Observations of strong ion-ion correlations in dense plasmas
Abstract
Using simultaneous spectrally, angularly, and temporally resolved x-ray scattering, we measure the pronounced ion-ion correlation peak in a strongly coupled plasma. Laser-driven shock-compressed aluminum at ~3× solid density is probed with high-energy photons at 17.9 keV created by molybdenum He-α emission in a laser-driven plasma source. The measured elastic scattering feature shows a well-pronounced correlation peak at a wave vector of k=4Å–1. The magnitude of this correlation peak cannot be described by standard plasma theories employing a linear screened Coulomb potential. Advanced models, including a strong short-range repulsion due to the inner structure of the aluminum ions are however in good agreement with the scattering data. These studies have demonstrated a new highly accurate diagnostic technique to directly measure the state of compression and the ion-ion correlations. Furthermore, we have since applied this new method in single-shot wave-number resolved S(k) measurements to characterize the physical properties of dense plasmas.
- Authors:
-
more »
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- AWE plc, Reading (United Kingdom); Univ. of Warwick, Coventry (United Kingdom)
- Univ. of California, Berkeley, CA (United States)
- Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of California, Los Angeles, CA (United States)
- Univ. of Warwick, Coventry (United Kingdom)
- Univ. of Oxford, Oxford (United Kingdom)
- GSI Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany)
- Max Planck Institut fur Physik komplexer Systeme, Dresden (Germany)
- Tessella, 26 The Quadrant, Abington (United Kingdom)
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Friedrich-Schiller-Univ., Jena (Germany)
- Publication Date:
- Research Org.:
- Univ. of California, Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1334521
- Grant/Contract Number:
- NA0000910
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physics of Plasmas
- Additional Journal Information:
- Journal Volume: 21; Journal Issue: 5; Journal ID: ISSN 1070-664X
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY; x-ray scattering; aluminum; elasticity; scattering measurements; molybdenum
Citation Formats
Ma, T., Fletcher, L., Pak, A., Chapman, D. A., Falcone, R. W., Fortmann, C., Galtier, E., Gericke, D. O., Gregori, G., Hastings, J., Landen, O. L., Le Pape, S., Lee, H. J., Nagler, B., Neumayer, P., Turnbull, D., Vorberger, J., White, T. G., Wunsch, K., Zastrau, U., Glenzer, S. H., and Doppner, T. Observations of strong ion-ion correlations in dense plasmas. United States: N. p., 2014.
Web. doi:10.1063/1.4872161.
Ma, T., Fletcher, L., Pak, A., Chapman, D. A., Falcone, R. W., Fortmann, C., Galtier, E., Gericke, D. O., Gregori, G., Hastings, J., Landen, O. L., Le Pape, S., Lee, H. J., Nagler, B., Neumayer, P., Turnbull, D., Vorberger, J., White, T. G., Wunsch, K., Zastrau, U., Glenzer, S. H., & Doppner, T. Observations of strong ion-ion correlations in dense plasmas. United States. https://doi.org/10.1063/1.4872161
Ma, T., Fletcher, L., Pak, A., Chapman, D. A., Falcone, R. W., Fortmann, C., Galtier, E., Gericke, D. O., Gregori, G., Hastings, J., Landen, O. L., Le Pape, S., Lee, H. J., Nagler, B., Neumayer, P., Turnbull, D., Vorberger, J., White, T. G., Wunsch, K., Zastrau, U., Glenzer, S. H., and Doppner, T. Thu .
"Observations of strong ion-ion correlations in dense plasmas". United States. https://doi.org/10.1063/1.4872161. https://www.osti.gov/servlets/purl/1334521.
@article{osti_1334521,
title = {Observations of strong ion-ion correlations in dense plasmas},
author = {Ma, T. and Fletcher, L. and Pak, A. and Chapman, D. A. and Falcone, R. W. and Fortmann, C. and Galtier, E. and Gericke, D. O. and Gregori, G. and Hastings, J. and Landen, O. L. and Le Pape, S. and Lee, H. J. and Nagler, B. and Neumayer, P. and Turnbull, D. and Vorberger, J. and White, T. G. and Wunsch, K. and Zastrau, U. and Glenzer, S. H. and Doppner, T.},
abstractNote = {Using simultaneous spectrally, angularly, and temporally resolved x-ray scattering, we measure the pronounced ion-ion correlation peak in a strongly coupled plasma. Laser-driven shock-compressed aluminum at ~3× solid density is probed with high-energy photons at 17.9 keV created by molybdenum He-α emission in a laser-driven plasma source. The measured elastic scattering feature shows a well-pronounced correlation peak at a wave vector of k=4Å–1. The magnitude of this correlation peak cannot be described by standard plasma theories employing a linear screened Coulomb potential. Advanced models, including a strong short-range repulsion due to the inner structure of the aluminum ions are however in good agreement with the scattering data. These studies have demonstrated a new highly accurate diagnostic technique to directly measure the state of compression and the ion-ion correlations. Furthermore, we have since applied this new method in single-shot wave-number resolved S(k) measurements to characterize the physical properties of dense plasmas.},
doi = {10.1063/1.4872161},
journal = {Physics of Plasmas},
number = 5,
volume = 21,
place = {United States},
year = {Thu Apr 24 00:00:00 EDT 2014},
month = {Thu Apr 24 00:00:00 EDT 2014}
}
Web of Science
Works referenced in this record:
Screening of ionic cores in partially ionized plasmas within linear response
journal, June 2010
- Gericke, D. O.; Vorberger, J.; Wünsch, K.
