Electric-field noise from carbon-adatom diffusion on a Au(110) surface: First-principles calculations and experiments
Abstract
The decoherence of trapped-ion quantum bits due to heating of their motional modes is a fundamental science and engineering problem. This heating is attributed to electric-field noise arising from processes on the trap-electrode surfaces. In this work, we address the source of this noise by focusing on the diffusion of carbon-containing adsorbates on the surface of Au(110). We show by detailed scanned probe microscopy and density functional theory how the carbon adatom diffusion on the gold surface changes the energy landscape, and how the adatom dipole moment varies with the diffusive motion. Lastly, a simple model for the diffusion noise, which varies quadratically with the variation of the dipole moment, qualitatively reproduces the measured noise spectrum, and the estimate of the noise spectral density is in accord with measured values.
- Authors:
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1336362
- Alternate Identifier(s):
- OSTI ID: 1346432
- Report Number(s):
- SAND2016-8969J
Journal ID: ISSN 2469-9926; PLRAAN; 647315
- Grant/Contract Number:
- AC04-94AL85000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review A
- Additional Journal Information:
- Journal Volume: 95; Journal Issue: 3; Journal ID: ISSN 2469-9926
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS
Citation Formats
Kim, E., Safavi-Naini, A., Hite, D. A., McKay, K. S., Pappas, D. P., Weck, P. F., and Sadeghpour, H. R. Electric-field noise from carbon-adatom diffusion on a Au(110) surface: First-principles calculations and experiments. United States: N. p., 2017.
Web. doi:10.1103/PhysRevA.95.033407.
Kim, E., Safavi-Naini, A., Hite, D. A., McKay, K. S., Pappas, D. P., Weck, P. F., & Sadeghpour, H. R. Electric-field noise from carbon-adatom diffusion on a Au(110) surface: First-principles calculations and experiments. United States. https://doi.org/10.1103/PhysRevA.95.033407
Kim, E., Safavi-Naini, A., Hite, D. A., McKay, K. S., Pappas, D. P., Weck, P. F., and Sadeghpour, H. R. Wed .
"Electric-field noise from carbon-adatom diffusion on a Au(110) surface: First-principles calculations and experiments". United States. https://doi.org/10.1103/PhysRevA.95.033407. https://www.osti.gov/servlets/purl/1336362.
@article{osti_1336362,
title = {Electric-field noise from carbon-adatom diffusion on a Au(110) surface: First-principles calculations and experiments},
author = {Kim, E. and Safavi-Naini, A. and Hite, D. A. and McKay, K. S. and Pappas, D. P. and Weck, P. F. and Sadeghpour, H. R.},
abstractNote = {The decoherence of trapped-ion quantum bits due to heating of their motional modes is a fundamental science and engineering problem. This heating is attributed to electric-field noise arising from processes on the trap-electrode surfaces. In this work, we address the source of this noise by focusing on the diffusion of carbon-containing adsorbates on the surface of Au(110). We show by detailed scanned probe microscopy and density functional theory how the carbon adatom diffusion on the gold surface changes the energy landscape, and how the adatom dipole moment varies with the diffusive motion. Lastly, a simple model for the diffusion noise, which varies quadratically with the variation of the dipole moment, qualitatively reproduces the measured noise spectrum, and the estimate of the noise spectral density is in accord with measured values.},
doi = {10.1103/PhysRevA.95.033407},
journal = {Physical Review A},
number = 3,
volume = 95,
place = {United States},
year = {Wed Mar 01 00:00:00 EST 2017},
month = {Wed Mar 01 00:00:00 EST 2017}
}
Web of Science
Works referenced in this record:
Scaling the Ion Trap Quantum Processor
journal, March 2013
- Monroe, C.; Kim, J.
- Science, Vol. 339, Issue 6124
Surface science for improved ion traps
journal, October 2013
- Hite, D. A.; Colombe, Y.; Wilson, A. C.
- MRS Bulletin, Vol. 38, Issue 10
Heating of trapped ions from the quantum ground state
journal, May 2000
- Turchette, Q. A.; King, B. E.
- Physical Review A, Vol. 61, Issue 6
Scaling and Suppression of Anomalous Heating in Ion Traps
journal, September 2006
- Deslauriers, L.; Olmschenk, S.; Stick, D.
