Towards stable and commercially available perovskite solar cells

Park, Nam-Gyu; Grätzel, Michael; Miyasaka, Tsutomu; Zhu, Kai; Emery, Keith

doi:10.1038/nenergy.2016.152

Title: Towards stable and commercially available perovskite solar cells

Journal Article · 17 October 2016 · Nature Energy

DOI: https://doi.org/10.1038/nenergy.2016.152 · OSTI ID:1329525

Park, Nam-Gyu ^[1]; Grätzel, Michael ^[2]; Miyasaka, Tsutomu ^[3]; Zhu, Kai ^[4]; Emery, Keith ^[4]

Sungkyunkwan Univ., Suwon (Republic of Korea). School of Chemical Engineering
Ecole Polytechnique Federale Lausanne (Switzlerland). Inst. of Chemical Sciences and Engineering
Toin Univ. of Yokohama (Japan)
National Renewable Energy Lab. (NREL), Golden, CO (United States)

Solar cells employing a halide perovskite with an organic cation now show power conversion efficiency of up to 22%. But, these cells are facing issues towards commercialization, such as the need to achieve long-term stability and the development of a manufacturing method for the reproducible fabrication of high-performance devices. We propose a strategy to obtain stable and commercially viable perovskite solar cells. A reproducible manufacturing method is suggested, as well as routes to manage grain boundaries and interfacial charge transport. Electroluminescence is regarded as a metric to gauge theoretical efficiency. We highlight how optimizing the design of device architectures is important not only for achieving high efficiency but also for hysteresis-free and stable performance. Here, we argue that reliable device characterization is needed to ensure the advance of this technology towards practical applications. We believe that perovskite-based devices can be competitive with silicon solar modules, and discuss issues related to the safe management of toxic material.

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Renewable Energy. Solar Energy Technologies Office

