Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe
Abstract
The coexistence and competition between superconductivity and electronic orders, such as spin or charge density waves, have been a central issue in high transition-temperature (Tc) superconductors. Unlike other iron-based superconductors, FeSe exhibits nematic ordering without magnetism whose relationship with its superconductivity remains unclear. Moreover, a pressure-induced fourfold increase of Tc has been reported, which poses a profound mystery. Here we report high-pressure magnetotransport measurements in FeSe up to ~15 GPa, which uncover the dome shape of magnetic phase superseding the nematic order. Above ~6 GPa the sudden enhancement of superconductivity (Tc ≤ 38.3 K) accompanies a suppression of magnetic order, demonstrating their competing nature with very similar energy scales. Above the magnetic dome, we find anomalous transport properties suggesting a possible pseudogap formation, whereas linear-in-temperature resistivity is observed in the normal states of the high-Tc phase above 6 GPa. In conclusion, the obtained phase diagram highlights unique features of FeSe among iron-based superconductors, but bears some resemblance to that of high-Tc cuprates.
- Authors:
-
[5];
[2]
- Chinese Academy of Sciences (CAS), Beijing (China)
- Univ. of Tokyo, Chiba (Japan)
- Chinese Academy of Sciences (CAS), Beijing (China); Yunnan Univ., Kunming (China)
- The Univ. of Electro-Communications, Tokyo (Japan)
- Kyoto Univ., Kyoto (Japan)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- The Univ. of Tokyo, Chiba (Japan)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1329162
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 7; Journal Issue: 12146; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; magnetic properties and materials; superconducting properties and materials
Citation Formats
Sun, J. P., Matsuura, K., Ye, G. Z., Mizukami, Y., Shimozawa, M., Matsubayashi, K., Yamashita, M., Watashige, T., Kasahara, S., Matsuda, Y., Yan, J. -Q., Sales, B. C., Uwatoko, Y., Cheng, J. -G., and Shibauchi, T. Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe. United States: N. p., 2016.
Web. doi:10.1038/ncomms12146.
Sun, J. P., Matsuura, K., Ye, G. Z., Mizukami, Y., Shimozawa, M., Matsubayashi, K., Yamashita, M., Watashige, T., Kasahara, S., Matsuda, Y., Yan, J. -Q., Sales, B. C., Uwatoko, Y., Cheng, J. -G., & Shibauchi, T. Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe. United States. https://doi.org/10.1038/ncomms12146
Sun, J. P., Matsuura, K., Ye, G. Z., Mizukami, Y., Shimozawa, M., Matsubayashi, K., Yamashita, M., Watashige, T., Kasahara, S., Matsuda, Y., Yan, J. -Q., Sales, B. C., Uwatoko, Y., Cheng, J. -G., and Shibauchi, T. Tue .
"Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe". United States. https://doi.org/10.1038/ncomms12146. https://www.osti.gov/servlets/purl/1329162.
@article{osti_1329162,
title = {Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe},
author = {Sun, J. P. and Matsuura, K. and Ye, G. Z. and Mizukami, Y. and Shimozawa, M. and Matsubayashi, K. and Yamashita, M. and Watashige, T. and Kasahara, S. and Matsuda, Y. and Yan, J. -Q. and Sales, B. C. and Uwatoko, Y. and Cheng, J. -G. and Shibauchi, T.},
abstractNote = {The coexistence and competition between superconductivity and electronic orders, such as spin or charge density waves, have been a central issue in high transition-temperature (Tc) superconductors. Unlike other iron-based superconductors, FeSe exhibits nematic ordering without magnetism whose relationship with its superconductivity remains unclear. Moreover, a pressure-induced fourfold increase of Tc has been reported, which poses a profound mystery. Here we report high-pressure magnetotransport measurements in FeSe up to ~15 GPa, which uncover the dome shape of magnetic phase superseding the nematic order. Above ~6 GPa the sudden enhancement of superconductivity (Tc ≤ 38.3 K) accompanies a suppression of magnetic order, demonstrating their competing nature with very similar energy scales. Above the magnetic dome, we find anomalous transport properties suggesting a possible pseudogap formation, whereas linear-in-temperature resistivity is observed in the normal states of the high-Tc phase above 6 GPa. In conclusion, the obtained phase diagram highlights unique features of FeSe among iron-based superconductors, but bears some resemblance to that of high-Tc cuprates.},
doi = {10.1038/ncomms12146},
journal = {Nature Communications},
number = 12146,
volume = 7,
place = {United States},
