Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2

Huang, Lunan; McCormick, Timothy M.; Ochi, Masayuki; Zhao, Zhiying; Suzuki, Michi -To; Arita, Ryotaro; Wu, Yun; Mou, Daixiang; Cao, Huibo; Yan, Jiaqiang; Trivedi, Nandini; Kaminski, Adam

doi:10.1038/nmat4685

Title: Spectroscopic evidence for a type II Weyl semimetallic state in MoTe₂

Abstract

In a type I Dirac or Weyl semimetal, the low-energy states are squeezed to a single point in momentum space when the chemical potential μ is tuned precisely to the Dirac/Weyl point. Recently, a type II Weyl semimetal was predicted to exist, where the Weyl states connect hole and electron bands, separated by an indirect gap. This leads to unusual energy states, where hole and electron pockets touch at the Weyl point. In this paper, we present the discovery of a type II topological Weyl semimetal state in pure MoTe₂, where two sets of Weyl points (W^±₂ , W^±₃) exist at the touching points of electron and hole pockets and are located at different binding energies above E_F. Using angle-resolved photoemission spectroscopy, modelling, density functional theory and calculations of Berry curvature, we identify the Weyl points and demonstrate that they are connected by different sets of Fermi arcs for each of the two surface terminations. We also find new surface ‘track states’ that form closed loops and are unique to type II Weyl semimetals. Lastly, this material provides an exciting, new platform to study the properties of Weyl fermions.

Authors:

Huang, Lunan ^[1]; McCormick, Timothy M. ^[2]; Ochi, Masayuki ^[3]; Zhao, Zhiying ^[4]; Suzuki, Michi -To ^[5]; Arita, Ryotaro ^[6]; Wu, Yun ^[1];

^[1]; Cao, Huibo ^[7]; Yan, Jiaqiang ^[8]; Trivedi, Nandini ^[2]; Kaminski, Adam ^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)
The Ohio State Univ., Columbus, OH (United States)
Osaka Univ., Osaka (Japan)
Univ. of Tennessee, Knoxville, TN (United States)
RIKEN Center for Emergent Matter Science (CEMS), Saitama (Japan)
RIKEN Center for Emergent Matter Science (CEMS), Saitama (Japan); Tohoku Univ., Miyagi (Japan)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

Publication Date:: 2016-07-11

Research Org.:: Ames Lab., Ames, IA (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Ames Lab. and Iowa State Univ., Ames, IA (United States); RIKEN Center for Emergent Matter Science (CEMS), Wako (Japan); The Ohio State Univ., Columbus, OH (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Simons Foundation (United States)

Contributing Org.:: Osaka Univ. (Japan); Univ. of Tennessee, Knoxville, TN (United States); Tohoku Univ., Sendai (Japan)

OSTI Identifier:: 1278751

Alternate Identifier(s):: OSTI ID: 1338564

Report Number(s):: IS-J-9004
Journal ID: ISSN 1476-1122; nmat4685

Grant/Contract Number:: AC02-07CH11358; DMR-1420451; NSF-DMR-1309461; 343227

Resource Type:: Accepted Manuscript

Journal Name:: Nature Materials

Additional Journal Information:: Journal Volume: 15; Journal Issue: 11; Journal ID: ISSN 1476-1122

Publisher:: Nature Publishing Group

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; topological insulators

Citation Formats


                    Huang, Lunan, McCormick, Timothy M., Ochi, Masayuki, Zhao, Zhiying, Suzuki, Michi -To, Arita, Ryotaro, Wu, Yun, Mou, Daixiang, Cao, Huibo, Yan, Jiaqiang, Trivedi, Nandini, and Kaminski, Adam. Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2.  United States: N. p., 2016. 
Web.  doi:10.1038/nmat4685.

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                    Huang, Lunan, McCormick, Timothy M., Ochi, Masayuki, Zhao, Zhiying, Suzuki, Michi -To, Arita, Ryotaro, Wu, Yun, Mou, Daixiang, Cao, Huibo, Yan, Jiaqiang, Trivedi, Nandini, & Kaminski, Adam. Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2.  United States.  https://doi.org/10.1038/nmat4685

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                    Huang, Lunan, McCormick, Timothy M., Ochi, Masayuki, Zhao, Zhiying, Suzuki, Michi -To, Arita, Ryotaro, Wu, Yun, Mou, Daixiang, Cao, Huibo, Yan, Jiaqiang, Trivedi, Nandini, and Kaminski, Adam. Mon .  
"Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2".  United States.  https://doi.org/10.1038/nmat4685.  https://www.osti.gov/servlets/purl/1278751.

