Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2

Gardner, D. R.; Bonnoit, C. J.; Chisnell, R.; Said, A. H.; Leu, B. M.; Williams, Travis J.; Luke, G. M.; Lee, Y. S.

doi:10.1103/PhysRevB.93.075123

Title: Inelastic x-ray scattering measurements of phonon dynamics in URu₂Si₂

Abstract

In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu₂Si₂. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the low temperature phase.

Authors:

Gardner, D. R. ^[1]; Bonnoit, C. J. ^[1]; Chisnell, R. ^[1]; Said, A. H. ^[2]; Leu, B. M. ^[2]; Williams, Travis J. ^[3]; Luke, G. M. ^[4]; Lee, Y. S. ^[1]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
McMaster Univ., Hamilton, ON (Canada); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
McMaster Univ., Hamilton, ON (Canada)

Publication Date:: Thu Feb 11 00:00:00 EST 2016

Research Org.:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1302920

Alternate Identifier(s):: OSTI ID: 1237785

Grant/Contract Number:: AC05-00OR22725; FG02-07ER46134; AC02-06CH11357

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 93; Journal Issue: 7; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Gardner, D. R., Bonnoit, C. J., Chisnell, R., Said, A. H., Leu, B. M., Williams, Travis J., Luke, G. M., and Lee, Y. S. Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2.  United States: N. p., 2016. 
Web.  doi:10.1103/PhysRevB.93.075123.

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                    Gardner, D. R., Bonnoit, C. J., Chisnell, R., Said, A. H., Leu, B. M., Williams, Travis J., Luke, G. M., & Lee, Y. S. Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2.  United States.  https://doi.org/10.1103/PhysRevB.93.075123

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                    Gardner, D. R., Bonnoit, C. J., Chisnell, R., Said, A. H., Leu, B. M., Williams, Travis J., Luke, G. M., and Lee, Y. S. Thu .  
"Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2".  United States.  https://doi.org/10.1103/PhysRevB.93.075123.  https://www.osti.gov/servlets/purl/1302920.

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@article{osti_1302920,

  title        = {Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2},

  author       = {Gardner, D. R. and Bonnoit, C. J. and Chisnell, R. and Said, A. H. and Leu, B. M. and Williams, Travis J. and Luke, G. M. and Lee, Y. S.},

  abstractNote = {In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu2Si2. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the low temperature phase.},

  doi          = {10.1103/PhysRevB.93.075123},

  journal      = {Physical Review B},

  number       = 7,

  volume       = 93,

  place        = {United States},

  year         = {Thu Feb 11 00:00:00 EST 2016},

  month        = {Thu Feb 11 00:00:00 EST 2016}

}

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Works referenced in this record:

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Works referencing / citing this record:

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
journal, January 2020

Mydosh, J. A.; Oppeneer, P. M.; Riseborough, P. S.
Journal of Physics: Condensed Matter, Vol. 32, Issue 14
DOI: 10.1088/1361-648x/ab5eba

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Title: Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2

Abstract

Citation Formats

Superconducting and Magnetic Transitions in the Heavy-Fermion System U Ru 2 Si 2 journal, December 1985

Partially gapped Fermi surface in the heavy-electron superconductor URu 2 Si 2 journal, January 1986

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of URu 2 Si 2 journal, November 2011

Hidden order behaviour in URu 2 Si 2 (A critical review of the status of hidden order in 2014) journal, May 2014

Hastatic order in the heavy-fermion compound URu2Si2 journal, January 2013

Modulated Spin Liquid: A New Paradigm for URu 2 Si 2 journal, March 2011

Helicity Order: Hidden Order Parameter in URu 2 Si 2 journal, January 2006

Interplay between spin-density wave and induced local moments in URu 2 Si 2 journal, July 2005

Hybridization Wave as the “Hidden Order” in URu 2 Si 2 journal, February 2011

Chirality density wave of the "hidden order" phase in URu2Si2 journal, February 2015

Emergent rank-5 nematic order in URu2Si2 journal, June 2012

Multipole order and global/site symmetry in the hidden-order phase of URu 2 Si 2 journal, November 2014

Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking journal, February 2009

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of URu 2 Si 2 journal, November 2010

