Fermi surface topology and hot spot distribution in the Kondo lattice system
Abstract
Rare-earth hexaborides have attracted considerable attention recently in connection to a variety of correlated phenomena including heavy fermions, superconductivity, and low-temperature magnetic phases. Here, we present high-resolution angle-resolved photoemission spectroscopy studies of trivalent CeB6 and divalent BaB6 rare-earth hexaborides. Here we find that the Fermi surface electronic structure of CeB6 consists of large oval-shaped pockets around the X points of the Brillouin zone, whereas the states around the zone center Γ point are strongly renormalized. Our first-principles calculations agree with our experimental results around the X points but not around the Γ point, indicating areas of strong renormalization located near Γ. The Ce quasiparticle states participate in the formation of hot spots at the Fermi surface, whereas the incoherent f states hybridize and lead to the emergence of dispersive features absent in the non-$$f$$ counterpart BaB6. Lastly, our results provide an understanding of the electronic structure in rare-earth hexaborides, which will be useful in elucidating the nature of the exotic low-temperature phases in these materials.
- Authors:
-
- Princeton Univ., NJ (United States). Dept. of Physics; Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Princeton Univ., NJ (United States). Dept. of Physics
- Univ. of California, Irvine, CA (United States). Dept. of Physics and Astronomy
- National Tsing Hua Univ., Hsinchu (Taiwan). Dept. of Physics
- National Tsing Hua Univ., Hsinchu (Taiwan). Dept. of Physics; Academia Sinica, Taipei (Taiwan)
- Temple Univ., Philadelphia, PA (United States). Dept. of Physics
- National Univ. of Singapore (Singapore). Graphene Research Centre, Dept. of Physics
- Northeastern Univ., Boston, MA (United States). Dept. of Physics
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Princeton Univ., NJ (United States). Dept. of Physics; Princeton Univ., NJ (United States). Princeton Center for Complex Materials
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); National Science Council, Taiwan
- OSTI Identifier:
- 1334118
- Alternate Identifier(s):
- OSTI ID: 1221700
- Report Number(s):
- LA-UR-15-26954
Journal ID: ISSN 1098-0121; PRBMDO
- Grant/Contract Number:
- AC52-06NA25396; FG02-07ER46352; FG02-01ER45872; AC02-05CH11231; NRF-NRFF2013-03; GBMF4547; DEFG02-01ER45872
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review. B, Condensed Matter and Materials Physics
- Additional Journal Information:
- Journal Volume: 92; Journal Issue: 10; Journal ID: ISSN 1098-0121
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; 36 MATERIALS SCIENCE
Citation Formats
Neupane, Madhab, Alidoust, Nasser, Belopolski, Ilya, Bian, Guang, Xu, Su-Yang, Kim, Dae-Jeong, Shibayev, Pavel P., Sanchez, Daniel S., Zheng, Hao, Chang, Tay-Rong, Jeng, Horng-Tay, Riseborough, Peter S., Lin, Hsin, Bansil, Arun, Durakiewicz, Tomasz, Fisk, Zachary, and Hasan, M. Zahid. Fermi surface topology and hot spot distribution in the Kondo lattice system CeB6. United States: N. p., 2015.
Web. doi:10.1103/PhysRevB.92.104420.
Neupane, Madhab, Alidoust, Nasser, Belopolski, Ilya, Bian, Guang, Xu, Su-Yang, Kim, Dae-Jeong, Shibayev, Pavel P., Sanchez, Daniel S., Zheng, Hao, Chang, Tay-Rong, Jeng, Horng-Tay, Riseborough, Peter S., Lin, Hsin, Bansil, Arun, Durakiewicz, Tomasz, Fisk, Zachary, & Hasan, M. Zahid. Fermi surface topology and hot spot distribution in the Kondo lattice system CeB6. United States. https://doi.org/10.1103/PhysRevB.92.104420
Neupane, Madhab, Alidoust, Nasser, Belopolski, Ilya, Bian, Guang, Xu, Su-Yang, Kim, Dae-Jeong, Shibayev, Pavel P., Sanchez, Daniel S., Zheng, Hao, Chang, Tay-Rong, Jeng, Horng-Tay, Riseborough, Peter S., Lin, Hsin, Bansil, Arun, Durakiewicz, Tomasz, Fisk, Zachary, and Hasan, M. Zahid. Fri .
