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Title: Effect of higher-order multipole moments on the Stark line shape

Abstract

Spectral line shapes are sensitive to plasma conditions and are often used to diagnose electron density of laboratory plasmas as well as astrophysical plasmas. Stark line-shape models take into account the perturbation of the radiator’s energy structure due to the Coulomb interaction with the surrounding charged particles. Solving this Coulomb interaction is challenging and is commonly approximated via a multipole expansion. Yet, most models include only up to the second term of the expansion (the dipole term). While there have been studies on the higher-order terms due to one of the species (i.e. either ions or electrons), there is no model that includes the terms beyond dipole from both species. Here, we investigate the importance of the higher-order multipole terms from both species on the Hβ line shape. First, we find that it is important to include higher order terms consistently from both ions and electrons to reproduce measured line-shape asymmetry. Next, we study the line shape convergence with the higher-order terms at 1017, 1018, and 1019 e/cc. We discover that the line shape calculated with the dipole-only approximation becomes inaccurate as density increases. It is necessary to include only up to the third (quadrupole) term to compute the line-shapemore » accurately within 2%. Since most existing models include only the dipole terms, the densities inferred with such models are in question. Finally, we investigate the impact of neglecting the quadrupole terms on density diagnostics. We find that the model without the quadrupole term slightly underestimates the density, and the discrepancy becomes as large as 12% at high densities. Although the case of study is limited to Hβ , we expect similar impact on other lines.« less

Authors:
 [1];  [2];  [3];  [1];  [1]
  1. Univ. of Texas, Austin, TX (United States)
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  3. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Publication Date:
Research Org.:
Univ. of Texas, Austin, TX (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Fusion Energy Sciences (FES)
OSTI Identifier:
1511676
Alternate Identifier(s):
OSTI ID: 1280206
Grant/Contract Number:  
NA0003843; SC0010623
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review A
Additional Journal Information:
Journal Volume: 94; Journal Issue: 2; Journal ID: ISSN 2469-9926
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
74 ATOMIC AND MOLECULAR PHYSICS

Citation Formats

Gomez, T. A., Nagayama, T., Kilcrease, D. P., Montgomery, M. H., and Winget, D. E. Effect of higher-order multipole moments on the Stark line shape. United States: N. p., 2016. Web. doi:10.1103/PhysRevA.94.022501.
Gomez, T. A., Nagayama, T., Kilcrease, D. P., Montgomery, M. H., & Winget, D. E. Effect of higher-order multipole moments on the Stark line shape. United States. https://doi.org/10.1103/PhysRevA.94.022501
Gomez, T. A., Nagayama, T., Kilcrease, D. P., Montgomery, M. H., and Winget, D. E. Tue . "Effect of higher-order multipole moments on the Stark line shape". United States. https://doi.org/10.1103/PhysRevA.94.022501. https://www.osti.gov/servlets/purl/1511676.
@article{osti_1511676,
title = {Effect of higher-order multipole moments on the Stark line shape},
author = {Gomez, T. A. and Nagayama, T. and Kilcrease, D. P. and Montgomery, M. H. and Winget, D. E.},
abstractNote = {Spectral line shapes are sensitive to plasma conditions and are often used to diagnose electron density of laboratory plasmas as well as astrophysical plasmas. Stark line-shape models take into account the perturbation of the radiator’s energy structure due to the Coulomb interaction with the surrounding charged particles. Solving this Coulomb interaction is challenging and is commonly approximated via a multipole expansion. Yet, most models include only up to the second term of the expansion (the dipole term). While there have been studies on the higher-order terms due to one of the species (i.e. either ions or electrons), there is no model that includes the terms beyond dipole from both species. Here, we investigate the importance of the higher-order multipole terms from both species on the Hβ line shape. First, we find that it is important to include higher order terms consistently from both ions and electrons to reproduce measured line-shape asymmetry. Next, we study the line shape convergence with the higher-order terms at 1017, 1018, and 1019 e/cc. We discover that the line shape calculated with the dipole-only approximation becomes inaccurate as density increases. It is necessary to include only up to the third (quadrupole) term to compute the line-shape accurately within 2%. Since most existing models include only the dipole terms, the densities inferred with such models are in question. Finally, we investigate the impact of neglecting the quadrupole terms on density diagnostics. We find that the model without the quadrupole term slightly underestimates the density, and the discrepancy becomes as large as 12% at high densities. Although the case of study is limited to Hβ , we expect similar impact on other lines.},
doi = {10.1103/PhysRevA.94.022501},
journal = {Physical Review A},
number = 2,
volume = 94,
place = {United States},
year = {Tue Aug 02 00:00:00 EDT 2016},
month = {Tue Aug 02 00:00:00 EDT 2016}
}

Journal Article:

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Cited by: 24 works
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Figures / Tables:

FIG. 1 FIG. 1: The double-peaked Hβ line shape. The asymmetry of the core is defined as the normalized difference of the intensity of the blue peak and red peak, (IbIr)/Ib, where the subscripts b and r denote the blue (∆E > 0) and red peak (∆E < 0), respectively.

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Works referencing / citing this record:

Study of Stark broadening of Li i 460 and 497 nm spectral lines with independent plasma diagnostics by Thomson scattering
journal, February 2018

  • Dzierżȩga, Krzysztof; Piȩta, Tomasz; Zawadzki, Witold
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ZEST: A Fast Code for Simulating Zeeman-Stark Line-Shape Functions
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Matrix Methods for Solving Hartree-Fock Equations in Atomic Structure Calculations and Line Broadening
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Laboratory Hydrogen-Beta Emission Spectroscopy for Analysis of Astrophysical White Dwarf Spectra
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Electron Broadening Operator Including Penetrating Collisions for Hydrogen
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H β and H γ Absorption-line Profile Inconsistencies in Laboratory Experiments Performed at White Dwarf Photosphere Conditions
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Electron broadening operator including penetrating collisions for hydrogen
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