Towards stable and commercially available perovskite solar cells

Park, Nam-Gyu; Grätzel, Michael; Miyasaka, Tsutomu; Zhu, Kai; Emery, Keith

doi:10.1038/nenergy.2016.152

Title: Towards stable and commercially available perovskite solar cells

Abstract

Solar cells employing a halide perovskite with an organic cation now show power conversion efficiency of up to 22%. But, these cells are facing issues towards commercialization, such as the need to achieve long-term stability and the development of a manufacturing method for the reproducible fabrication of high-performance devices. We propose a strategy to obtain stable and commercially viable perovskite solar cells. A reproducible manufacturing method is suggested, as well as routes to manage grain boundaries and interfacial charge transport. Electroluminescence is regarded as a metric to gauge theoretical efficiency. We highlight how optimizing the design of device architectures is important not only for achieving high efficiency but also for hysteresis-free and stable performance. Here, we argue that reliable device characterization is needed to ensure the advance of this technology towards practical applications. We believe that perovskite-based devices can be competitive with silicon solar modules, and discuss issues related to the safe management of toxic material.

Authors:

Park, Nam-Gyu ^[1]; Grätzel, Michael ^[2]; Miyasaka, Tsutomu ^[3]; Zhu, Kai ^[4]; Emery, Keith ^[4]

Sungkyunkwan Univ., Suwon (Republic of Korea). School of Chemical Engineering
Ecole Polytechnique Federale Lausanne (Switzlerland). Inst. of Chemical Sciences and Engineering
Toin Univ. of Yokohama (Japan)
National Renewable Energy Lab. (NREL), Golden, CO (United States)

Publication Date:: 2016-10-17

Research Org.:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Org.:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office

OSTI Identifier:: 1329525

Report Number(s):: NREL/JA-5900-66413
Journal ID: ISSN 2058-7546

Grant/Contract Number:: AC36-08GO28308

Resource Type:: Accepted Manuscript

Journal Name:: Nature Energy

Additional Journal Information:: Journal Volume: 1; Journal Issue: 11; Journal ID: ISSN 2058-7546

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 14 SOLAR ENERGY; 36 MATERIALS SCIENCE; solar cells; perovskite; manufacturing; grain boundaries; interfacial charge transport

Citation Formats


                    Park, Nam-Gyu, Grätzel, Michael, Miyasaka, Tsutomu, Zhu, Kai, and Emery, Keith. Towards stable and commercially available perovskite solar cells.  United States: N. p., 2016. 
Web.  doi:10.1038/nenergy.2016.152.

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                    Park, Nam-Gyu, Grätzel, Michael, Miyasaka, Tsutomu, Zhu, Kai, & Emery, Keith. Towards stable and commercially available perovskite solar cells.  United States.  https://doi.org/10.1038/nenergy.2016.152

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                    Park, Nam-Gyu, Grätzel, Michael, Miyasaka, Tsutomu, Zhu, Kai, and Emery, Keith. Mon .  
"Towards stable and commercially available perovskite solar cells".  United States.  https://doi.org/10.1038/nenergy.2016.152.  https://www.osti.gov/servlets/purl/1329525.

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@article{osti_1329525,

  title        = {Towards stable and commercially available perovskite solar cells},

  author       = {Park, Nam-Gyu and Grätzel, Michael and Miyasaka, Tsutomu and Zhu, Kai and Emery, Keith},

  abstractNote = {Solar cells employing a halide perovskite with an organic cation now show power conversion efficiency of up to 22%. But, these cells are facing issues towards commercialization, such as the need to achieve long-term stability and the development of a manufacturing method for the reproducible fabrication of high-performance devices. We propose a strategy to obtain stable and commercially viable perovskite solar cells. A reproducible manufacturing method is suggested, as well as routes to manage grain boundaries and interfacial charge transport. Electroluminescence is regarded as a metric to gauge theoretical efficiency. We highlight how optimizing the design of device architectures is important not only for achieving high efficiency but also for hysteresis-free and stable performance. Here, we argue that reliable device characterization is needed to ensure the advance of this technology towards practical applications. We believe that perovskite-based devices can be competitive with silicon solar modules, and discuss issues related to the safe management of toxic material.},