- Physical Review E, Vol. 81, Issue 6
Theory of x-ray scattering in high-pressure electrides
journal, November 2012
- Fortmann, C.; Niemann, C.; Glenzer, S. H.
- Physical Review B, Vol. 86, Issue 17
The experimental plan for cryogenic layered target implosions on the National Ignition Facility—The inertial confinement approach to fusion
journal, May 2011
- Edwards, M. J.; Lindl, J. D.; Spears, B. K.
- Physics of Plasmas, Vol. 18, Issue 5
Derivation of the static structure factor in strongly coupled non-equilibrium plasmas for X-ray scattering studies
journal, May 2007
- Gregori, G.; Ravasio, A.; Höll, A.
- High Energy Density Physics, Vol. 3, Issue 1-2
Cryogenic thermonuclear fuel implosions on the National Ignition Facility
journal, May 2012
- Glenzer, S. H.; Callahan, D. A.; MacKinnon, A. J.
- Physics of Plasmas, Vol. 19, Issue 5
Demonstration of self-seeding in a hard-X-ray free-electron laser
journal, August 2012
- Amann, J.; Berg, W.; Blank, V.
- Nature Photonics, Vol. 6, Issue 10, p. 693-698
Characterization of strongly-bent HAPG crystals for von-Hámos x-ray spectrographs
journal, October 2013
- Zastrau, U.; Woldegeorgis, A.; Förster, E.
- Journal of Instrumentation, Vol. 8, Issue 10
Theoretical model of x-ray scattering as a dense matter probe
journal, February 2003
- Gregori, G.; Glenzer, S. H.; Rozmus, W.
- Physical Review E, Vol. 67, Issue 2
Strongly coupled plasma physics and high energy-density matter
journal, May 2004
- Murillo, M. S.
- Physics of Plasmas, Vol. 11, Issue 5
Effective ion–ion potentials in warm dense matter
journal, March 2013
- Vorberger, J.; Gericke, D. O.
- High Energy Density Physics, Vol. 9, Issue 1
Strongly coupled plasmas: high-density classical plasmas and degenerate electron liquids
journal, October 1982
- Ichimaru, Setsuo
- Reviews of Modern Physics, Vol. 54, Issue 4
The upgrade to the OMEGA laser system
journal, January 1995
- Boehly, T. R.; Craxton, R. S.; Hinterman, T. H.
- Review of Scientific Instruments, Vol. 66, Issue 1
X-ray line measurements with high efficiency Bragg crystals
journal, October 2004
- Pak, A.; Gregori, G.; Knight, J.
- Review of Scientific Instruments, Vol. 75, Issue 10
Aluminium at terapascal pressures
journal, July 2010
- Pickard, Chris J.; Needs, R. J.
- Nature Materials, Vol. 9, Issue 8
Ion structure in warm dense matter: Benchmarking solutions of hypernetted-chain equations by first-principle simulations
journal, January 2009
- Wünsch, K.; Vorberger, J.; Gericke, D. O.
- Physical Review E, Vol. 79, Issue 1
The ice layer in Uranus and Neptune—diamonds in the sky?
journal, July 1981
- Ross, Marvin
- Nature, Vol. 292, Issue 5822
Structure of strongly coupled multicomponent plasmas
journal, May 2008
- Wünsch, K.; Hilse, P.; Schlanges, M.
- Physical Review E, Vol. 77, Issue 5
Dissociation of CH4 at High Pressures and Temperatures: Diamond Formation in Giant Planet Interiors?
journal, October 1999
- Benedetti, L. R.
- Science, Vol. 286, Issue 5437
K-shell spectra from Ag, Sn, Sm, Ta, and Au generated by intense femtosecond laser pulses
journal, May 2007
- Seely, John F.; Holland, Glenn E.; Hudson, Lawrence T.
- High Energy Density Physics, Vol. 3, Issue 1-2
Ion structure in dense plasmas: MSA versus HNC
journal, May 2009
- Wünsch, K.; Vorberger, J.; Gregori, G.
- Journal of Physics A: Mathematical and Theoretical, Vol. 42, Issue 21
Femtosecond Visualization of Lattice Dynamics in Shock-Compressed Matter
journal, October 2013
- Milathianaki, D.; Boutet, S.; Williams, G. J.
- Science, Vol. 342, Issue 6155
Interaction of photons with plasmas and liquid metals - photoabsorption and scattering
journal, December 1999
- Chihara, Junzo
- Journal of Physics: Condensed Matter, Vol. 12, Issue 3
X-Ray Scattering Measurements of Strong Ion-Ion Correlations in Shock-Compressed Aluminum
journal, February 2013
- Ma, T.; Döppner, T.; Falcone, R. W.
- Physical Review Letters, Vol. 110, Issue 6
Three-dimensional HYDRA simulations of National Ignition Facility targets
journal, May 2001
- Marinak, M. M.; Kerbel, G. D.; Gentile, N. A.
- Physics of Plasmas, Vol. 8, Issue 5
Works referencing / citing this record:
Measurement of temperature and density using non-collective X-ray Thomson scattering in pulsed power produced warm dense plasmas
journal, May 2018
- Valenzuela, J. C.; Krauland, C.; Mariscal, D.
- Scientific Reports, Vol. 8, Issue 1
Electron-ion collision-frequency for x-ray Thomson scattering in dense plasmas
journal, January 2016
- Faussurier, Gérald; Blancard, Christophe
- Physics of Plasmas, Vol. 23, Issue 1
Measurement of ionic structure in isochorically heated graphite from X-ray Thomson scattering
journal, February 2019
- Lv, Min; Hu, Zhimin; Hou, Yong
- Physics of Plasmas, Vol. 26, Issue 2