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2 journal, January 2011

Cyclotron resonance study of quasiparticle mass and scattering rate in the hidden-order and superconducting phases of URu 2 Si 2 journal, December 2013

Cyclotron Resonance in the Hidden-Order Phase of URu 2 Si 2 journal, July 2012

NMR Study of In-Plane Twofold Ordering in URu 2 Si 2 journal, June 2013

Thermal expansion and specific heat of monocrystalline U Ru 2 Si 2 journal, December 1986

Thermal Transport in the Hidden-Order State of URu 2 Si 2 journal, April 2005

Phonon Thermal Transport of URu 2 Si 2 : Broken Translational Symmetry and Strong-Coupling of the “Hidden Order” to the Lattice journal, October 2006

Γ 3 -Type Lattice Instability and the Hidden Order of URu 2 Si 2 journal, January 2013

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 journal, June 2014

X-ray backscattering study of crystal lattice distortion in hidden order of URu 2 Si 2 journal, September 2014

Magnetic excitations in the heavy-fermion superconductor URu 2 Si 2 journal, June 1991

Search for hidden orbital currents and observation of an activated ring of magnetic scattering in the heavy fermion superconductor URu 2 Si 2 journal, April 2004

Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2 journal, January 2007

Itinerant spin excitations near the hidden order transition in URu 2 Si 2 journal, April 2009

Neutron scattering study of URu 2 − x Re x Si 2 ( x = 0.10 ): Driving order towards quantum criticality journal, December 2012

Neutron scattering studies on URu 2 Si 2 journal, July 2014

Symmetry and correlations underlying hidden order in URu 2 Si 2 journal, January 2015

Lattice dynamics of the heavy-fermion compound URu 2 Si 2 journal, January 2015

A Study of Elastic Properties of URu 2 Si 2 in Comparison with the Non-5 f Contribution of ThRu 2 Si 2 journal, December 2012

Elastic properties of the heavy fermion superconductor URu2Si2 journal, February 1994

Scattering of Neutrons by an Anharmonic Crystal journal, December 1962

Phonon Lifetime Investigation of Anharmonicity and Thermal Conductivity of UO 2 by Neutron Scattering and Theory journal, April 2013

Observation of the Thermal Conductivity due to Spins in the One-Dimensional Antiferromagnetic Ising-Like Spin System A Co X 3 ( A = Rb, Cs; X = Cl, Br) journal, June 2014

Magnetic heat transport in R 2 Cu O 4 ( R = La , Pr, Nd, Sm, Eu, and Gd) journal, March 2006

Magnetic phase transitions and magnetoelectric coupling of GdFe O 3 single crystals probed by low-temperature heat transport journal, January 2011

Thermal Conductivity of Ho 2 Ti 2 O 7 along the [111] Direction journal, May 2013

Evidence for a large magnetic heat current in insulating layered cuprates journal, May 2003

Imaging the Three-Dimensional Fermi-Surface Pairing near the Hidden-Order Transition in URu 2 Si 2 Using Angle-Resolved Photoemission Spectroscopy journal, September 2013

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu 2 Si 2 journal, January 2020

Title: Inelastic x-ray scattering measurements of phonon dynamics in URu₂Si₂

Superconducting and Magnetic Transitions in the Heavy-Fermion System U ${Ru}_{2}$ ${Si}_{2}$
journal, December 1985

Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$
journal, January 1986

Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$
journal, November 2011

Hidden order behaviour in URu ₂ Si ₂ (A critical review of the status of hidden order in 2014)
journal, May 2014

Hastatic order in the heavy-fermion compound URu2Si2
journal, January 2013

Modulated Spin Liquid: A New Paradigm for ${URu}_{2} {Si}_{2}$
journal, March 2011

Helicity Order: Hidden Order Parameter in ${URu}_{2} {Si}_{2}$
journal, January 2006

Interplay between spin-density wave and induced local moments in ${URu}_{2} {Si}_{2}$
journal, July 2005

Hybridization Wave as the “Hidden Order” in ${URu}_{2} {Si}_{2}$
journal, February 2011

Chirality density wave of the "hidden order" phase in URu2Si2
journal, February 2015