  doi          = {10.1038/nenergy.2016.152},

  journal      = {Nature Energy},

  number       = 11,

  volume       = 1,

  place        = {United States},

  year         = {2016},

  month        = {10}

}

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Molecular Engineering of the Fullerene‐Based Electron Transport Layer Materials for Improving Ambient Stability of Perovskite Solar Cells
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Ab initio study of the dynamics of electron trapping and detrapping processes in the CH ₃ NH ₃ PbI ₃ perovskite
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Skillfully deflecting the question: a small amount of piperazine-1,4-diium iodide radically enhances the thermal stability of CsPbI ₃ perovskite
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Influence of Grain Size on Phase Transitions in Halide Perovskite Films
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Stavrakas, Camille; Zelewski, Szymon J.; Frohna, Kyle
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Benchmarking Chemical Stability of Arbitrarily Mixed 3D Hybrid Halide Perovskites for Solar Cell Applications
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García‐Fernández, Alberto; Juarez‐Perez, Emilio J.; Castro‐García, Socorro
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Interface Engineering in n‐i‐p Metal Halide Perovskite Solar Cells
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Yang, Zhi; Dou, Jinjuan; Wang, Minqiang
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Liu, Tiefeng; Jiang, Youyu; Qin, Minchao
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Impacts of alkaline on the defects property and crystallization kinetics in perovskite solar cells
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Chen, Yihua; Li, Nengxu; Wang, Ligang
Nature Communications, Vol. 10, Issue 1
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Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells
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Alharbi, Essa A.; Alyamani, Ahmed Y.; Kubicki, Dominik J.
Nature Communications, Vol. 10, Issue 1
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Reduction of lead leakage from damaged lead halide perovskite solar modules using self-healing polymer-based encapsulation
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Jiang, Yan; Qiu, Longbin; Juarez-Perez, Emilio J.
Nature Energy, Vol. 4, Issue 7
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Imperfections and their passivation in halide perovskite solar cells
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Chen, Bo; Rudd, Peter N.; Yang, Shuang
Chemical Society Reviews, Vol. 48, Issue 14
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Stable, color-tunable 2D SCN-based perovskites: revealing the critical influence of an asymmetric pseudo-halide on constituent ions
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Li, Chia-Hsin; Tsai, Chang-Che; Liao, Ming-Yun
Nanoscale, Vol. 11, Issue 6
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Ultrafast carrier dynamics of metal halide perovskite nanocrystals and perovskite-composites
journal, January 2019

Mondal, Navendu; De, Apurba; Das, Somnath
Nanoscale, Vol. 11, Issue 20
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Potassium ions as a kinetic controller in ionic double layers for hysteresis-free perovskite solar cells
journal, January 2019

