DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Magneto-Optical Signature of Massless Kane Electrons in Cd 3 As 2

Abstract

Here, we report on optical reflectivity experiments performed on Cd3As2 over a broad range of photon energies and magnetic fields. The presence of 3D massless charge carriers are clearly indicated in the observed response. The specific cyclotron resonance absorption in the quantum limit implies that we are probing massless Kane electrons rather than symmetry-protected 3D Dirac particles. Furthermore, the latter may appear at a smaller energy scale and are not directly observed in our infrared experiments.

Authors:
 [1];  [2];  [3];  [4];  [5];  [3];  [6];  [7];  [7];  [8];  [8];  [9];  [10];  [9];  [11];  [11];  [12];  [13];  [1];  [2] more »;  [2];  [2];  [2];  [14] « less
  1. Univ. of Geneva (Switzerland). Dept. of Quantum Matter Physics
  2. Centre National de la Recherche Scientifique (CNRS), Grenoble (France). National Lab. of Intense Magnetic Fields
  3. Univ. of Paris-Sud, Orsay (France). Lab. of Solid State Physics (LPS)
  4. Univ. of Geneva (Switzerland). GAP-Biophotonics
  5. Centre National de la Recherche Scientifique (CNRS), Grenoble (France). National Lab. of Intense Magnetic Fields; Brno Univ. of Technology (Czech Republic)
  6. Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.
  7. Masaryk Univ., Brno (Czech Republic). Central European Inst. of Technology (CEITEC)
  8. Univ. of Montpellier (France). Charles Coulomb Lab.
  9. Johns Hopkins Univ., Baltimore, MD (United States). Inst. for Quantum Matter
  10. Johns Hopkins Univ., Baltimore, MD (United States). Inst. for Quantum Matter; Univ. of California, Berkeley, CA (United States). Dept. of Physics
  11. Academy of Sciences of Moldova, Chisinau (Moldova). Inst. of Applied Physics
  12. Princeton Univ., NJ (United States). Dept. of Chemistry
  13. Princeton Univ., NJ (United States). Inst. of Physics
  14. Centre National de la Recherche Scientifique (CNRS), Grenoble (France). National Lab. of Intense Magnetic Fields; Charles Univ., Prague (Czech Republic). Inst. of Physics
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1336158
Alternate Identifier(s):
OSTI ID: 1325842
Report Number(s):
BNL-112683-2016-JA
Journal ID: ISSN 0031-9007; PRLTAO; R&D Project: PO016; KC0202020
Grant/Contract Number:  
SC00112704; FG02-08ER46544; SC0012704
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Letters
Additional Journal Information:
Journal Volume: 117; Journal Issue: 13; Journal ID: ISSN 0031-9007
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Akrap, A., Hakl, M., Tchoumakov, S., Crassee, I., Kuba, J., Goerbig, M. O., Homes, C. C., Caha, O., Novák, J., Teppe, F., Desrat, W., Koohpayeh, S., Wu, L., Armitage, N. P., Nateprov, A., Arushanov, E., Gibson, Q. D., Cava, R. J., van der Marel, D., Piot, B. A., Faugeras, C., Martinez, G., Potemski, M., and Orlita, M. Magneto-Optical Signature of Massless Kane Electrons in Cd3As2. United States: N. p., 2016. Web. doi:10.1103/PhysRevLett.117.136401.
Akrap, A., Hakl, M., Tchoumakov, S., Crassee, I., Kuba, J., Goerbig, M. O., Homes, C. C., Caha, O., Novák, J., Teppe, F., Desrat, W., Koohpayeh, S., Wu, L., Armitage, N. P., Nateprov, A., Arushanov, E., Gibson, Q. D., Cava, R. J., van der Marel, D., Piot, B. A., Faugeras, C., Martinez, G., Potemski, M., & Orlita, M. Magneto-Optical Signature of Massless Kane Electrons in Cd3As2. United States. https://doi.org/10.1103/PhysRevLett.117.136401
Akrap, A., Hakl, M., Tchoumakov, S., Crassee, I., Kuba, J., Goerbig, M. O., Homes, C. C., Caha, O., Novák, J., Teppe, F., Desrat, W., Koohpayeh, S., Wu, L., Armitage, N. P., Nateprov, A., Arushanov, E., Gibson, Q. D., Cava, R. J., van der Marel, D., Piot, B. A., Faugeras, C., Martinez, G., Potemski, M., and Orlita, M. Wed . "Magneto-Optical Signature of Massless Kane Electrons in Cd3As2". United States. https://doi.org/10.1103/PhysRevLett.117.136401. https://www.osti.gov/servlets/purl/1336158.
@article{osti_1336158,
title = {Magneto-Optical Signature of Massless Kane Electrons in Cd3As2},
author = {Akrap, A. and Hakl, M. and Tchoumakov, S. and Crassee, I. and Kuba, J. and Goerbig, M. O. and Homes, C. C. and Caha, O. and Novák, J. and Teppe, F. and Desrat, W. and Koohpayeh, S. and Wu, L. and Armitage, N. P. and Nateprov, A. and Arushanov, E. and Gibson, Q. D. and Cava, R. J. and van der Marel, D. and Piot, B. A. and Faugeras, C. and Martinez, G. and Potemski, M. and Orlita, M.},
abstractNote = {Here, we report on optical reflectivity experiments performed on Cd3As2 over a broad range of photon energies and magnetic fields. The presence of 3D massless charge carriers are clearly indicated in the observed response. The specific cyclotron resonance absorption in the quantum limit implies that we are probing massless Kane electrons rather than symmetry-protected 3D Dirac particles. Furthermore, the latter may appear at a smaller energy scale and are not directly observed in our infrared experiments.},
doi = {10.1103/PhysRevLett.117.136401},
journal = {Physical Review Letters},
number = 13,
volume = 117,
place = {United States},
year = {Wed Sep 21 00:00:00 EDT 2016},
month = {Wed Sep 21 00:00:00 EDT 2016}
}

