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Title: Low vibration high numerical aperture automated variable temperature Raman microscope

Abstract

Raman micro-spectroscopy is well suited for studying a variety of properties and has been applied to wide- ranging areas. Combined with tuneable temperature, Raman spectra can offer even more insights into the properties of materials. However, previous designs of variable temperature Raman microscopes have made it extremely challenging to measure samples with low signal levels due to thermal and positional instability as well as low collection efficiencies. Thus, contemporary Raman microscope has found limited applicability to probing the subtle physics involved in phase transitions and hysteresis. This paper describes a new design of a closed-cycle, Raman microscope with full polarization rotation. High collection efficiency, thermal and mechanical stability are ensured by both deliberate optical, cryogenic, and mechanical design. Measurements on two samples, Bi2Se3 and V2O3, which are known as challenging due to low thermal conductivities, low signal levels and/or hysteretic effects, are measured with previously undemonstrated temperature resolution.

Authors:
 [1];  [2];  [3];  [4];  [4];  [4];  [5];  [5];  [5];  [2];  [3]
  1. Univ. of Toronto, ON (Canada)
  2. Montana Instruments, Bozeman, MT (United States)
  3. Boston College, Chestnut Hill, MA (United States)
  4. Univ. of California, San Diego, CA (United States)
  5. Brookhaven National Lab. (BNL), Upton, NY (United States)
Publication Date:
Research Org.:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1303003
Alternate Identifier(s):
OSTI ID: 1245502
Report Number(s):
BNL-112459-2016-JA
Journal ID: ISSN 0034-6748; R&D Project: PO010; KC0201060
Grant/Contract Number:  
SC00112704
Resource Type:
Accepted Manuscript
Journal Name:
Review of Scientific Instruments
Additional Journal Information:
Journal Volume: 87; Journal Issue: 4; Journal ID: ISSN 0034-6748
Publisher:
American Institute of Physics (AIP)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Raman microscope; Cryo Optic; Low vibration; High NA

Citation Formats

Tian, Y., Reijnders, A. A., Osterhoudt, G. B., Valmianski, I., Ramirez, J. G., Urban, C., Zhong, R., Schneeloch, J., Gu, G., Henslee, I., and Burch, K. S. Low vibration high numerical aperture automated variable temperature Raman microscope. United States: N. p., 2016. Web. doi:10.1063/1.4944559.
Tian, Y., Reijnders, A. A., Osterhoudt, G. B., Valmianski, I., Ramirez, J. G., Urban, C., Zhong, R., Schneeloch, J., Gu, G., Henslee, I., & Burch, K. S. Low vibration high numerical aperture automated variable temperature Raman microscope. United States. doi:10.1063/1.4944559.
Tian, Y., Reijnders, A. A., Osterhoudt, G. B., Valmianski, I., Ramirez, J. G., Urban, C., Zhong, R., Schneeloch, J., Gu, G., Henslee, I., and Burch, K. S. Tue . "Low vibration high numerical aperture automated variable temperature Raman microscope". United States. doi:10.1063/1.4944559. https://www.osti.gov/servlets/purl/1303003.
@article{osti_1303003,
title = {Low vibration high numerical aperture automated variable temperature Raman microscope},
author = {Tian, Y. and Reijnders, A. A. and Osterhoudt, G. B. and Valmianski, I. and Ramirez, J. G. and Urban, C. and Zhong, R. and Schneeloch, J. and Gu, G. and Henslee, I. and Burch, K. S.},
abstractNote = {Raman micro-spectroscopy is well suited for studying a variety of properties and has been applied to wide- ranging areas. Combined with tuneable temperature, Raman spectra can offer even more insights into the properties of materials. However, previous designs of variable temperature Raman microscopes have made it extremely challenging to measure samples with low signal levels due to thermal and positional instability as well as low collection efficiencies. Thus, contemporary Raman microscope has found limited applicability to probing the subtle physics involved in phase transitions and hysteresis. This paper describes a new design of a closed-cycle, Raman microscope with full polarization rotation. High collection efficiency, thermal and mechanical stability are ensured by both deliberate optical, cryogenic, and mechanical design. Measurements on two samples, Bi2Se3 and V2O3, which are known as challenging due to low thermal conductivities, low signal levels and/or hysteretic effects, are measured with previously undemonstrated temperature resolution.},
doi = {10.1063/1.4944559},
journal = {Review of Scientific Instruments},
number = 4,
volume = 87,
place = {United States},
year = {2016},
month = {4}
}

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    Works referencing / citing this record:

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