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@article{osti_1278751,

  title        = {Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2},

  author       = {Huang, Lunan and McCormick, Timothy M. and Ochi, Masayuki and Zhao, Zhiying and Suzuki, Michi -To and Arita, Ryotaro and Wu, Yun and Mou, Daixiang and Cao, Huibo and Yan, Jiaqiang and Trivedi, Nandini and Kaminski, Adam},

  abstractNote = {In a type I Dirac or Weyl semimetal, the low-energy states are squeezed to a single point in momentum space when the chemical potential μ is tuned precisely to the Dirac/Weyl point. Recently, a type II Weyl semimetal was predicted to exist, where the Weyl states connect hole and electron bands, separated by an indirect gap. This leads to unusual energy states, where hole and electron pockets touch at the Weyl point. In this paper, we present the discovery of a type II topological Weyl semimetal state in pure MoTe2, where two sets of Weyl points (W±2 , W±3) exist at the touching points of electron and hole pockets and are located at different binding energies above EF. Using angle-resolved photoemission spectroscopy, modelling, density functional theory and calculations of Berry curvature, we identify the Weyl points and demonstrate that they are connected by different sets of Fermi arcs for each of the two surface terminations. We also find new surface ‘track states’ that form closed loops and are unique to type II Weyl semimetals. Lastly, this material provides an exciting, new platform to study the properties of Weyl fermions.},

  doi          = {10.1038/nmat4685},

  journal      = {Nature Materials},

  number       = 11,

  volume       = 15,

  place        = {United States},

  year         = {2016},

  month        = {7}

}

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Armitage, N. P.; Mele, E. J.; Vishwanath, Ashvin
arXiv
DOI: 10.48550/arxiv.1705.01111

Unconventional quantum Hall effects in two-dimensional massive spin-1 fermion systems
text, January 2017

Xu, Yong; Duan, L. -M.
arXiv
DOI: 10.48550/arxiv.1705.05780

Flux growth in a horizontal configuration: an analogue to vapor transport growth
text, January 2017

Yan, J. -Q.; Sales, B. C.; Susner, M. A.
arXiv
DOI: 10.48550/arxiv.1706.02339

The semiclassical theory of anomalous transport in type-II topological Weyl semimetals
text, January 2017

McCormick, Timothy M.; McKay, Robert C.; Trivedi, Nandini
arXiv
DOI: 10.48550/arxiv.1707.06222

Imaginary part of Hall conductivity in tilted doped Weyl semimetal with both broken time reversal and inversion symmetry
text, January 2018

Mukherjee, S. P.; Carbotte, J. P.
arXiv
DOI: 10.48550/arxiv.1803.05366

Low-Temperature Eutectic Synthesis of PtTe2 with Weak Antilocalization and Controlled Layer Thinning
text, January 2018

Hao, Song; Zeng, Junwen; Xu, Tao
arXiv
DOI: 10.48550/arxiv.1808.02283

Quasiparticle Properties under Interactions in Weyl and Nodal Line Semimetals
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Kang, Jing; Zou, Jianfei; Li, Kai
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DOI: 10.48550/arxiv.1903.00170

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DOI: 10.48550/arxiv.1903.10612

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Li, Yupeng; Xu, Zhu-An
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DOI: 10.48550/arxiv.1907.04493

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Liu, D. F.; Liang, A. J.; Liu, E. K.
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DOI: 10.48550/arxiv.1909.09580

Angle-resolved photoemission spectroscopy and its application to topological materials
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Lv, Baiqing; Qian, Tian; Ding, Hong
arXiv
DOI: 10.48550/arxiv.2106.09797

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Title: Spectroscopic evidence for a type II Weyl semimetallic state in MoTe2

Abstract

Citation Formats

New type of Weyl semimetal with quadratic double Weyl fermions journal, January 2016

Topological nodal semimetals journal, December 2011

Generalized Gradient Approximation Made Simple journal, October 1996

A topological Dirac insulator in a quantum spin Hall phase journal, April 2008

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples journal, December 2015

Evolution of the Fermi surface of Weyl semimetals in the transition metal pnictide family journal, November 2015

Prediction of Weyl semimetal in orthorhombic MoTe 2 journal, October 2015

Type-II Weyl semimetals journal, November 2015

Structured Weyl Points in Spin-Orbit Coupled Fermionic Superfluids journal, December 2015

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation journal, November 2006

Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy journal, March 2014

Gravitation and the Electron journal, April 1929

Observation of Weyl nodes in TaAs journal, August 2015

Discovery of a Weyl fermion state with Fermi arcs in niobium arsenide journal, August 2015

Dirac node arcs in PtSn4 journal, April 2016

wannier90: A tool for obtaining maximally-localised Wannier functions journal, May 2008

Weyl semimetal phase in the non-centrosymmetric compound TaAs journal, August 2015

Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi journal, January 2014

Weyl Semimetal in a Topological Insulator Multilayer journal, September 2011

Nanostructured Carbon Allotropes with Weyl-like Loops and Points journal, September 2015

Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface journal, March 2011

Maximally localized generalized Wannier functions for composite energy bands journal, November 1997

Maximally localized Wannier functions for entangled energy bands journal, December 2001

Discovery of a Weyl fermion semimetal and topological Fermi arcs journal, July 2015

Weyl Semimetal in a Topological Insulator Multilayer text, January 2011

Discovery of a Three-dimensional Topological Dirac Semimetal, Na3Bi text, January 2013

Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs text, January 2015

Type-II Weyl Semimetals text, January 2015

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples text, January 2015

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation text, January 2006

In-Plane 2H-1T′ MoTe 2 Homojunctions Synthesized by Flux-Controlled Phase Engineering journal, February 2017

Weyl Semimetals as Hydrogen Evolution Catalysts journal, March 2017

A Simple Method for Synthesis of High-Quality Millimeter-Scale 1T′ Transition-Metal Telluride and Near-Field Nanooptical Properties journal, August 2017

Single-Crystalline Nanobelts Composed of Transition Metal Ditellurides journal, June 2018

Discovery of Superconductivity in 2M WS 2 with Possible Topological Surface States journal, June 2019

Optical Response of MoTe2 and WTe2 Weyl Semimetals: Distinguishing between Bulk and Surface Contributions journal, January 2020

Nonsaturating Magnetoresistance and Nontrivial Band Topology of Type‐II Weyl Semimetal NbIrTe 4 journal, July 2019

Novel 2D Layered Molybdenum Ditelluride Encapsulated in Few-Layer Graphene as High-Performance Anode for Lithium-Ion Batteries journal, February 2018

Highly Active, Durable Ultrathin MoTe 2 Layers for the Electroreduction of CO 2 to CH 4 journal, March 2018

Discovery of a new type of topological Weyl fermion semimetal state in MoxW1−xTe2 journal, December 2016

Signature of type-II Weyl semimetal phase in MoTe2 journal, January 2017

Weyl semimetals, Fermi arcs and chiral anomalies journal, October 2016

Lorentz-violating type-II Dirac fermions in transition metal dichalcogenide PtTe2 journal, August 2017

Signatures of the topological s +− superconducting order parameter in the type-II Weyl semimetal T d-MoTe2 journal, October 2017

Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2 journal, November 2017

Evidence for topological type-II Weyl semimetal WTe2 journal, December 2017

Spin-momentum locking and spin-orbit torques in magnetic nano-heterojunctions composed of Weyl semimetal WTe2 journal, September 2018

Temperature-driven topological transition in 1T'-MoTe2 journal, January 2018

Pressure-induced superconductivity in MoP journal, May 2018

Searching for topological Fermi arcs via quasiparticle interference on a type-II Weyl semimetal MoTe2 journal, August 2018

Electronic band tuning under pressure in MoTe2 topological semimetal journal, August 2019

Spatially dispersive circular photogalvanic effect in a Weyl semimetal journal, July 2019

Efficient topological materials discovery using symmetry indicators journal, February 2019

Visualizing electronic structures of quantum materials by angle-resolved photoemission spectroscopy journal, August 2018

Observation of unconventional chiral fermions with long Fermi arcs in CoSi journal, March 2019

Quasiparticle Properties under Interactions in Weyl and Nodal Line Semimetals journal, February 2019

Composition and temperature-dependent phase transition in miscible Mo1−xWxTe2 single crystals journal, March 2017

Metastable phase control of two-dimensional transition metal dichalcogenides on metal substrates journal, January 2018

Robust topological nodal lines in halide carbides journal, January 2019

Mobility spectrum analytical approach for the type-II Weyl semimetal T d -MoTe 2 journal, February 2018

Thermoelectric transport in torsional strained Weyl semimetals journal, February 2019

Magneto-resistance in pristine and irradiated TaAs 2 journal, April 2019

Field-effect transistor based on surface negative refraction in Weyl nanowire journal, January 2020