Journal Article:

Citation Metrics:
Cited by: 87 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Crystal growth and characterization of II3V2 compounds
journal, January 1980


Spin magnetic moment and spin resonance of conduction electrons in α-Sn-type semiconductors
journal, October 1971


Transient reflectance of photoexcited Cd 3 As 2
journal, June 2015

  • Weber, C. P.; Arushanov, Ernest; Berggren, Bryan S.
  • Applied Physics Letters, Vol. 106, Issue 23
  • DOI: 10.1063/1.4922528

Magneto-optical oscillations in Cd 3 As 2
journal, April 1981


Interband optical conductivity of the [001]-oriented Dirac semimetal Cd 3 As 2
journal, March 2016


Three-dimensional Dirac semimetal and quantum transport in Cd 3 As 2
journal, September 2013


Collective Modes of the Massless Dirac Plasma
journal, May 2009


Classification of stable three-dimensional Dirac semimetals with nontrivial topology
journal, September 2014

  • Yang, Bohm-Jung; Nagaosa, Naoto
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5898

Three-dimensional Dirac fermions in quasicrystals as seen via optical conductivity
journal, June 2013


Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2
journal, May 2014

  • Neupane, Madhab; Xu, Su-Yang; Sankar, Raman
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4786

II3V2 compounds and alloys
journal, January 1992


Band structure of CdGe As 2 near k = 0
journal, December 1974


Magneto-optical conductivity of Weyl semimetals
journal, June 2013


Optical verification of the valence band structure of cadmium arsenide
journal, February 1980


How Perfect Can Graphene Be?
journal, September 2009


Magnetoplasma reflectivity studies on Cd3As2
journal, February 1984

  • Schleijpen, H. M. A.; von Ortenberg, M.; Gelten, M. J.
  • International Journal of Infrared and Millimeter Waves, Vol. 5, Issue 2
  • DOI: 10.1007/BF01417648

Effet Shubnikov de Haas dans Cd3As2: Forme de la surface de Fermi et modele non parabolique de la bande de conduction
journal, June 1969


Infrared and microwave magnetoplasma effects in semiconductors
journal, September 1970


Experimental Realization of a Three-Dimensional Dirac Semimetal
journal, July 2014


Observation of three-dimensional massless Kane fermions in a zinc-blende crystal
journal, January 2014

