Towards stable and commercially available perovskite solar cells
Abstract
Solar cells employing a halide perovskite with an organic cation now show power conversion efficiency of up to 22%. But, these cells are facing issues towards commercialization, such as the need to achieve long-term stability and the development of a manufacturing method for the reproducible fabrication of high-performance devices. We propose a strategy to obtain stable and commercially viable perovskite solar cells. A reproducible manufacturing method is suggested, as well as routes to manage grain boundaries and interfacial charge transport. Electroluminescence is regarded as a metric to gauge theoretical efficiency. We highlight how optimizing the design of device architectures is important not only for achieving high efficiency but also for hysteresis-free and stable performance. Here, we argue that reliable device characterization is needed to ensure the advance of this technology towards practical applications. We believe that perovskite-based devices can be competitive with silicon solar modules, and discuss issues related to the safe management of toxic material.
- Authors:
-
- Sungkyunkwan Univ., Suwon (Republic of Korea). School of Chemical Engineering
- Ecole Polytechnique Federale Lausanne (Switzlerland). Inst. of Chemical Sciences and Engineering
- Toin Univ. of Yokohama (Japan)
- National Renewable Energy Lab. (NREL), Golden, CO (United States)
- Publication Date:
- Research Org.:
- National Renewable Energy Laboratory (NREL), Golden, CO (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office
- OSTI Identifier:
- 1329525
- Report Number(s):
- NREL/JA-5900-66413
Journal ID: ISSN 2058-7546
- Grant/Contract Number:
- AC36-08GO28308
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Energy
- Additional Journal Information:
- Journal Volume: 1; Journal Issue: 11; Journal ID: ISSN 2058-7546
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; 36 MATERIALS SCIENCE; solar cells; perovskite; manufacturing; grain boundaries; interfacial charge transport
Citation Formats
Park, Nam-Gyu, Grätzel, Michael, Miyasaka, Tsutomu, Zhu, Kai, and Emery, Keith. Towards stable and commercially available perovskite solar cells. United States: N. p., 2016.
Web. doi:10.1038/nenergy.2016.152.
Park, Nam-Gyu, Grätzel, Michael, Miyasaka, Tsutomu, Zhu, Kai, & Emery, Keith. Towards stable and commercially available perovskite solar cells. United States. https://doi.org/10.1038/nenergy.2016.152
Park, Nam-Gyu, Grätzel, Michael, Miyasaka, Tsutomu, Zhu, Kai, and Emery, Keith. Mon .
"Towards stable and commercially available perovskite solar cells". United States. https://doi.org/10.1038/nenergy.2016.152. https://www.osti.gov/servlets/purl/1329525.
@article{osti_1329525,
title = {Towards stable and commercially available perovskite solar cells},
author = {Park, Nam-Gyu and Grätzel, Michael and Miyasaka, Tsutomu and Zhu, Kai and Emery, Keith},
abstractNote = {Solar cells employing a halide perovskite with an organic cation now show power conversion efficiency of up to 22%. But, these cells are facing issues towards commercialization, such as the need to achieve long-term stability and the development of a manufacturing method for the reproducible fabrication of high-performance devices. We propose a strategy to obtain stable and commercially viable perovskite solar cells. A reproducible manufacturing method is suggested, as well as routes to manage grain boundaries and interfacial charge transport. Electroluminescence is regarded as a metric to gauge theoretical efficiency. We highlight how optimizing the design of device architectures is important not only for achieving high efficiency but also for hysteresis-free and stable performance. Here, we argue that reliable device characterization is needed to ensure the advance of this technology towards practical applications. We believe that perovskite-based devices can be competitive with silicon solar modules, and discuss issues related to the safe management of toxic material.},
doi = {10.1038/nenergy.2016.152},
journal = {Nature Energy},
number = 11,
volume = 1,
place = {United States},
year = {2016},
month = {10}
}
Web of Science
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Beyond efficiency: phenothiazine, a new commercially viable substituent for hole transport materials in perovskite solar cells
journal, January 2019
- Maciejczyk, Michal R.; Chen, Ruihao; Brown, Alasdair
- Journal of Materials Chemistry C, Vol. 7, Issue 28
Inorganic–organic halide perovskites for new photovoltaic technology
journal, August 2017
- Li, Dongmei; Shi, Jiangjian; Xu, Yuzhuan
- National Science Review, Vol. 5, Issue 4
Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells.
text, January 2019
- Alharbi, Essa A.; Alyamani, Ahmed Y.; Kubicki, Dominik
- Apollo - University of Cambridge Repository
Performance Loss Analysis and Design Space Optimization of Perovskite Solar Cells
text, January 2018
- Agarwal, Sumanshu; Nair, Pradeep R.
- arXiv
Shape-Pure, Nearly Monodispersed CsPbBr 3 Nanocubes Prepared Using Secondary Aliphatic Amines
journal, November 2018
- Imran, Muhammad; Ijaz, Palvasha; Baranov, Dmitry
- Nano Letters, Vol. 18, Issue 12
Role of Acid–Base Equilibria in the Size, Shape, and Phase Control of Cesium Lead Bromide Nanocrystals
journal, January 2018
- Almeida, Guilherme; Goldoni, Luca; Akkerman, Quinten
- ACS Nano, Vol. 12, Issue 2
Study on the Property of Electron-Transport Layer in the Doped Formamidinium Lead Iodide Perovskite Based on DFT
journal, November 2019
- Diao, Xin-Feng; Tang, Yan-lin; Xie, Quan
- ACS Omega, Vol. 4, Issue 22
Ultrafast and broadband photodetectors based on a perovskite/organic bulk heterojunction for large-dynamic-range imaging
journal, March 2020
- Li, Chenglong; Wang, Hailu; Wang, Fang
- Light: Science & Applications, Vol. 9, Issue 1
Tailoring vertical phase distribution of quasi-two-dimensional perovskite films via surface modification of hole-transporting layer
journal, February 2019
- Liu, Tiefeng; Jiang, Youyu; Qin, Minchao
- Nature Communications, Vol. 10, Issue 1
Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells
journal, July 2019
- Alharbi, Essa A.; Alyamani, Ahmed Y.; Kubicki, Dominik J.
- Nature Communications, Vol. 10, Issue 1
Carrier lifetime enhancement in halide perovskite via remote epitaxy
journal, September 2019
- Jiang, Jie; Sun, Xin; Chen, Xinchun
- Nature Communications, Vol. 10, Issue 1
Hazard potential of perovskite solar cell technology for potential implementation of “safe-by-design” approach
journal, March 2019
- Bae, Su-Yong; Lee, Su Young; Kim, Ji-wan
- Scientific Reports, Vol. 9, Issue 1
Perspective: Theory and simulation of hybrid halide perovskites
journal, June 2017
- Whalley, Lucy D.; Frost, Jarvist M.; Jung, Young-Kwang
- The Journal of Chemical Physics, Vol. 146, Issue 22
Facile and noninvasive passivation, doping and chemical tuning of macroscopic hybrid perovskite crystals
journal, March 2020
- Kirmani, Ahmad R.; Mansour, Ahmed E.; Yang, Chen
- PLOS ONE, Vol. 15, Issue 3