Grant/Contract Number:: AC36-08GO28308

OSTI ID:: 1329525

Report Number(s):: NREL/JA-5900-66413

Journal Information:: Nature Energy, Vol. 1, Issue 11; ISSN 2058-7546

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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On-device lead sequestration for perovskite solar cells Li, Xun; Zhang, Fei; He, Haiying Nature, Vol. 578, Issue 7796 https://doi.org/10.1038/s41586-020-2001-x	journal	February 2020
Pressure responses of halide perovskites with various compositions, dimensionalities, and morphologies Li, Mei; Liu, Tianbiao; Wang, Yonggang Matter and Radiation at Extremes, Vol. 5, Issue 1 https://doi.org/10.1063/1.5133653	journal	January 2020
Charge Transfer in Mixed-Phase TiO2 Photoelectrodes for Perovskite Solar Cells Nikolskaia, Anna; Vildanova, Marina; Kozlov, Sergey Sustainability, Vol. 12, Issue 3 https://doi.org/10.3390/su12030788	journal	January 2020
Integrated Perovskite/Bulk‐Heterojunction Organic Solar Cells Liu, Yongsheng; Chen, Yongsheng Advanced Materials, Vol. 32, Issue 3 https://doi.org/10.1002/adma.201805843	journal	February 2019
Recent progressive efforts in perovskite solar cells toward commercialization Kim, Byeong Jo; Lee, Sangwook; Jung, Hyun Suk Journal of Materials Chemistry A, Vol. 6, Issue 26 https://doi.org/10.1039/c8ta02159g	journal	January 2018
Large metal halide perovskite crystals for field-effect transistor applications Matsushima, Toshinori; Leyden, Matthew R.; Fujihara, Takashi Applied Physics Letters, Vol. 115, Issue 12 https://doi.org/10.1063/1.5116411	journal	September 2019
Challenges for commercializing perovskite solar cells Rong, Yaoguang; Hu, Yue; Mei, Anyi Science, Vol. 361, Issue 6408 https://doi.org/10.1126/science.aat8235	journal	September 2018
High-Temperature Ionic Epitaxy of Halide Perovskite Thin Film and the Hidden Carrier Dynamics Wang, Yiping; Sun, Xin; Chen, Zhizhong Advanced Materials, Vol. 29, Issue 35 https://doi.org/10.1002/adma.201702643	journal	July 2017
On the Current–Voltage Hysteresis in Perovskite Solar Cells: Dependence on Perovskite Composition and Methods to Remove Hysteresis Kang, Dong‐Ho; Park, Nam‐Gyu Advanced Materials, Vol. 31, Issue 34 https://doi.org/10.1002/adma.201805214	journal	February 2019
Broadband Extrinsic Self‐Trapped Exciton Emission in Sn‐Doped 2D Lead‐Halide Perovskites Yu, Jiancan; Kong, Jintao; Hao, Wei Advanced Materials https://doi.org/10.1002/adma.201806385	journal	December 2018
Insight into the Interfacial Elastic Contact in Stacking Perovskite Solar Cells Shao, Yingying; Zhang, Chunyang; Wang, Shi Advanced Materials Interfaces, Vol. 6, Issue 7 https://doi.org/10.1002/admi.201900157	journal	February 2019
Performance Enhancement of Perovskite Solar Cells Induced by Lead Acetate as an Additive Tang, Guanqi; You, Peng; Tai, Qidong Solar RRL, Vol. 2, Issue 6 https://doi.org/10.1002/solr.201800066	journal	April 2018
Discrete SnO ₂ Nanoparticle‐Modified Poly(3,4‐Ethylenedioxythiophene):Poly(Styrenesulfonate) for Efficient Perovskite Solar Cells Jia, Pengcheng; Bi, Wentao; Huang, Xin Solar RRL, Vol. 3, Issue 10 https://doi.org/10.1002/solr.201900162	journal	July 2019
A non-equilibrium Ti ⁴⁺ doping strategy for an efficient hematite electron transport layer in perovskite solar cells Zhu, Weidong; Zhang, Qianni; Zhang, Chunfu Dalton Transactions, Vol. 47, Issue 18 https://doi.org/10.1039/c8dt00692j	journal	January 2018
Beyond efficiency: phenothiazine, a new commercially viable substituent for hole transport materials in perovskite solar cells Maciejczyk, Michal R.; Chen, Ruihao; Brown, Alasdair Journal of Materials Chemistry C, Vol. 7, Issue 28 https://doi.org/10.1039/c8tc05773g	journal	January 2019
Inorganic–organic halide perovskites for new photovoltaic technology Li, Dongmei; Shi, Jiangjian; Xu, Yuzhuan National Science Review, Vol. 5, Issue 4 https://doi.org/10.1093/nsr/nwx100	journal	August 2017
Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells. Alharbi, Essa A.; Alyamani, Ahmed Y.; Kubicki, Dominik Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.43116	text	January 2019
Performance Loss Analysis and Design Space Optimization of Perovskite Solar Cells Agarwal, Sumanshu; Nair, Pradeep R. arXiv https://doi.org/10.48550/arxiv.1803.04171	text	January 2018
Shape-Pure, Nearly Monodispersed CsPbBr ₃ Nanocubes Prepared Using Secondary Aliphatic Amines Imran, Muhammad; Ijaz, Palvasha; Baranov, Dmitry Nano Letters, Vol. 18, Issue 12 https://doi.org/10.1021/acs.nanolett.8b03598	journal	November 2018
Role of Acid–Base Equilibria in the Size, Shape, and Phase Control of Cesium Lead Bromide Nanocrystals Almeida, Guilherme; Goldoni, Luca; Akkerman, Quinten ACS Nano, Vol. 12, Issue 2 https://doi.org/10.1021/acsnano.7b08357	journal	January 2018
Study on the Property of Electron-Transport Layer in the Doped Formamidinium Lead Iodide Perovskite Based on DFT Diao, Xin-Feng; Tang, Yan-lin; Xie, Quan ACS Omega, Vol. 4, Issue 22 https://doi.org/10.1021/acsomega.9b03015	journal	November 2019
Ultrafast and broadband photodetectors based on a perovskite/organic bulk heterojunction for large-dynamic-range imaging Li, Chenglong; Wang, Hailu; Wang, Fang Light: Science & Applications, Vol. 9, Issue 1 https://doi.org/10.1038/s41377-020-0264-5	journal	March 2020
Tailoring vertical phase distribution of quasi-two-dimensional perovskite films via surface modification of hole-transporting layer Liu, Tiefeng; Jiang, Youyu; Qin, Minchao Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08843-5	journal	February 2019
Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells Alharbi, Essa A.; Alyamani, Ahmed Y.; Kubicki, Dominik J. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10985-5	journal	July 2019
Carrier lifetime enhancement in halide perovskite via remote epitaxy Jiang, Jie; Sun, Xin; Chen, Xinchun Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-12056-1	journal	September 2019
Hazard potential of perovskite solar cell technology for potential implementation of “safe-by-design” approach Bae, Su-Yong; Lee, Su Young; Kim, Ji-wan Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-018-37229-8	journal	March 2019
Perspective: Theory and simulation of hybrid halide perovskites Whalley, Lucy D.; Frost, Jarvist M.; Jung, Young-Kwang The Journal of Chemical Physics, Vol. 146, Issue 22 https://doi.org/10.1063/1.4984964	journal	June 2017
Facile and noninvasive passivation, doping and chemical tuning of macroscopic hybrid perovskite crystals Kirmani, Ahmad R.; Mansour, Ahmed E.; Yang, Chen PLOS ONE, Vol. 15, Issue 3 https://doi.org/10.1371/journal.pone.0230540	journal	March 2020

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