Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces
Abstract
Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field confinement, enhancement, and scattering almost independently allows nonlinear frequency conversion efficiencies to be enhanced by many orders of magnitude compared to bulk materials. Also, the subwavelength length scale renders phase matching issues irrelevant. Compared with plasmonic nanostructures, dielectric resonator metamaterials show great promise for enhanced nonlinear optical processes due to their larger mode volumes. Here, we present, for the first time, resonantly enhanced second-harmonic generation (SHG) using gallium arsenide (GaAs) based dielectric metasurfaces. Using arrays of cylindrical resonators we observe SHG enhancement factors as large as 104 relative to unpatterned GaAs. At the magnetic dipole resonance, we measure an absolute nonlinear conversion efficiency of ~2 × 10–5 with ~3.4 GW/cm2 pump intensity. In conclusion, the polarization properties of the SHG reveal that both bulk and surface nonlinearities play important roles in the observed nonlinear process.
- Authors:
-
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Friedrich-Schiller-Univ. Jena, Jena (Germany)
- Publication Date:
- Research Org.:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1326369
- Report Number(s):
- SAND-2016-9155J
Journal ID: ISSN 1530-6984; 647439
- Grant/Contract Number:
- AC04-94AL85000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Letters
- Additional Journal Information:
- Journal Volume: 16; Journal Issue: 9; Journal ID: ISSN 1530-6984
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; dielectric metasurfaces; GaAs; III−V semiconductors; monolithic; resonantly enhanced; Second-harmonic generation
Citation Formats
Liu, Sheng, Sinclair, Michael B., Saravi, Sina, Keeler, Gordon A., Yang, Yuanmu, Reno, John, Peake, Gregory M., Setzpfandt, Frank, Staude, Isabelle, Pertsch, Thomas, and Brener, Igal. Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces. United States: N. p., 2016.
Web. doi:10.1021/acs.nanolett.6b01816.
Liu, Sheng, Sinclair, Michael B., Saravi, Sina, Keeler, Gordon A., Yang, Yuanmu, Reno, John, Peake, Gregory M., Setzpfandt, Frank, Staude, Isabelle, Pertsch, Thomas, & Brener, Igal. Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces. United States. https://doi.org/10.1021/acs.nanolett.6b01816
Liu, Sheng, Sinclair, Michael B., Saravi, Sina, Keeler, Gordon A., Yang, Yuanmu, Reno, John, Peake, Gregory M., Setzpfandt, Frank, Staude, Isabelle, Pertsch, Thomas, and Brener, Igal. Mon .
"Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces". United States. https://doi.org/10.1021/acs.nanolett.6b01816. https://www.osti.gov/servlets/purl/1326369.
@article{osti_1326369,
title = {Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces},
author = {Liu, Sheng and Sinclair, Michael B. and Saravi, Sina and Keeler, Gordon A. and Yang, Yuanmu and Reno, John and Peake, Gregory M. and Setzpfandt, Frank and Staude, Isabelle and Pertsch, Thomas and Brener, Igal},
abstractNote = {Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field confinement, enhancement, and scattering almost independently allows nonlinear frequency conversion efficiencies to be enhanced by many orders of magnitude compared to bulk materials. Also, the subwavelength length scale renders phase matching issues irrelevant. Compared with plasmonic nanostructures, dielectric resonator metamaterials show great promise for enhanced nonlinear optical processes due to their larger mode volumes. Here, we present, for the first time, resonantly enhanced second-harmonic generation (SHG) using gallium arsenide (GaAs) based dielectric metasurfaces. Using arrays of cylindrical resonators we observe SHG enhancement factors as large as 104 relative to unpatterned GaAs. At the magnetic dipole resonance, we measure an absolute nonlinear conversion efficiency of ~2 × 10–5 with ~3.4 GW/cm2 pump intensity. In conclusion, the polarization properties of the SHG reveal that both bulk and surface nonlinearities play important roles in the observed nonlinear process.},
doi = {10.1021/acs.nanolett.6b01816},
journal = {Nano Letters},
number = 9,
volume = 16,
place = {United States},
year = {Mon Aug 08 00:00:00 EDT 2016},
month = {Mon Aug 08 00:00:00 EDT 2016}
}
Web of Science
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conference, January 2018
- Arbabi, Ehsan; Arbabi, Amir; Kamali, Seyedeh Mahsa
- CLEO: Science and Innovations, Conference on Lasers and Electro-Optics
All-dielectric nanophotonics: the quest for better materials and fabrication techniques
preprint, January 2017
- Baranov, Denis G.; Zuev, Dmitry A.; Lepeshov, Sergey I.
- arXiv
Gradient metasurfaces: a review of fundamentals and applications
text, January 2017
- Ding, Fei; Pors, Anders; Bozhevolnyi, Sergey I.
- arXiv
Thermal tuning capabilities of semiconductor metasurface resonators
preprint, January 2018
- Lewi, Tomer; Butakov, Nikita A.; Schuller, Jon A.
- arXiv
Giant nonlinear response at the nanoscale driven by bound states in the continuum
text, January 2018
- Carletti, Luca; Koshelev, Kirill; De Angelis, Costantino
- arXiv
Reconfiguring structured light beams using nonlinear metasurfaces
text, January 2018
- Xu, Yun; Sun, Jingbo; Frantz, Jesse
- arXiv
All-dielectric metasurfaces with trapped modes: group-theoretical description
text, January 2018
- Yu, Pengchao; Kupriianov, Anton S.; Dmitriev, Victor
- arXiv
Coherent Control of the Non-instantaneous Nonlinear Power-law Response in Resonant Nanostructures
text, January 2019
- Bahar, Eyal; Arieli, Uri; Mrejen, Michael
- arXiv
Boosting third-harmonic generation by a mirror-enhanced anapole resonator
journal, July 2018
- Xu, Lei; Rahmani, Mohsen; Zangeneh Kamali, Khosro
- Light: Science & Applications, Vol. 7, Issue 1
Ultrafast all-optical tuning of direct-gap semiconductor metasurfaces
journal, May 2017
- Shcherbakov, Maxim R.; Liu, Sheng; Zubyuk, Varvara V.
- Nature Communications, Vol. 8, Issue 1
An all-dielectric metasurface as a broadband optical frequency mixer
journal, June 2018
- Liu, Sheng; Vabishchevich, Polina P.; Vaskin, Aleksandr
- Nature Communications, Vol. 9, Issue 1
Numerical Study on Mie Resonances in Single GaAs Nanomembranes
journal, June 2019
- Raya, Andrés M.; Fuster, David; Llorens, José M.
- Nanomaterials, Vol. 9, Issue 6