasting physics in wire array z pinch sources of 1-20 keV emission on the Z facility
journal, May 2014

  • Ampleford, D. J.; Jones, B.; Jennings, C. A.
  • Physics of Plasmas, Vol. 21, Issue 5
  • DOI: 10.1063/1.4876621

Tungsten wire-array Z-pinch experiments at 200 TW and 2 MJ
journal, May 1998

  • Spielman, R. B.; Deeney, C.; Chandler, G. A.
  • Physics of Plasmas, Vol. 5, Issue 5
  • DOI: 10.1063/1.872881

Time-Integrated Synthetic X-Ray Spectroscopy for Stainless Steel Wire Array $Z$-Pinches
journal, April 2010

  • Dasgupta, Arati; Giuliani, John L.; Davis, Jack
  • IEEE Transactions on Plasma Science, Vol. 38, Issue 4
  • DOI: 10.1109/TPS.2010.2040841

Investigation of K‐shell emission from moderate‐Z, low‐η (‐velocity), Z‐pinch implosions
journal, July 1996

  • Thornhill, J. W.; Whitney, K. G.; Davis, J.
  • Journal of Applied Physics, Vol. 80, Issue 2
  • DOI: 10.1063/1.362923

Large diameter (45–80mm) nested stainless steel wire arrays at the Z accelerator
journal, February 2008

  • Coverdale, C. A.; Deeney, C.; LePell, P. D.
  • Physics of Plasmas, Vol. 15, Issue 2
  • DOI: 10.1063/1.2840641

Simulation study of 3–5 keV x-ray conversion efficiency from Ar K-shell vs. Ag L-shell targets on the National Ignition Facility laser
journal, May 2015

  • Kemp, G. E.; Colvin, J. D.; Fournier, K. B.
  • Physics of Plasmas, Vol. 22, Issue 5
  • DOI: 10.1063/1.4921250

Basic considerations for scaling Z ‐pinch x‐ray emission with atomic number
journal, February 1990

  • Whitney, K. G.; Thornhill, J. W.; Apruzese, J. P.
  • Journal of Applied Physics, Vol. 67, Issue 4
  • DOI: 10.1063/1.345642

Doppler measurement of implosion velocity in fast Z -pinch x-ray sources
journal, November 2011


National Ignition Facility laser performance status
journal, January 2007

  • Haynam, C. A.; Wegner, P. J.; Auerbach, J. M.
  • Applied Optics, Vol. 46, Issue 16
  • DOI: 10.1364/AO.46.003276

Deuterium gas-puff Z-pinch implosions on the Z accelerator
journal, May 2007

  • Coverdale, C. A.; Deeney, C.; Velikovich, A. L.
  • Physics of Plasmas, Vol. 14, Issue 5
  • DOI: 10.1063/1.2710207

A Review of the Gas-Puff <inline-formula> <tex-math notation="LaTeX">$Z$ </tex-math></inline-formula>-Pinch as an X-Ray and Neutron Source
journal, August 2015


Computational modeling of Krypton gas puffs with tailored mass density profiles on Za)
journal, May 2015

  • Jennings, C. A.; Ampleford, D. J.; Lamppa, D. C.
  • Physics of Plasmas, Vol. 22, Issue 5
  • DOI: 10.1063/1.4921154

Works referencing / citing this record:

The effects of microstructure on propagation of laser-driven radiative heat waves in under-dense high-Z plasma
journal, March 2018

  • Colvin, J. D.; Matsukuma, H.; Brown, K. C.
  • Physics of Plasmas, Vol. 25, Issue 3
  • DOI: 10.1063/1.5012523