Kim, Seul-Gi; Li, Cheng; Guerrero, Antonio
Journal of Materials Chemistry A, Vol. 7, Issue 32
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Sulfur-fused perylene diimide electron transport layers allow >400 h operational lifetime of methylammonium lead iodide photovoltaics
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Nakayama, Hidenori; Zheng, Yonghao; Schneider, Julia A.
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Advances in modelling and simulation of halide perovskites for solar cell applications
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Yu, Chol-Jun
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Giant Rashba splitting in 2D organic-inorganic halide perovskites measured by transient spectroscopies
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Science Advances, Vol. 3, Issue 7
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Lee, Chia-Chen; Chen, Chih-I; Liao, Yu-Te
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Materials chemistry and engineering in metal halide perovskite lasers
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Liu, Yongsheng; Chen, Yongsheng
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Recent progressive efforts in perovskite solar cells toward commercialization
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Large metal halide perovskite crystals for field-effect transistor applications
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Matsushima, Toshinori; Leyden, Matthew R.; Fujihara, Takashi
Applied Physics Letters, Vol. 115, Issue 12
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Challenges for commercializing perovskite solar cells
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Rong, Yaoguang; Hu, Yue; Mei, Anyi
Science, Vol. 361, Issue 6408
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High-Temperature Ionic Epitaxy of Halide Perovskite Thin Film and the Hidden Carrier Dynamics
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Wang, Yiping; Sun, Xin; Chen, Zhizhong
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Kang, Dong‐Ho; Park, Nam‐Gyu
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Yu, Jiancan; Kong, Jintao; Hao, Wei
Advanced Materials
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Insight into the Interfacial Elastic Contact in Stacking Perovskite Solar Cells
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Shao, Yingying; Zhang, Chunyang; Wang, Shi
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Chemical stability and instability of inorganic halide perovskites
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Zhou, Yuanyuan; Zhao, Yixin
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Inorganic–organic halide perovskites for new photovoltaic technology
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Li, Dongmei; Shi, Jiangjian; Xu, Yuzhuan
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Atomic-level passivation mechanism of ammonium salts enabling highly efficient perovskite solar cells.
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Alharbi, Essa A.; Alyamani, Ahmed Y.; Kubicki, Dominik
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Performance Loss Analysis and Design Space Optimization of Perovskite Solar Cells
text, January 2018

Agarwal, Sumanshu; Nair, Pradeep R.
arXiv
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Imran, Muhammad; Ijaz, Palvasha; Baranov, Dmitry
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Role of Acid–Base Equilibria in the Size, Shape, and Phase Control of Cesium Lead Bromide Nanocrystals
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Almeida, Guilherme; Goldoni, Luca; Akkerman, Quinten
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Study on the Property of Electron-Transport Layer in the Doped Formamidinium Lead Iodide Perovskite Based on DFT
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Diao, Xin-Feng; Tang, Yan-lin; Xie, Quan
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Li, Chenglong; Wang, Hailu; Wang, Fang
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Liu, Tiefeng; Jiang, Youyu; Qin, Minchao
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DOI: 10.1038/s41467-019-08843-5

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Nature Communications, Vol. 10, Issue 1
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Carrier lifetime enhancement in halide perovskite via remote epitaxy
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Nature Communications, Vol. 10, Issue 1
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Hazard potential of perovskite solar cell technology for potential implementation of “safe-by-design” approach
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Bae, Su-Yong; Lee, Su Young; Kim, Ji-wan
Scientific Reports, Vol. 9, Issue 1
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Perspective: Theory and simulation of hybrid halide perovskites
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Whalley, Lucy D.; Frost, Jarvist M.; Jung, Young-Kwang
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Facile and noninvasive passivation, doping and chemical tuning of macroscopic hybrid perovskite crystals
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Kirmani, Ahmad R.; Mansour, Ahmed E.; Yang, Chen
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Detection of X-ray photons by solution-processed lead halide perovskites
journal, May 2015

Organometal Halide Perovskites as Visible-Light Sensitizers for Photovoltaic Cells
journal, May 2009

Grain boundary dominated ion migration in polycrystalline organic–inorganic halide perovskite films
journal, January 2016

Efficient and stable large-area perovskite solar cells with inorganic charge extraction layers
journal, October 2015

Understanding the rate-dependent J–V hysteresis, slow time component, and aging in CH ₃ NH ₃ PbI ₃ perovskite solar cells: the role of a compensated electric field
journal, January 2015

Organolead Halide Perovskites for Low Operating Voltage Multilevel Resistive Switching
journal, May 2016

Origin and elimination of photocurrent hysteresis by fullerene passivation in CH3NH3PbI3 planar heterojunction solar cells
journal, December 2014

Efficient luminescent solar cells based on tailored mixed-cation perovskites
journal, January 2016

Highly Reproducible Perovskite Solar Cells with Average Efficiency of 18.3% and Best Efficiency of 19.7% Fabricated via Lewis Base Adduct of Lead(II) Iodide
journal, July 2015

Solvent engineering for high-performance inorganic–organic hybrid perovskite solar cells
journal, July 2014