- Physical Review Letters, Vol. 97, Issue 10
Temperature Dependence of Electric Field Noise above Gold Surfaces
journal, October 2008
- Labaziewicz, Jaroslaw; Ge, Yufei; Leibrandt, David R.
- Physical Review Letters, Vol. 101, Issue 18
Insensitivity of the rate of ion motional heating to trap-electrode material over a large temperature range
journal, January 2014
- Chiaverini, J.; Sage, J. M.
- Physical Review A, Vol. 89, Issue 1
Zero-point cooling and low heating of trapped ions
journal, October 2004
- Deslauriers, L.; Haljan, P. C.; Lee, P. J.
- Physical Review A, Vol. 70, Issue 4
Simplified motional heating rate measurements of trapped ions
journal, September 2007
- Epstein, R. J.; Seidelin, S.; Leibfried, D.
- Physical Review A, Vol. 76, Issue 3
Reduction of heating rate in a microfabricated ion trap by pulsed-laser cleaning
journal, December 2011
- Allcock, D. T. C.; Guidoni, L.; Harty, T. P.
- New Journal of Physics, Vol. 13, Issue 12
100-Fold Reduction of Electric-Field Noise in an Ion Trap Cleaned with In Situ Argon-Ion-Beam Bombardment
journal, September 2012
- Hite, D. A.; Colombe, Y.; Wilson, A. C.
- Physical Review Letters, Vol. 109, Issue 10
Surface noise analysis using a single-ion sensor
journal, June 2014
- Daniilidis, N.; Gerber, S.; Bolloten, G.
- Physical Review B, Vol. 89, Issue 24
Microscopic model of electric-field-noise heating in ion traps
journal, August 2011
- Safavi-Naini, A.; Rabl, P.; Weck, P. F.
- Physical Review A, Vol. 84, Issue 2
Micro-fabricated stylus ion trap
journal, August 2013
- Arrington, Christian L.; McKay, Kyle S.; Baca, Ehren D.
- Review of Scientific Instruments, Vol. 84, Issue 8
Measurements of trapped-ion heating rates with exchangeable surfaces in close proximity
journal, January 2017
- Hite, D. A.; McKay, K. S.; Kotler, S.
- MRS Advances, Vol. 2, Issue 41
Diffusion of oxygen on tungsten (110)
journal, March 1977
- Butz, R.; Wagner, H.
- Surface Science, Vol. 63
On the coverage dependence of the surface diffusion constant
journal, October 1980
- Asada, Hiromu; Masuda, Makihiko
- Surface Science, Vol. 99, Issue 3
Surface diffusion of K on Pd{111}: Coverage dependence of the diffusion coefficient determined with the Boltzmann–Matano method
journal, March 1998
- Šnábl, M.; Ondřejček, M.; Cháb, V.
- The Journal of Chemical Physics, Vol. 108, Issue 10
Collective surface diffusion: An experimentalist's view
journal, November 2005
- Naumovets, A. G.
- Physica A: Statistical Mechanics and its Applications, Vol. 357, Issue 2
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996
- Kresse, G.; Furthmüller, J.
- Physical Review B, Vol. 54, Issue 16, p. 11169-11186
Atoms, molecules, solids, and surfaces: Applications of the generalized gradient approximation for exchange and correlation
journal, September 1992
- Perdew, John P.; Chevary, J. A.; Vosko, S. H.
- Physical Review B, Vol. 46, Issue 11
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Projector augmented-wave method
journal, December 1994
- Blöchl, P. E.
- Physical Review B, Vol. 50, Issue 24, p. 17953-17979
From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999
- Kresse, G.; Joubert, D.
- Physical Review B, Vol. 59, Issue 3, p. 1758-1775
High-precision sampling for Brillouin-zone integration in metals
journal, August 1989
- Methfessel, M.; Paxton, A. T.
- Physical Review B, Vol. 40, Issue 6
Special points for Brillouin-zone integrations
journal, June 1976
- Monkhorst, Hendrik J.; Pack, James D.
- Physical Review B, Vol. 13, Issue 12, p. 5188-5192
Lattice Constants and Thermal Expansion of Gold up to 878 °C by X-Ray Method
journal, January 1963
- Dutta, B. N.; Dayal, B.