Quasiparticle interference on type-I and type-II Weyl semimetal surfaces: a review journal, January 2018

Quasiparticle scattering in type-II Weyl semimetal MoTe 2 journal, February 2018

Type I superconductivity in Dirac materials journal, July 2018

New developments in laser-based photoemission spectroscopy and its scientific applications: a key issues review journal, April 2018

Quantum oscillations in the type-II Dirac semi-metal candidate PtSe 2 journal, April 2018

Electronic properties of candidate type-II Weyl semimetal WTe 2 . A review perspective journal, March 2019

Nonlocal transport in superconducting heterostructures based on Weyl semimetals journal, August 2019

Giant optical activity and Kerr effect in type-I and type-II Weyl semimetals journal, August 2019

Enhanced interaction effects in the vicinity of the topological transition journal, October 2019

Layer-dependent spin-orbit torques generated by the centrosymmetric transition metal dichalcogenide β − MoTe 2 journal, November 2019

Electrodynamics of tilted Dirac and Weyl materials: A unique platform for unusual surface plasmon polaritons journal, November 2019

Asymmetric mass acquisition in LaBi: Topological semimetal candidate journal, August 2016

Hall effect within the colossal magnetoresistive semimetallic state of MoTe 2 journal, September 2016

Observation of Fermi arcs in the type-II Weyl semimetal candidate WTe 2 journal, September 2016

Title: Spectroscopic evidence for a type II Weyl semimetallic state in MoTe₂

New type of Weyl semimetal with quadratic double Weyl fermions
journal, January 2016

Topological nodal semimetals
journal, December 2011

Generalized Gradient Approximation Made Simple
journal, October 1996

A topological Dirac insulator in a quantum spin Hall phase
journal, April 2008

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
journal, December 2015

Evolution of the Fermi surface of Weyl semimetals in the transition metal pnictide family
journal, November 2015

Prediction of Weyl semimetal in orthorhombic ${MoTe}_{2}$
journal, October 2015

Type-II Weyl semimetals
journal, November 2015

Structured Weyl Points in Spin-Orbit Coupled Fermionic Superfluids
journal, December 2015

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation
journal, November 2006

Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy
journal, March 2014

Gravitation and the Electron
journal, April 1929

Observation of Weyl nodes in TaAs
journal, August 2015

Discovery of a Weyl fermion state with Fermi arcs in niobium arsenide
journal, August 2015

Dirac node arcs in PtSn4
journal, April 2016

wannier90: A tool for obtaining maximally-localised Wannier functions
journal, May 2008

Weyl semimetal phase in the non-centrosymmetric compound TaAs
journal, August 2015

Discovery of a Three-Dimensional Topological Dirac Semimetal, Na3Bi
journal, January 2014

Weyl Semimetal in a Topological Insulator Multilayer
journal, September 2011

Nanostructured Carbon Allotropes with Weyl-like Loops and Points
journal, September 2015

Dimensional crossover in topological matter: Evolution of the multiple Dirac point in the layered system to the flat band on the surface
journal, March 2011

Maximally localized generalized Wannier functions for composite energy bands
journal, November 1997

Maximally localized Wannier functions for entangled energy bands
journal, December 2001

Discovery of a Weyl fermion semimetal and topological Fermi arcs
journal, July 2015

Weyl Semimetal in a Topological Insulator Multilayer
text, January 2011

Discovery of a Three-dimensional Topological Dirac Semimetal, Na3Bi
text, January 2013

Discovery of a Weyl Fermion Semimetal and Topological Fermi Arcs
text, January 2015

Type-II Weyl Semimetals
text, January 2015

Use of frit-disc crucibles for routine and exploratory solution growth of single crystalline samples
text, January 2015

Ab initio calculation of the anomalous Hall conductivity by Wannier interpolation
text, January 2006

In-Plane 2H-1T′ MoTe ₂ Homojunctions Synthesized by Flux-Controlled Phase Engineering
journal, February 2017

Weyl Semimetals as Hydrogen Evolution Catalysts
journal, March 2017

A Simple Method for Synthesis of High-Quality Millimeter-Scale 1T′ Transition-Metal Telluride and Near-Field Nanooptical Properties
journal, August 2017

Single-Crystalline Nanobelts Composed of Transition Metal Ditellurides
journal, June 2018

Discovery of Superconductivity in 2M WS 2 with Possible Topological Surface States
journal, June 2019

Optical Response of MoTe2 and WTe2 Weyl Semimetals: Distinguishing between Bulk and Surface Contributions
journal, January 2020

