Negative pressures and spallation in water drops subjected to nanosecond shock waves

Stan, Claudiu A.; Willmott, Philip R.; Stone, Howard A.; Koglin, Jason E.; Liang, Mengning; Aquila, Andrew L.; Robinson, Joseph S.; Gumerlock, Karl L.; Blaj, Gabriel; Sierra, Raymond G.; Boutet, Sebastien; Guillet, Serge A. H.; Curtis, Robin H.; Vetter, Sharon L.; Loos, Henrik; Turner, James L.; Decker, Franz -Josef

doi:10.1021/acs.jpclett.6b00687

Title: Negative pressures and spallation in water drops subjected to nanosecond shock waves

Journal Article · 16 May 2016 · Journal of Physical Chemistry Letters

DOI: https://doi.org/10.1021/acs.jpclett.6b00687 · OSTI ID:1295510

Stan, Claudiu A. ^[1]; Willmott, Philip R. ^[2]; Stone, Howard A. ^[3]; Koglin, Jason E. ^[1]; Liang, Mengning ^[1]; Aquila, Andrew L. ^[1]; Robinson, Joseph S. ^[1]; Gumerlock, Karl L. ^[1]; Blaj, Gabriel ^[1]; Sierra, Raymond G. ^[1]; Boutet, Sebastien ^[1]; Guillet, Serge A. H. ^[1]; Curtis, Robin H. ^[1]; Vetter, Sharon L. ^[1]; Loos, Henrik ^[1]; Turner, James L. ^[1]; Decker, Franz -Josef ^[1]

SLAC National Accelerator Lab., Menlo Park, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Paul Scherrer Institute, Villigen (Switzerland)
Princeton Univ., Princeton, NJ (United States)

Most experimental studies of cavitation in liquid water at negative pressures reported cavitation at tensions significantly smaller than those expected for homogeneous nucleation, suggesting that achievable tensions are limited by heterogeneous cavitation. We generated tension pulses with nanosecond rise times in water by reflecting cylindrical shock waves, produced by X-ray laser pulses, at the internal surface of drops of water. Depending on the X-ray pulse energy, a range of cavitation phenomena occurred, including the rupture and detachment, or spallation, of thin liquid layers at the surface of the drop. When spallation occurred, we evaluated that negative pressures below –100 MPa were reached in the drops. As a result, we model the negative pressures from shock reflection experiments using a nucleation-and-growth model that explains how rapid decompression could outrun heterogeneous cavitation in water, and enable the study of stretched water close to homogeneous cavitation pressures.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1295510

Report Number(s):: SLAC-PUB--16782

Journal Information:: Journal of Physical Chemistry Letters, Journal Name: Journal of Physical Chemistry Letters Journal Issue: 11 Vol. 7; ISSN 1948-7185

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEAR CHEMISTRY
X-ray lasers
cavitation
dynamic decompression
heterogeneous nucleation
stretched water

Title: Negative pressures and spallation in water drops subjected to nanosecond shock waves

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