- physica status solidi (b), Vol. 3, Issue 3
Adsorbate-substrate and adsorbate-adsorbate interactions of Na and K adlayers on Al(111)
journal, December 1992
- Neugebauer, Jörg; Scheffler, Matthias
- Physical Review B, Vol. 46, Issue 24
Influence of monolayer contamination on electric-field-noise heating in ion traps
journal, February 2013
- Safavi-Naini, A.; Kim, E.; Weck, P. F.
- Physical Review A, Vol. 87, Issue 2
ORDER-DISORDER PHASE TRANSITION OF Au(110)-(1x2) RECONSTRUCTION
journal, November 1988
- Nguyen, H. Q.; Kuk, Y.; Silverman, P. J.
- Le Journal de Physique Colloques, Vol. 49, Issue C6
First-principles calculations of clean Au(110) surfaces and chemisorption of atomic oxygen
journal, January 2009
- Landmann, M.; Rauls, E.; Schmidt, W. G.
- Physical Review B, Vol. 79, Issue 4
Reconstruction of charged surfaces: General trends and a case study of Pt(110) and Au(110)
journal, December 2003
- Lozovoi, Alexander Y.; Alavi, Ali
- Physical Review B, Vol. 68, Issue 24
Surface diffusion model of adsorption-induced field emission flicker noise
journal, April 1971
- Kleint, Ch.
- Surface Science, Vol. 25, Issue 2
Current fluctuations from small regions of adsorbate covered field emitters
journal, July 1973
- Gomer, Robert
- Surface Science, Vol. 38, Issue 2
Spectral analysis of adsorbate induced field-emission flicker noise
journal, December 1985
- Gesley, M. A.; Swanson, L. W.
- Physical Review B, Vol. 32, Issue 12
Ion-trap measurements of electric-field noise near surfaces
journal, December 2015
- Brownnutt, M.; Kumph, M.; Rabl, P.
- Reviews of Modern Physics, Vol. 87, Issue 4
Controlling trapping potentials and stray electric fields in a microfabricated ion trap through design and compensation
journal, July 2012
- Charles Doret, S.; Amini, Jason M.; Wright, Kenneth
- New Journal of Physics, Vol. 14, Issue 7
Individual-Ion Addressing with Microwave Field Gradients
journal, April 2013
- Warring, U.; Ospelkaus, C.; Colombe, Y.
- Physical Review Letters, Vol. 110, Issue 17
Works referencing / citing this record:
Trapped-ion quantum computing: Progress and challenges
journal, June 2019
- Bruzewicz, Colin D.; Chiaverini, John; McConnell, Robert
- Applied Physics Reviews, Vol. 6, Issue 2
Crystallographic orientation dependence of work function: carbon adsorption on Au surfaces
journal, February 2019
- Jooya, H. Z.; Fan (言 詯), X.; McKay, K. S.
- Molecular Physics, Vol. 117, Issue 15-16
Radio-frequency microplasmas with energies suited to in situ selective cleaning of surface adsorbates in ion microtraps
journal, February 2019
- Akhtar, Mariam; Wilpers, Guido; Choonee, Kaushal
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 52, Issue 5
van der Waals-corrected density functional study of electric field noise heating in ion traps caused by electrode surface adsorbates
journal, May 2019
- Ray, Keith G.; Rubenstein, Brenda M.; Gu, Wenze
- New Journal of Physics, Vol. 21, Issue 5
Crystallographic orientation dependence of work function: carbon adsorption on Au surfaces
text, January 2019
- Jooya, H. Z.; 詯), X. Fan (言; McKay, K. S.
- Taylor & Francis
Crystallographic orientation dependence of work function: carbon adsorption on Au surfaces
text, January 2019
- Jooya, H. Z.; 詯), X. Fan (言; McKay, K. S.
- Figshare
Distance scaling of electric-field noise in a surface-electrode ion trap
text, January 2017
- Sedlacek, J. A.; Greene, A.; Stuart, J.
- arXiv
Evidence for multiple mechanisms underlying surface electric-field noise in ion traps
text, January 2018
- Sedlacek, J. A.; Stuart, J.; Slichter, D. H.
- arXiv
Crystallographic orientation dependence of work function: Carbon adsorption on Au surfaces
text, January 2019
- Jooya, H. Z.; Fan, X.; McKay, K. S.
- arXiv
Distance scaling and polarization of electric-field noise in a surface ion trap
text, January 2019
- An, Da; Matthiesen, Clemens; Urban, Erik
- arXiv