year = {Tue Jul 19 00:00:00 EDT 2016},
month = {Tue Jul 19 00:00:00 EDT 2016}
}
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Figures / Tables:
Figure 1: Temperature–pressure phase diagram of bulk FeSe. The structural (Ts, blue), magnetic (Tm, green), and superconducting transition temperatures (Tc, red and black) as a function of hydrostatic pressure in high-quality single crystals determined by anomalies in resistivity ρ(T)
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Pressure Induced Stripe-order Antiferromagnetism and First-order Phase Transition in FeSe
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- arXiv
Nematic quantum critical point without magnetism in FeSe1-xSx superconductors
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- arXiv
Observation of Ising spin-nematic order and its close relationship to the superconductivity in FeSe single crystals
text, January 2016
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- arXiv
Interplay of nematic and magnetic orders in FeSe under pressure
text, January 2016
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- arXiv
High-temperature superconductivity in one-unit-cell FeSe films
text, January 2017
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- arXiv
Dome of magnetic order inside the nematic phase of sulfur-substituted FeSe under pressure
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- arXiv
BCS-like critical fluctuations with limited overlap of Cooper pairs in FeSe
text, January 2017
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- arXiv
Suppression of electronic correlations by chemical pressure from FeSe to FeS
text, January 2017
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- arXiv
Flux growth in a horizontal configuration: an analogue to vapor transport growth
text, January 2017
- Yan, J. -Q.; Sales, B. C.; Susner, M. A.
- arXiv
Two distinct superconducting pairing states divided by the nematic end point in FeSe$_{1-x}$S$_{x}$
text, January 2017
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- arXiv
NMR evidence for static local nematicity and its cooperative interplay with low-energy magnetic fluctuations in FeSe under pressure
text, January 2017
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- arXiv
Unusual Effects of Be doping in the Iron Based Superconductor FeSe
text, January 2018
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- arXiv
Observation of orbital ordering and origin of the nematic order in FeSe
text, January 2018
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- arXiv
Theoretical study of impurity-induced magnetism in FeSe
text, January 2018
- Martiny, Johannes H. J.; Kreisel, Andreas; Andersen, Brian M.
- arXiv
Synergy and competition between superconductivity and antiferromagnetism in FeSe under pressure
text, January 2018
- Chen, Guan-Yu; Wang, Enyu; Zhu, Xiyu
- arXiv
Charge carrier dynamics of FeSe thin film investigated by terahertz magneto-optical spectroscopy
text, January 2019
- Yoshikawa, Naotaka; Takayama, Masayuki; Shikama, Naoki
- arXiv
Ionic-liquid-gating induced protonation and superconductivity in FeSe, FeSe0.93S0.07, ZrNCl, 1T-TaS2, and Bi2Se3
text, January 2019
- Cui, Y.; Hu, Z.; Zhang, J. S.
- arXiv
Orbital transmutation and the electronic spectrum of FeSe in the nematic phase
text, January 2019
- Christensen, Morten H.; Fernandes, Rafael M.; Chubukov, Andrey V.
- arXiv
Maximizing T c by tuning nematicity and magnetism in FeSe1−x S x superconductors
journal, October 2017
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- Nature Communications, Vol. 8, Issue 1
Reemergence of high-Tc superconductivity in the (Li1-xFe x )OHFe1-ySe under high pressure
journal, January 2018
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Tunable critical temperature for superconductivity in FeSe thin films by pulsed laser deposition
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Simple analytical model of the effect of high pressure on the critical temperature and other thermodynamic properties of superconductors
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Control of structural transition in FeSe1−xTex thin films by changing substrate materials
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Enhancement of Superconductivity Linked with Linear-in-Temperature/Field Resistivity in Ion-Gated FeSe Films
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- arXiv
Lattice-shifted nematic quantum critical point in $FeSe_{1−x}S_{x}$
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- Nature Research
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