Itinerant and localized magnetization dynamics in antiferromagnetic Ho

Rettig, L.; Dornes, C.; Thielemann-Kuhn, N.; Pontius, N.; Zabel, H.; Schlagel, D. L.; Lograsso, T. A.; Chollet, M.; Robert, A.; Sikorski, M.; Song, S.; Glownia, J. M.; SchuBler-Langeheine, C.; Johnson, S. L.; Staub, U.

doi:10.1103/PhysRevLett.116.257202

Title: Itinerant and localized magnetization dynamics in antiferromagnetic Ho

Journal Article · 20 June 2016 · Physical Review Letters

DOI: https://doi.org/10.1103/PhysRevLett.116.257202 · OSTI ID:1278746

Rettig, L. ^[1]; Dornes, C. ^[2]; Thielemann-Kuhn, N. ^[3]; Pontius, N. ^[4]; Zabel, H. ^[5]; Schlagel, D. L. ^[6]; Lograsso, T. A. ^[7]; Chollet, M. ^[8]; Robert, A. ^[8]; Sikorski, M. ^[8]; Song, S. ^[8]; Glownia, J. M. ^[8]; SchuBler-Langeheine, C. ^[4]; Johnson, S. L. ^[2]; Staub, U. ^[1]

Paul Scherrer Inst. (PSI), Villigen (Switzerland)
ETH Zurich, Zurich (Switzerland)
Helmholtz-Zentrum Berlin fur Materialien und Energie GmbH, Berlin (Germany); Univ. Potsdam, Potsdam-Golm (Germany)
Helmholtz-Zentrum Berlin fur Materialien und Energie GmbH, Berlin (Germany)
Ruhr-Univ. Bochum, Bochum (Germany)
Ames Lab., Ames, IA (United States)
Iowa State Univ., Ames, IA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States)

Using femtosecond time-resolved resonant magnetic x-ray diffraction at the Ho L₃ absorption edge, we investigate the demagnetization dynamics in antiferromagnetically ordered metallic Ho after femtosecond optical excitation. Here, tuning the x-ray energy to the electric dipole (E1, 2p → 5d) or quadrupole (E2, 2p → 4f) transition allows us to selectively and independently study the spin dynamics of the itinerant 5d and localized 4f electronic subsystems via the suppression of the magnetic (2 1 3–τ) satellite peak. We find demagnetization time scales very similar to ferromagnetic 4f systems, suggesting that the loss of magnetic order occurs via a similar spin-flip process in both cases. The simultaneous demagnetization of both subsystems demonstrates strong intra-atomic 4f–5d exchange coupling. In addition, an ultrafast lattice contraction due to the release of magneto-striction leads to a transient shift of the magnetic satellite peak.

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Research Organization:: Ames Laboratory (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-07CH11358; AC02-76SF00515

OSTI ID:: 1278746

Alternate ID(s):: OSTI ID: 1258705

Report Number(s):: IS-J--8844

Journal Information:: Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 25 Vol. 116; ISSN 0031-9007; ISSN PRLTAO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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