Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2

Huang, Lunan; McCormick, Timothy M.; Ochi, Masayuki; Zhao, Zhiying; Suzuki, Michi -To; Arita, Ryotaro; Wu, Yun; Mou, Daixiang; Cao, Huibo; Yan, Jiaqiang; Trivedi, Nandini; Kaminski, Adam

doi:10.1038/nmat4685

Title: Spectroscopic evidence for a type II Weyl semimetallic state in MoTe₂

Journal Article · 10 July 2016 · Nature Materials

DOI: https://doi.org/10.1038/nmat4685 · OSTI ID:1278751

Huang, Lunan ^[1]; McCormick, Timothy M. ^[2]; Ochi, Masayuki ^[3]; Zhao, Zhiying ^[4]; Suzuki, Michi -To ^[5]; Arita, Ryotaro ^[6]; Wu, Yun ^[1];

^[1]; Cao, Huibo ^[7]; Yan, Jiaqiang ^[8]; Trivedi, Nandini ^[2]; Kaminski, Adam ^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)
The Ohio State Univ., Columbus, OH (United States)
Osaka Univ., Osaka (Japan)
Univ. of Tennessee, Knoxville, TN (United States)
RIKEN Center for Emergent Matter Science (CEMS), Saitama (Japan)
RIKEN Center for Emergent Matter Science (CEMS), Saitama (Japan); Tohoku Univ., Miyagi (Japan)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

In a type I Dirac or Weyl semimetal, the low-energy states are squeezed to a single point in momentum space when the chemical potential μ is tuned precisely to the Dirac/Weyl point. Recently, a type II Weyl semimetal was predicted to exist, where the Weyl states connect hole and electron bands, separated by an indirect gap. This leads to unusual energy states, where hole and electron pockets touch at the Weyl point. Here we present the discovery of a type II topological Weyl semimetal state in pure MoTe₂, where two sets of Weyl points (W^±₂ , W^±₃) exist at the touching points of electron and hole pockets and are located at different binding energies above E_F. Using angle-resolved photoemission spectroscopy, modelling, density functional theory and calculations of Berry curvature, we identify the Weyl points and demonstrate that they are connected by different sets of Fermi arcs for each of the two surface terminations. We also find new surface ‘track states’ that form closed loops and are unique to type II Weyl semimetals. Lastly, this material provides an exciting, new platform to study the properties of Weyl fermions.

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Research Organization:: Ames Lab. and Iowa State Univ., Ames, IA (United States); Ames Laboratory (AMES), Ames, IA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); RIKEN Center for Emergent Matter Science (CEMS), Wako (Japan); The Ohio State Univ., Columbus, OH (United States)

Sponsoring Organization:: National Science Foundation (NSF) (United States); Simons Foundation (United States); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Contributing Organization:: Osaka Univ. (Japan); Tohoku Univ., Sendai (Japan); Univ. of Tennessee, Knoxville, TN (United States)

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1278751

Report Number(s):: IS-J--9004; nmat4685

Journal Information:: Nature Materials, Journal Name: Nature Materials Journal Issue: 11 Vol. 15; ISSN 1476-1122

