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Title: Quantum Oscillations at Integer and Fractional Landau Level Indices in Single-Crystalline ZrTe5

Abstract

A three-dimensional (3D) Dirac semimetal (DS) is an analogue of graphene, but with linear energy dispersion in all (three) momentum directions. 3D DSs have been a fertile playground in discovering novel quantum particles, for example Weyl fermions, in solid state systems. Many 3D DSs were theoretically predicted and experimentally confirmed. Here, we report here the results in exfoliated ZrTe5 thin flakes from the studies of aberration-corrected scanning transmission electron microscopy and low temperature magneto-transport measurements. We observed several unique results. First, a π Berry phase was obtained from the Landau fan diagram of the Shubnikov-de Haas oscillations in the longitudinal conductivity σxx. Second, the longitudinal resistivity ρxx shows a linear magnetic field dependence in the quantum limit regime. Most surprisingly, quantum oscillations were also observed at fractional Landau level indices N = 5/3 and 7/5, demonstrating strong electron-electron interaction effects in ZrTe5.

Authors:
 [1];  [2];  [2];  [3];  [3];  [2];  [1];  [1]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Georgia Inst. of Technology, Atlanta, GA (United States). School of Physics
  3. Univ. of Tennessee, Knoxville, TN (United States). Dept. of Physics and Astronomy
Publication Date:
Research Org.:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA)
OSTI Identifier:
1332915
Report Number(s):
SAND2016-10784J
Journal ID: ISSN 2045-2322; srep35357; TRN: US1601868
Grant/Contract Number:  
AC04-94AL85000; DMR-1350002; FG02-07ER46451
Resource Type:
Accepted Manuscript
Journal Name:
Scientific Reports
Additional Journal Information:
Journal Volume: 6; Journal ID: ISSN 2045-2322
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Citation Formats

Yu, W., Jiang, Y., Yang, J., Dun, Z. L., Zhou, H. D., Jiang, Z., Lu, P., and Pan, W. Quantum Oscillations at Integer and Fractional Landau Level Indices in Single-Crystalline ZrTe5. United States: N. p., 2016. Web. doi:10.1038/srep35357.
Yu, W., Jiang, Y., Yang, J., Dun, Z. L., Zhou, H. D., Jiang, Z., Lu, P., & Pan, W. Quantum Oscillations at Integer and Fractional Landau Level Indices in Single-Crystalline ZrTe5. United States. https://doi.org/10.1038/srep35357
Yu, W., Jiang, Y., Yang, J., Dun, Z. L., Zhou, H. D., Jiang, Z., Lu, P., and Pan, W. Fri . "Quantum Oscillations at Integer and Fractional Landau Level Indices in Single-Crystalline ZrTe5". United States. https://doi.org/10.1038/srep35357. https://www.osti.gov/servlets/purl/1332915.
@article{osti_1332915,
title = {Quantum Oscillations at Integer and Fractional Landau Level Indices in Single-Crystalline ZrTe5},
author = {Yu, W. and Jiang, Y. and Yang, J. and Dun, Z. L. and Zhou, H. D. and Jiang, Z. and Lu, P. and Pan, W.},
abstractNote = {A three-dimensional (3D) Dirac semimetal (DS) is an analogue of graphene, but with linear energy dispersion in all (three) momentum directions. 3D DSs have been a fertile playground in discovering novel quantum particles, for example Weyl fermions, in solid state systems. Many 3D DSs were theoretically predicted and experimentally confirmed. Here, we report here the results in exfoliated ZrTe5 thin flakes from the studies of aberration-corrected scanning transmission electron microscopy and low temperature magneto-transport measurements. We observed several unique results. First, a π Berry phase was obtained from the Landau fan diagram of the Shubnikov-de Haas oscillations in the longitudinal conductivity σxx. Second, the longitudinal resistivity ρxx shows a linear magnetic field dependence in the quantum limit regime. Most surprisingly, quantum oscillations were also observed at fractional Landau level indices N = 5/3 and 7/5, demonstrating strong electron-electron interaction effects in ZrTe5.},
doi = {10.1038/srep35357},
journal = {Scientific Reports},
number = ,
volume = 6,
place = {United States},
year = {Fri Oct 14 00:00:00 EDT 2016},
month = {Fri Oct 14 00:00:00 EDT 2016}
}

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Works referenced in this record:

Experimental observation of the quantum Hall effect and Berry's phase in graphene
journal, November 2005

  • Zhang, Yuanbo; Tan, Yan-Wen; Stormer, Horst L.
  • Nature, Vol. 438, Issue 7065, p. 201-204
  • DOI: 10.1038/nature04235

Dirac versus Weyl Fermions in Topological Insulators: Adler-Bell-Jackiw Anomaly in Transport Phenomena
journal, December 2013


Quantum magnetoresistance
journal, August 1998


Giant Resistivity Anomaly in ZrTe 5
journal, August 1980

  • Okada, Shigeto; Sambongi, Takashi; Ido, Masayuki
  • Journal of the Physical Society of Japan, Vol. 49, Issue 2
  • DOI: 10.1143/JPSJ.49.839