  • Orlita, M.; Basko, D. M.; Zholudev, M. S.
  • Nature Physics, Vol. 10, Issue 3
  • DOI: 10.1038/nphys2857

Chiral tunnelling and the Klein paradox in graphene
journal, August 2006

  • Katsnelson, M. I.; Novoselov, K. S.; Geim, A. K.
  • Nature Physics, Vol. 2, Issue 9
  • DOI: 10.1038/nphys384

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2
journal, November 2014

  • Liang, Tian; Gibson, Quinn; Ali, Mazhar N.
  • Nature Materials, Vol. 14, Issue 3
  • DOI: 10.1038/nmat4143

A stable three-dimensional topological Dirac semimetal Cd3As2
journal, May 2014

  • Liu, Z. K.; Jiang, J.; Zhou, B.
  • Nature Materials, Vol. 13, Issue 7
  • DOI: 10.1038/nmat3990

Landau quantization and quasiparticle interference in the three-dimensional Dirac semimetal Cd3As2
journal, June 2014

  • Jeon, Sangjun; Zhou, Brian B.; Gyenis, Andras
  • Nature Materials, Vol. 13, Issue 9
  • DOI: 10.1038/nmat4023

Band structure of indium antimonide
journal, January 1957


The Crystal and Electronic Structures of Cd 3 As 2 , the Three-Dimensional Electronic Analogue of Graphene
journal, March 2014

  • Ali, Mazhar N.; Gibson, Quinn; Jeon, Sangjun
  • Inorganic Chemistry, Vol. 53, Issue 8
  • DOI: 10.1021/ic403163d

How perfect can graphene be?
text, January 2009


Magneto-optical conductivity of Weyl semimetals
text, January 2013


Three-dimensional Dirac fermions in quasicrystals as seen via optical conductivity
text, January 2013


Experimental Realization of a Three-Dimensional Dirac Semimetal
text, January 2013


Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd$_3$As$_2$
text, January 2014


Chiral tunneling and the Klein paradox in graphene
text, January 2006


Works referencing / citing this record:

Route towards Dirac and Weyl antiferromagnetic spintronics: Route towards Dirac and Weyl antiferromagnetic spintronics
journal, March 2017

  • Šmejkal, Libor; Jungwirth, Tomáš; Sinova, Jairo
  • physica status solidi (RRL) - Rapid Research Letters, Vol. 11, Issue 4
  • DOI: 10.1002/pssr.201700044

Chiral Landau levels in Weyl semimetal NbAs with multiple topological carriers
journal, May 2018


Electronic and optical properties of topological semimetal Cd3As2
journal, April 2017

  • Mosca Conte, Adriano; Pulci, Olivia; Bechstedt, Friedhelm
  • Scientific Reports, Vol. 7, Issue 1
  • DOI: 10.1038/srep45500

Surface plasmons in Weyl semimetals
journal, August 2018


Hybridization of topological surface states with a flat band
journal, January 2020

  • Krishtopenko, Sergey S.; Antezza, Mauro; Teppe, Frédéric
  • Journal of Physics: Condensed Matter, Vol. 32, Issue 16
  • DOI: 10.1088/1361-648x/ab6741

Optical spectroscopy study of the topological property in PrSb
journal, September 2019


Ferromagnetic state above room temperature in a proximitized topological Dirac semimetal
journal, December 2019


Magneto-optical conductivity of double Weyl semimetals
journal, August 2017


Surface superconductivity in a three-dimensional Cd 3 As 2 semimetal at the interface with a gold contact
journal, March 2019


Collisionless Transport Close to a Fermionic Quantum Critical Point in Dirac Materials
journal, September 2018


Electrodynamic response of type II Weyl semimetals
text, January 2016


Weyl and Dirac Semimetals in Three Dimensional Solids
text, January 2017


Magneto-optical conductivity of double Weyl semimetals
text, January 2017


From Dirac semimetals to topological phases in three dimensions: a coupled wire construction
text, January 2017


Chiral Landau levels in Weyl semimetal NbAs with multiple topological carriers
text, January 2018


Ferromagnetic state above room temperature in a proximitized topological Dirac semimetal
text, January 2019