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Quantum oscillations and nontrivial topological state in a compensated semimetal TaP 2 Wang, Hongyuan; Su, Hao; Zhang, Jiuyang Physical Review B, Vol. 100, Issue 11 https://doi.org/10.1103/physrevb.100.115127	journal	September 2019
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Observation of large topologically trivial Fermi arcs in the candidate type-II Weyl semimetal WT e 2 Bruno, F. Y.; Tamai, A.; Wu, Q. S. Physical Review B, Vol. 94, Issue 12 https://doi.org/10.1103/physrevb.94.121112	journal	September 2016
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Experimental evidence for type-II Dirac semimetal in PtSe 2 Zhang, Kenan; Yan, Mingzhe; Zhang, Haoxiong Physical Review B, Vol. 96, Issue 12 https://doi.org/10.1103/physrevb.96.125102	journal	September 2017
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Double Andreev reflections in type-II Weyl semimetal-superconductor junctions Hou, Zhe; Sun, Qing-Feng Physical Review B, Vol. 96, Issue 15 https://doi.org/10.1103/physrevb.96.155305	journal	October 2017
Quasiparticle interference of surface states in the type-II Weyl semimetal WTe 2 Zhang, Wenhan; Wu, Quansheng; Zhang, Lunyong Physical Review B, Vol. 96, Issue 16 https://doi.org/10.1103/physrevb.96.165125	journal	October 2017
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Semiclassical theory of anomalous transport in type-II topological Weyl semimetals McCormick, Timothy M.; McKay, Robert C.; Trivedi, Nandini Physical Review B, Vol. 96, Issue 23 https://doi.org/10.1103/physrevb.96.235116	journal	December 2017
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Correlated triple-Weyl semimetals with Coulomb interactions Zhang, Shi-Xin; Jian, Shao-Kai; Yao, Hong Physical Review B, Vol. 96, Issue 24 https://doi.org/10.1103/physrevb.96.241111	journal	December 2017
Enhanced ultrafast relaxation rate in the Weyl semimetal phase of MoTe 2 measured by time- and angle-resolved photoelectron spectroscopy Crepaldi, A.; Autès, G.; Gatti, G. Physical Review B, Vol. 96, Issue 24 https://doi.org/10.1103/physrevb.96.241408	journal	December 2017
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Berry curvature dipole in Weyl semimetal materials: An ab initio study Zhang, Yang; Sun, Yan; Yan, Binghai Physical Review B, Vol. 97, Issue 4 https://doi.org/10.1103/physrevb.97.041101	journal	January 2018
Dimensionality-driven orthorhombic MoT e 2 at room temperature He, Rui; Zhong, Shazhou; Kim, Hyun Ho Physical Review B, Vol. 97, Issue 4 https://doi.org/10.1103/physrevb.97.041410	journal	January 2018
Doping and tilting on optics in noncentrosymmetric multi-Weyl semimetals Mukherjee, S. P.; Carbotte, J. P. Physical Review B, Vol. 97, Issue 4 https://doi.org/10.1103/physrevb.97.045150	journal	January 2018
Heat capacity evidence for conventional superconductivity in the type-II Dirac semimetal PdTe 2 Physical Review B, Vol. 97, Issue 5 https://doi.org/10.1103/physrevb.97.054515	journal	February 2018
Universal scattering response across the type-II Weyl semimetal phase diagram Rüßmann, P.; Weber, A. P.; Glott, F. Physical Review B, Vol. 97, Issue 7 https://doi.org/10.1103/physrevb.97.075106	journal	February 2018
Saddle-like topological surface states on the T T ′ X family of compounds ( T , T ′ = Transition metal, X = Si , Ge) Singh, Bahadur; Zhou, Xiaoting; Lin, Hsin Physical Review B, Vol. 97, Issue 7 https://doi.org/10.1103/physrevb.97.075125	journal	February 2018
Dynamics of out-of-equilibrium electron and hole pockets in the type-II Weyl semimetal candidate WTe 2 Caputo, M.; Khalil, L.; Papalazarou, E. Physical Review B, Vol. 97, Issue 11 https://doi.org/10.1103/physrevb.97.115115	journal	March 2018
Magnetic properties of type-I and type-II Weyl semimetals in the superconducting state Rosenstein, Baruch; Shapiro, B. Ya.; Li, Dingping Physical Review B, Vol. 97, Issue 14 https://doi.org/10.1103/physrevb.97.144510	journal	April 2018
Floquet Weyl semimetals in light-irradiated type-II and hybrid line-node semimetals Chen, Rui; Zhou, Bin; Xu, Dong-Hui Physical Review B, Vol. 97, Issue 15 https://doi.org/10.1103/physrevb.97.155152	journal	April 2018
Topological surface Fermi arcs in the magnetic Weyl semimetal Co 3 Sn 2 S 2 Xu, Qiunan; Liu, Enke; Shi, Wujun Physical Review B, Vol. 97, Issue 23 https://doi.org/10.1103/physrevb.97.235416	journal	June 2018
Origin of magnetoresistance suppression in thin γ − MoT e 2 Zhong, Shazhou; Tiwari, Archana; Nichols, George Physical Review B, Vol. 97, Issue 24 https://doi.org/10.1103/physrevb.97.241409	journal	June 2018
Quantum oscillations in type-II Dirac semimetal PtTe 2 Fu, Dongzhi; Bo, Xiangyan; Fei, Fucong Physical Review B, Vol. 97, Issue 24 https://doi.org/10.1103/physrevb.97.245109	journal	June 2018