Nonsaturating Magnetoresistance and Nontrivial Band Topology of Type‐II Weyl Semimetal NbIrTe ₄
journal, July 2019

Novel 2D Layered Molybdenum Ditelluride Encapsulated in Few-Layer Graphene as High-Performance Anode for Lithium-Ion Batteries
journal, February 2018

Highly Active, Durable Ultrathin MoTe ₂ Layers for the Electroreduction of CO ₂ to CH ₄
journal, March 2018

Discovery of a new type of topological Weyl fermion semimetal state in MoxW1−xTe2
journal, December 2016

Signature of type-II Weyl semimetal phase in MoTe2
journal, January 2017

Weyl semimetals, Fermi arcs and chiral anomalies
journal, October 2016

Lorentz-violating type-II Dirac fermions in transition metal dichalcogenide PtTe2
journal, August 2017

Signatures of the topological s +− superconducting order parameter in the type-II Weyl semimetal T d-MoTe2
journal, October 2017

Extremely high magnetoresistance and conductivity in the type-II Weyl semimetals WP2 and MoP2
journal, November 2017

Evidence for topological type-II Weyl semimetal WTe2
journal, December 2017

Spin-momentum locking and spin-orbit torques in magnetic nano-heterojunctions composed of Weyl semimetal WTe2
journal, September 2018

Temperature-driven topological transition in 1T'-MoTe2
journal, January 2018

Pressure-induced superconductivity in MoP
journal, May 2018

Searching for topological Fermi arcs via quasiparticle interference on a type-II Weyl semimetal MoTe2
journal, August 2018

Electronic band tuning under pressure in MoTe2 topological semimetal
journal, August 2019

Spatially dispersive circular photogalvanic effect in a Weyl semimetal
journal, July 2019

Efficient topological materials discovery using symmetry indicators
journal, February 2019

Visualizing electronic structures of quantum materials by angle-resolved photoemission spectroscopy
journal, August 2018

Observation of unconventional chiral fermions with long Fermi arcs in CoSi
journal, March 2019

Quasiparticle Properties under Interactions in Weyl and Nodal Line Semimetals
journal, February 2019

Composition and temperature-dependent phase transition in miscible Mo1−xWxTe2 single crystals
journal, March 2017

Metastable phase control of two-dimensional transition metal dichalcogenides on metal substrates
journal, January 2018

Robust topological nodal lines in halide carbides
journal, January 2019

Mobility spectrum analytical approach for the type-II Weyl semimetal T _d -MoTe ₂
journal, February 2018

Thermoelectric transport in torsional strained Weyl semimetals
journal, February 2019

Magneto-resistance in pristine and irradiated TaAs ₂
journal, April 2019

Field-effect transistor based on surface negative refraction in Weyl nanowire
journal, January 2020

Quasiparticle interference on type-I and type-II Weyl semimetal surfaces: a review
journal, January 2018

Quasiparticle scattering in type-II Weyl semimetal MoTe ₂
journal, February 2018

Type I superconductivity in Dirac materials
journal, July 2018

New developments in laser-based photoemission spectroscopy and its scientific applications: a key issues review
journal, April 2018

Quantum oscillations in the type-II Dirac semi-metal candidate PtSe ₂
journal, April 2018

Electronic properties of candidate type-II Weyl semimetal WTe ₂ . A review perspective
journal, March 2019

Nonlocal transport in superconducting heterostructures based on Weyl semimetals
journal, August 2019

Giant optical activity and Kerr effect in type-I and type-II Weyl semimetals
journal, August 2019

Enhanced interaction effects in the vicinity of the topological transition
journal, October 2019

Layer-dependent spin-orbit torques generated by the centrosymmetric transition metal dichalcogenide $β - {MoTe}_{2}$
journal, November 2019

Electrodynamics of tilted Dirac and Weyl materials: A unique platform for unusual surface plasmon polaritons
journal, November 2019

Asymmetric mass acquisition in LaBi: Topological semimetal candidate
journal, August 2016

Hall effect within the colossal magnetoresistive semimetallic state of ${MoTe}_{2}$
journal, September 2016

Observation of Fermi arcs in the type-II Weyl semimetal candidate ${WTe}_{2}$
journal, September 2016

Type-II Dirac fermions in the ${PtSe}_{2}$ class of transition metal dichalcogenides
journal, September 2016

Observation of Fermi arc and its connection with bulk states in the candidate type-II Weyl semimetal ${WTe}_{2}$
journal, December 2016