"Fermi surface topology and hot spot distribution in the Kondo lattice system CeB6". United States. https://doi.org/10.1103/PhysRevB.92.104420. https://www.osti.gov/servlets/purl/1334118.
@article{osti_1334118,
title = {Fermi surface topology and hot spot distribution in the Kondo lattice system CeB6},
author = {Neupane, Madhab and Alidoust, Nasser and Belopolski, Ilya and Bian, Guang and Xu, Su-Yang and Kim, Dae-Jeong and Shibayev, Pavel P. and Sanchez, Daniel S. and Zheng, Hao and Chang, Tay-Rong and Jeng, Horng-Tay and Riseborough, Peter S. and Lin, Hsin and Bansil, Arun and Durakiewicz, Tomasz and Fisk, Zachary and Hasan, M. Zahid},
abstractNote = {Rare-earth hexaborides have attracted considerable attention recently in connection to a variety of correlated phenomena including heavy fermions, superconductivity, and low-temperature magnetic phases. Here, we present high-resolution angle-resolved photoemission spectroscopy studies of trivalent CeB6 and divalent BaB6 rare-earth hexaborides. Here we find that the Fermi surface electronic structure of CeB6 consists of large oval-shaped pockets around the X points of the Brillouin zone, whereas the states around the zone center Γ point are strongly renormalized. Our first-principles calculations agree with our experimental results around the X points but not around the Γ point, indicating areas of strong renormalization located near Γ. The Ce quasiparticle states participate in the formation of hot spots at the Fermi surface, whereas the incoherent f states hybridize and lead to the emergence of dispersive features absent in the non-$f$ counterpart BaB6. Lastly, our results provide an understanding of the electronic structure in rare-earth hexaborides, which will be useful in elucidating the nature of the exotic low-temperature phases in these materials.},
doi = {10.1103/PhysRevB.92.104420},
journal = {Physical Review. B, Condensed Matter and Materials Physics},
number = 10,
volume = 92,
place = {United States},
year = {Fri Sep 18 00:00:00 EDT 2015},
month = {Fri Sep 18 00:00:00 EDT 2015}
}
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Works referenced in this record:
Low-Temperature Anomalies and Ferromagnetism of
journal, December 1997
- Degiorgi, L.; Felder, E.; Ott, H. R.
- Physical Review Letters, Vol. 79, Issue 25
Heavy fermion semiconductors
journal, May 2000
- Riseborough, Peter S.
- Advances in Physics, Vol. 49, Issue 3
Electronic Structure of Strongly Correlated Systems
journal, January 2011
- Antonov, V. N.; Bekenov, L. V.; Yaresko, A. N.
- Advances in Condensed Matter Physics, Vol. 2011
Colloquium: Topological insulators
journal, November 2010
- Hasan, M. Z.; Kane, C. L.
- Reviews of Modern Physics, Vol. 82, Issue 4, p. 3045-3067
Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2
journal, May 2014
- Neupane, Madhab; Xu, Su-Yang; Sankar, Raman
- Nature Communications, Vol. 5, Issue 1
Topological Kondo Insulators
journal, March 2010
- Dzero, Maxim; Sun, Kai; Galitski, Victor
- Physical Review Letters, Vol. 104, Issue 10
Correlated Topological Insulators with Mixed Valence
journal, February 2013
- Lu, Feng; Zhao, JianZhou; Weng, Hongming
- Physical Review Letters, Vol. 110, Issue 9
Surface and bulk electronic structure of the strongly correlated system SmB and implications for a topological Kondo insulator
journal, September 2013
- Xu, N.; Shi, X.; Biswas, P. K.