A Fast Deposition-Crystallization Procedure for Highly Efficient Lead Iodide Perovskite Thin-Film Solar Cells
journal, July 2014

Predicting the Open-Circuit Voltage of CH ₃ NH ₃ PbI ₃ Perovskite Solar Cells Using Electroluminescence and Photovoltaic Quantum Efficiency Spectra: the Role of Radiative and Non-Radiative Recombination
journal, September 2014

Organometal halide perovskite solar cells: degradation and stability
journal, January 2016

Influence of Electrode Interfaces on the Stability of Perovskite Solar Cells: Reduced Degradation Using MoO _x /Al for Hole Collection
journal, April 2016

Formamidinium and Cesium Hybridization for Photo- and Moisture-Stable Perovskite Solar Cell
journal, September 2015

Outdoor Performance and Stability under Elevated Temperatures and Long-Term Light Soaking of Triple-Layer Mesoporous Perovskite Photovoltaics
journal, May 2015

The light and shade of perovskite solar cells
journal, August 2014

Lead-free organic–inorganic tin halide perovskites for photovoltaic applications
journal, January 2014

Highly efficient planar perovskite solar cells through band alignment engineering
journal, January 2015

Unravelling the Effects of Grain Boundary and Chemical Doping on Electron–Hole Recombination in CH ₃ NH ₃ PbI ₃ Perovskite by Time-Domain Atomistic Simulation
journal, March 2016

Lead-Free Halide Perovskite Solar Cells with High Photocurrents Realized Through Vacancy Modulation
journal, September 2014

Perovskite Photovoltaics: Rare Functions of Organo Lead Halide in Solar Cells and Optoelectronic Devices
journal, June 2015

Efficient charge extraction and slow recombination in organic–inorganic perovskites capped with semiconducting single-walled carbon nanotubes
journal, January 2016

Solar cell efficiency tables (version 47): Solar cell efficiency tables
journal, November 2015

Impact of microstructure on local carrier lifetime in perovskite solar cells
journal, April 2015

Toxicity of organometal halide perovskite solar cells
journal, February 2016

Lewis Acid–Base Adduct Approach for High Efficiency Perovskite Solar Cells
journal, January 2016

Some Thermodynamics of Photochemical Systems
journal, June 1967

A vacuum flash–assisted solution process for high-efficiency large-area perovskite solar cells
journal, June 2016

Efficient Hybrid Solar Cells Based on Meso-Superstructured Organometal Halide Perovskites
journal, October 2012

The perils of solar cell efficiency measurements
journal, May 2012

Perovskite photonic sources
journal, April 2016

Ion Migration and the Role of Preconditioning Cycles in the Stabilization of the J - V Characteristics of Inverted Hybrid Perovskite Solar Cells
journal, October 2015

Rain on Methylammonium Lead Iodide Based Perovskites: Possible Environmental Effects of Perovskite Solar Cells
journal, April 2015

Degradation Mechanisms of Solution-Processed Planar Perovskite Solar Cells: Thermally Stimulated Current Measurement for Analysis of Carrier Traps
journal, November 2015

Organic–inorganic hybrid lead halide perovskites for optoelectronic and electronic applications
journal, January 2016

Charge Transfer Dynamics between Carbon Nanotubes and Hybrid Organic Metal Halide Perovskite Films
journal, January 2016

How should you measure your excitonic solar cells?
journal, January 2012

Lead Iodide Perovskite Sensitized All-Solid-State Submicron Thin Film Mesoscopic Solar Cell with Efficiency Exceeding 9%
journal, August 2012

A Fast Deposition-Crystallization Procedure for Highly Efficient Lead Iodide Perovskite Thin-Film Solar Cells
journal, July 2014

Detection of X-ray photons by solution-processed lead halide perovskites
text, January 2015

Unique Seamlessly Bonded CNT@Graphene Hybrid Nanostructure Introduced in an Interlayer for Efficient and Stable Perovskite Solar Cells
journal, June 2018

Semimetallicity and Negative Differential Resistance from Hybrid Halide Perovskite Nanowires
journal, January 2019