Temperature-induced inversion of the spin-photogalvanic effect in WTe 2 and MoTe 2 Lim, Sejoon; Rajamathi, Catherine R.; Süß, Vicky Physical Review B, Vol. 98, Issue 12 https://doi.org/10.1103/physrevb.98.121301	journal	September 2018
Phase transition and electronic structure evolution of MoTe 2 induced by W substitution Jin, Wencan; Schiros, Theanne; Lin, Yi Physical Review B, Vol. 98, Issue 14 https://doi.org/10.1103/physrevb.98.144114	journal	October 2018
Continuously tunable topological pump in high-dimensional cold atomic gases Yang, Yan-Bin; Duan, L. -M.; Xu, Yong Physical Review B, Vol. 98, Issue 16 https://doi.org/10.1103/physrevb.98.165128	journal	October 2018
Importance of electron correlations in understanding photoelectron spectroscopy and Weyl character of MoTe 2 Aryal, Niraj; Manousakis, Efstratios Physical Review B, Vol. 99, Issue 3 https://doi.org/10.1103/physrevb.99.035123	journal	January 2019
Emergence of topologically protected states in the MoTe 2 Weyl semimetal with layer-stacking order Schneeloch, John A.; Duan, Chunruo; Yang, Junjie Physical Review B, Vol. 99, Issue 16 https://doi.org/10.1103/physrevb.99.161105	journal	April 2019
Fragility of Fermi arcs in Dirac semimetals Wu, Yun; Jo, Na Hyun; Wang, Lin-Lin Physical Review B, Vol. 99, Issue 16 https://doi.org/10.1103/physrevb.99.161113	journal	April 2019
Phononic Weyl points and one-way topologically protected nontrivial phononic surface arc states in noncentrosymmetric WC-type materials Xie, Qing; Li, Jiangxu; Ullah, Sami Physical Review B, Vol. 99, Issue 17 https://doi.org/10.1103/physrevb.99.174306	journal	May 2019
Optical evidence of the type-II Weyl semimetals MoTe 2 and WTe 2 Kimura, Shin-ichi; Nakajima, Yuki; Mita, Zenjiro Physical Review B, Vol. 99, Issue 19 https://doi.org/10.1103/physrevb.99.195203	journal	May 2019
Single pair of Weyl fermions in the half-metallic semimetal EuC d 2 A s 2 Wang, Lin-Lin; Jo, Na Hyun; Kuthanazhi, Brinda Physical Review B, Vol. 99, Issue 24 https://doi.org/10.1103/physrevb.99.245147	journal	June 2019
Experimental Observation of Anisotropic Adler-Bell-Jackiw Anomaly in Type-II Weyl Semimetal WTe 1.98 Crystals at the Quasiclassical Regime Lv, Yang-Yang; Li, Xiao; Zhang, Bin-Bin Physical Review Letters, Vol. 118, Issue 9 https://doi.org/10.1103/physrevlett.118.096603	journal	March 2017
Multiple Types of Topological Fermions in Transition Metal Silicides Tang, Peizhe; Zhou, Quan; Zhang, Shou-Cheng Physical Review Letters, Vol. 119, Issue 20 https://doi.org/10.1103/physrevlett.119.206402	journal	November 2017
Fermiology and Superconductivity of Topological Surface States in PdTe 2 Clark, O. J.; Neat, M. J.; Okawa, K. Physical Review Letters, Vol. 120, Issue 15 https://doi.org/10.1103/physrevlett.120.156401	journal	April 2018
Bulk Fermi Surfaces of the Dirac Type-II Semimetallic Candidates M Al 3 (Where M = V , Nb, and Ta) Chen, K. -W.; Lian, X.; Lai, Y. Physical Review Letters, Vol. 120, Issue 20 https://doi.org/10.1103/physrevlett.120.206401	journal	May 2018
Evidence of a Coulomb-Interaction-Induced Lifshitz Transition and Robust Hybrid Weyl Semimetal in T d − MoTe 2 Xu, N.; Wang, Z. W.; Magrez, A. Physical Review Letters, Vol. 121, Issue 13 https://doi.org/10.1103/physrevlett.121.136401	journal	September 2018
Spin-Resolved Electronic Response to the Phase Transition in MoTe 2 Weber, Andrew P.; Rüßmann, Philipp; Xu, Nan Physical Review Letters, Vol. 121, Issue 15 https://doi.org/10.1103/physrevlett.121.156401	journal	October 2018
Higher-Order Topology, Monopole Nodal Lines, and the Origin of Large Fermi Arcs in Transition Metal Dichalcogenides X Te 2 ( X = Mo , W ) Wang, Zhijun; Wieder, Benjamin J.; Li, Jian Physical Review Letters, Vol. 123, Issue 18 https://doi.org/10.1103/physrevlett.123.186401	journal	October 2019
Mechanical control of crystal symmetry and superconductivity in Weyl semimetal MoTe 2 Heikes, Colin; Liu, I-Lin; Metz, Tristin Physical Review Materials, Vol. 2, Issue 7 https://doi.org/10.1103/physrevmaterials.2.074202	journal	July 2018
Thickness dependent electronic structure of exfoliated mono- and few-layer 1 T ′ − MoTe 2 Pawlik, A. -S.; Aswartham, S.; Morozov, I. Physical Review Materials, Vol. 2, Issue 10 https://doi.org/10.1103/physrevmaterials.2.104004	journal	October 2018
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe 2 Zhang, M. Y.; Wang, Z. X.; Li, Y. N. Physical Review X, Vol. 9, Issue 2 https://doi.org/10.1103/physrevx.9.021036	journal	May 2019
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Title: Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2

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Title: Spectroscopic evidence for a type II Weyl semimetallic state in MoTe₂