- Physical Review B, Vol. 88, Issue 12
Surface electronic structure of the topological Kondo-insulator candidate correlated electron system SmB6
journal, December 2013
- Neupane, M.; Alidoust, N.; Xu, S-Y.
- Nature Communications, Vol. 4, Issue 1
Observation of possible topological in-gap surface states in the Kondo insulator SmB6 by photoemission
journal, December 2013
- Jiang, J.; Li, S.; Zhang, T.
- Nature Communications, Vol. 4, Issue 1
Low-temperature surface conduction in the Kondo insulator SmB
journal, November 2013
- Wolgast, Steven; Kurdak, Çağlıyan; Sun, Kai
- Physical Review B, Vol. 88, Issue 18
Topological surface state in the Kondo insulator samarium hexaboride
journal, March 2014
- Kim, D. J.; Xia, J.; Fisk, Z.
- Nature Materials, Vol. 13, Issue 5
Angle-resolved Photoemission Spectroscopy Study on the Surface States of the Correlated Topological Insulator YbB6
journal, August 2014
- Xia, M.; Jiang, J.; Ye, Z. R.
- Scientific Reports, Vol. 4, Issue 1
Non-Kondo-like Electronic Structure in the Correlated Rare-Earth Hexaboride
journal, January 2015
- Neupane, Madhab; Xu, Su-Yang; Alidoust, Nasser
- Physical Review Letters, Vol. 114, Issue 1
Magnetic and transport properties of pure and carbon‐doped divalent RE hexaboride single crystals
journal, January 1980
- Tarascon, J. M.; Etourneau, J.; Dordor, P.
- Journal of Applied Physics, Vol. 51, Issue 1
Topological Crystalline Kondo Insulator in Mixed Valence Ytterbium Borides
journal, January 2014
- Weng, Hongming; Zhao, Jianzhou; Wang, Zhijun
- Physical Review Letters, Vol. 112, Issue 1
De Haas-van Alphen study of the hexaborides of La, Ce, Pr, and Nd; First results
journal, November 1982
- van Deursen, A. P. J.; Fisk, Z.; de Vroomen, A. R.
- Solid State Communications, Vol. 44, Issue 5
Quantum Interference in the Spin-Polarized Heavy Fermion Compound : Evidence for Topological Deformation of the Fermi Surface in Strong Magnetic Fields
journal, July 1998
- Harrison, N.; Hall, D. W.; Goodrich, R. G.
- Physical Review Letters, Vol. 81, Issue 4
Fermi surface properties of low-concentration de Haas–van Alphen
journal, November 2000
- Teklu, A. A.; Goodrich, R. G.; Harrison, N.
- Physical Review B, Vol. 62, Issue 19
Magnetic-field dependence of the paramagnetic to the high-temperature magnetically ordered phase transition in
journal, July 2000
- Hall, Donavan; Fisk, Z.; Goodrich, R. G.
- Physical Review B, Vol. 62, Issue 1
Zero-field magnetic structure in reinvestigated by neutron diffraction and muon spin relaxation
journal, December 2003
- Zaharko, O.; Fischer, P.; Schenck, A.
- Physical Review B, Vol. 68, Issue 21
Extension of the temperature-magnetic field phase diagram of
journal, February 2004
- Goodrich, R. G.; Young, David P.; Hall, Donavan
- Physical Review B, Vol. 69, Issue 5
Itinerant magnetism in the Kondo crystal as indicated by polarized neutron scattering
journal, March 2005
- Plakhty, V. P.; Regnault, L. P.; Goltsev, A. V.
- Physical Review B, Vol. 71, Issue 10
Resonant magnetic exciton mode in the heavy-fermion antiferromagnet CeB6
journal, January 2012
- Friemel, G.; Li, Yuan; Dukhnenko, A. V.
- Nature Communications, Vol. 3, Issue 1
Intense low-energy ferromagnetic fluctuations in the antiferromagnetic heavy-fermion metal CeB6
journal, May 2014
- Jang, Hoyoung; Friemel, G.; Ollivier, J.