Solution‐Processable Perovskite Solar Cells toward Commercialization: Progress and Challenges
journal, April 2019

A Review of Perovskites Solar Cell Stability
journal, February 2019

Humidity‐Tolerant Roll‐to‐Roll Fabrication of Perovskite Solar Cells via Polymer‐Additive‐Assisted Hot Slot Die Deposition
journal, March 2019

Tailoring the Functionality of Organic Spacer Cations for Efficient and Stable Quasi‐2D Perovskite Solar Cells
journal, April 2019

Wearable Large-Scale Perovskite Solar-Power Source via Nanocellular Scaffold
journal, September 2017

Organic-Inorganic Hybrid Halide Perovskites for Memories, Transistors, and Artificial Synapses
journal, May 2018

Cerium and Ytterbium Codoped Halide Perovskite Quantum Dots: A Novel and Efficient Downconverter for Improving the Performance of Silicon Solar Cells
journal, September 2017

In Situ Real-Time Study of the Dynamic Formation and Conversion Processes of Metal Halide Perovskite Films
journal, January 2018

Toward Perovskite Solar Cell Commercialization: A Perspective and Research Roadmap Based on Interfacial Engineering
journal, June 2018

Perovskite Nanoparticle Composite Films by Size Exclusion Lithography
journal, July 2018

Extending the Photovoltaic Response of Perovskite Solar Cells into the Near‐Infrared with a Narrow‐Bandgap Organic Semiconductor
journal, September 2019

A‐Site Management for Highly Crystalline Perovskites
journal, November 2019

Combining Efficiency and Stability in Mixed Tin–Lead Perovskite Solar Cells by Capping Grains with an Ultrathin 2D Layer
journal, March 2020

Transition from Positive to Negative Photoconductance in Doped Hybrid Perovskite Semiconductors
journal, August 2019

Recent Progress on the Long-Term Stability of Perovskite Solar Cells
journal, February 2018

Additional Organic‐Solvent‐Rinsing Process to Enhance Perovskite Photovoltaic Performance
journal, July 2019

Perovskite Tandem Solar Cells
journal, May 2017

Direct Evidence of Ion Diffusion for the Silver-Electrode-Induced Thermal Degradation of Inverted Perovskite Solar Cells
journal, March 2017

Understanding and Eliminating Hysteresis for Highly Efficient Planar Perovskite Solar Cells
journal, May 2017

Efficient and Hysteresis-Free Perovskite Solar Cells Based on a Solution Processable Polar Fullerene Electron Transport Layer
journal, August 2017

Low-Temperature Solution-Processed CuCrO ₂ Hole-Transporting Layer for Efficient and Photostable Perovskite Solar Cells
journal, January 2018

A New Perspective on the Role of A-Site Cations in Perovskite Solar Cells
journal, January 2018

Room-Temperature Vapor Deposition of Cobalt Nitride Nanofilms for Mesoscopic and Perovskite Solar Cells
journal, January 2018

Roll-to-Roll Slot Die Coated Perovskite for Efficient Flexible Solar Cells
journal, October 2018

Fusing Nanowires into Thin Films: Fabrication of Graded‐Heterojunction Perovskite Solar Cells with Enhanced Performance
journal, May 2019

Processing‐Performance Evolution of Perovskite Solar Cells: From Large Grain Polycrystalline Films to Single Crystals
journal, April 2020

Wide‐Bandgap Perovskite/Gallium Arsenide Tandem Solar Cells
journal, December 2019

Electron‐Beam‐Related Studies of Halide Perovskites: Challenges and Opportunities
journal, February 2020

Development of Dopant‐Free Organic Hole Transporting Materials for Perovskite Solar Cells
journal, April 2020

A Purified, Solvent‐Intercalated Precursor Complex for Wide‐Process‐Window Fabrication of Efficient Perovskite Solar Cells and Modules
journal, May 2019

A Scalable Methylamine Gas Healing Strategy for High‐Efficiency Inorganic Perovskite Solar Cells
journal, March 2019