Emergent rank-5 nematic order in URu2Si2
journal, June 2012

Multipole order and global/site symmetry in the hidden-order phase of ${URu}_{2} {Si}_{2}$
journal, November 2014

Hidden order in URu2Si2 originates from Fermi surface gapping induced by dynamic symmetry breaking
journal, February 2009

Similarity of the Fermi Surface in the Hidden Order State and in the Antiferromagnetic State of ${URu}_{2} {Si}_{2}$
journal, November 2010

Rotational Symmetry Breaking in the Hidden-Order Phase of URu2Si2
journal, January 2011

Cyclotron resonance study of quasiparticle mass and scattering rate in the hidden-order and superconducting phases of ${URu}_{2}$ Si $_{2}$
journal, December 2013

Cyclotron Resonance in the Hidden-Order Phase of ${URu}_{2} {Si}_{2}$
journal, July 2012

NMR Study of In-Plane Twofold Ordering in ${URu}_{2} {Si}_{2}$
journal, June 2013

Thermal expansion and specific heat of monocrystalline U ${Ru}_{2}$ ${Si}_{2}$
journal, December 1986

Thermal Transport in the Hidden-Order State of ${URu}_{2} {Si}_{2}$
journal, April 2005

Phonon Thermal Transport of ${URu}_{2} {Si}_{2}$ : Broken Translational Symmetry and Strong-Coupling of the “Hidden Order” to the Lattice
journal, October 2006

Γ ₃ -Type Lattice Instability and the Hidden Order of URu ₂ Si ₂
journal, January 2013

Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2
journal, June 2014

X-ray backscattering study of crystal lattice distortion in hidden order of URu ₂ Si ₂
journal, September 2014

Magnetic excitations in the heavy-fermion superconductor ${URu}_{2}$ ${Si}_{2}$
journal, June 1991

Search for hidden orbital currents and observation of an activated ring of magnetic scattering in the heavy fermion superconductor ${URu}_{2} {Si}_{2}$
journal, April 2004

Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2
journal, January 2007

Itinerant spin excitations near the hidden order transition in URu ₂ Si ₂
journal, April 2009

Neutron scattering study of URu $_{2 - x}$ Re $_{x}$ Si $_{2}$ ( $x = 0.10$ ): Driving order towards quantum criticality
journal, December 2012

Neutron scattering studies on URu ₂ Si ₂
journal, July 2014

Symmetry and correlations underlying hidden order in ${URu}_{2} {Si}_{2}$
journal, January 2015

Lattice dynamics of the heavy-fermion compound ${URu}_{2} {Si}_{2}$
journal, January 2015

A Study of Elastic Properties of URu ₂ Si ₂ in Comparison with the Non-5 f Contribution of ThRu ₂ Si ₂
journal, December 2012

Elastic properties of the heavy fermion superconductor URu2Si2
journal, February 1994

Scattering of Neutrons by an Anharmonic Crystal
journal, December 1962

Phonon Lifetime Investigation of Anharmonicity and Thermal Conductivity of ${UO}_{2}$ by Neutron Scattering and Theory
journal, April 2013

Observation of the Thermal Conductivity due to Spins in the One-Dimensional Antiferromagnetic Ising-Like Spin System A Co X ₃ ( A = Rb, Cs; X = Cl, Br)
journal, June 2014

Magnetic heat transport in $R_{2} Cu O_{4}$ ( $R = La$ , Pr, Nd, Sm, Eu, and Gd)
journal, March 2006

Magnetic phase transitions and magnetoelectric coupling of GdFe $O_{3}$ single crystals probed by low-temperature heat transport
journal, January 2011

Thermal Conductivity of ${Ho}_{2} {Ti}_{2} O_{7}$ along the [111] Direction
journal, May 2013

Evidence for a large magnetic heat current in insulating layered cuprates
journal, May 2003

Imaging the Three-Dimensional Fermi-Surface Pairing near the Hidden-Order Transition in ${URu}_{2} {Si}_{2}$ Using Angle-Resolved Photoemission Spectroscopy
journal, September 2013

Hidden order and beyond: an experimental—theoretical overview of the multifaceted behavior of URu ₂ Si ₂
journal, January 2020