- Nature Materials, Vol. 13, Issue 7
Dense Kondo behavior in CeB6 and its alloys
journal, February 1983
- Komatsubara, T.; Sato, N.; Kunii, S.
- Journal of Magnetism and Magnetic Materials, Vol. 31-34
Magnetic Phase Diagrams of the Dense Kondo Compounds CeB 6 and Ce 0.5 La 0.5 B 6
journal, October 1995
- Nakamura, Shintaro; Goto, Terutaka; Kunii, Satoru
- Journal of the Physical Society of Japan, Vol. 64, Issue 10
Electrical resistivity and magnetoresistance of CeB6
journal, November 1980
- Takase, A.; Kojima, K.; Komatsubara, T.
- Solid State Communications, Vol. 36, Issue 5
Anomalous femtosecond quasiparticle dynamics of hidden order state in URu Si
journal, October 2011
- Dakovski, Georgi L.; Li, Yinwan; Gilbertson, Steve M.
- Physical Review B, Vol. 84, Issue 16
Imaging the Three-Dimensional Fermi-Surface Pairing near the Hidden-Order Transition in Using Angle-Resolved Photoemission Spectroscopy
journal, September 2013
- Meng, Jian-Qiao; Oppeneer, Peter M.; Mydosh, John A.
- Physical Review Letters, Vol. 111, Issue 12
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Projector augmented-wave method
journal, December 1994
- Blöchl, P. E.
- Physical Review B, Vol. 50, Issue 24, p. 17953-17979
From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999
- Kresse, G.; Joubert, D.
- Physical Review B, Vol. 59, Issue 3, p. 1758-1775
Ab initio molecular dynamics for open-shell transition metals
journal, November 1993
- Kresse, G.; Hafner, J.
- Physical Review B, Vol. 48, Issue 17
Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996
- Kresse, G.; Furthmüller, J.
- Computational Materials Science, Vol. 6, Issue 1, p. 15-50
Contribution à l'étude des borures à teneur élevée en bore
journal, January 1954
- Blum, P.; Bertaut, F.
- Acta Crystallographica, Vol. 7, Issue 1
Fermi Surface and Cyclotron Mass of CeB 6
journal, October 1989
- Ōnuki, Yoshichika; Komatsubara, Takemi; H. P. Reinders, Paul
- Journal of the Physical Society of Japan, Vol. 58, Issue 10
Imaging the Formation of High-Energy Dispersion Anomalies in the Actinide
journal, November 2012
- Das, Tanmoy; Durakiewicz, Tomasz; Zhu, Jian-Xin
- Physical Review X, Vol. 2, Issue 4
Metamagnetism and soliton excitations in the modulated ferromagnetic Ising chain CoV O
journal, September 2011
- Kimber, Simon A. J.; Mutka, Hannu; Chatterji, Tapan
- Physical Review B, Vol. 84, Issue 10
Works referencing / citing this record:
Nesting-driven multipolar order in CeB6 from photoemission tomography
journal, March 2016
- Koitzsch, A.; Heming, N.; Knupfer, M.
- Nature Communications, Vol. 7, Issue 1
Multipolar phases and magnetically hidden order: review of the heavy-fermion compound Ce 1− x La x B 6
journal, May 2016
- Cameron, Alistair S.; Friemel, Gerd; Inosov, Dmytro S.
- Reports on Progress in Physics, Vol. 79, Issue 6
Doping-induced redistribution of magnetic spectral weight in the substituted hexaborides and
journal, February 2018
- Nikitin, S. E.; Portnichenko, P. Y.; Dukhnenko, A. V.
- Physical Review B, Vol. 97, Issue 7
Multipolar phases and magnetically hidden order: Review of the heavy-fermion compound Ce(1-x)La(x)B6
text, January 2015
- Cameron, A. S.; Friemel, G.; Inosov, D. S.
- arXiv