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Title: Ultrathin IBAD MgO films for epitaxial growth on amorphous substrates and sub-50 nm membranes

Here, a fabrication process has been developed for high energy ion beam assisted deposition (IBAD) biaxial texturing of ultrathin (~1 nm) MgO films, using a high ion-to-atom ratio and post-deposition annealing instead of a homoepitaxial MgO layer. These films serve as the seed layer for epitaxial growth of materials on amorphous substrates such as electron/X-ray transparent membranes or nanocalorimetry devices. Stress measurements and atomic force microscopy of the MgO films reveal decreased stress and surface roughness, while X-ray diffraction of epitaxial overlayers demonstrates the improved crystal quality of films grown epitaxially on IBAD MgO. The process simplifies the synthesis of IBAD MgO, fundamentally solves the “wrinkle” issue induced by the homoepitaxial layer on sub-50 nm membranes, and enables studies of epitaxial materials in electron/X-ray transmission and nanocalorimetry.
Authors:
 [1] ;  [2] ;  [3] ;  [1] ;  [4] ;  [1]
  1. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)
  2. Univ. of California, Berkeley, CA (United States)
  3. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States); CNRS-Univ. de Rouen, St. Etienne du Rouvray (France)
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Santa Cruz, CA (United States)
Publication Date:
Report Number(s):
LBNL-1006527
Journal ID: ISSN 0003-6951; ir:1006527
Grant/Contract Number:
AC02-05CH11231
Type:
Published Article
Journal Name:
Applied Physics Letters
Additional Journal Information:
Journal Volume: 109; Journal Issue: 19; Journal ID: ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)
Research Org:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Epitaxy; Ion beam assisted deposition; Thin film growth; Atomic force microscopy; X-ray diffraction
OSTI Identifier:
1337585
Alternate Identifier(s):
OSTI ID: 1331404; OSTI ID: 1372677

Wang, Siming, Antonakos, C., Bordel, C., Bouma, D. S., Fischer, P., and Hellman, F.. Ultrathin IBAD MgO films for epitaxial growth on amorphous substrates and sub-50 nm membranes. United States: N. p., Web. doi:10.1063/1.4966956.
Wang, Siming, Antonakos, C., Bordel, C., Bouma, D. S., Fischer, P., & Hellman, F.. Ultrathin IBAD MgO films for epitaxial growth on amorphous substrates and sub-50 nm membranes. United States. doi:10.1063/1.4966956.
Wang, Siming, Antonakos, C., Bordel, C., Bouma, D. S., Fischer, P., and Hellman, F.. 2016. "Ultrathin IBAD MgO films for epitaxial growth on amorphous substrates and sub-50 nm membranes". United States. doi:10.1063/1.4966956.
@article{osti_1337585,
title = {Ultrathin IBAD MgO films for epitaxial growth on amorphous substrates and sub-50 nm membranes},
author = {Wang, Siming and Antonakos, C. and Bordel, C. and Bouma, D. S. and Fischer, P. and Hellman, F.},
abstractNote = {Here, a fabrication process has been developed for high energy ion beam assisted deposition (IBAD) biaxial texturing of ultrathin (~1 nm) MgO films, using a high ion-to-atom ratio and post-deposition annealing instead of a homoepitaxial MgO layer. These films serve as the seed layer for epitaxial growth of materials on amorphous substrates such as electron/X-ray transparent membranes or nanocalorimetry devices. Stress measurements and atomic force microscopy of the MgO films reveal decreased stress and surface roughness, while X-ray diffraction of epitaxial overlayers demonstrates the improved crystal quality of films grown epitaxially on IBAD MgO. The process simplifies the synthesis of IBAD MgO, fundamentally solves the “wrinkle” issue induced by the homoepitaxial layer on sub-50 nm membranes, and enables studies of epitaxial materials in electron/X-ray transmission and nanocalorimetry.},
doi = {10.1063/1.4966956},
journal = {Applied Physics Letters},
number = 19,
volume = 109,
place = {United States},
year = {2016},
month = {11}
}

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