Three-dimensional Dirac semimetal and quantum transport in Cd 3 As 2
journal, September 2013


Observation of Fermi arc surface states in a topological metal
journal, December 2014


Transport evidence for the three-dimensional Dirac semimetal phase in ZrT e 5
journal, March 2016


Gating of high-mobility InAs metamorphic heterostructures
journal, December 2014

  • Shabani, J.; McFadden, A. P.; Shojaei, B.
  • Applied Physics Letters, Vol. 105, Issue 26
  • DOI: 10.1063/1.4905370

Thermoelectric power of HfTe5 and ZrTe5
journal, June 1982


Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi
journal, January 2014


Quantum Oscillations and Hall Anomaly of Surface States in the Topological Insulator Bi2Te3
journal, July 2010


High-field Shubnikov–de Haas oscillations in the topological insulator Bi 2 Te 2 Se
journal, July 2012


Extremely high electron mobility in a phonon-glass semimetal
journal, April 2013

  • Ishiwata, S.; Shiomi, Y.; Lee, J. S.
  • Nature Materials, Vol. 12, Issue 6
  • DOI: 10.1038/nmat3621

Electronic structure of Zr Te 5
journal, July 1982


Room Temperature Giant and Linear Magnetoresistance in Topological Insulator Bi 2 Te 3 Nanosheets
journal, June 2012


Magnetoinfrared Spectroscopy of Landau Levels and Zeeman Splitting of Three-Dimensional Massless Dirac Fermions in ZrTe 5
journal, October 2015


Experimental Realization of a Three-Dimensional Dirac Semimetal
journal, July 2014


Quantum Transport Evidence for the Three-Dimensional Dirac Semimetal Phase in Cd 3 As 2
journal, December 2014


Chiral magnetic effect in ZrTe5
journal, February 2016

  • Li, Qiang; Kharzeev, Dmitri E.; Zhang, Cheng
  • Nature Physics, Vol. 12, Issue 6
  • DOI: 10.1038/nphys3648

Ti insertion in the M Te 5 ( M = Zr, Hf) structure type: Hf 0.78 Ti 0.22 Te 5
journal, February 2012

  • Yu, Jaemin; Yun, Hoseop
  • Acta Crystallographica Section E Structure Reports Online, Vol. 68, Issue 3
  • DOI: 10.1107/S1600536812006691

Effect of elastic tension on the electrical resistance of HfTe 5 and ZrTe 5
journal, January 1989


Quantized Hall Effect and Shubnikov–de Haas Oscillations in Highly Doped Bi 2 Se 3 : Evidence for Layered Transport of Bulk Carriers
journal, May 2012


Two-dimensional surface state in the quantum limit of a topological insulator
journal, November 2010

  • Analytis, James G.; McDonald, Ross D.; Riggs, Scott C.
  • Nature Physics, Vol. 6, Issue 12
  • DOI: 10.1038/nphys1861

Quantum Linear Magnetoresistance in Multilayer Epitaxial Graphene
journal, October 2010

  • Friedman, Adam L.; Tedesco, Joseph L.; Campbell, Paul M.
  • Nano Letters, Vol. 10, Issue 10
  • DOI: 10.1021/nl101797d

A stable three-dimensional topological Dirac semimetal Cd3As2
journal, May 2014

  • Liu, Z. K.; Jiang, J.; Zhou, B.
  • Nature Materials, Vol. 13, Issue 7
  • DOI: 10.1038/nmat3990

Detection of Berry's Phase in a Bulk Rashba Semiconductor
journal, December 2013


Topological semimetal and Fermi-arc surface states in the electronic structure of pyrochlore iridates
journal, May 2011


Single crystals of transition metal trichalcogenides
journal, January 1983


Two-dimensional gas of massless Dirac fermions in graphene
journal, November 2005

  • Novoselov, K. S.; Geim, A. K.; Morozov, S. V.
  • Nature, Vol. 438, Issue 7065, p. 197-200
  • DOI: 10.1038/nature04233

The Crystal Structure of HfTe5.
journal, January 1973


Observation of a three-dimensional topological Dirac semimetal phase in high-mobility Cd3As2
journal, May 2014

  • Neupane, Madhab; Xu, Su-Yang; Sankar, Raman
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms4786

Works referencing / citing this record:

Type I superconductivity in Dirac materials
journal, July 2018

  • Shapiro, B. Ya; Shapiro, I.; Li, Dingping
  • Journal of Physics: Condensed Matter, Vol. 30, Issue 33
  • DOI: 10.1088/1361-648x/aad305

Magnetic properties of type-I and type-II Weyl semimetals in the superconducting state
journal, April 2018


The Property, Preparation and Application of Topological Insulators: A Review
journal, July 2017


Type I superconductivity in Dirac materials
text, January 2018