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Title: Solid-state electrochemistry on the nanometer and atomic scales: the scanning probe microscopy approach

Energy technologies of the 21st century require an understanding and precise control over ion transport and electrochemistry at all length scales – from single atoms to macroscopic devices. Our short review provides a summary of recent studies dedicated to methods of advanced scanning probe microscopy for probing electrochemical transformations in solids at the meso-, nano- and atomic scales. In this discussion we present the advantages and limitations of several techniques and a wealth of examples highlighting peculiarities of nanoscale electrochemistry.
Authors:
 [1] ;  [2] ;  [2] ;  [2] ;  [2] ;  [2]
  1. National Inst. of Standards and Technology, Gaithersburg, MD (United States); Univ. of Maryland, College Park, MD (United States)
  2. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Publication Date:
Grant/Contract Number:
AC05-00OR22725
Type:
Accepted Manuscript
Journal Name:
Nanoscale
Additional Journal Information:
Journal Volume: 8; Journal Issue: 29; Journal ID: ISSN 2040-3364
Publisher:
Royal Society of Chemistry
Research Org:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)
Sponsoring Org:
USDOE Office of Science (SC)
Country of Publication:
United States
Language:
English
Subject:
77 NANOSCIENCE AND NANOTECHNOLOGY
OSTI Identifier:
1286973

Strelcov, Evgheni, Yang, Sang Mo, Jesse, Stephen, Balke, Nina, Vasudevan, Rama K., and Kalinin, Sergei V.. Solid-state electrochemistry on the nanometer and atomic scales: the scanning probe microscopy approach. United States: N. p., Web. doi:10.1039/C6NR01524G.
Strelcov, Evgheni, Yang, Sang Mo, Jesse, Stephen, Balke, Nina, Vasudevan, Rama K., & Kalinin, Sergei V.. Solid-state electrochemistry on the nanometer and atomic scales: the scanning probe microscopy approach. United States. doi:10.1039/C6NR01524G.
Strelcov, Evgheni, Yang, Sang Mo, Jesse, Stephen, Balke, Nina, Vasudevan, Rama K., and Kalinin, Sergei V.. 2016. "Solid-state electrochemistry on the nanometer and atomic scales: the scanning probe microscopy approach". United States. doi:10.1039/C6NR01524G. https://www.osti.gov/servlets/purl/1286973.
@article{osti_1286973,
title = {Solid-state electrochemistry on the nanometer and atomic scales: the scanning probe microscopy approach},
author = {Strelcov, Evgheni and Yang, Sang Mo and Jesse, Stephen and Balke, Nina and Vasudevan, Rama K. and Kalinin, Sergei V.},
abstractNote = {Energy technologies of the 21st century require an understanding and precise control over ion transport and electrochemistry at all length scales – from single atoms to macroscopic devices. Our short review provides a summary of recent studies dedicated to methods of advanced scanning probe microscopy for probing electrochemical transformations in solids at the meso-, nano- and atomic scales. In this discussion we present the advantages and limitations of several techniques and a wealth of examples highlighting peculiarities of nanoscale electrochemistry.},
doi = {10.1039/C6NR01524G},
journal = {Nanoscale},
number = 29,
volume = 8,
place = {United States},
year = {2016},
month = {4}
}